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At least 937 records · Page 52

Development of Laser-Induced Breakdown Spectroscopy for the Californium-252 Supply Program

Calibration-free–laser-induced breakdown spectroscopy (CF-LIBS) is suggested as an alternative to traditional LIBS because it does not rely on calibration curves and instead relies on previously reported parameters called transition probabilities. Transition probabilities are fundamental parameters that describe the probability a specific transition from an upper energy to a lower energy will occur. These values act as internal calibrations and allow concentrations to be calculated based on the plasma temperature and electron density, which can be determined from Saha-Boltzmann methods. CF-LIBS provides the ability to perform elemental concentration estimations on samples without the need for chemical dilutions and only nanograms of material are ablated into the plasma. These benefits can be applied remotely inside hot cells, glove boxes, and radiation hoods through optical fibers. This report summarizes recent efforts to develop CF-LIBS methods for future applications within Oak Ridge National Laboratory’s radioisotope production portfolio, such as the Cf-252 Supply Program. Summaries are provided for the developed Python scripts for data analysis and two studies employing these programs to determine unreported transition probabilities of relevant lanthanides. Additionally, a review of fiber-delivered LIBS and a discussion of a LIBS fiber probe design are provided.

07 ISOTOPE AND RADIATION SOURCES↗

Serf studies of mass motions arising in flares

It is believed that radio type IVs, co-spatial with dense hot plasmoids, may be the result of a plasma radiation emission mechanism. The injection of mass into the corona was recently observed in chromospheric and coronal lines with magnetic field changes and also at very high speeds into loops. The start time of coronal loop transients, if extrapolated to the chromosphere, in most cases precedes flare H-alpha or X-ray emission. Observational inferences from polarization and other studies are seen as favoring the three-dimensional bubble over the planar loop as a description of coronal mass motions.

Wagner, W. J.↗

The laboratory simulation of unmagnetized supernova remnants Absence of a blast wave

Supernova remnants are experimentally simulated by irradiating spherical targets with eight-beam carbon dioxide laser in a chamber containing finite amounts of neutral gas, the gas being ionized by radiation from the hot target. The expansion velocities of the target plasmas are approximately the same as the expansion velocities of supernova ejecta and the experiment is successfully scaled to the case of a supernova remnant in an unmagnetized, low-density, interstellar medium. No sweep-up of the ambient plasma is detected, indicating that no hydrodynamic shock wave is formed to couple the target ejecta to the ambient gas. The experiment implies that if supernova ejecta couple to the interstellar medium, magnetic-field effects may be crucial to the physical description.

Borovsky, J. E.↗

Optical Microvariability of Blazars

We present the results of optical differential photometry of five blazers [PKS0219+428 (3C66A), PKS 0235+164 (AO 0235+16), H0414+019, PKS 0851+202 (OJ 187) and QSO 1807+698 (3C 371)] that were observed on 7 nights between November 05, 1997 and December 29, 1998, using the B and the V band filters. We have detected microvariations in four blazers (3C66A, AO 0235+16, H0414+019, and OJ 287). In addition, the light curve of AO 0235+16 has displayed a mini-flare when the brightness of this source was decreasing. Night-to-night variations have also been detected in 3C66A, H0414+019, and OJ 287. The results of our observations are discussed in the framework of accretion disk phenomena (magnetic flares or hot spots in accretion disks) and jet phenomena (plasma instabilities in jets).

Ghosh, K. K.↗

Multicomponent, Rare-Earth-Doped Thermal-Barrier Coatings

Multicomponent, rare-earth-doped, perovskite-type thermal-barrier coating materials have been developed in an effort to obtain lower thermal conductivity, greater phase stability, and greater high-temperature capability, relative to those of the prior thermal-barrier coating material of choice, which is yttria-partially stabilized zirconia. As used here, "thermal-barrier coatings" (TBCs) denotes thin ceramic layers used to insulate air-cooled metallic components of heat engines (e.g., gas turbines) from hot gases. These layers are generally fabricated by plasma spraying or physical vapor deposition of the TBC materials onto the metal components. A TBC as deposited has some porosity, which is desirable in that it reduces the thermal conductivity below the intrinsic thermal conductivity of the fully dense form of the material. Undesirably, the thermal conductivity gradually increases because the porosity gradually decreases as a consequence of sintering during high-temperature service. Because of these and other considerations such as phase transformations, the maximum allowable service temperature for yttria-partially stabilized zirconia TBCs lies in the range of about 1,200 to 1,300 C. In contrast, the present multicomponent, rare-earth-doped, perovskite-type TBCs can withstand higher temperatures.

Miller, Robert A.↗

A superconfiguration calculation of opacity with consistent bound and continuum electron treatments using green’s functions

One of the challenges in calculating the opacity of dense plasmas is the difficulty in consistently modeling electrons bound to nuclei and those that exist within the continuum of free states in electronic structure models. We address this issue by adapting the green's function approach, originally developed for use in average atom calculations, to the determination of superconfiguration (SC) electronic structure. The spectra created using these SCs indicate that a consistent treatment of continuum electronic structure is important for phenomena involving electrons near ionization thresholds, such as the pressure ionization of bound states and the opacity due to transitions near bound-free edges. Though important for dense plasmas, the detailed incorporation of continuum electrons into structure calculations does not have significant impact on the recent discrepancies between the predicted and measured opacity of hot, dense iron (Bailey et al 2015 Nature517 56). Here we find that the inclusion of plasma effects through an ion-sphere model along with our treatment of continuum electronic states gives a description of pressure ionization in hot, dense aluminum that is in better agreement with experiment than methods that rely on perturbative descriptions of the plasma environment (Hoarty et al 2013 Phys. Rev. Lett.110 265003).

74 ATOMIC AND MOLECULAR PHYSICS↗

A suite of neutron time-of-flight detectors to measure hot-spot motion in direct-drive inertial confinement fusion experiments on OMEGA

A suite of six neutron time of flight detectors capable of measuring the primary DT neutron energy spectrum has recently been completed on the OMEGA Laser System. The detectors are positioned along multiple quasi-orthogonal lines of sight (LOS’s) in either a stand-alone, collinear, or antipodal configuration. The collinear detector configuration enables one to measure the neutron velocity along the detector LOS independent of the neutron-production history, while the antipodal detector configuration enables one to directly measure of the hot-spot velocity along the detector axis and Gamow velocity shift due to the plasma ion temperature. Using these six measurements of the primary DT neutron energy spectrum, the neutron-averaged hot-spot velocity and Gamow velocity shift of DT fusion neutrons have been measured in cryogenic experiments on OMEGA for the first time. Finally, the detector suite is operable between DT neutron yields of 1 × 10 13 to 2 × 10 14 with an uncertainty of ~14 km/s in the neutron-averaged hot-spot velocity measurement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A different view of plasma flow inside P/Halley

The Giotto spacecraft carried two different instruments - the JPA and the IMS - for the observation of hot ions in the coma of P/Halley. Although there are many similarities in the time and distance profiles of the plasma flow parameters (bulk velocity, number density, and temperature) computed from the two data sets, there are also some significant differences, especially at cometocentric distances less than 500,000 km. The principal discrepancies between the JPA results presented by Formisano et al. (1990) and the IMS observations are: (1) the IMS did not detect the levelling off of the speed and temperature profiles that Formisano et al. interpreted as flow stabilization; (2) the IMS detected differential north-south flow between the solar wind and cometary ions for only a brief interval when the magnetic field was oriented nearly southward, whereas Formisano et al. reported more extensive differential north-south flow that was independent of the direction of the field; (3) the JPA ion densities were factors of 2 to 4 higher than the IMS ion densities which, in turn, were an order of magnitude greater than theoretical values.

Neugebauer, M.↗

Correlation of auroral hiss and upward electron beams near the polar cusp

Data were obtained from the DE-1 high-altitude plasma instrument (HAPI) and plasma wave instrument (PWI) during outbound passes through the polar cusp near local noon. The observed distribution functions of electron beams are fitted by drifting Maxwellian functions and the observed distribution functions of hot background electrons by isotropic Maxwellian functions. In addition, the cold plasma density is inferred from knowledge of the electron plasma frequency and the measured density of the warm plasma, including the electron beam distribution. The empirically fitted plasma parameters, including density, temperature and drifting energy, are used to solve the linear dispersion equation for the resulting whistler mode emissions. Because the whistler mode becomes quasi-electrostatic for wave-normal angles near the resonance cone, the electrostatic approximation is used for the whistler mode dispersion relation. The results of wave instability analyses are then compared with the wave observations. A ray tracing of cusp hiss emission is conducted to locate the wave source region (at about one earth-radius).

Lin, C. S.↗

Trailing Shield For Welding On Pipes

Trailing shield ensures layer of inert gas covers hot, newly formed bead between two tubes or pipes joined by plasma arc welding. Inert gas protects weld bead from oxidation by air until cooler and less vulnerable to oxidation. Intended for use on nickel-base alloy pipes, on which weld beads remain hot enough to oxidize after primary inert-gas purge from welding-torch cup has passed.

Coby, John B., Jr.↗

Plasma Science in Planetary Entry

Spacecraft entering a planetary atmosphere dissipate a great deal of energy into the surrounding gas. In the frame of reference of the vehicle, the atmospheric gas suddenly decelerates from hypersonic (Mach ~5-50) to subsonic velocities. The kinetic energy of the gas is rapidly converted to thermal and chemical energy, forming a bow shock behind which a plasma with energies on the order of one electron volt (eV) is produced. The resulting shock layer relaxes from strong thermal non-equilibrium that is translationally hot but internally cold and un-ionized toward a thermochemically equilibrated plasma over a distance of a few centimeters. Composition is dependent upon the planetary atmosphere – Air for Earth, CO2/N2 for Mars and Venus, N2/CH4 for Titan and H2/He/CH4 for Saturn, Neptune and Jupiter. Typical velocities of entry may range from 3-7 km/s (4-25 MJ/kg) for Titan/Mars, 8-14 km/s (30-100 MJ/kg) for Earth/Venus, and 25-40 km/s (300-800 MJ/kg) for outer planets. The equilibrium plasmas produced from these conditions are highly dissociated (up to and above 99%) and ionized (0.1- 15%), with temperatures from 7,000-15,000K and pressures from 0.1-1.0 bar. Understanding the behavior of these plasmas – the way in which they approach equilibrium, how they radiate, and how they interact with materials – is an active area of research necessitated by requirements to predict and test the performance of thermal protection systems (TPS) that enable spacecraft to deliver scientific instruments, and people, to foreign worlds and back to Earth. The endeavor is a multi-physics problem, with key processes highlighted in Fig. 1. This white paper describes the current state of the art in simulating shock layer plasmas both computationally and in ground test facilities. Gaps requiring further research and development are identified.

Cruden, Brett A.↗

Hot electrons between cold walls

We consider electron cooling in a collisionless plasma slab between two cold and freely emitting walls. Numerical calculations suggest a counterintuitive behavior of this system: the cooling rate slows down and eventually stops, leaving the system with a significant fraction of its initial thermal energy. Analytical treatment within the Vlasov–Poisson model reveals a set of steady-states with a two-component distribution of electrons: the primary electrons trapped within the potential wells and the secondary electrons forming the counterstreaming beams. We show that such steady-states are linearly stable with respect to one-dimensional perturbations. Establishment of a particular steady-state depends on initial conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Absorption of relativistic multi-picosecond laser pulses in wire arrays

We study the interaction of intense multi-picosecond laser pulses with arrays of carbon wires attached to solid substrates. Here, we find that laser absorption in wire arrays resembles that in flat targets with very large uniform plasma density gradients. Performing two-dimensional particle-in-cell simulations, we optimize target parameters like wire thickness and -distance for energy absorption of a 2picosecond laser pulse with a large focal spot; this has implications for x-ray- and charged particle source development.

43 PARTICLE ACCELERATORS↗

Non-perturbative quarkonium dissociation rates in strongly coupled quark-gluon plasma

Heavy quarks and quarkonia are versatile probes of the transport properties of the hot QCD medium produced in ultra-relativistic heavy-ion collisions (URHICs). A robust description of heavy-flavor transport coefficients requires a microscopic approach that treats the open and hidden heavy-flavor sectors on the same footing. Here, we employ the quantum many-body T -matrix formalism to evaluate the dissociation rates of heavy quarkonia in the quark-gluon plasma (QGP). The basic ingredient is the heavy-light T -matrix, which utilizes a nonperturbative driving kernel constrained by lattice-QCD data. Its resummation in a ladder series provides a much enhanced interaction strength compared to a previously used perturbative coupling to the quasiparticle partons in the QGP. The in-medium quarkonium properties, particularly their temperature-dependent binding energies, are obtained from selfconsistent calculations with the same interaction kernel, including interference effects (also referred to as the imaginary part of the heavy-quark potential) as well as off-shell parton spectral functions. We systematically investigate the interplay of these effects and elaborate on the connections to the dipole approximation used in effective field theory.

effective field theories of QCD↗

Electrostatic emissions between electron gyroharmonics in the outer magnetosphere

A scheme was constructed and a theoretical model was developed to classify electrostatic emissions. All of the emissions appear to be generated by the same basic mechanism: an unstable electron plasma distribution consisting of cold electrons (less than 100 eV) and hot loss cone electrons (about 1 keV). Each emission class is associated with a particular range of model parameters; the wide band electric field data can thus be used to infer the density and temperature of the cold plasma component. The model predicts that gyroharmonic emissions near the plasma frequency require large cold plasma densities.

Hubbard, R. F.↗

The plasma environment of Uranus

An overview of the observational results on the plasma environment at Uranus is given, and the implications of these observations for magnetospheric physics at Uranus are discussed. During the Voyager 2 encounter with Uranus, an extended magnetosphere filled with a tenuous plasma was detected. This low-energy plasma was found to consist of protons and electrons, with no significant heavy ion contribution, and with a density in the regions sampled by the spacecraft of at most three electrons per cubic centimeter. The plasma electrons and ions exhibit both a thermal component (with temperatures of tens of eV) and a hot component (with temperatures of a few keV). The thermal ion component is observed both inside and outside an L-shell value near 5, whereas the hot ion and electron component is excluded from the region inside of that L-shell. The source of the thermal component of the plasma is either the planetary ionosphere or the neutral hydrogen corona surrounding Uranus, whereas the hot component is convected in from the magnetotail, with probably an ionospheric source.

Belcher, J. W.↗

Interaction of SPI pellets with plasma on JET and associated disruptions

Abstract The presented data refer to the Shattered Pellet Injector (SPI) experiments carried out at JET in 2019–2020. This paper is a full journal version of the data originally presented as posters at TMPDM_2020 and EPS_2021. This paper presents various aspects of the interaction of pellets with plasma and associated disruptions. The experiment was performed with I p = (1.1–3.1) MA plasmas and mainly with Ne + D 2 pellet composition, but also with Ar pellets. The Current Quench (CQ) time, τ 80−20 , is the key characteristic of mitigation effectiveness. A pellet with a high content of Ne or Ar can reduce the CQ duration below the upper required JET threshold. Plasmas with high (thermal + internal poloidal magnetic) pre-disruptive plasma energy require a high content of Ne pellets to obtain a short CQ duration. Pellets with a small amount of Ne (and accordingly large amount of D), instead of causing a mitigated CQ, create the conditions for a ‘cold’ Vertical Displacement Events (VDE). The SPI was applied to plasma with different status: mainly to normal (‘healthy’) plasma, i.e. not prone to disruption, post-disruptive and VDE plasma. This study shows that SPI effectiveness in terms of CQ duration and, accordingly, EM loads does not depend on the state of the plasma, whether it is ‘healthy’ or post-disruptive plasma. SPI has been shown to reduce the axisymmetric vertical vessel reaction forces by about (30–40) % compared to unmitigated disruptions. On JET, the VDE, whether ‘hot’ or ‘cold’, always creates the conditions for a toroidal asymmetry in the plasma, so the VDE on the JET is referred to as Asymmetric VDE (AVDE). The interrupting of VDE and prevention of AVDE with SPI has been demonstrated. Thus, the effectiveness of disruption mitigation using SPI has been confirmed.

Gerasimov, S. N. (ORCID:0009000237937211)↗