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NASA NTRSDate not supplied

Linear Polarizer Design for Application in the Far-Ultraviolet Spectral Range

New mission concepts that are under consideration by NASA call for the design and implementation of Far Ultraviolet (FUV) polarizer technologies that have not been developed yet. A team that includes members from the NASA Goddard Space Flight Center (GSFC), Arizona State University (ASU), and Woodruff Consulting, worked on the design and development of a polarizer design that produce very high extinction ratios in the FUV spectral range (100-200 nm). This polarizer consists of reflecting light through a series of mirrors from a combination of two silicon carbide (SiC) and two lithium fluoride (LiF) crystals positioned at angles of incidence (relative to surface normal) close to the average LiF Brewster’s angle in the FUV. The output is a highly linearly polarized beam. This polarizer concept was fabricated and tested in the existing McPherson 225 Vacuum Ultraviolet (VUV) spectrometer located in the Optics Branch at NASA-GSFC. Initial testing using a MgF2 crystal at the Brewster’s angle as an analyzer has shown that this design can produce state-of-the-art extinction ratios at the Hydrogen Lyman-Alpha (Ly-α) wavelength of 121.6 nm, and that the measured extinction ratio of the two crossed polarizers, ≈114, is mostly limited by the MgF2 analyzer. A polarizer with such a performance at this wavelength has never been reported and it signifies a breakthrough in FUV polarization technology. The levels of effectiveness paired with the polarizer’s compact design allows for a new polarizer capability that would one day be implemented in a future FUV spectropolarimetry space mission.

Far Ultraviolet (FUV)↗
NASA NTRSDate not supplied

Exploring Environmental and Aerosol Impacts on Maritime Tropical Convection using Airborne Radiometer, Radar, Lidar, and Dropsondes

The field deployment phase of NASA’s Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) took place around the Philippines during August–October 2019, with the primary goal of jointly investigating aerosols and tropical meteorology at the micro-β to meso-β scales. A suite of instruments was deployed on NASA’s P-3B Orion aircraft to accomplish this mission, including: the Advanced Microwave Precipitation Radiometer (AMPR), Airborne Precipitation and cloud Radar 3rd Generation (APR-3), High Spectral Resolution Lidar 2 (HSRL2), and Advanced Vertical Atmospheric Profiling System (AVAPS) dropsondes. To examine potential aerosol influences on maritime tropical convection, P-3 flight segments throughout CAMP2Ex were binned into similar environmental groups using “low,” “medium,” and “high” values of nine AVAPS-derived parameters with known physical connections to convective frequency and/or intensity. Aerosol concentrations in each flight segment were evaluated using three HSRL2 variables at 355 and 532 nm: aerosol backscatter, aerosol extinction, and aerosol optical thickness. A set of radiometer- and radar-derived variables directly related to convective frequency and/or intensity was used to characterize convection, which included: AMPR-derived integrated cloud liquid water; polarization-corrected temperatures at 10.7, 19.35, 37.1, and 85.5 GHz; peak equivalent radar reflectivity factor (ZH); peak height of 30-dBZ ZH; and the number of radar data columns with composite ZH > 30 dBZ. The ZH analyses were performed using both Ku- and Ka-band APR-3 data. For each flight segment, correlation coefficients were calculated between each convective parameter and aerosol concentrations within the “low,” “medium,” and “high” groups for each environmental variable. The environmental stratification thresholds were then varied in a series of sensitivity tests. Several noteworthy correlations were observed between the convective and aerosol parameters within the environmental groups, especially when stratifying the environments based on their 850–500-hPa temperature lapse rate, 700–500-hPa temperature lapse rate, and K-Index. The convective parameters were often correlated most strongly with 355-nm extinction, 532-nm extinction, and 532-nm backscatter, while the presence of precipitation-sized liquid and ice hydrometeors contributed to some unexpected negative correlations. In general, as environmental conditions became more favorable for convection, a stronger correlation was observed between the convective parameters and aerosol concentrations. However, a “Goldilocks” zone of medium aerosol concentration was correlated most strongly with the convective parameters in many cases. These results stress the importance of considering environmental and aerosol conditions together when evaluating their impacts on convection. This presentation will provide a detailed discussion of these results and their implications, a summary of the limitations associated with such an analysis, and suggestions for future work.

Corey G. Amiot↗
NASA NTRSDate not supplied

Satellite-Assisted Particulate Matter (SAPM) for the Models, In situ, and Remote Sensing of Aerosols (MIRA) Working Group

Models, In situ, and Remote sensing of Aerosols (MIRA) is an international working group that provides a forum for collaborations amongst these three atmospheric aerosol communities. MIRA consists of a collection of interdisciplinary and independently funded Topic/Project groups with clear goals and generally characterized by requests for additional scientific data. The Satellite-Assisted Particulate Matter (SAPM) Topic group focuses on the study of fine particulate matter (PM2.5), as it is a major contributor to air pollution and negatively impacts human health. Our group aims to provide intercomparisons of various methods and techniques for estimating surface PM2.5 assisted by satellite remote sensors (passive and active), global aerosol models, and in situ aerosol measurements. The overall motivation of our work is to enhance PM2.5 coverage beyond in situ ground stations, which can be limited. In this presentation, we provide an overview of various PM2.5 estimation approaches by current SAPM team members, as each approach has its own strengths and limitations. One approach uses near-surface aerosol extinction retrievals from the spaceborne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and an assumed value of mass extinction efficiency to derive PM2.5 concentrations (Toth et al 2019). A study using this method found a promising agreement (R=0.60; slope=0.89) with U.S. Environmental Protection Agency (EPA) in situ PM2.5 measurements over the contiguous United States (CONUS) for a 12-year (2007-2018) period (Toth et al 2022). In a different approach combining spaceborne lidar and a model, the Cloud Aerosol Transport System (CATS) lidar and Goddard Earth Observing System (GEOS) model are blended in an ensemble variational assimilation scheme to retrieve aerosol extinction and convert speciated mass concentrations to total PM2.5. A recent study (Matus et al in prep.) found agreement within 2 μg/m3 over the CONUS on the 2016 annual mean when compared to EPA ground-based measurements. Another study explored trends in city aerosol optical depth (AOD) from a spaceborne passive remote sensor, Moderate Resolution Imaging Spectroradiometer (MODIS), and found that these trends agree well with trends in city surface PM2.5, which provides confidence in the use of city AOD for city PM2.5 trend studies (Vohra et al 2021). In a follow-on study, steep and significant trends (~2.5 to 7.8% a-1) in AOD are found for several South Asian cities (e.g., Bangalore and Hyderabad), suggesting rapid growth in PM2.5 (Vohra et al 2022). Also in this presentation, we report results on our current collective SAPM study of India, a country that exhibits high levels of PM2.5 pollution. We show the temporal (i.e., seasonal) and spatial variability of PM2.5 over India using the CALIOP and CATS+model approaches, comparisons between the estimated PM2.5 from the retrieval schemes, and validation with in situ PM2.5 ground-based observations from the Central Pollution Control Board in India. This region provides us with an excellent case study to test our PM2.5 retrievals in heavily polluted scenes and over a complex and varying topography. The SAPM Topic group actively seeks international participants/collaborators in our group, including those working with in situ aerosol measurements (e.g., ACTRIS). We are interested in aerosol datasets in order to either improve our PM2.5 estimates from various approaches (e.g., using in situ mass scattering/absorption coefficient and aerosol hygroscopic properties for various aerosol species) and/or validate the PM2.5 estimates (e.g., using in situ ground-based PM2.5 concentrations).

Travis D Toth↗
NASA NTRSDate not supplied

Variable Lidar Ratios for Marine and Dusty Marine Using MODIS AOD Constrained Retrievals and GOCART Model Simulations and their Impact on Level 2 CALIPSO Data Products in Version 5

The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard CALIPSO provided global measurements of attenuated backscatter profiles of various tropospheric aerosol species from June 2006 through June 2023. Extinction profiles are retrieved from these backscatter measurements by assuming a value for the extinction-to-backscatter or lidar ratio (LR). Up until version V4.51 of the data products, only a constant global value for each of the species has been used, spatially and temporally. However, it has been well known from various ground-based measurements that LRs of each aerosol species can potentially vary spatially as well seasonally. For the forthcoming Version 5 of the CALIPSO products, the CALIPSO team will implement variable lidar ratios at 532 nm for the species classified as “marine” and “dusty marine”. Here we present the essential elements of this scheme, which involves estimating lidar ratios by constraining Fernald solutions for the CALIOP particulate backscatter profiles using aerosol optical depths (AOD) from collocated MODIS retrievals. To account for the lack of measurements in various regions and seasons (e.g., Arctic winters), we leverage collocated model sea-salt volume fractions (SSVF) simulated by the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model and use an empirical relationship between the SSVF and LR to build hybrid climatological maps for the entire globe, i.e., using the modelled values when reliable values of the constrained LRs are not available. Initial evaluation of the resulting extinction profiles and corresponding AODs, both globally and in specific regions are presented using a limited amount of data. The primary improvement in AOD occurs in the coastal areas, like the Arabian Sea and Bay of Bengal. The estimated marine LR values in these regions are significantly higher than the constant value of 23 sr used in previous data releases, likely due to mixing with offshore pollution which results in higher AODs. Initial validation results using the CALIPSO Ocean Derived Column Optical Depth (ODCOD) retrievals and ground-based AERONET AOD measurements are presented.

CALIPSO↗
NASA NTRSDate not supplied

Spaceborne Lidar Retrievals of PM2.5 for Air Quality Studies and Applications

Fine particulate matter (PM2.5) substantially contributes to air pollution and negatively affects human health. While many studies have investigated the use of passive column-integrated aerosol optical depth to infer surface PM2.5, the use of lidar observations for air quality characterization is not nearly as extensive. Lidar measurements are critical, however, due to the vertical aerosol information they provide, including near the surface. In this presentation, we first provide an overview of various lidar-based approaches for estimating PM2.5 concentrations and then discuss how lidar measurements can assist other air quality applications. For example, estimates of PM2.5 have been obtained in a physics-based approach through CALIOP near-surface aerosol extinction retrievals, assumptions on the mass extinction efficiency, and incorporating other parameters (an aerosol hygroscopic growth factor and PM2.5/PM10 ratio). Application of this algorithm over the contiguous United States (CONUS) from 2006 to 2018 yielded larger PM2.5 values over the eastern and western CONUS (~10-15 μg/m³) and lower PM2.5 levels in the central CONUS (~5 μg/m³). These spatial patterns were similar to those from gridded PM2.5 concentrations obtained through in situ measurements at ground stations operated by the US Environmental Protection Agency. In another approach, the Cloud Aerosol Transport System (CATS) lidar was used with the Goddard Earth Observing System (GEOS) model in a 1D ensemble-based variational technique to obtain PM2.5 over the US and Europe, and the spatial patterns of the CATS/GEOS based PM2.5 concentrations generally captured those from surface stations (with corresponding hourly EPA PM2.5 vs CATS PM2.5 statistics of R=0.4 and bias=1.5 μg/m³). In our recent work, as part of the Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group, we have applied both the CALIOP and CATS/GEOS based approaches over the highly polluted country of India during the post-monsoon season (September-October 2016). We derived elevated levels of two-month mean PM2.5 (~100 μg/m³) in northern India, especially near New Delhi. These high PM2.5 concentrations in the Indo-Gangetic plain are driven in large part from the seasonal burning of crop residue and meteorological conditions typical at this time of the year, such as low wind speeds and a shallow boundary layer. While the satellite-derived PM2.5 moderately replicates (R = ~0.7-0.9) the spatial variability in the two-month mean of surface in situ PM2.5 from monitoring sites operated by the Central and State Pollution Control Boards, we show results from specific scenes for which there are large deviations between the satellite-derived PM2.5 and in situ measurements. Other current work on this topic focuses on developing PM2.5 estimates using airborne high spectral resolution lidar measurements through machine learning regression algorithms and involves several parameters (e.g., aerosol extinction, color ratio, lidar ratio). Application of this method over major metropolitan areas in the US and Asia have resulted in high correlations (R = 0.93) with surface measurements. This airborne lidar approach can be adapted to spaceborne lidar measurements, and all three of these approaches can be applied to ESA’s EarthCARE Atmospheric Lidar instrument, setting the stage for the future Cloud Aerosol Lidar for Global Scale Observations of the Ocean-Land Atmosphere System (CALIGOLA) mission. Ultimately, beyond estimates of PM2.5, the aerosol vertical distribution from lidars can benefit studies involving passive sensor approaches for PM2.5 proxies (including from geostationary satellites), wildfire smoke plume injection heights, volcanic emissions (e.g., ash height retrievals), and aerosol/air quality model assimilation, evaluation, and forecasts.

Travis D Toth↗
NASA NTRSDate not supplied

Particulate Emission and Optical Measurements in n-Heptane Low-Swirl Non-Premixed Flames at Elevated Pressures

A series of ground combustion tests conducted at elevated pressures demonstrates in-chamber optical measurements of soot emissions, combined with conventional gaseous and particle emissions sampling techniques. Utilizing a micro-radial-entry counter-swirl (MRX) burner, we successfully stabilized an n-heptane low-swirl, non-premixed spray flame across a wide range of equivalence ratios at pressures reaching 250 psia. Our optical diagnostics feature a temporally gated diffused-backlight illumination extinction imaging (DBI-EI) system, equipped with a 470-nm strobe high-intensity LED array as the illumination source, along with a line-of-sight telecentric camera. By accessing the flame tube, the pulsed DBI-EI provides illuminating optical extinction images, enabling experimental estimation of soot volume fractions within the reaction zone. This imaging technique will allow for real-time observation of soot formation dynamics occurring above the air-blast fuel injector. To further enhance our analysis, we employed simultaneous gaseous and particulate extractive diagnostics, interpreting in-flame particulate information through CO2 sampling, exhaust particle sizing, and particle counting. The processed dataset reveals a promising application of DBI-EI for propulsion emission analysis in high-pressure environments, where optical beam-steering effects can significantly impact results. This report is essential to bridging the divide between in-flame optical diagnostics and exhaust extractive measurements. By achieving an understanding of non-premixed combustion emission characteristics, we attempt to provide invaluable data for computer code validation, advancing the field of combustion research and supporting the development of cleaner, more efficient engines.

high-pressure flame↗
NASA NTRSDate not supplied

Particulate Emission and Optical Measurements in n-Heptane Low-Swirl Non-Premixed Flames at Elevated Pressures

A series of ground combustion tests conducted at elevated pressures demonstrates in-chamber optical measurements of soot emissions, combined with conventional gaseous and particle emissions sampling techniques. Utilizing a micro-radial-entry counter-swirl (MRX) burner, we successfully stabilized an n-heptane low-swirl, non-premixed spray flame across a wide range of equivalence ratios at pressures reaching 250 psia. Our optical diagnostics feature a temporally gated diffused-backlight illumination extinction imaging (DBI-EI) system, equipped with a 470-nm strobe high-intensity LED array as the illumination source, along with a line-of-sight telecentric camera. By accessing the flame tube, the pulsed DBI-EI provides illuminating optical extinction images, enabling experimental estimation of soot volume fractions within the reaction zone. This imaging technique will allow for real-time observation of soot formation dynamics occurring above the air-blast fuel injector. To further enhance our analysis, we employed simultaneous gaseous and particulate extractive diagnostics, interpreting in-flame particulate information through CO2 sampling, exhaust particle sizing, and particle counting. The processed dataset reveals a promising application of DBI-EI for propulsion emission analysis in high-pressure environments, where optical beam-steering effects can significantly impact results. This report is essential to bridging the divide between in-flame optical diagnostics and exhaust extractive measurements. By achieving an understanding of non-premixed combustion emission characteristics, we attempt to provide invaluable data for computer code validation, advancing the field of combustion research and supporting the development of cleaner, more efficient engines.

high-pressure flame↗
NASA NTRS1960

The Atmosphere and Haze of Mars

The 'blue haze' is an absorbing smoke, dark as soot in reflection, red in transmission. Its currently accepted explanation by pure scattering (omnidirectional or forward) is untenable, as it would either increase the surface brightness of fall to obscure the surface details. The limb darkening of Mars is mainly the results of absorption by the smoke. The opacity of the Martian atmosphere increases from the red toward the violet. The extinction by the Martian atmosphere is greater than that by the terrestrial at all wavelengths, but only about 20 per cent of the Martian extinction is due to scattering. Dollfus' polarimeteric estimate, corrected for self-absorption, corresponds to a martian atmospheric pressure of 87 mm Hg. The photochemical breakup of carbon dioxide and the escape of oxygen must lead to considerable concentrations of carbon monoxide in the martian atmosphere.

HAZE↗
NASA NTRS1972

Effects of normal acceleration on transient burning rate augmentation of an aluminized solid propellant

Instantaneous burning rate data for a polybutadiene acrylic acid propellant, containing 16 weight percent aluminum, were calculated from the pressure histories of a test motor with 96.77 sq cm of burning area and a 5.08-cm-thick propellant web. Additional acceleration tests were conducted with reduced propellant web thicknesses of 3.81, 2.54, and 1.27 cm. The metallic residue collected from the various web thickness tests was characterized by weight and shape and correlated with the instantaneous burning rate measurements. Rapid depressurization extinction tests were conducted in order that surface pitting characteristics due to localized increased burning rate could be correlated with the residue analysis and the instantaneous burning rate data. The acceleration-induced burning rate augmentation was strongly dependent on propellant distance burned, or burning time, and thus was transient in nature. The results from the extinction tests and the residue analyses indicate that the transient rate augmentation was highly dependent on local enhancement of the combustion zone heat feedback to the surface by the growth of molten residue particles on or just above the burning surface. The size, shape, and number density of molten residue particles, rather than the total residue weight, determined the acceleration-induced burning rate augmentation.

Northam, G. B.↗
NASA NTRS1972

Ultraviolet photometry of the eclipsing variable CW Cephei

A series of photometric observations was made of the eclipsing variable CW Cephei on the OAO 2. Approximate elements were derived from the eclipse depths and shape of the secondary. Persistent asymmetries and anomalous light variations, larger than the expected experimental error, were also found, subsequent ground-based observations show H alpha entirely in emission, indicating the presence of an extended gaseous system surrounding one or both components. A detailed comparison was made of the flux distribution of the binary relative to that for the nominally unreddened stars delta Pic, BlIII, and eta Aur, B3V, to investigate the effects of interstellar extinction. The resultant extinction curves, normalized at a wavelength of 3330 A, show a relatively smooth increase with decreasing wavelength.

Sobieski, S.↗
NASA NTRS1972

Ultraviolet photometry of globular clusters

Filter photometry measurements of the integrated light from several globular clusters between 1500 and 4000 A are discussed. The techniques and problems associated with carrying out photometry of faint extended sources with the OAO-2 instrumentation are described first. The energy distribution for globular clusters determined from these data are corrected for interstellar extinction on the basis of B-V color excesses and a mean ultraviolet extinction curve. The results are compared with synthetic cluster calculations. The ultraviolet energy distribution is primarily determined by the number of stars at the blue end of the horizontal branch.

Welch, G. A.↗
NASA NTRS1972

Reflectance of aqueous solutions

The optical properties and optical constants of water and aqueous solutions were studied to develop an accurate tabulation of graphical representations of the optical constants through a broad spectrum. Manuscripts of articles are presented concerning extinction coefficients, relative specular reflectance, and temperature effect on the water spectrum. Graphs of absolute reflectance, phase shifts, index of refraction, and extinction coefficients for water, heavy water and aqueous solutions are included.

Querry, M. R.↗
NASA NTRS1972

Photochemistry chemical kinetics in the interstellar medium.

Gas phase processes involving interstellar molecules are considered. The primary process is photodissociation in the ambient radiation field. In obscured regions, a combination of Johnson's (1965) and Stecher's (1969) Perseus extinction curves was used to obtain the radiation field as a function of the extinction at 5,500 A. On the basis of laboratory measurements, it is concluded that the molecules of water, ammonia, methane, and formaldehyde have lifetimes less than one hundred years.

Donn, B.↗
NASA NTRS1973

Interstellar grains.

Questions of interstellar extinction are discussed together with the spatial distribution of dust, the scattering of light by grains, diffuse interstellar absorption lines, and questions of interstellar polarization. Theoretical extinction curves are considered, giving attention to ice grains, graphite grains, polycyclic hydrocarbons, silicate grains, core-mantle grains, mixtures of grains, and the total amount of dust. Aspects of grain temperature and grain potential are examined along with processes on grain surfaces, the scattering of X rays by interstellar grains, the origin and destruction of grains, and the dust in the HII regions.

Aannestad, P. A.↗
NASA NTRS1974

An interdisciplinary study of the estaurine and coastal oceanography of Block Island Sound and adjacent New York coastal waters

ERTS-1 photographic data products have been analyzed using additive color viewing and electronic image analysis techniques. Satellite data were compared to water sample data collected simultaneously with the data of ERTS-1 coverage in New York Bight. Prediction of the absolute value of total suspended particles can be made using composites of positives of MSS bands 5 and 6 which have been precisely made using the step wedge supplied on the imagery. Predictions of the relative value of the extinction coefficient can be made using bands 4 and 5. Thematic charts of total suspended particles (particles per litre) and extinction coefficient provide scientists conducting state and federal water sampling programs in New York Bight with data which improves the performance of these programs.

Yost, E.↗
NASA NTRS1973

On the distance to Cygnus X-1

Interstellar extinction of 50 stars in the immediate vicinity of Cyg X-1 is compared with color excess of HDE 226868. The fact that HDE 226868 has extinction drastically exceeding that of all stars in the field at less than 1 kpc is believed to be in conflict with the model of Trimble et al. (1973) in which the primary is a luminous undermassive star and with other similar models. Uniform extrapolation of the reddening yields a distance estimate of (2.5 plus or minus 0.4) kpc for Cygnus X-1, in agreement with the spectroscopic modulus for an O9 star.

Margon, B.↗
NASA NTRS1974

The local complex of O and B stars. I - Distribution of stars and interstellar dust

The O-B5 stars, supergiants, young clusters, and associations within 1 kpc of the sun populate two flat systems inclined to each other by 19 to 22 deg. The historical background, statistical significance, composition, spatial arrangement of the contents, and interstellar extinction in the two belts are discussed. A more or less random distribution in space and in age characterizes the O-B5 stars of the 'galactic belt', which is aligned nearly along the Milky Way. The 'Gould belt' is inclined to the Milky Way (north in Sco-Oph and south in Orion), and exhibits a projected distribution of O-B5 stars in its mean plane that resembles a 'dragonfly', with five major features defining it. A crude 'diameter' of the system is 750 to 1000 pc, and the sun's position is eccentric, lying toward Ophiuchus. The nuclear age of the system, while not unique, may be characterized as 30 m.y. from the spectral type of the broad main-sequence turnup near B2-5. Most of the O-B2 stars and youngest stellar groups near the sun belong to the Gould belt, but both belts have approximately equal space densities of B3-B5 stars and similar average values of interstellar extinction.-

Stothers, R.↗
NASA NTRS1974

A dust-shell model of the infrared object HD 45677

A dust-shell model of the infrared star HD-45677 was constructed by means of a generalization of the mathematical techniques of Huang. The model shows that an isotropically scattering, uniform-density spherical circumstellar dust shell is able to account for the observed emergent energy distribution. The extinction properties of the grains required depend on the energy distribution incident on the inner boundary of the shell such that gray grains are needed if the stellar temperature is about 13,000 K and a reciprocal wavelength extinction law is indicated for a star of 20,000 K. This model for HD 45677 is compared with that of Dyck and Milkey, who propose free-free emission from a circumstellar gas shell to account for the observed infrared excess.

Apruzese, J. P.↗