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At least 937 records · Page 52
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Electroluminescence and cathodoluminescence from polyethylene and polypropylene films: Spectra reconstruction from elementary components and underlying mechanisms

The mechanisms of electroluminescence from large band gap polymers used as insulation in electric components are still under debate. It becomes important to unravel the underlying physics of the emission because of increasing thermo-electric stress and a possible relationship between electroluminescence and field withstand. We report herein on the cathodoluminescence spectra of polyethylene and polypropylene films as a way to uncover the nature of its contributions to electroluminescence emission. It is shown that spectra from the two materials are structured around four elementary components, each of them being associated with a specific process contributing to the overall emission with different weights depending on excitation conditions and on materials. The cathodoluminescence and electroluminescence spectra of each material are reconstructed from the four spectral components and their relative contribution are discussed. It is shown that electroluminescence from polyethylene and polypropylene has the same origin pointing towards generic mechanisms in both.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Hydrodynamic model for expansion and collisional relaxation of x-ray laser-excited multi-component nanoplasma

The irradiation of an atomic cluster with a femtosecond x-ray free-electron laser pulse results in a nanoplasma formation. This typically occurs within a few hundred femtoseconds. By this time the x-ray pulse is over, and the direct photoinduced processes no longer contributing. All created electrons within the nanoplasma are thermalized. The nanoplasma thus formed is a mixture of atoms, electrons, and ions of various charges. While expanding, it is undergoing electron impact ionization and three-body recombination. Below we present a hydrodynamic model to describe the dynamics of such multi-component nanoplasmas. The model equations are derived by taking the moments of the corresponding Boltzmann kinetic equations. We include the equations obtained, together with the source terms due to electron impact ionization and three-body recombination, in our hydrodynamic solver. Model predictions for a test case, expanding spherical Ar nanoplasma, are obtained. With this model, we complete the two-step approach to simulate x-ray created nanoplasmas, enabling computationally efficient simulations of their picosecond dynamics. Moreover, the hydrodynamic framework including collisional processes can be easily extended for other source terms and then applied to follow relaxation of any finite non-isothermal multi-component nanoplasma with its components relaxed into local thermodynamic equilibrium.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Mutual interaction between high and low stereo-regularity components for crystallization and melting behaviors of polypropylene blend fibers

Crystallization and melting behaviors of blend fibers of two types of polypropylene (PP), i.e. high stereo-regularity/high molecular weight PP (HPP) and low stereo-regularity/low molecular weight PP (LPP), was investigated. Blend fibers consisting of various HPP/LPP compositions were prepared through the melt spinning process. Differential scanning calorimetry (DSC), temperature modulated DSC (TMDSC) and wide-angle X-ray diffraction (WAXD) analysis were applied for clarifying the crystallization and melting behaviors of individual components. In the DSC measurement of blend fibers with high LPP composition, continuous endothermic heat was detected between the melting peaks of LPP at around 40 °C and that of HPP at around 160 °C. Such endothermic heat was more distinct for the blend fibers with higher LPP composition indicating that the melting of LPP in the heating process was hindered because of the presence of HPP crystals. On the other hand, heat of crystallization was detected at around 90 °C in the case of blend fibers with LPP content of 30 to 70 wt%, indicating that the crystallization of HPP component was taking place during the heating of as-spun blend fibers in the DSC measurement. Through the TMDSC analysis, re-organization of the crystalline structure through the simultaneous melting and re-crystallization was detected in the cases of HPP and blend fibers, whereas re-crystallization was not detected during the melting of LPP fibers. In the WAXD analysis during the heating of fibers, amount of a-form crystal was almost constant up to the melting in the case of single component HPP fibers, whereas there was a distinct increase of the intensity of crystalline reflections from around 100 °C, right after the melting of LPP in the case of blend fibers. These results suggested that the crystallization of HPP in the spinning process as well as during the conditioning process after spinning was hindered by the presence of LPP.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Nonlinear low frequency electrostatic structures in a magnetized two-component auroral plasma

Finite amplitude nonlinear ion-acoustic solitons, double layers, and supersolitons in a magnetized two-component plasma composed of adiabatic warm ions fluid and energetic nonthermal electrons are studied by employing the Sagdeev pseudopotential technique and assuming the charge neutrality condition at equilibrium. The model generates supersoliton structures at supersonic Mach numbers regime in addition to solitons and double layers, whereas in the unmagnetized two-component plasma case only, soliton and double layer solutions can be obtained. Further investigation revealed that wave obliqueness plays a critical role for the evolution of supersoliton structures in magnetized two-component plasmas. In addition, the effect of ion temperature and nonthermal energetic electron tends to decrease the speed of oscillation of the nonlinear electrostatic structures. The present theoretical results are compared with Viking satellite observations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Connected components of irreducible maps and 1D quantum phases

We investigate elementary topological properties of sets of completely positive (CP) maps that arise in quantum Perron-Frobenius theory. We prove that the set of primitive CP maps of fixed Kraus rank is path-connected and we provide a complete classification of the connected components of irreducible CP maps at given Kraus rank and fixed peripheral spectrum in terms of a multiplicity index. These findings are then applied to analyse 1D quantum phases by studying equivalence classes of translational invariant matrix product states that correspond to the connected components of the respective CP maps. Our results extend the previously obtained picture in that they do not require blocking of physical sites, they lead to analytic paths, and they allow us to decompose into ergodic components and to study the breaking of translational symmetry.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Achromatic registration of quadrature components of the optical spectrum in spectral domain optical coherence tomography

We have thoroughly investigated the method of simultaneous reception of spectral components with the achromatised quadrature phase shift between two portions of a reference wave, designed for the effective suppression of the 'mirror' artefact in the resulting image obtained by means of spectral domain optical coherence tomography (SD OCT). We have developed and experimentally tested a phase-shifting element consisting of a beam divider, which splits the reference optical beam into the two beams, and of delay lines being individual for each beam, which create a mutual phase difference of π/2 in the double pass of the reference beam. The phase shift achromatism over a wide spectral range is achieved by using in the delay lines the individual elements with different dispersion characteristics. The ranges of admissible adjustment parameters of the achromatised delay line are estimated for exact and inexact conformity of the geometric characteristics of its components to those calculated. A possibility of simultaneous recording of the close-to-quadrature spectral components with a single linear photodetector element is experimentally confirmed. The suppression of the artefact mirror peak in the OCT-signal by an additional 9 dB relative to the level of its suppression is experimentally achieved when the air delay line is used. Two-dimensional images of the surface positioned at an angle to the axis of the probe beam are obtained with the correction of the 'mirror' artefact while maintaining the dynamic range of the image. (laser biophotonics)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Consistent dynamics of the components of an elliptically polarised wave with zero mean amplitudes in a nonlinear isotropic gyrotropic medium in the adiabatic approximation

The adiabatic approximation is used to obtain an analytical solution to a nonintegrable problem of propagation of a plane elliptically polarised light wave with zero mean amplitudes of orthogonal circularly polarised field components through an isotropic gyrotropic medium with local and nonlocal components of Kerr nonlinearity and second-order group velocity dispersion. We describe the aperiodic evolution of bound (attributable to the medium nonlinearity) paired states, which are responsible for the propagation of two orthogonal polarisation components – cnoidal waves with significantly different periods. (nonlinear optical phenomena)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

High-power gas-discharge excimer ArF, KrCl, KrF and XeCl lasers utilising two-component gas mixtures without a buffer gas

Results of an experimental study of the influence of a gas mixture (laser active medium) composition on an output energy and total efficiency of gas-discharge excimer lasers on ArF* (193 nm), KrCl* (222 nm), KrF* (248 nm) and XeCl* (308 nm) molecules operating without a buffer gas are presented. The optimal ratios of gas components (from the viewpoint of a maximum output energy) of an active medium are found, which provide an efficient operation of laser sources. It is experimentally confirmed that for gas-discharge excimer lasers on halogenides of inert gases the presence of a buffer gas in an active medium is not a necessary condition for efficient operation. For the first time, in two-component gas mixtures of repetitively pulsed gas-discharge excimer lasers on electron transitions of excimer molecules ArF*, KrCl*, KrF* and XeCl*, the pulsed energy of laser radiation obtained under pumping by a transverse volume electric discharge in a low-pressure gas mixture without a buffer gas reached up to 170 mJ and a high pulsed output power (of up to 24 MW) was obtained at a FWHM duration of the KrF-laser pulse of 7 ns. The maximal total efficiency obtained in the experiment with two-component gas mixtures of KrF and XeCl lasers was 0.8%. (lasers)

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2026

Initial Assessment of 3D-Printed Molybdenum Lattices as a Substrate for Liquid Metal Plasma-Facing Components

Many liquid metal plasma-facing component concepts for fusion reactors require a capillary porous material to wick the liquid metal to the surface of the component. In this work, samples of 3D-printed molybdenum lattices designed to have pore sizes ranging from 100 to 1000 µm were fabricated by two different suppliers. The dimensions of the lattice structures were characterized using an optical microscope, revealing that the lattice walls were almost systematically thicker than they were designed to be and in turn the pores are all smaller than they were designed to be. In many cases the pores were completely clogged. Several spectroscopic techniques were used to characterize the chemical composition of the materials, collectively indicating the presence of a thick layer of oxygen-rich material extending more than 1 µm below the surface. Compression testing revealed significant asymmetry in the mechanical behavior depending on which direction the force was applied relative to the print direction. Lastly, lithium wetting tests of several lattice samples were performed, and a sample with ~250-µm pores was found to soak up lithium quickly after initial wetting of the surface occurred. The implications of these results for future liquid metal plasma-facing component design are discussed.

Parsons, Matthew S. [Princeton Plasma Physics Labo↗
DOE OSTI2013

A tidally stripped stellar component of the Magellanic bridge

Deep photometry of the Small Magellanic Cloud (SMC) stellar periphery (R = 4°, 4.2 kpc) is used to study its line-of-sight depth with red clump (RC) stars. The RC luminosity function is affected little by young (≲1 Gyr) blue-loop stars in these regions because their main-sequence counterparts are not observed in the color-magnitude diagrams. The SMCs eastern side is found to have a large line-of-sight depth (∼23 kpc) while the western side has a much shallower depth (∼10 kpc), consistent with previous photographic plate photometry results. We use a model SMC RC luminosity function to deconvolve the observed RC magnitudes and construct the density function in distance for our fields. Three of the eastern fields show a distance bimodality with one component at the 'systemic' ∼67 kpc SMC distance and a second component at ∼55 kpc. Our data are not reproduced well by the various extant Magellanic Cloud and Stream simulations. However, the models predict that the known H I Magellanic Bridge (stretching from the SMC eastward toward the Large Magellanic Cloud, LMC) has a decreasing distance with angle from the SMC and should be seen in both the gaseous and stellar components. From comparison with these models, we conclude that the most likely explanation for our newly identified ∼55 kpc stellar structure in the eastern SMC is a stellar counterpart of the H I Magellanic Bridge that was tidally stripped from the SMC ∼200 Myr ago during a close encounter with the LMC. This discovery has important implications for microlensing surveys of the SMC.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

OGLE-2013-BLG-0102LA,B: MICROLENSING BINARY WITH COMPONENTS AT STAR/BROWN DWARF AND BROWN DWARF/PLANET BOUNDARIES

We present an analysis of the gravitational microlensing event OGLE-2013-BLG-0102. The light curve of the event is characterized by a strong short-term anomaly superposed on a smoothly varying lensing curve with a moderate magnification A {sub max} ∼ 1.5. It is found that the event was produced by a binary lens with a mass ratio between the components of q = 0.13 and the anomaly was caused by the passage of the source trajectory over a caustic located away from the barycenter of the binary. Based on the analysis of the effects on the light curve due to the finite size of the source and the parallactic motion of the Earth, we determine the physical parameters of the lens system. The measured masses of the lens components are M {sub 1} = 0.096 ± 0.013 M {sub ☉} and M {sub 2} = 0.012 ± 0.002 M {sub ☉}, which correspond to near the hydrogen-burning and deuterium-burning mass limits, respectively. The distance to the lens is 3.04 ± 0.31 kpc and the projected separation between the lens components is 0.80 ± 0.08 AU.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

TITANIUM ISOTOPE SOURCE RELATIONS AND THE EXTENT OF MIXING IN THE PROTO-SOLAR NEBULA EXAMINED BY INDEPENDENT COMPONENT ANALYSIS

The Ti isotope variations observed in hibonites represent some of the largest isotope anomalies observed in the solar system. Titanium isotope compositions have previously been reported for a wide variety of different early solar system materials, including calcium, aluminum rich inclusions (CAIs) and CM hibonite grains, some of the earliest materials to form in the solar system, and bulk meteorites which formed later. These data have the potential to allow mixing of material to be traced between many different regions of the early solar system. We have used independent component analysis to examine the mixing end-members required to produce the compositions observed in the different data sets. The independent component analysis yields results identical to a linear regression for the bulk meteorites. The components identified for hibonite suggest that most of the grains are consistent with binary mixing from one of three highly anomalous nucleosynthetic sources. Comparison of these end-members show that the sources which dominate the variation of compositions in the meteorite parent body forming regions was not present in the region in which the hibonites formed. This suggests that the source which dominates variation in Ti isotope anomalies between the bulk meteorites was not present when the hibonite grains were forming. One explanation is that the bulk meteorite source may not be a primary nucleosynthetic source but was created by mixing two or more of the hibonite sources. Alternatively, the hibonite sources may have been diluted during subsequent nebula processing and are not a dominant solar system signatures.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Facility for high heat flux testing of irradiated fusion materials and components using infrared plasma arc lamps

A new high-heat flux testing facility using water-wall stabilized high-power high-pressure argon Plasma Arc Lamps (PALs) has been developed for fusion applications. It can handle irradiated plasma facing component materials and mock-up divertor components. Two PALs currently available at ORNL can provide maximum incident heat fluxes of 4.2 and 27 MW/m2 over a heated area of 9x12 and 1x10 cm2, respectively, which are fusion-prototypical steady state heat flux conditions. The facility will be described and the main differences between the photon-based high-heat flux testing facilities, such as PALs, and the e-beam and particle beam facilities more commonly used for fusion HHF testing are discussed. The components of the test chamber were designed to accommodate radiation safety and materials compatibility requirements posed by high-temperature exposure of low levels irradiated tungsten articles. Issues related to the operation and temperature measurements during testing are presented and discussed.

Sabau, Adrian S↗
DOE OSTI2018

Two distinct components of the delayed single electron noise in liquid xenon emission detectors

Single electron noise which persists for many milliseconds is known to follow ionizing events in liquid/gas xenon emission detectors. Due to the long timescale, this noise can be mistaken for a genuine signal. Therefore, it is a limiting background to the low-energy threshold of dark matter searches, and could prevent discovery-class searches for MeV scale hidden sector dark matter. A systematic study reveals distinct fast and slow components to the noise. The fast component is compatible with the hypothesis of electrons which were trapped below the liquid surface, and can be reduced by increasing the electric field across the liquid/gas interface. However, the slow component increases linearly with electric field. Hypotheses for the origin of this effect are discussed, and techniques for mitigation are suggested.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Characterization of UV optical components for photon detector calibration in liquid argon TPCs

Large liquid argon time projection chambers (LArTPCs)require stable and well-characterized delivery of ultraviolet (UV)light for in situ calibration of photosensors at cryogenictemperatures. This article reports bench-top and cryogenicmeasurements of the optical components used in a UV lightcalibration system, including multi-mode fused-silica fibers,SMA-to-SMA connectors, optical fiber feedthroughs, andlight-diffuser assemblies. Light loss in several fiber types and SMAconnectors was measured across wavelengths from275–970 mm. In addition,light-loss measurements of the tested fibers after severalliquid-nitrogen thermal cycles showed no statistically significantdegradation relative to baseline measurements, and high-rate pulsedexposure (30–90 million pulses from a275 nm LED) likewise showed nomeasurable aging in jacketed fibers. A compact, palm-sized,3D-printed PEEK diffuser housing with stacked UV-grade fused-silicadiffusers yields Lambertian emission and the most uniform angulardistribution. Optical components exhibiting improved UV transmissionwere deployed successfully in multiple DUNE small- and large-scaleprototypes, demonstrating reliable operation of UV light calibrationsystem. These findings inform component selection and calibrationprocedures for achieving reliable, uniform UV light delivery inlarge-scale cryogenic detectors such as DUNE.

Behera, B. [South Dakota Sch. Mines Tech.] (ORCID:↗
DOE OSTI2025

The ability of Salmonella enterica subsp. enterica strains to form biofilms on abiotic surfaces and their susceptibility to selected essential oil components

Abstract The ability of Salmonella enterica subsp. enterica to persist and form biofilms on different surfaces can constitute a source of food contamination, being an issue of global concern. The objective of this study was to understand the biofilm formation profile of 14 S. enterica strains among different serovars and sources and to evaluate the ability of essential oil (EO) components (carveol, citronellol, and citronellal) to disinfect the biofilms formed on stainless steel and polypropylene surfaces. All the strains were able to form biofilms with counts between 5.34 to 6.78 log CFU cm−2. Then, the minimum inhibitory concentration (MIC) and minimum bactericidal concentration (MBC) of EO components were evaluated on two selected strains. All compounds inhibited the growth of Salmonella Typhimurium (strain 1; MIC = 800–1000 µg ml−1) and Salmonella Enteritidis (strain 5; MIC = 400–1000 µg ml−1) and only carveol showed bactericidal activity against strains 1 and 5 (MBC = 1200 µg ml−1). Biofilms were exposed to the EO components at 10 × MIC for 30 min and polypropylene surfaces were more difficult to disinfect showing reductions between 0.9 and <1.2 log CFU cm−2. In general, the S. enterica biofilms demonstrated a significant tolerance to disinfection, demonstrating their high degree of recalcitrance on food processing surfaces.

Pérez-Lavalle, Liliana (ORCID:0000000344825031)↗
DOE OSTI2024

Negative components in the representation $\frac{𝑑^{2}⁡(𝜎⁢𝐸)}{𝑑⁡𝐸^2}$ of heavy-ion fusion cross sections

Negative components are observed in the representation $\frac{𝑑^{2}⁡(𝜎⁢𝐸)}{𝑑⁡𝐸^2}$ in heavy-ion fusions related to recent studies of noticeable oscillations in the high-energy region of the fusion excitation functions. A modified multiGaussian model has been developed, which includes contributions for both positive and negative components in the $\frac{𝑑^{2}⁡(𝜎⁢𝐸)}{𝑑⁡𝐸^2}$ representation. The model reproduces the heavy-ion fusion excitation functions very well, including oscillations. The property of these negative components in the $\frac{𝑑^{2}⁡(𝜎⁢𝐸)}{𝑑⁡𝐸^2}$ spectrum and the reaction mechanism of fusion at energies above the Coulomb barrier are investigated. Finally, the model also reproduces well light heavy-ion fusion reactions between 12 C and 16 O at high energy; results imply that the compound nucleus channel effect may have an important contribution at the high energy region for all fusion systems.

low & intermediate energy heavy-ion reactions↗
DOE OSTI2018

Possible determination of high-lying single-particle components with ( p , d ) reactions

A detailed feasibility study on deducing the high-lying single particle components (HLSPCs), which are important but used to be ignored, in the ground and low-lying excited states of even-even light nuclei is performed by analyses of (p, d) reactions with 12 C, 24 Mg, 28 Si, and 40 Ca targets at 51.93 MeV. Coupled reaction channel analyses have been made for (p, d) transitions to the j-forbidden excited states in 11 C (5/2 – ; 4.32 MeV), 23 Mg (7/2 + ; 2.05 MeV), 27 Si (7/2 + ; 2.16 MeV), and 39 Ca (9/2 – ; 3.64 MeV), including the major allowed transition components together with direct components of HLSPCs. Spectroscopic amplitudes of the HLSPCs are deduced by fitting the angular distributions of the ground and the j-forbidden excited states simultaneously. Lastly, the present analysis demonstrates for the first time that information about HLSPCs in atomic nuclei can be obtained from analysis of (p, d) reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗