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At least 937 records · Page 52

Remote Sensing of Tropospheric Aerosols from Space: Past, Present, and Future

Aerosol particles originate from man-made sources such as urban/industrial activities,rurning associated with land use processes, wind-blown dust, and natural sources. Their interaction with sunlight and their effect on cloud microphysics forms a major uncertainty in predicting climate change. Furthermore, the lifetime of only a few days causes high spatial variability in aerosol optical and radiative properties that requires global observations from space. Remote sensing of aerosol properties from space is reviewed both for present and planned national and international satellite sensors. Techniques that are being used to enhance our ability to characterize the global distribution of aerosol properties include well-calibrated multispectral radiometers, multispectral polarimeters, and multi-angle spectroradiometers. Though most of these sensor systems rely primarily on visible to mid-infrared spectral channels, the availability of of thermal channels to aid in cloud screening is an important additional piece of information that is not always incorporated into the sensor design. In this paper we describe the various satellite sensor systems being developed by Europe, Japan, and the U.S., and highlight the advantages and disadvantages of each of these systems for aerosol applications. An important underlying theme is that the remote sensing of aerosol properties, especially aerosol size distribution and single scattering albedo, is exceedingly difficult. As a consequence, no one sensor system is capable of providing totally unambiguous information, and hence a careful intercomparison of derived products from different sensors, together with a comprehensive network of ground-based sun-photometer and sky radiometer systems, are required to advance our quantitative understanding of global aerosol characteristics.

King, Michael D.↗

A Principal Component-Based Radiative Transfer Forward Model (PCRTM) for Vertically in Homogeneous Cloud

A principal-component based radiative transfer model (PCRTM) is developed for simulating the infrared spectral radiance at the top of the atmosphere (TOA). The PCRTM approach removes the redundancy in radiative transfer calculation in high resolution infrared spectra, and saves significant amount of computational time with great accuracy. In PCRTM, both ice and water clouds are treated as effective transmissivity and reflectivity stored in a pre-calculated lookup tables. These quantities are calculated using cloud single scattering properties such as cloud optical depth, cloud particle size, cloud phase, etc. The cloud can be inserted into any pressure layer in the PCRTM model (up to 100 layers). The effective temperature of each cloud layer is treated as a function of its optical depth. To test the accuracy of this approximation, the results are compared with the more rigorous DISORT model, which treats cloud as a plane parallel layer. The root-mean-square error of PCRTM, with respect to DISORT results, is generally less than 0.5 K in brightness temperature. However, the CPU time required by PCRTM was approximately two orders of magnitude less than that required by DISORT.

Li, Hui↗

Impact of Assimilated and Interactive Aerosol on Tropical Cyclogenesis

This article investigates the impact 3 of Saharan dust on the development of tropical cyclones in the Atlantic. A global data assimilation and forecast system, the NASA GEOS-5, is used to assimilate all satellite and conventional data sets used operationally for numerical weather prediction. In addition, this new GEOS-5 version includes assimilation of aerosol optical depth from the Moderate Resolution Imaging Spectroradiometer (MODIS). The analysis so obtained comprises atmospheric quantities and a realistic 3-d aerosol and cloud distribution, consistent with the meteorology and validated against Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and CloudSat data. These improved analyses are used to initialize GEOS-5 forecasts, explicitly accounting for aerosol direct radiative effects and their impact on the atmospheric dynamics. Parallel simulations with/without aerosol radiative effects show that effects of dust on static stability increase with time, becoming highly significant after day 5 and producing an environment less favorable to tropical cyclogenesis.

dust↗

Observation of the Spectrally Invariant Properties of Clouds in Cloudy-to-Clear Transition Zones During the MAGIC Field Campaign

We use the spectrally invariant method to study the variability of cloud optical thickness τau and droplet effective radius r(sub eff) in transition zones (between the cloudy and clear sky columns) observed from Solar Spectral Flux Radiometer (SSFR) and Shortwave Array Spectroradiometer-Zenith (SASZe) during the Marine ARM GPCI Investigation of Clouds (MAGIC) field campaign. The measurements from the SSFR and the SASZe are different, however inter-instrument differences of self-normalized measurements (divided by their own spectra at a fixed time) are small. The spectrally invariant method approximates the spectra in the cloud transition zone as a linear combination of definitely clear and cloudy spectra, where the coefficients, slope and intercept, characterize the spectrally invariant properties of the transition zone. Simulation results from the SBDART (Santa Barbara DISORT Atmospheric Radiative Transfer) model demonstrate that (1) the slope of the visible band is positively correlated with the cloud optical thickness τ while the intercept of the near-infrared band has high negative correlation with the cloud drop effective radius r(sub eff)even without the exact knowledge of τau; (2) the above relations hold for all Solar Zenith Angle (SZA) and for cloud-contaminated skies. In observations using redundant measurements from SSFR and SASZe, we find that during cloudy-to-clear transitions, (a) the slopes of the visible band decrease, and (b) the intercepts of the near-infrared band remain almost constant near cloud edges. The findings in simulations and observations suggest that, while the optical thickness decreases during the cloudy-to-clear transition, the cloud drop effective radius does not change when cloud edges are approached. These results support the hypothesis that inhomogeneous mixing dominates near cloud edges in the studied cases.

spectral invariance↗

The role of polar stratospheric clouds on total ozone minihole events

Using seven years of data from tha SAM 2 (Stratospheric Aerosol Measurement 2) and TOMS (Total Ozone Mapping Spectrometer) instruments, along with 70 mbar temperatures extracted from an NMC analysis, the effect of the austral spring polar stratospheric clouds (PSC) on the formation of total ozone miniholes is investigated. A total ozone minihole event is designated as the rapid decrease of more than 20 DU of total ozone over a time period of a day and a spatial extent of approximately 1000 by 1000 km. The severe decrease of total ozone during these minihole events could be explained in part by PSC being formed at altitudes of 10 to 24 km and preventing scattered UV radiation from ozone below the cloud from reaching the TOMS instrument. A result of the cloud's opaqueness is that the total ozone retrieval from TOMS data would underestimate the ozone column in the vicinity of the PSC. The approach to investigate the effect of PSC on total ozone was to use SAM 2 aerosol extinction values in conjunction with NMC stratospheric temperatures to determine if PSC are present during total ozone minihole events occurring during August and September, 1979 to 1986. The minihole events during these seven years were divided into two types: type 1, where the minihole region of 24 hour darkness from regions exposed to sunlight, and type 2, where the minihole occurred 5 to 10 degrees north of the terminator. The presence of PSC in a given region was ascertained by a maximum aerosol extinction greater than .006/km occurring with a temperature less than 189 K. It is found that PSC are consistently present with type 2 minihole events. This is contrasted with PSC rarely occurring in the same vicinity of type 2 miniholes. Also observed of that type 1 minihole events have minimum total ozone values which are on the average 3 to 10 DU smaller than type 2 miniholes. It can be concluded that care must be taken when trying to deduce a dynamical explanation of minihole events near the polar terminator and the role of PSC must be accounted for in type 1 minihole formation.

Sabutis, Joseph L.↗

Spatially Complete Global Surface Albedos Derived from Terra/MODIS Data

Spectral land surface albedo is an important parameter for describing the radiative properties of the Earth. Accordingly it reflects the consequences of natural and human interactions, such as anthropogenic, meteorological, and phenological effects, on global and local climatological trends. Consequently, albedos are integral parts in a variety of research areas, such as general circulation models (GCMs), energy balance studies, modeling of land use and land use change, and biophysical, oceanographic, and meteorological studies. , Over five years of land surface anisotropy, diffuse bihemispherical (white-sky) albedo and direct beam directional hemispherical (black-sky) albedo from observations acquired by the MODIS instruments aboard NASA s Terra and Aqua satellite platforms have provided researchers with unprecedented spatial, spectral, and temporal information on the land surface s radiative characteristics. However, roughly 30% of the global land surface, on an annual equal-angle basis, is obscured due to persistent and transient cloud cover, while another 207% is obscured due to ephemeral and seasonal snow effects. This precludes the MOD43B3 albedo products from being directly used in some remote sensing and ground-based applications, climate models, and global change research projects. To provide researchers with the requisite spatially complete global snow-free land surface albedo dataset, an ecosystem-dependent temporal interpolation technique was developed to fill missing or lower quality data and snow covered values from the official MOD43B3 dataset with geophysically realistic values. The method imposes pixel-level and local regional ecosystem-dependent phenological behavior onto retrieved pixel temporal data in such a way as to maintain pixel-level spatial and spectral detail and integrity. The phenological curves are derived from statistics based on the MODIS MOD12Q1 IGBP land cover classification product geolocated with the MOD43B3 data.

King, Michael D.↗

The impacts of immersion ice nucleation parameterizations on Arctic mixed-phase stratiform cloud properties and the Arctic radiation budget in GEOS-5

The influence of four different immersion freezing parameterizations on Arctic clouds and the top-of-the atmosphere (TOA) and surface radiation fluxes is investigated in the fifth version of the National Aeronautics and Space Administration (NASA) Goddard Earth Observing System (GEOS-5) with sea surface temperature, sea ice fraction and aerosol emissions held fixed. The different parameterizations were derived from a variety of sources, including classical nucleation theory, field and laboratory measurements. Despite the large spread in the ice-nucleating particle (INP) concentrations in the parameterizations, the cloud properties and radiative fluxes had a tendency to form two groups, with the lower INP concentration category producing larger water path and low-level cloud fraction during winter and early spring, whereas the opposite occurred during the summer season. The stability of the lower troposphere was found to strongly correlate with low-cloud fraction, and along with the effect of ice nucleation, ice sedimentation and melting rates, appears to explain the spring-to-summer reversal pattern in the relative magnitude of the cloud properties between the two categories of simulations. The strong modulation effect of the liquid phase on immersion freezing led to the successful simulation of the characteristic Arctic cloud structure, with a layer rich in supercooled water near cloud top and ice and snow at lower levels. Comparison with satellite retrievals and in situ data suggest that simulations with low INP concentrations more realistically represent Arctic clouds and radiation.

Arctic↗

Measurement of the Vertical Distribution of Aerosol by Globally Distributed MP Lidar Network Sites

The global distribution of aerosol has an important influence on climate through the scattering and absorption of shortwave radiation and through modification of cloud optical properties. Current satellite and other data already provide a great amount of information on aerosol distribution. However there are critical parameters that can only be obtained by active optical profiling. For aerosol, no passive technique can adequately resolve the height profile of aerosol. The aerosol height distribution is required for any model for aerosol transport and the height resolved radiative heating/cooling effect of aerosol. The Geoscience Laser Altimeter System (GLAS) is an orbital lidar to be launched by 2002. GLAS will provide global measurements of the height distribution of aerosol. The sampling will be limited by nadir only coverage. There is a need for local sites to address sampling, and accuracy factors. Full time measurements of the vertical distribution of aerosol are now being acquired at a number of globally distributed MP (micro pulse) lidar sites. The MP lidar systems provide profiling of all significant cloud and aerosol to the limit of signal attenuation from compact, eye safe instruments. There are currently six sites in operation and over a dozen planned. At all sites there are a complement of passive aerosol and radiation measurements supporting the lidar data. Four of the installations are at Atmospheric Radiation Measurement program sites. The aerosol measurements, retrievals and data products from the network sites will be discussed. The current and planned application of data to supplement satellite aerosol measurements is covered.

Spinhirne, James↗

Impact of Aerosols on Convective Clouds and Precipitation

Aerosols are a critical.factor in the atmospheric hydrological cycle and radiation budget. As a major agent for clouds to form and a significant attenuator of solar radiation, aerosols affect climate in several ways. Current research suggests that aerosols have a major impact on the dynamics, microphysics, and electrification properties of continental mixed-phase convective clouds. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing a significant source of cloud condensation nuclei (CCN). Such pollution . effects on precipitation potentially have enormous climatic consequences both in terms of feedbacks involving the land surface via rainfall as well as the surface energy budget and changes in latent heat input to the atmosphere. Basically, aerosol concentrations can influence cloud droplet size distributions, the warm-rain process, the cold-rain process, cloud-top heights, the depth of the mixed-phase region, and the occurrence of lightning. Recently, many cloud resolution models (CRMs) have been used to examine the role of aerosols on mixed-phase convective clouds. These modeling studies have many differences in terms of model configuration (two- or three-dimensional), domain size, grid spacing (150-3000 m), microphysics (two-moment bulk, simple or sophisticated spectral-bin), turbulence (1st or 1.5 order turbulent kinetic energy (TKE)), radiation, lateral boundary conditions (i.e., closed, radiative open or cyclic), cases (isolated convection, tropical or midlatitude squall lines) and model integration time (e.g., 2.5 to 48 hours). Among these modeling studies, the most striking difference is that cumulative precipitation can either increase or decrease in response to higher concentrations of CCN. In this presentation, we review past efforts and summarize our current understanding of the effect of aerosols on convective precipitation processes. Specifically, this paper addresses the following topics: observational evidence of the effect of aerosols on precipitation processes, and results from (CRM) simulations. Note that this presentation is mainly based on a recent paper published in Geophy. Rev. (Tao et al. 2012).

Tao, Wei-Kuo↗

Origin and evolution of the zodiacal dust cloud

The astrophysical importance of the zodiacal cloud became more apparent. The most useful source of information on the structure of the zodiacal cloud is the Infrared Astronomical Satellite (IRAS) observations. A substantial fraction of the extensive IRAS data set was analyzed. Also, a numerical model was developed (SIMUL) that allows to calculate the distribution of night-sky brightness that would be produced by any particular distribution of dust particle orbits. This model includes the effects of orbital perturbations by both the planets and solar radiation, it reproduces the exact viewing geometry of the IRAS telescope, and allows for the eccentricity of the Earth's orbit. SIMUL now is used to model not just the solar system dust bands discovered by IRAS but the whole zodiacal cloud.

Dermott, S. F.↗

Time scales for molecule formation by ion-molecule reactions

Analytical solutions are obtained for nonlinear differential equations governing the time-dependence of molecular abundances in interstellar clouds. Three gas-phase reaction schemes are considered separately for the regions where each dominates. The particular case of CO, and closely related members of the Oh and CH families of molecules, is studied for given values of temperature, density, and the radiation field. Nonlinear effects and couplings with particular ions are found to be important. The time scales for CO formation range from 100,000 to a few million years, depending on the chemistry and regime. The time required for essentially complete conversion of C(+) to CO in the region where the H3(+) chemistry dominates is several million years. Because this time is longer than or comparable to dynamical time scales for dense interstellar clouds, steady-state abundances may not be observed in such clouds.

Langer, W. D.↗

NASA/GEWEX SRB Surface Radiation Budget Fluxes Through the Prism of Weather States

The NASA/GEWEX Surface Radiation Budget Version 4 (SRB Rel4) product is now publicly available, covering the period from July 1983 through June 2017. This supersedes the SRB Rel3 (Stackhouse et al., 2011) product which has been used in the community for a wide variety of applications, including climate model validation, agriculture, solar energy, and architecture. SRB Rel4 uses the newly recalibrated and processed ISCCP HXS product as its primary input for cloud and radiance data, replacing ISCCP DX with a ninefold increase in pixel count (10km instead of 30km). This version retains a 1°x1° resolution but benefits from a much larger number of samples per grid box than the SRB Rel3. ISCCP also provides an atmospheric temperature and moisture dataset known as nnHIRS which we use here, along with Seaflux and Landflux surface and near-surface meteorological parameters. Rel4 incorporates several important algorithm improvements. These include recalculated shortwave (SW) atmospheric transmissivities and reflectivities yielding a somewhat less transmissive atmosphere. Both shortwave and longwave (LW) now also include variable aerosol composition and radiative properties, allowing for the use of a detailed aerosol history from the Max Planck Institute Aerosol Climatology (MACv1). LW and SW algorithms now produce pristine sky fluxes, allowing the aerosol flux effects to be quantified. For SW, ocean albedo and snow/ice albedo are improved from Release 3. Total solar irradiance is now variable, and reduced to an average of 1361 Wm-2. The radiative treatment of ice cloud is improved. For the LW, a climatological monthly varying spectral surface emissivity is added. Here we evaluate the SRB Rel4 top of atmosphere (TOA) and surface fluxes in the context of weather states and oceanic regions. Weather states (Tselioudis et al., 2013, Tselioudis et al., 2021) are defined by K-means clustering 2-D histograms of satellite-retrieved cloud optical depths and cloud top pressures. The most recent (Tselioudis et al., 2021) weather states derived from the International Satellite Cloud Climatology Project (ISCCP) H-series data results in eight cloud weather states and one clear sky weather state, for a total of nine weather states. We examine the statistics of SRB Rel4 fluxes for each weather state and a variety of relevant land and ocean regions. We compare to similar analyses performed on CERES EBAF and SYN1Deg flux products, and validate against Baseline Surface Radiometer Network (BSRN) land stations and Pacific Marine Environmental Laboratory (PMEL) ocean buoy data. It is demonstrated that the weather state concept is valuable when examining the comparative strengths and weaknesses of satellite radiative flux algorithms.

Atmospheric Radiation↗

Aerosol, radiation, and climate

Airborne, spaceborne, and ground-based measurements are used to study the radiative and climatic effects of aerosols. The data, which are modelled with a hierarchy of radiation and climate models, and their implications are summarized. Consideration is given to volcanic aerosols, polar stratospheric clouds, and the Arctic haze. It is shown that several types of aerosols (volcanic particles and the Arctic haze) cause significant alterations to the radiation budget of the regions where they are located.

Pollack, J. B.↗

Parameterization of sub-grid scale convection

The following topics are discussed: an overview of the cumulus parameterization problem; interactions between explicit and implicit processes in mesoscale models; effects of model grid size on the cumulus parameterization problem; parameterizing convective effects on momentum fields in mesoscale models; differences between slantwise and vertical cumulus parameterization; experiments with different closure hypotheses; and coupling cumulus parameterizations to boundary layer, stable cloud, and radiation schemes.

Frank, William↗

Aerosol Loading and Radiation Budget Perturbations in Densely Populated and Highly Polluted Indo-Gangetic Plain by COVID-19: Influences on Cloud Properties and Air Temperature

Aerosols emitted in densely populated and industrialized Indo-Gangetic Plain, one of the most polluted regions in the world, modulate regional climate, monsoon, and Himalayan glacier retreat. Thus, this region is important for understanding aerosol perturbations and their resulting impacts on atmospheric changes during COVID-19 lockdown period, a natural experimental condition created by the pandemic. By analyzing 5 years (2016–2020) data of aerosols and performing a radiative transfer calculation, we found that columnar and near-surface aerosol loadings decreased, leading to reductions in radiative cooling at the surface and top of the atmosphere and atmospheric warming during lockdown period. Further, satellite data analyses showed increases in cloud optical thickness and cloud-particle effective radius and decrease in lower tropospheric air temperature during lockdown period. These results indicate critical influences of COVID-19 lockdown on regional climate and water cycle over Indo-Gangetic Plain, emphasizing need for further studies from modeling perspectives.

P Khatri↗

Theoretical and Observational Determination of Global and Regional Radiation Budget, Forcing and Feedbacks at the Top-of-Atmosphere and Surface

Report consists of: 1. List of accomplishments 2. List of publications 3. Abstracts of published or submitted papers and 4. Subject invention disclosure. The accomplishments of the grant listed are: 1. Improved the third-order turbulence closure in cloud resolving models to remove the liquid water oscillation. 2. Used the University of California-Los Angeles (UCLA) large-eddy simulation (LES) model to provide data for radiation transfer testing. 3. Revised shortwave k-distribution models based on HITRAN 2000. 4. Developed a gamma-weighted two-stream radiative transfer model for radiation budget estimate applications. 5. Estimated the effect of spherical geometry to the earth radiation budget. 6. Estimated top-of-atmosphere irradiance over snow and sea ice surfaces. 7. Estimated the aerosol direct radiative effect at the top of the atmosphere. 8. Estimated the top-of-atmosphere reflectance of the clear-sky molecular atmosphere over ocean. 9. Developed and validated new set of Angular Distribution Models for the CERES TRMM satellite instrument (tropical) 10. Developed and validated new set of Angular Distribution Models for the CERES Terra satellite instrument (global) 11. Quantified the top-of-atmosphere direct radiative effect of aerosols over global oceans from merged CERES and MODIS observations 12 Clarified the definition of TOA flux reference level for radiation budget studies 13. Developed new algorithm for unfaltering CERES measured radiances 14. Used multiangle POLDER measurements to produce narrowband angular distribution models and examine the effect of scene identification errors on TOA albedo estimates 15. Developed and validated a novel algorithm called the Multidirectional Reflectance Matching (MRM) model for inferring TOA albedos from ice clouds using multi-angle satellite measurements. 16. Developed and validated a novel algorithm called the Multidirectional Polarized Reflectance Matching (MPRM) model for inferring particle shapes from ice clouds using multi-angle polarized satellite measurements. 17. Developed 4 advanced light scattering models including the three-dimensional (3D) uniaxial perfectly matched layer (UPML) finite-difference time-domain (FDTD) model. 18. Develop sunglint in situ measurement and study reflectance distribution in the sunglint area. 19. Lead a balloon-borne radiometer TOA albedo validation effort. 20. Developed a CERES surface UVB, UVA, and UV index product.

Loeb, Norman G.↗

Toward the characterization of upper tropospheric clouds using Atmospheric Infrared Sounder and Microwave Limb Sounder observations

We estimate the accuracy of cloud top altitude (Z) retrievals from the Atmospheric Infrared Sounder (AIRS) and Advanced Microwave Sounding Unit (AMSU) observing suite (ZA) on board the Earth Observing System Aqua platform. We compare ZA with coincident measurements of Z derived from the micropulse lidar and millimeter wave cloud radar at the Atmospheric Radiation Measurement (ARM) program sites of Nauru and Manus islands (ZARM) and the inferred Z from vertically resolved Microwave Limb Sounder (MLS) ice water content (IWC) retrievals. The mean difference in ZA minus ZARM plus or minus one standard deviation ranges from −2.2 to 1.6 km ± 1.0 to 4.2 km for all cases of AIRS effective cloud fraction (f A) > 0.15 at Manus Island using the cloud radar only. The range of mean values results from using different approaches to determine ZARM, day/night differences, and the magnitude of f A; the variation about the mean decreases for increasing values of f A. Analysis of ZARM from the micropulse lidar at Nauru Island for cases restricted to 0.05 ≤ f A ≤ 0.15 indicates a statistically significant improvement in ZA − ZARM over the cloud radar-derived values at Manus Island. In these cases the ZA − ZARM difference is −1.1 to 2.1 km ± 3.0 to 4.5 km. These results imply that the operational ZA is quantitatively useful for constraining cirrus altitude despite the nominal 45 km horizontal resolution. Mean differences of cloud top pressure (PCLD) inferred from coincident AIRS and MLS ice water content (IWC) retrievals depend upon the method of defining AIRS PCLD (as with the ARM comparisons) over the MLS spatial scale, the peak altitude and maximum value of MLS IWC, and f A. AIRS and MLS yield similar vertical frequency distributions when comparisons are limited to f A > 0.1 and IWC > 1.0 mg m−3. Therefore the agreement depends upon the opacity of the cloud, with decreased agreement for optically tenuous clouds. Further, the mean difference and standard deviation of AIRS and MLS PCLD are highly dependent on the MLS tangent altitude. For MLS tangent altitudes greater than 146 hPa, the strength of the limb technique, the disagreement becomes statistically significant. This implies that AIRS and MLS “agree” in a statistical sense at lower tangent altitudes and “disagree” at higher tangent altitudes. These results provide important insights on upper tropospheric cloudiness as observed by nadir-viewing AIRS and limb-viewing MLS.

Wu, Dong L.↗