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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Impact of Newly Measured 𝛽-Delayed Neutron Emitters around 78 Ni on Light Element Nucleosynthesis in the Neutrino Wind Following a Neutron Star Merger

Neutron emission probabilities and half-lives of 37 𝛽-delayed neutron emitters from 75 Ni to 92 Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and six half-lives for the first time that supersede theoretical estimates. These nuclei lie in the path of the weak 𝑟 process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars synthesizing elements in the 𝐴∼80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and have been identified in the AT2017gfo event, associated to the gravitational wave detection GW170817. Abundance calculations based on over 17,000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50%–70% in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal poor stars and thus is significant in the comparison with other possible astrophysical processes contributing to the light-element production. These results underline the importance of including experimental decay data for very neutron-rich 𝛽 -delayed neutron emitters into 𝑟 -process models.

59 ≤ A ≤ 89↗
DOE OSTI2026

Scintillation of liquid nitrogen

Liquid nitrogen is commonly used in cryogenic applications and is a promising medium for the direct immersion cooling of sensors used for nuclear and particle physics experiments. The scintillation properties of gaseous nitrogen are well-documented, but little is known about the scintillation of liquid nitrogen. If present, scintillation light from interactions of ambient radioactivity could produce backgrounds for rare event searches such as the direct detection of dark matter. Using a coincidence-tagged alpha decay, we demonstrate that liquid nitrogen exhibits measurable, albeit very faint, scintillation. Assuming the same scintillation wavelengths as gaseous nitrogen, we estimate a relative scintillation yield of $Y_{\liquidn}/Y^{\STP}_{\gasn} =$ \num[uncertainty-descriptors={stat,sys}]{0.0142(0.0005)(0.0030)} with respect to gaseous nitrogen at standard temperature and pressure. Considering the average scintillation yield from alpha decays in gaseous nitrogen, this implies a scintillation yield for alpha decays in liquid nitrogen of $Y_{\liquidn} = \qty[]{2.39(0.56)}{photons~per~MeV}$. To our knowledge this is the first measurement of scintillation in liquid nitrogen.

Pagani, Luca (ORCID:0000000234692581)↗
DOE OSTI2019

Using Correlations to Cs-137 to Reduce Uncertainty in SRS Tank Farm Tc-99 and I-129 Inventories - 19266

Performance Assessment (PA) modeling of the Saltstone Disposal Facility (SDF) shows that iodine-129 (I-129) dominates peaks of potential future doses, followed by contributions from technetium-99 (Tc-99). While these radionuclides are important from a PA perspective, they are relatively unimportant from a safety analysis or occupational exposure perspective. As such, the storage of Tc-99 and I-129 within liquid waste at Savannah River Site (SRS) have not been well tracked, resulting in considerable uncertainty in the estimated inventories of Tc-99 and I-129 used for PA modeling. Alternatively, cesium-137 (Cs-137) is considered a high-risk radionuclide from an occupational exposure perspective and is well characterized. Within the liquid waste at SRS, analyses have shown that concentrations of Cs-137 are closely correlated to both Tc-99 and I-129. These correlations and the abundance of Cs-137 data were leveraged to significantly reduce inventory uncertainty for waste destined to be disposed at the SDF. Previous attempts to mathematically define these correlations had two flaws: (1) the defined correlations failed to address the impact of the relatively short half-life of Cs-137 compared to the long half-lives of Tc-99 and I-129, and (2) the analyses relied on a small number of samples. To address the issue of the decay rate from the short half-life, all Cs-137 concentrations were decayed to a single future date. To improve the number of samples used to develop the correlations, a literature review was performed resulting in a larger data set. The data underwent a validation process, then the correlations were updated. The resulting correlations were used to improve inventory estimates for Tc-99 and I-129 for an ongoing revision to the SDF PA. (author)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2019

Nuclear properties for astrophysical and radioactive-ion-beam applications (II)

We tabulate the ground-state odd-proton and odd-neutron spins and parities, proton and neutron pairing gaps, one- and two-neutron separation energies, quantities related to β-delayed one- and two-neutron emission probabilities, average energy and average number of emitted neutrons, β-decay energy release and half-life with respect to Gamow–Teller decay with a phenomenological treatment of first-forbidden decays, one- and two-proton separation energies, and α-decay energy release and half-life for 9318 nuclei ranging from {sup 16}O to {sup 339}136 and extending from the proton drip line to the neutron drip line. This paper is a new and improved version of Atomic Data And Nuclear Data Tables [66 131 (1997)]. The starting point of our present work is the new study (FRDM(2012)) of nuclear ground-state masses and deformations based on the finite-range droplet model and folded-Yukawa single-particle potential published in a previous issue of Atomic Data And Nuclear Data Tables [109–110, 1 (2016)]. The β-delayed neutron-emission probabilities and Gamow–Teller β-decay rates are obtained from a quasi-particle random-phase approximation with single-particle levels and wave functions at the calculated nuclear ground-state shapes as input quantities. A development since 1997 is we now use a Hauser–Feshbach approach to account for (n, γ) competition and treat first-forbidden decay in a phenomenological approach.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Kilonovae Across the Nuclear Physics Landscape: The Impact of Nuclear Physics Uncertainties on r-process-powered Emission

Merging neutron stars produce “kilonovae”—electromagnetic transients powered by the decay of unstable nuclei synthesized via rapid neutron capture (the r-process) in material that is gravitationally unbound during inspiral and coalescence. Kilonova emission, if accurately interpreted, can be used to characterize the masses and compositions of merger-driven outflows, helping to resolve a long-standing debate about the origins of r-process material in the Universe. We explore how the uncertain properties of nuclei involved in the r-process complicate the inference of outflow properties from kilonova observations. Using r-process simulations, we show how nuclear physics uncertainties impact predictions of radioactive heating and element synthesis. For a set of models that span a large range in both predicted heating and final abundances, we carry out detailed numerical calculations of decay product thermalization and radiation transport in a kilonova ejecta with a fixed mass and density profile. The light curves associated with our models exhibit great diversity in their luminosities, with peak brightness varying by more than an order of magnitude. We also find variability in the shape of the kilonova light curves and their color, which in some cases runs counter to the expectation that increasing levels of lanthanide and/or actinide enrichment will be correlated with longer, dimmer, redder emission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Updates to the Hanford Soil Inventory Model (SIM Version 2) for FY 2025

Update SIM to newest version (SIMv2.3). SIM is being updated to reflect the updates to the tank leak inventories performed in ECF-HANFORD-24-0061. This update is also being done to publish the site inventories in both 2001 decayed and back-decayed formats. This is particularly needed for modeling that requires inventory data from before 2001 that includes decay information for radionuclides.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2015

The future of RADCALC- the radioactive material and waste transportation software program - 15154

This paper provides a thorough review of RADCALC, the U.S. Department of Energy (DOE)-developed software tool to assist DOE sites in making radioactive material and waste packaging and transportation determinations in compliance with applicable Federal regulations and DOE Orders and Standards. There are more than 400 registered users of the RADCALC tool across the DOE complex. DOE has also authorized a limited number of users from certain universities and foreign countries. DOE periodically upgrades the software consistent with changing domestic and international requirements, as well as needs unique to DOE. Due to recent changes in regulatory requirements by the Department of Transportation (DOT), it is necessary that the current version of RADCALC should be updated in a timely manner. Prior to investing funds in software upgrades, DOE decided to evaluate the nature of changes required and level of operational support and looked for alternatives for meeting sites' operational needs. DOE formed a joint review team consisting of experts from Energy Facility Contractors Group (EFCOG) sites, commercial waste treatment facilities and the National Laboratories. This team evaluated the RADCALC software, commercially available software packages, and internal DOE site-developed programs against an established set of criteria. The team also reviewed and prioritized regulatory changes and user-recommended enhancements. Based on extensive review, the team recommended that DOE continue to support RADCALC noting that RADCALC is a cost-effective, technically robust tool that can perform complicated radioactive material shipping determinations. The tool promotes accuracy, consistency, and completeness between shipments by a single shipper, between shippers at a given site, and between sites. The isotopic coverage, decay algorithm and the range of calculations are without compare either within DOE or in industry in a tool of this kind. The team also recommended that DOE should actively promote RADCALC use throughout the DOE complex and consider cooperative arrangements with the Department of Defense or other government entities that may have similar needs. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS1979

Post-development image intensification by autoradiography

A method of post-development intensification of photographic images using a newly developed autoradiographic procedure is described. Radioactive Thiourea-S35 is combined with silver in the developed emulsion, which is then contact printed with a receiver emulsion. The beta decay from S35 produces an enhanced autoradiographic image. The laboratory technique is described and results of astronomical applications are presented.

Askins, B. S.↗
DOE OSTI2020

Beta-delayed charged-particle spectroscopy using TexAT

β-delayed charged-particle emission is a sensitive probe of three-body decays in light nuclei. Time Projection Chambers (TPCs) offer a significant advantage over traditional charged-particle spectroscopy techniques due to a low-energy threshold and a high-geometric efficiency (≈ 4π) which are essential for use with radioactive ion beams where the beam intensities are limited. The technique for high-sensitivity spectroscopy of β-delayed charged-particle emission is shown to be possible using the Texas Active Target (TexAT) TPC in conjunction with the General Electronics for TPCs (GET) system. The benchmark case studied was that of 12 N β-decay to the first α-unbound state in 12 C, the Hoyle state. Here, half-life and branching ratio measurements are presented and are in good agreement with previous studies. The efficacy of using TPCs to study such a near-threshold state and disentangle the three-body dynamics of the decay products is demonstrated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Personnel Qualification and Certification Program in Pressure Decay Leak Testing on the RT-100 Type (B) Cask - 17229

The requirements for qualifications and certification of leak test personnel on Type (B) shipping casks have been more clearly defined with the recent release of ANSI N14.5-2014, Leak Tests on Radioactive Packages for Shipment. The latest version creates a standardized approach for qualifying and certifying personnel to conduct pre-shipment leakage tests on Type (B) packages. The U.S Nuclear Regulatory Commission (NRC) is currently updating the Regulatory Guide R.G 7.4, Leakage Tests on Packages for shipment of Radioactive Material, to endorse ANSI N14.5-2014. According to ANSI N14.5-2014, leakage testing shall be performed in accordance with written procedures by qualified and certified personnel in accordance with the requirements of ASNT SNT-TC-1A-2006, Recommended Practice for Personnel Qualification and Certification in Nondestructive Testing. This is a significant modification to the old standard, ANSI N14.5-1997, which simply states that pressure leak testing shall be conducted by trained and certified personnel without reference to any specific certification standards or regulations. SNT-TC-1A published by the American Society for Nondestructive Testing (ASNT) has several advantages to employers; namely, it allows for a Limited NDT Level II certification program. Limited certifications are especially valuable for personnel who possess limited experience and wish to become a certified Limited NDT Level II in a specific technique on a specific cask using a specific procedure and equipment. Robatel Technologies recently developed a comprehensive qualification and training program based on the recommendations of SNT-TC-1A for Exelon Corporation to certify their employees to a Limited NDT Level II in Pressure Decay Leak Testing on the RT-100 Cask. The project scope included the development of a training and qualification program (Written practice), writing a pressure decay leak test procedure, the design of a pressure decay leak test manifold, and the delivery of classroom training. The written practice outlines the requirements to ensure that personnel participating in the program have the necessary qualification, experience, and training to become certified in the leak test method. The program will give Exelon the liberty to conduct their own leak testing on the RT- 100 without the need to rely on outside resources for leak testing. When fully implemented, the program is expected to improve productivity and eliminate schedule delays, along with substantial economic benefits. Following the appropriate standards and industry best practices, the project was successfully completed and scheduled to be fully implemented by Exelon's Nuclear Stations by the end of 2016. (authors)

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2025

Binding energies, charge radii, spins, and moments: Odd-odd Ag isotopes and discovery of a new isomer

We report on the masses and hyperfine structure of ground and isomeric states in 114,116,118,120 Ag isotopes, measured with the phase-imaging ion-cyclotron-resonance technique (PI-ICR) with the JYFLTRAP mass spectrometer and the collinear laser spectroscopy beamline at the Ion Guide Isotope Separator On-Line facility, Jyväskylä, Finland. We measured the masses and excitation energies, electromagnetic moments, and charge radii, and firmly established the nuclear spins of the long-lived states. A new isomer was discovered in 118 Ag and the half-lives of 118 Ag long-lived states were reevaluated. We unambiguously pinned down the level ordering of all long-lived states, placing the inversion of the 𝐼 = 0 − and 𝐼 = 4 + states at 𝐴 = 118 (𝑁 = 71). As a result, we compared the electromagnetic moments of each state to empirical single-particle moments to identify the dominant configuration where possible.

90 ≤ A ≤ 149↗
DOE OSTI2013

Measurement of cross sections for the {sup 232}Th(P,4n){sup 229}Pa reaction at low proton energies

The alpha-emitters {sup 225}Ac and {sup 213}Bi are of great interest for alpha-radioimmunotherapy which uses radioisotopes attached to cancer-seeking antibodies to efficiently treat various types of cancers. Both radioisotopes are daughters of the long-lived {sup 229}Th(t{sub 1/2} = 7880y). {sup 229}Th can be produced by proton irradiation of {sup 232}Th and {sup 230}Th, either directly or through production of isobars that beta-decay into {sup 229}Th. To obtain excitation functions, {sup 232}Th and {sup 230}Th have been irradiated at the On-Line Test Facility at the Holifield Radioactive Ion Beam Facility at ORNL. Benchmark tests conducted with Cu and Ni foils show very good agreement with literature results. The experiments with thorium targets were focused on the production of {sup 229}Pa and its daughter {sup 225}Ac from both {sup 232}Th and {sup 230}Th. Differential cross-sections for production of {sup 229}Pa and other Pa isotopes have been obtained.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Simulation of charge readout with segmented tiles in nEXO

nEXO is a proposed experiment to search for the neutrino-less double beta decay (0νββ) of 136 Xe in a tonne-scale liquid xenon time projection chamber (TPC). The nEXO TPC will be equipped with charge collection tiles to form the anode. In this work, the charge reconstruction performance of this anode design is studied with a dedicated simulation package. A multi-variate method and a deep neural network are developed to distinguish simulated 0νββ signals from backgrounds arising from trace levels of natural radioactivity in the detector materials. These simulations indicate that the nEXO TPC with charge-collection tiles shows promising capability to discriminate the 0νββ signal from backgrounds. Furthermore, the estimated half-life sensitivity for 0νββ decay is improved by 20 32)% with the multi-variate (deep neural network) methods considered here, e sensitivity estimated in the nEXO pre-conceptual design report.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Proton branching ratios of 23 Mg levels

Background: The anomalous 22 Ne abundance measured in certain presolar graphite grains is thought to arise from the decay of 22 Na that was synthesized at high temperatures in core-collapse supernovae. To better interpret this abundance anomaly, the primary destruction mechanism of 22 Na, the 22 Na(p,γ) 23 Mg reaction, must be better understood. Purpose: Determine proton branching ratios of several 23 Mg excited states that play a role in the high-temperature 22 Na(p,γ) 23 Mg reaction rate. Methods: Particle decays of 23 Mg excited states populated with the previously reported 24 Mg(p,d) 23 Mg transfer reaction measurement [Kwag et al., Eur. Phys. J. A 56, 108 (2020)] were analyzed to extract proton branching ratios. The reaction was studied using a 31-MeV proton beam from the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory and 24 Mg solid targets. Results: Proton branching ratios of several 23 Mg excited states in the energy range of Ex = 8.044 - 9.642 MeV were experimentally determined for the first time for the p0 and p1'(p1+p2+p3) decay channels. Conclusions: These new branching ratios for 23 Mg levels can provide an experimental foundation for an improved high-temperature rate of the 22 Na(p,γ) 23 Mg reaction needed to understand production of anomalously high 22 Ne abundance in core-collapse supernovae.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Identification of new transitions and levels in 163 Gd from $β$-decay studies

Background: Neutron-rich nuclei in the mass region around A = 160 have been and will continue to be of interest for the study of nuclear structure because of the rapid onset of deformation between 88 and 90 neutrons. The observation of detailed changes in nuclear structures within this mass region has provided and will continue to provide insight into the nuclear force. Purpose: Investigations of γ rays emitted following Eu 163 β -decay to Gd 163 have been performed for evaluation of the nuclear structure of Gd 163 . Method: Data were collected at the LeRIBSS station of the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory with an array of four Clover HPGe detectors for γ -rays and two plastic scintillators for β detection. The γ rays were identified as belonging to Gd 163 via mass selection and γ – γ – β , x-ray- γ , or γ – γ coincidences. Results: In total 107 new γ -ray transitions were observed in Gd 163 from 53 newly identified levels. Conclusions: We report the structure of Gd 163 has been identified for the first time. This structure has been evaluated in comparison to projected shell model, and potential energy surface calculations with good agreement.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Abatement of Xenon and Iodine Emissions from Medical Isotope Production Facilities

The capability of the International Monitoring System (IMS) to detect xenon from underground nuclear explosions is dependent on the radioactive xenon background. Adding to the background, medical isotope production (MIP) by fission releases several important xenon isotopes including xenon-133 and iodine-133 that decays to xenon-133. The amount of xenon released from these facilities may be equivalent to or exceed that released from an underground nuclear explosion. Thus the release of gaseous fission products within days of irradiation makes it difficult to distinguish MIP emissions from a nuclear explosion. In addition, recent shortages in molybdenum-99 have created interest and investment opportunities to design and build new MIP facilities in the United States and throughout the world. Due to the potential increase in the number of MIP facilities, a discussion of abatement technologies provides insight into how the problem of emission control from MIP facilities can be tackled. A review of practices is provided to delineate methods useful for abatement of medical isotopes.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2015

Instrument for precision long-term β-decay rate measurements

We describe an experimental setup for making precision measurements of relative β-decay rates of {sup 22}Na, {sup 36}Cl, {sup 54}Mn, {sup 60}Co, {sup 90}Sr, {sup 133}Ba, {sup 137}Cs, {sup 152}Eu, and {sup 154}Eu. The radioactive samples are mounted in two automated sample changers that sequentially position the samples with high spatial precision in front of sets of detectors. The set of detectors for one sample changer consists of four Geiger-Müller (GM) tubes and the other set of detectors consists of two NaI scintillators. The statistical uncertainty in the count rate is few times 0.01% per day for the GM detectors and about 0.01% per hour on the NaI detectors. The sample changers, detectors, and associated electronics are housed in a sealed chamber held at constant absolute pressure, humidity, and temperature to isolate the experiment from environmental variations. The apparatus is designed to accumulate statistics over many years in a regulated environment to test recent claims of small annual variations in the decay rates. We demonstrate that absent this environmental regulation, uncontrolled natural atmospheric pressure variations at our location would imprint an annual signal of 0.1% on the Geiger-Müller count rate. However, neither natural pressure variations nor plausible indoor room temperature variations cause a discernible influence on our NaI scintillator detector count rate.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2014

Laboratory studies on the removal of radon-born lead from KamLAND's organic liquid scintillator

We studied the removal of radioactivity from liquid scintillator in preparation of a low background phase of KamLAND. We describe the methods and techniques developed to measure and efficiently extract radon decay products from liquid scintillator. Lastly, we report the radio-isotope reduction factors obtained when applying various extraction methods. During this study, distillation was identified as the most efficient method for removing radon daughters from liquid scintillator.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗