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DOE OSTI2023

Mid-infrared spectroscopy with a broadly tunable thin-film lithium niobate optical parametric oscillator

Mid-infrared spectroscopy, an important technique for sensing molecules, has encountered barriers from sources either limited in tuning range or excessively bulky for widespread use. We present a compact, efficient, and broadly tunable optical parametric oscillator surmounting these challenges. Leveraging dispersion-engineered thin-film lithium niobate-on-sapphire photonics and a singly resonant cavity allows broad, controlled tuning over an octave from 1.5–3.3 µm. The device generates >25mW of mid-infrared light at 3.2 µm with 15% conversion efficiency. The ability to precisely control the device’s mid-infrared emission enables spectroscopy of methane and ammonia, demonstrating our approach’s relevance for sensing. Our work signifies an important advance in nonlinear photonics miniaturization, bringing practical field applications of high-speed, broadband mid-infrared spectroscopy closer to reality.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2024

Subphotospheric Emission from Short Gamma-Ray Bursts: Protons Mold the Multimessenger Signals

Abstract The origin of the observed Band-like photon spectrum in short gamma-ray bursts (sGRBs) is a long-standing mystery. We carry out the first general relativistic magnetohydrodynamic simulation of an sGRB jet with initial magnetizationσ 0 = 150 in dynamical ejecta from a binary merger. From this simulation, we identify regions along the jet of efficient energy dissipation due to magnetic reconnection and collisionless subshocks. Taking into account electron and proton acceleration processes, we solve for the first time the coupled transport equations for photons, electrons, protons, neutrinos, and intermediate particle species up to close to the photosphere (i.e., up to 1 × 10 12 cm), accounting for all relevant radiative and cooling processes. We find that the subphotospheric multimessenger signals carry strong signatures of the hadronic interactions and their resulting particle cascades. Importantly, the spectral energy distribution of photons is significantly distorted with respect to the Wien one, commonly assumed below the photosphere. Our findings suggest that the bulk of the nonthermal photon spectrum observed in sGRBs can stem from hadronic processes occurring below the photosphere and previously neglected, with an accompanying energy flux of neutrinos peaking in the GeV energy range.

Astronomy & Astrophysics↗

NASA NTRS2002

Pulsar Polar Cap Heating and Surface Thermal X-ray Emission: Inverse Compton Radiation Pair Fronts - 2

We investigate the production of electron-positron pairs by inverse Compton scattered (ICS) photons above a pulsar polar cap (PC) and calculate surface heating by returning positrons. This paper is a continuation of our self-consistent treatment of acceleration, pair dynamics, and electric field screening above pulsar PCs. We calculate the altitude of the inverse Compton pair-formation fronts, the flux of returning positrons, and present the heating efficiencies and X-ray luminosities. We revise pulsar death lines implying cessation of pair formation, and present them in surface magnetic field-period space. We find that virtually all known radio pulsars are capable of producing pairs by resonant and nonresonant ICS photons radiated by particles accelerated above the PC in a pure star-centered dipole field, so that our ICS pair death line coincides with empirical radio pulsar death. Our calculations show that ICS pairs are able to screen the accelerating electric field only for high PC surface temperatures and magnetic fields. We argue that such screening at ICS pair fronts occurs locally, slowing but not turning off acceleration of particles until screening can occur at a curvature radiation (CR) pair front at higher altitude. In the case where no screening occurs above the PC surface, we anticipate that the pulsar gamma-ray luminosity will be a substantial fraction of its spin-down luminosity. The X-ray luminosity resulting from PC heating by ICS pair fronts is significantly lower than the PC heating luminosity from CR pair fronts, which dominates for most pulsars. PC heating from ICS pair fronts is highest in millisecond pulsars, which cannot produce CR pairs, and may account for observed thermal X-ray components in the spectra of these old pulsars.

Harding, Alice K.↗

NASA NTRS1994

Multiwavelength tests of the dusty torus model for Seyfert galaxies

We present a compilation of emission properties for a sample of 116 Seyfert galaxies based on both previously unpublished data and measurements available in the literature. These measurements include fluxes in the emission lines (O III) lambda(5007) and H-beta, as well as the infrared (25-60 microns), ultraviolet (1450 A), soft (0.2-4 keV), and hard (2-10 keV) X-ray continua. These are used to try to distinguish between isotropic and anisotropic emission properties of Seyfert galaxies. The distribution functions of (O III) lambda 5007 infrared, and hard X-ray continuum are similar for Seyfert 1's and Seyfert 2's, consistent with these properties being isotropic. The ultraviolet and soft X-ray continua of Seyfert 2's are underluminous relative to the type 1's suggesting photons at these energies escape from the central source anisotropically. There is a correlation between the ultraviolet continuum and emission-line fluxes in Seyfert 1's consistent with the idea that the central engine is responsible for powering the line emission. No such correlation is found for the Seyfert 2's. Instead, the scatter in the plot of ultraviolet continuum versus line emission suggests the true nuclear continuum luminosity is not seen at Earth in these objects. These properties are consistent with those expected in the dusty torus model.

Mulchaey, John S.↗

DOE OSTI2024

Spectroscopic search for optical emission lines from dark matter decay

We search for narrow-line optical emission from dark matter decay by stacking dark-sky spectra from the Dark Energy Spectroscopic Instrument (DESI) at the redshift of nearby galaxies from DESI’s Bright Galaxy and Luminous Red Galaxy samples. Our search uses regions separated by 5 to 20 arcsec from the centers of the galaxies, corresponding to an impact parameter of approximately 50 kpc. No unidentified spectral line shows up in the search, and we place a line flux limit of 10 −19 ergs/s/cm 2 /arcsec 2 on emissions in the wavelength range of 2000–9000⁢ Å. This places the tightest constraints yet on the two-photon decay of dark matter in the mass range of 5 to 12 eV, with a particle lifetime exceeding 3 × 10 25 s. Furthermore, this detection limit also implies that the line surface brightness contributed from all dark matter along the line of sight is at least 2 orders of magnitude lower than the measured extragalactic background light (EBL), ruling out the possibility that narrow optical-line emission from dark matter decay is a major source of the EBL.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS2011

Suzaku Detection of Diffuse Hard X-Ray Emission Outside Vela X

Vela X is a large, 3 deg x 2 deg, radio-emitting pulsar wind nebula (PWN) powered by the Vela pulsar in the Vela supernova remnant. Using four Suzaku/XIS observations pointed just outside Vela X, we find hard X-ray emission extending throughout the fields of view. The hard X-ray spectra are well represented by a power-law. The photon index is measured to be constant at Gamma approximates 2.4, similar to that of the southern outer part of Vela X. The power-law flux decreases with increasing distance from the pulsar. These properties lead us to propose that the hard X-ray emission is associated with the Vela PWN. The larger X-ray extension found in this work strongly suggests that distinct populations relativistic electrons form the X-ray PWN and Vela X, as was recently inferred from multiwavelength spectral modeling of Vela X.

Katsuda, Satoru↗

NASA NTRS2019

The Orbital Variation of Non-Thermal X-Ray Emission from eta Carinae

The collision of strong stellar winds in massive binary systems creates powerful shocks,which accelerates a small amount of particles to relativistic energies at the shock interface.This process is important in fundamental astrophysics in two ways;i) some particles may contribute to cosmic-rays observed around the Earth, whose origin is not well known, andii) it provides a good laboratory for particle acceleration physics as the shock occurs steadily in a predictable environment.Some relativistic particles collide with stellar photons or ambient material near the binary systemand emit non-thermal X-rays and gamma-rays, which are good probes of particle acceleration.This emission had been searched for decades but not found convincingly without sensitive high-energy telescopes.The NuSTAR telescope observed the enigmatic supermassive binary system eta Carinae multiple times after 2014 and found conclusive evidence of non-thermal emission from the star in the extremely hard X-ray band.This emission is prominent between 20-50 keV, below which thermal emission from shock colliding plasma dominates.It is relatively stable throughout the binary orbit, but it disappears near periastron when the wind colliding activity shuts off.This variation indicates that the non-thermal X-ray emission originates from the head-on wind-wind collision.The flat spectrum is consistent with inverse-Compton of stellar UV photons by accelerated electrons.The spectrum smoothly connects to a gamma-ray spectrum of a Fermi source detected around eta Carinae,suggesting that acceleration occurs up to the GeV energy.This result provide the strongest evidence so far that particle acceleration occurs at the wind colliding shock of a massive colliding wind binary system.

Hamaguchi, Kenji↗

DOE OSTI2022

Core–Shell Covalently Linked Graphitic Carbon Nitride–Melamine–Resorcinol–Formaldehyde Microsphere Polymers for Efficient Photocatalytic CO 2 Reduction to Methanol

Photocatalytic reduction of CO 2 with light and H 2 O to form CH 3 OH is a promising route to mitigate carbon emissions and climate changes. Although semiconducting metal oxides are potential photocatalysts for this reaction, low photon efficiency and leaching of environmental unfriendly, toxic metals limit their applicability. Here, we report a metal-free, core-shell photocatalysts consisting of graphitic carbon nitride (g-C 3 N 4 , CN) covalently linked to melamine-resorcinol-formaldehyde (MRF) microsphere polymers for this reaction. Cova-lent linkage enabled efficient separation of photo-generated carriers and photocatalysis. Using 100 mg of a photocatalyst containing 15 wt.% CN, a CH 3 OH yield of 0.99 μmol·h -1 was achieved at a reaction temperature of 80 °C and 0.5 MPa with external quantum efficiencies ranging from 5.5% at 380 nm to 1.7% at 550 nm. The yield was about 20 and 10 times higher than that of its components CN and MRF, respectively. Characterization with XPS, TEM, and bulk and surface elemental analyses supported a core-shell structure and charge transfer at C-N bond at the CN-MRF interface between the methoxy group in the 2,4-trishydroxylmethyl-1,3-diphenol part of MRF and the terminal amino groups in the CN. This enhanced ligand-to-ligand charge transfer resulted in 67% of photo-excited internal charge transferred from CN to hy-droxymethylamino group in MRF, whose amino group was the catalytic site for CO 2 photocatalytic reduction to CH 3 OH. Furthermore, this study provides a series of new metal-free photocatalyst designs and insights into the molecular-level structure-mediated photocatalytic response

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Mid-IR UAV-based sensing platform with deep learning to Identify and Quantify Gaseous Emission in Gas Flares

This report details the development and evaluation of a Mid-Infrared (Mid-IR) Unmanned Aerial Vehicle (UAV)-based sensing platform integrated with deep learning algorithms for the identification and quantification of gaseous emissions in gas flares. The project, spearheaded by Omega Optics, Inc., aimed to address environmental monitoring challenges by leveraging advanced photonic technologies and autonomous UAV operations. The research focused on designing, optimizing, and fabricating photonic crystal waveguides and grating couplers to enhance the sensitivity and accuracy of gas detection. A comprehensive drone-based system was developed, featuring a miniaturized sensor, GPS module, and microcontroller communication network for real-time gas concentration monitoring. The system's adaptive sampling algorithm, implemented using the Robot Operating System (ROS), enables autonomous detection and localization of gas emission sources. Preliminary results demonstrate the platform's capability to detect and monitor gas emissions with high precision, cost-effectiveness, and scalability. Future work will expand upon this foundation by introducing 3D wind model-based learning for dynamic environmental conditions and further enhancing the user interface and data processing algorithms to support broader environmental monitoring applications. Overall, this project represents a significant step forward in UAV-based environmental sensing technologies, offering robust solutions for detecting and mitigating the impacts of gaseous emissions on public health and safety.

47 OTHER INSTRUMENTATION↗

NASA NTRS1984

Hydrogen on Venus - Exospheric distribution and escape

The spatial distribution of suprathermal H in the Venus atmosphere is calculated using an approximate numerical solution of the time-independent Boltzmann equation. Sources of suprathermal H are specified on the basis of Pioneer Venus measurements. Reactions involving H2 are neglected. The computed densities of suprathermal H are in satisfactory agreement with profiles derived from analysis of Lyman-alpha airglow by Mariners 5 and 10 and Veneras 11 and 12. The dayside emission at radial distances larger than 18,000 km is attributed to scattering of solar photons by fast H atoms produced primarily on the nightside near midnight. The nightside ionosphere, and consequently the source of suprathermal H, are both expected to vary in response to changes in the solar wind.

Rodriguez, J. M.↗

NASA NTRS1986

The central engine of quasars and active galactic nuclei Hadronic interactions of shock-accelerated relativistic protons

The detailed dynamics are presented of a model for AGNs and QSOs based on spherically symmetric accretion onto a black hole and dissipation of the accretion energy in a collisionless shock. The basic assumptions and equations relevant for the model are presented, and the relations between the physical parameters are given in terms of the shock parameters. The latter are calculated for varying Mach numbers, and the resulting scaling laws are discussed and compared to the data, in particular the recently discovered correlations between luminosity and mass. The model can naturally produce ultrarelativistic electrons with flat spectra, a feature which, when coupled with e(+)-e(-) pair production, can account for the observed continuum radiation from these objects over essentially the whole electromagnetic spectrum. The model also predicts the emission of high-energy neutrinos with a luminosity roughly equal to that of the photons.

Kazanas, D.↗

NASA NTRS1987

Prospects for gamma-ray line observations of individual supernovae

The gamma-ray line emission from individual type I and type II supernovae are studied using numerical simulations and photon propagation codes to predict the flux levels and line shapes. For both types, the gamma ray lines with the highest flux from an individual event are the 0.847 and 1.238 MeV lines from the Ni-56 to Co-56 to Fe-56 decay chain. For type I supernovae, the 0.847 MeV line peaks at about 70 days after event onset. The historical record indicates an approximate discovery rate of once in 10 years for balloon-borne instruments, once in two to three years for the Gamma-Ray Observatory, and once in one to two years for a proposed space mission. The 0.847 MeV line flux from type II supernovae peaks at about 600 days after event onset at a low level which restricts observations to the events in the Galaxy and its nearest neighbors. The expected line shape is narrower than for type I supernovae.

Gehrels, Neil↗

NASA NTRS2012

The Galactic Centre Mini-Spiral in the MM-Regime

Context: The mini-spiral is a feature of the interstellar medium in the central approx.2 pc of the Galactic center. It is composed of several streamers of dust and ionised and atomic gas with temperatures between a few 100 K to 10(exp 4) K. There is evidence that these streamers are related to the so-called circumnuclear disk of molecular gas and are ionized by photons from massive, hot stars in the central parsec. Aims: We attempt to constrain the emission mechanisms and physical properties of the ionized gas and dust of the mini-spiral region with the help of our multiwavelength data sets. Methods: Our observations were carried out at 1.3 mm and 3 mm with the mm interferometric array CARMA in California in March and April 2009, with the MIR instrument VISIR at ESO's VLT in June 2006, and the NIR Bry with VLT NACO in August 2009. Results: We present high resolution maps of the mini-spiral, and obtain a spectral index of 0.5 +/- 0.25 for Sgr A *, indicating an inverted synchrotron spectrum. We find electron densities within the range 0.8-1.5 x 10(exp 4)/cu cm for the mini-spiral from the radio continuum maps, along with a dust mass contribution of approx. 0.25 Mo from the MIR dust continuum. and extinctions ranging from 1.8-3 at 2.16 microns in the Bry line. Conclusions: We observe a mixture of negative and positive spectral indices in our 1.3 mm and 3 mm observations of the extended emission of the mini-spiral, which we interpret as evidence that there are a range of contributions to the thermal free-free emission by the ionized gas emission and by dust at 1.3 mm.

Kunneriath, D.↗

NASA NTRS2018

NICER Observes the Effects of an X-Ray Burst on the Accretion Environment in Aql X-1

Accretion disks around neutron stars regularly undergo sudden strong irradiation by Type I X-raybursts powered by unstable thermonuclear burning on the stellar surface. We investigate the impacton the disk during one of the first X-ray burst observations with the Neutron Star Interior CompositionExplorer (NICER) on the International Space Station. The burst is seen from Aql X-1 during the hardspectral state. In addition to thermal emission from the neutron star, the burst spectrum exhibits anexcess of soft X-ray photons below 1 keV, where NICER's sensitivity peaks. We interpret the excessas a combination of reprocessing by the strongly photoionized disk and enhancement of the pre-burstpersistent flux, possibly due to Poynting Robertson drag or coronal reprocessing. This is the firstsuch detection for a short sub-Eddington burst. As these bursts are observed frequently, NICER willbe able to study how X-ray bursts affect the disk and corona for a range of accreting neutron starsystems and disk states.

Keek, L.↗

DOE OSTI2026

X-ray Response of the Fully-Depleted, p-Channel SiSeRO-CCD

We present an X-ray characterization of a fully depleted, 725 $μ$m thick p-channel SiSeRO CCD. Measurements with a $^{55}$Fe source yield an energy resolution of $54 \pm 0.9$ eV ($14.6 \pm 0.25 e^{-}$) at 5.9 keV for single-pixel events, demonstrating that the SiSeRO amplifier preserves the intrinsic charge resolution of the CCD under multi-sample non-destructive readout. Characterization with a $^{241}$Am source extends the response to higher-energy photons, with reconstructed spectral features observed between 9-26 keV and the 59.5 keV $γ$ emission. These measurements, together with a muon-derived diffusion calibration, show that charge transport and diffusion are consistent with interactions spanning the full sensor depth. These results demonstrate that the SiSeRO CCD simultaneously achieves sub-electron noise performance and efficient charge collection in a thick, fully depleted silicon detector. This combination enables X-ray spectroscopy across a broad energy range while maintaining sensitivity to faint signals.

Cuevas-Zepeda, Julian↗

NASA NTRS1986

Measuring interstellar dust grains from the haloes of binary X-ray sources

A method for determining the location, size distribution, and composition of interstellar dust grains from the haloes of binary X-ray sources is described. The method is based on the time dependence of the halo X-ray emission during an eclipse of the point source. The distance of the dust cloud is inferred directly from observations of the growth of the dark circle around the eclipsed point source. Grain size distribution in the interstellar dust clouds is derived from the halo brightness profile at a given photon energy. The composition of the grains is obtained by observing the spectral features in the total optical depth due to X-ray scattering near the photoionization thresholds of the elements in the grains. The haloes become dim just below the ionization threshold, and sharply increase in function brightness as the photon energy increases beyond the absorption edge of the relevant atom. The method makes it possible to observe and analyze the halo emission during eclipse even without imaging the source. It is suggested that haloes probably account for the soft X-rays observed during eclipses and dips observed in sources including 4U1915-05 and X1755-338.

Xu, Y.↗

NASA NTRS2019

Observation of inverse Compton emission from a long γ-ray burst

Long-duration γ-ray bursts (GRBs) originate from ultra-relativistic jets launched from the collapsing cores of dying massive stars. They are characterized by an initial phase of bright and highly variable radiation in the kiloelectronvolt-to-megaelectronvolt band, which is probably produced within the jet and lasts from milliseconds to minutes, known as the prompt emission. Subsequently, the interaction of the jet with the surrounding medium generates shock waves that are responsible for the afterglow emission, which lasts from days to months and occurs over a broad energy range from the radio to the gigaelectronvolt bands. The afterglow emission is generally well explained as synchrotron radiation emitted by electrons accelerated by the external shock. Recently, intense long-lasting emission between 0.2 and 1 teraelectronvolts was observed from GRB 190114C. Here we report multifrequency observations of GRB 190114C, and study the evolution in time of the GRB emission across 17 orders of magnitude in energy, from 5 × 10^(−6) to 10^(12) electronvolts. We find that the broadband spectral energy distribution is double-peaked, with the teraelectronvolt emission constituting a distinct spectral component with power comparable to the synchrotron component. This component is associated with the afterglow and is satisfactorily explained by inverse Compton up-scattering of synchrotron photons by high-energy electrons. We find that the conditions required to account for the observed teraelectronvolt component are typical for GRBs, supporting the possibility that inverse Compton emission is commonly produced in GRBs.

P. Veres↗

NASA NTRS1972

Mariner 6 and 7 ultraviolet spectrometer experiment - Implications of CO2/+/, CO, and O airglow.

The Mariner 6 and 7 UV spectrometer experiments observed intense emissions from CO, O, and CO2(+) in the Martian airglow. Analysis shows that they are excited predominantly by the absorption of solar EUV photons by CO2 and constitute a major energy-loss mechanism for the thermosphere. Models of the thermospheric temperature profile and the airglow layer that demonstrate the effects of neutral chemistry and ionospheric composition are developed. With their aid, the observed CO Cameron-band emission scale height of 19 (plus or minus 4.5) km is shown to suggest an exospheric temperature of 315 (plus or minus 75) K. Consideration of other data suggests a 'best' value of about 350 K. Within the uncertainties in the excitation efficiencies and in the thermospheric cooling mechanisms, the observations are consistent with the measured electron density. There is no indication in the data that the ionosphere is modified by the solar wind below 200 km.

Stewart, A. I.↗