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At least 937 records · Page 52

AST Development in M2FCT (ASTWG and iDWG) Update to 21CTP [Slides]

Accelerated Stress Tests (ASTs) are required to evaluate fuel cell component durability in a reasonable time. Current DOE and FCTT ASTs are light duty focused with 5000 – 8000 hour durability requirements. Heavy duty ASTs need to reflect the 25000+ hour durability requirement. Interim solution is to extend the duration of the current light duty ASTs: Catalyst AST has been extended from 30,000 cycles to 90,000 cycles (From 50 hours to 150 hours). We need to understand Heavy duty stressors and tailor ASTs for heavy duty applications: Longer lifetimes; Higher efficiencies – Higher loadings - Potentially higher operating temperatures and voltages; Heat rejection during low speed hill climbs – Higher operating temperature; Longer Idling times – Higher operating voltages and drier operation; Take into account different hybridization strategies (Vary size of battery).

30 DIRECT ENERGY CONVERSION↗

The Strange Case of Ground-Coupled Airwaves on Seismoacoustic Stations at Local to Near-Regional Scales

Here we investigate the application of ground-coupled airwaves observed by seismoacoustic stations at local to near-regional scales to detect signals of interest and determine back-azimuth information. Ground-coupled airwaves are created from incident pressure waves traveling through the atmosphere that couple to the earth and transmit as a seismic wave with retrograde elliptical motion. Previous studies at sub-local scales (<10 km from a source of interest) found the back-azimuth to the source could be accurately determined from seismoacoustic signals recorded by acoustic and 3-component seismic sensors spatially separated on the order of 10 to 150 m. The potential back-azimuth directions are estimated from the coherent signals between the acoustic and vertical seismic data, via a propagation-induced phase shift of the seismoacoustic signal. A unique solution is then informed by the particle motion of the 3-component seismic station, which was previously found to be less accurate than the seismoacoustic-sensor method. We investigate the applicability of this technique to greater source-receiver distances, from 50-100 km and up to 400 km, which contains pressure waves with tropospheric and stratospheric ray paths, respectively. Specifically, we analyze seismoacoustic sources with ground truth from rocket motor fuel elimination events at the Utah Test and Training Range (UTTR) as well as a 2020 rocket launch in Southern California. From these sources we observe evidence that while coherent signals can be seen from both sources on multiple seismoacoustic station pairs, the determined ground-coupled airwave back-azimuths are more complicated than results at more local scales. Our findings suggest more complex factors including incidence angle, coupling location, subsurface material, and atmospheric propagation effects need to be fully investigated before the ground-coupled airwave back-azimuth determination method can be applied or assessed at these further distances.

58 GEOSCIENCES↗

Advanced Coolant Enclosure Solutions for Micro Gas Cooled Reactors with Enhanced Efficiency and Safety

Argonne’s advanced high-pressure, high-temperature gas enclosures solutions were developed and tested for Light Water Reactor (LWR) fuel applications wherein pressure, temperature, fuel and working fluid are substantially different when compared to the operating conditions typical of gas cooled reactors (GCR). For LWR applications the coolant sleeve pressure exerted on the inner and outer walls of the sleeve may be equalized by pressurizing the fuel rod (e.g., with helium gas) to compensate for the coolant high pressure exerted on the outer walls of the sleeve. This results in a lower differential pressure. Micro-GCRs are reactor systems operated at elevated temperatures and pressure with gas as a working fluid. HolosGen’s Holos-Quad represent a type of Micro-GCR wherein the core is sleeved to segregate the fuel and other components from the working fluid.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Idaho National Laboratory Water Assessment

Established in 1949, Idaho National Laboratory (INL) is part of the U.S. Department of Energy’s (DOE) complex of national laboratories. INL performs work in each of the strategic goal areas of the department: energy, national security, science, and environment, and is the nation’s center for nuclear energy research and development. Located in southeastern Idaho, its physical footprint includes 569,180 acres of federally owned land. A water balance for the fiscal year (FY) 2022 year was conducted for INL to identify major water using equipment and calculate the end-use categories. FY 2022 was selected as the evaluation year per the DOE Sustainability Performance Office. This report provides an analysis of facilities on the INL Site operated by Battelle Energy Alliance, LLC (BEA). This water balance report focused on the Advanced Test Reactor (ATR) Complex, Materials and Fuels Complex, Idaho Falls campus, and Central Facilities Area campuses, which consumed 98% of the 540,611 thousand gallons (kGal) of water used by INL in FY 2022. The resulting water balance identified the use categories for 75.3% of the FY 2022 water consumption.

99 GENERAL AND MISCELLANEOUS↗

Mechanics of the Ring Tension Test (RTT): A Finite Element-based Investigation

The ring tension test (RTT) is an experimental method for determining mechanical behavior in a material’s circumferential or hoop direction. It is a crucial test for testing anisotropic materials with tube geometry, such as nuclear fuel cladding or irradiated pipes. Several RTT configurations exist, each with their own advantages and disadvantages. However, this test is significantly more complex than traditional tensile testing and can be especially sensitive to small differences and inconsistencies in the test setup and geometry, ultimately affecting the derived mechanical properties. Previous research has focused on method development, and little work has been done on understanding the subtle differences between an ideal test and experiments, specifically when the tests are performed on highly irradiated materials in hot cells. In this work, a finite element-based investigation of the RTT is conducted. Two promising test configurations are investigated, comparing their ability to determine accurate material strengths through plastic deformation. Several non-ideal conditions and uncontrollable effects which are likely to occur during experimental testing such as machining tolerances, variations of specimen geometry from nominal dimensions, rotation of specimens and fixturing, and other test setup discrepancies are studied. The sensitivity of measured strengths to these conditions is presented. A mechanics-based approach to describing and correcting raw data to determine actual strengths is also included for one of the configurations, resulting in a robust correction method with highly accurate material strength measurements. Based on these analyses, the hemicylindrical mandrel configuration is recommended with a gauge region oriented at a 45° angle.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Improved Fuel Cycle Capability of Griffin for Fast Reactor Applications

Griffin is a MOOSE based reactor multiphysics analysis application jointly developed by Idaho National Laboratory and Argonne National Laboratory under the Department of Energy Office of Nuclear Energy Nuclear Energy Advanced Modeling and Simulation Program. This fiscal year, the fuel cycle capability has been significantly extended by improving the assembly shuffling option to allow flexible fuel reloading in the multi-cycle depletion calculation and incorporating decay between cycles. An equilibrium core calculation capability was also implemented to find an equilibrium core. Additionally, an enrichment search capability was added to determine the enrichment condition that allows a core to reach an equilibrium cycle with the end-of-cycle k-effective meeting a user-specified target value. The updated fuel management capability has been extensively tested using the three-dimensional ABTR problem with different batch schemes, exhibiting reasonable solutions in terms of manual shuffling, equilibrium cycle, and enrichment search calculations. The cross section generation workflow capability for fast reactors was further verified to produce microscopic cross sections as well as Griffin core inputs for an ring-heterogeneous configuration. Rigorous verification tests using the ABTR problem demonstrated that the RH core calculations, with cross sections and Griffin inputs generated from the cross section workflow of Griffin, produced accurate solution for fast reactor problems. In addition, an option to convert delay neutron parameter data generated from MC 2 -3 in the DLAYXS format into XML format was added to support transient calculations using MC 2 -3-generated data.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE Advanced Gas Reactor Fuel Development and Qualification Program Overview

Slides discussing the DOE Advanced Gas Reactor Fuel Development and Qualification Program Overview to include focus on LEU UCO TRISO fuel in cylindrical compacts, with data for fuel qualification in support of reactor licensing and a path to establish a domestic commercial TRISO fuel fabrication capability. Timelines from 2004 through 2029. Major program highlights include: Developed fuel performance models based on past observed behavior, Study to understand differences between US and German (“good”) fuel, Developed and improved fuel fabrication and characterization methods, Fabricated lab-scale fuel (AGR-1) with very high quality; excellent in-pile and post-irradiation high-temperature fuel performance, Scale-up coating fabrication (AGR-2) with excellent in-pile performance, AGR-3/4 fuel fabrication and irradiation experiment to assess FP transport behavior, Scale-up matrix fabrication (AGR-5/6/7); & fuel performance evaluation in progress.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ATR NEXSHARE Fact Sheet

This fact sheet will provide information for the database of experimental facilities supported by the IAEA as outlined below: NEXSHARE: As part of the Nuclear Harmonization and Standardization Initiative (NHSI), the IAEA proposes to establish a Network for global cooperation and resource sharing for experiments and code validation between experimental facilities, SMRs design organizations, International Organizations and Technical Support Organizations (TSOs). The proposed Network, NEXSHARE, will be done in collaboration with the OECD/NEA. EXPERIMENTAL FACILITY DATABASE: As part of this activity, the IAEA is compiling a database of experimental facilities applicable to SMRs (including water cooled, high temperature gas cooled, molten salt and fast neutron spectrum reactors). This database will also form part of NEXSHARE and will be documented in an IAEA publication.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TREAT Accomplishments FY21

No abstract. These highlight slides will be included on the website https://transient.inl.gov/SitePages/Home.aspx as information of work accomplished.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Determination of Average Burnup in AGR-3/4 Compacts 1-4 and 7-4

The Advanced Gas Reactor (AGR) Fuel Development and Qualification Program third and fourth irradiation experiments (AGR-3/4), originally planned as separate tests, were combined in one test train for irradiation in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). The irradiation test began on December 14, 2011, and ended on April 12, 2014 (Collin 2016). The originally planned AGR-3 and AGR-4 irradiation experiments were both focused on obtaining data on fission product transport to support the improvement of modeling. The AGR-3 experimental plan was focused on gaseous and metallic fission product release from the kernels and diffusion in the coatings during irradiation and post-irradiation safety testing. The AGR-4 experimental plan was focused on diffusivities and sorptivities in the compact matrix and reactor graphite. These two goals were combined in the AGR-3/4 irradiation, which consisted of 12 independently monitored capsules that each contained four AGR-3/4 compacts in a single stack surrounded by an inner ring of matrix or graphite and an outer ring of graphite. Two capsule types were used: a standard capsule and a so-called fuel body, in which the outer graphite ring included a floor and cap that fully enclosed the fuel. The fuel body design supported post-irradiation safety testing of the intact fuel and ring assembly to provide data on fission product transport and release from the matrix and graphite at accident temperatures.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Radial Deconsolidation and Leach-Burn-Leach of AGR-3/4 Compact 1-4 and 10-4

The Advanced Gas Reactor (AGR) Fuel Development and Qualification Program third and fourth irradiation experiments (AGR-3/4), originally planned as separate tests, were combined in one test train for irradiation in the Advanced Test Reactor at Idaho National Laboratory (INL). The irradiation test began on December 14, 2011 and ended on April 12, 2014 (Collin 2016). The originally planned AGR-3 and AGR-4 irradiation experiments were both focused on obtaining data on fission product transport to support the improvement of modeling. The AGR-3 experimental plan was focused on gaseous and metallic fission product release from the kernels and diffusion in the coatings during irradiation and postirradiation safety testing. The AGR-4 experimental plan was focused on diffusivities and sorptivities in the compact matrix and reactor graphite (Petti et al. 2005). These two goals were combined in the AGR-3/4 irradiation, which consisted of twelve independently monitored capsules that each contained four AGR-3/4 compacts in a single stack surrounded by an inner ring of matrix or graphite and an outer ring of graphite. There were two capsule types: a standard capsule and a “fuel body”, in which the outer graphite ring included a floor and cap that fully enclosed the fuel (Stempien et al. 2018a). The fuel body design supported post-irradiation safety testing of the intact fuel and ring assembly to provide data on fission product transport and release from matrix and graphite at accident temperatures (Demkowicz 2017).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Rapid prediction of fuel research octane number and octane sensitivity using the AFIDA constant-volume combustion chamber

Current research octane number (RON) and motor octane number (MON) gasoline performance characterization techniques use dated, complex engine testing methodology and limit researchers’ ability to easily characterize small volumes of experimental fuels. A novel methodology is presented that correlates measured ignition delay (ID) time to RON in an Advanced Fuel Ignition Delay Analyzer (AFIDA) constant-volume combustion chamber device at a single pressure/temperature condition, with an r2 of 0.99 and standard error (SE) of 1.0. The correlation of the slope of the ID time between two additional temperature points to octane sensitivity (S) produces an r2 of 0.97 and SE of 0.69; however, fuels with S>12 are indistinguishable. These results are based on methodology calibration using 31 primary and toluene reference fuels containing 0%-40% ethanol with RON values ranging from 85 to 113. Validation of these methods using a 102-sample fuel matrix spanning an array of base fuels and additive chemistry designed to test the robust applicability of the method, along with pump gasoline and high-octane surrogate blend samples, demonstrates an r2 of 0.94 and SE of 1.3 for the RON correlation over all samples, whereas the equivalent S correlation produces an r2 of 0.78 and SE of 1.2 by excluding two additives, 3-pentanone and diisobutylene, which displayed poor S correlation results. This novel AFIDA analysis method can be performed in 1 h and with 40 mL of fuel, offering significant improvements in time and volume requirements over traditional techniques.

33 ADVANCED PROPULSION SYSTEMS↗

Progress Report on SFR Metallic Fuel Data Qualification

This report summarizes the progress of SFR metallic fuel qualification related activities, which are focused on providing quality assurance relevant information applicable to experiments irradiated during the Integral Fast Reactor (IFR) program. An overview of the metallic fuel performance data and the associated databases, including the EBR-II Fuels Irradiation & Physics Database (FIPD), Out-of-Pile Transient Database (OPTD), and TREAT Experimental Relational Database (TREXR) is included. The legacy data in the databases, including as-built, post-irradiation examination (PIE), operating parameters, and out-of-pile experiment post-test data are introduced. The SFR metallic fuel Quality Assurance Program Plan (QAPP) and its implementation to qualify these legacy data is described in detail. Important PIE data QA documents and the specifications of seven types of PIE measurements (contact profilometry, laser profilometry, neutron radiography, gamma scan, fission gas release fission gas chemistry, and metallography) are provided. Examples of the implementation of the QAPP to qualify each of those types of PIE data are provided.

Mo, Kun [Argonne National Laboratory (ANL), Argonn↗

Report on RIA Relevant Modified Burst Testing of ATF Cladding Materials

The mechanical performance of accident-tolerant fuel (ATF) cladding candidates in light-water reactors (LWRs) must be similar to or better than that of current conventional nuclear fuel claddings to reduce dose to the public and ensure a that the core coolable geometry is maintained during a postulated reactivity-initiated accident (RIA) in light-water reactors (LWRs). During an RIA event, the rapid thermal expansion of nuclear fuel can deform the cladding once the fuel–cladding gap closes. In some cases, the pellet–cladding mechanical interaction (PCMI) can induce mechanical failure in ATF candidates. Thus, the mechanical response of ATF cladding must be investigated by mimicking the conditions of RIA and potentially performing Transient Reactor Test (TREAT) experiments to establish or verify the safety envelope. The work presented in this report investigated the failure behavior of as-received, hydrided, and chromium-coated (Cr-coated) Zircaloy-4 (Zry-4) cladding tube under strain-driven mechanical conditions, mimicking postulated RIA loading conditions. Mechanical testing was performed at 300°C via modified burst test (MBT) equipment with pulse width control previously developed under the Department of Energy’s (DOE’s) Advanced Fuel Campaign (AFC). The mechanical strains were determined using 2D digital image correlation (DIC) techniques. The base Zry-4 acquired by Cameco Inc. was in stress-relieved annealed (SRA) condition. Because of the observed large deformation of the cladding tubes, the failure strain definition was updated for the MBT, which can also be applied to other tube tests where significant bulging (out-of-plane deformation) is present. The failure strain was determined to be affected by the speed of the test or the RIA event. As the RIA-like event duration decreased from 75 to 15 ms, the failure strain decreased 5, 7 and 1% for as-received, hydrided, and Cr-coated specimens, respectively. Fractography on the Cr-coated specimens indicated the presence of two failure mechanisms: (i) crenulation at the outer surface of the coating due to the tensile tractional forces along with coatings grain microstructure and (ii) formation of critical defect at the coating/cladding interface that initiated coating rupture after severe plastic deformation of the Zry- 4 substrate. Based on the MBT results and fractography observations, performing mechanical property testing at high strain rates—in particular on Cr-coated tubes—and semi-integral TREAT experiments are required future efforts to ensure ATF cladding performance during transients. The testing recommended would also inform the development of long-term generalized cladding technologies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗