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At least 937 records · Page 52

Collisional effects in laser detection of tropospheric OH

The use of laser-induced fluorescence to measure OH in the troposphere is discussed. It is noted that quantitative laser detection of OH requires knowledge of collisional processes affecting the measurements and interference effects due to OH generated by laser photolytic processes. Collisions induce quenching of the excited A-state, as well as vibrational and rotational energy transfer in the excited and ground states. It is noted that the state-specific nature of these processes is important, especially the rotational level dependence of quenching and vibrational transfer in excited OH. Also important is the temperature dependence according to which quenching cross sections sharply increase with decreasing temperature. Laboratory experiments studying these collisional processes are described, and their implications for laser detection of tropospheric OH are examined.

Crosley, David R.↗

Inside the supernova: A powerful convective engine

We present an extensive study of the inception of supernova explosions by following the evolution of the cores of two massive stars (15 and 25 Solar mass) in multidimension. Our calculations begin at the onset of core collapse and stop several hundred milliseconds after the bounce, at which time successful explosions of the appropriate magnitude have been obtained. Similar to the classical delayed explosion mechanism of Wilson, the explosion is powered by the heating of the envelope due to neutrinos emitted by the protoneutron star as it radiates the gravitational energy liberated by the collapse. However, as was shown by Herant, Benz, & Colgate, this heating generates strong convection outside the neutrinosphere, which we demonstrate to be critical to the explosion. By breaking a purely stratified hydrostatic equilibrium, convection moves the nascent supernova away from a delicate radiative equilibrium between neutrino emission and absorption, Thus, unlike what has been observed in one-dimensional calculations, explosions are rendered quite insensitive to the details of the physical input parameters such as neutrino cross sections or nuclear equation of state parameters. As a confirmation, our comparative one-dimensional calculations with identical microphysics, but in which convection cannot occur, lead to dramatic failures. Guided by our numerical results, we have developed a paradigm for the supernova explosion mechanism. We view a supernova as an open cycle thermodynamic engine in which a reservoir of low-entropy matter (the envelope) is thermally coupled and physically connected to a hot bath (the protoneutron star) by a neutrino flux, and by hydrodynamic instabilities. This paradigm does not invoke new or modified physics over previous treatments, but relies on compellingly straightforward thermodynamic arguments. It provides a robust and self-regulated explosion mechanism to power supernovae that is effective under a wide range of physical parameters.

Herant, Marc↗

Validation of the NOνA experiment 2023-tuning on simulated neutrino-matter interactions

NOνA is a long-baseline neutrino oscillation experiment that utilizes a two-detector design to study the oscillations of muon neutrinos into electron neutrinos over a baseline of 810 km. The Near Detector (ND) measures the neutrino beam spectrum and composition before oscillation, which is then compared to the oscillated neutrino energy spectrum observed in the Far Detector (FD). In the ND, the neutrinos are detected through their interactions with the heavy target nuclei within the detector. NOνA employs the GENIE neutrino event generator for simulating these neutrino-nucleus interactions. However, the default GENIE prediction does not adequately reproduce the ND data. To address this, NOνA developed a tune of the neutrino interaction models within GENIE version 3:0:6 to minimize discrepancies between the simulated predictions and the observed data in the ND. This dissertation tests the NOνA’s 2023 tune of the GENIE neutrino cross-section simulations by performing a data/simulations comparison for the ND. The analysis employed datasets comprising $2.55\times10^{21}$ protons-on-target (POT) in neutrino beam mode and $1.14\times10^{21}$ POT in antineutrino beam mode. The NOνA tuning of neutrino-matter interaction simulations matches with ND data within the $1\sigma$ error band, overestimating muon neutrino and antineutrino charged current interactions by approximately 6 % and 9 %, respectively. Discrepancies were observed in the energy region dominated by Quasi-Elastic-like interactions. Systematic uncertainties associated with the modeling of the neutrino cross-section, particularly those pertaining Quasi-Elastic like interactions, contributed considerably to the overall error in the simulations. Furthermore, the reconstruction algorithm used in NOνA for particle classification demonstrated significant misidentifications between charged pions and protons, as well as a tendency to overlook additional pions or protons in multi-particle simulated events.

Cortés Parra, Camilo Andrés↗

Confirmation of PNNL Quantitative Infrared Cross-Sections for Isobutane

The Pacific Northwest National Laboratory (PNNL) gas-phase database is a compilation of quantitative experimental (5, 25, 50 °C) infrared spectra of ca. 500 molecules, designed for in situ, standoff or remote sensing of gases and vapors at or near atmospheric pressure. The data are characterized by calibration on both the wavenumber and intensity axes. Recent papers have called into question the PNNL intensity values for isobutane, (2-methylpropane, HC(CH 3 ) 3 ) suggesting discrepancies of 30 to 40%. In this study we re-measure and re-examine the intensity values of isobutane using both similar and alternate methods to those used to generate the original PNNL database spectra. Here, indirect confirmation from literature data of homologous molecules and direct confirmation from new results confirm that for many band integrals across the isobutane spectrum, the original PNNL data are indeed accurate to within the reported 3% experimental uncertainty.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Development and experimental evaluation of an acoustic flow meter prototype for measuring air flow

Here, this study outlines the development and testing of a flow meter prototype specifically designed for use in nuclear reactor environments. The meter uses flow-induced vibration to measure flow rates and is designed for remote monitoring in harsh environments where radiation can damage electronics. The device generates a vibration signal produced by a feedback system when fluid flows out of an orifice and interacts with a downstream wedge. The frequency of the vibration signal corresponds directly to flow rate and velocity. The study investigates geometric parameters intrinsic to the prototype, such as orifice height, width, edge distance, and chamber length. Different configurations were also tested, including a bypass loop with variable cross-sections around the device. The investigation results reveal the impact of these geometric parameters on the vibration signal output, providing valuable insights for future design improvements and enhancing the effectiveness of flow metering systems used in nuclear reactor applications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Large inverse Faraday effect for Rydberg states of free atoms and isolated donors in semiconductors

We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect and propose the appearance of the effect in two such systems: Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms are characterized by a large orbital radius. This large radius gives such excited states a large angular moment, which when driven with circularly polarized light translates to a large effective magnetic field $\mathscr{B}$ eff . We calculate this effect to generate effective magnetic fields of O⁡(1⁢ µ⁢T)×($\frac{ω}{1THz}$) -1 ⁢ ($\frac{\mathscr{I}}{10Wcm^{-2}}$)⁢n 4 in the Rydberg states of atoms such as Rb and Cs for off-resonant photon beams with frequency ω and intensity $\mathscr{I}$ expressed in units of the denominators and n the principal quantum number. Additionally, terahertz spectroscopy of phosphorus-doped silicon reveals a large cross section for excitation of shallow dopants to Rydberg-like states, which even for small n have the potential to be driven similarly with circularly polarized light to produce an even larger magnetization. Our theoretical calculations estimate $\mathscr{B}$ eff as O⁡(10 2 T) for Si:P with a beam intensity of 10 8 Wcm -2 .

36 MATERIALS SCIENCE↗

Moment extraction using an unfolding protocol without binning

Deconvolving (“unfolding”) detector distortions is a critical step in the comparison of cross-section measurements with theoretical predictions in particle and nuclear physics. However, most existing approaches require histogram binning while many theoretical predictions are at the level of statistical moments. We develop a new approach to directly unfold distribution moments as a function of another observable without having to first discretize the data. Our moment unfolding technique uses machine learning and is inspired by Boltzmann weight factors and generative adversarial networks (GANs). We demonstrate the performance of this approach using jet substructure measurements in collider physics. With this illustrative example, we find that our moment unfolding protocol is more precise than bin-based approaches and is as or more precise than completely unbinned methods.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A semiempirical method for obtaining fuselage normal areas from fuselage Mach sliced areas

An aircraft designed to meet low sonic boom or shaped ground overpressure signature requirements has a volume and lift equivalent area distribution which is in close agreement with the equivalent areas of a desired theoretical curve. Final-stage design modifications of the aircraft's geometry to meet this requirement are usually made through adjustments to the fuselage normal cross-section areas that are derived from the corresponding fuselage equivalent areas by iterative methods. The time required to obtain a good agreement between the desired low-boom area distribution and the conceptual aircraft total area distribution can be reduced by using a semi-empirical method which eliminates much of the final trial-and-error iteration previously employed. Fuselages from conceptual aircraft designed to generate low sonic boom ground overpressures at cruise Mach numbers of 2.0 and 3.0 were used as examples to examine the method's capabilities and limitations. Results indicated that the method has merit as a design tool consistent with other linear theory methods.

Mack, Robert J.↗

Additive manufacturing and testing of a ceramic heat exchanger for high-temperature and high-pressure applications for concentrating solar power

Heat exchangers with excellent corrosion and oxidation resistances are essential for the next-generation concentrating solar power (CSP) plants using a molten salt heat transfer fluid and a supercritical CO 2 Brayton power cycle that can operate at temperatures > 700 °C for higher efficiencies. Techniques were developed for additively manufacturing ceramic materials for applications involving high temperature, high pressure, and high corrosion resistance as needed for the CSP application. Based on a previous ceramic heat exchanger design with its cross-section geometry of the flow channels optimized for heat transfer and mechanical strength, lab-scale prototype heat exchangers, with integrated headers and incorporated flow channel dimensional compensations, were fabricated by using the binder jetting process. The printed prototype heat exchangers were successfully densified through the processes of liquid polymer infiltration and pyrolysis. In addition, thermophysical properties of the densified silicon carbide parts were measured to provide necessary design information. Experimental heat transfer testing of the lab-scale prototype heat exchanger was conducted, and the experimental data agreed reasonably well with the simulated results. Furthermore, this agreement provides validation of the simulation models for their applicability to the development of a full-scale ceramic heat exchanger.

14 SOLAR ENERGY↗

Substituent Effects on the Electronic Spectroscopy of Four-Carbon Criegee Intermediates

Atmospheric ozonolysis of biogenic and anthropogenic alkenes generates zwitterionic carbonyl oxide intermediates (R 1 R 2 C=O + O – ), known as Criegee intermediates, with different structural motifs and conformations. This study reports a systematic laboratory study of substituent effects on the electronic spectroscopy of four-carbon Criegee intermediates (CIs) with methyl–ethyl (MECI) and isopropyl (IPCI) groups, which are isomers produced in ozonolysis of asymmetric branched alkenes. The four-carbon CIs are separately generated by an alternative synthetic route, and spectroscopically characterized on the strong π* ← π transition associated with the carbonyl oxide group in a pulsed supersonic expansion with VUV photoionization at 118 nm and UV-induced depletion of the m/z 88 signal. The resultant broad and unstructured UV spectral features for MECI and IPCI are peaked at ca. 320 and 330 nm, respectively, with large absorption cross-sections of ca. 10 –17 cm 2 . Comparisons are made with the four-carbon CIs formed in isoprene ozonolysis, methyl vinyl ketone oxide (MVK-oxide) and methacrolein oxide (MACR-oxide), which have the same backbone connectivity as MECI and IPCI but have extended conjugation across the vinyl and carbonyl groups. A remarkable 50 nm shift of the peak absorption to longer wavelength is observed for MVK-oxide and MACR-oxide compared to MECI and IPCI, respectively. Furthermore, vertical excitation energies computed theoretically agree well with the experimental findings, confirming that the spectral shifts are caused by the extended π conjugation in the isoprene-derived Criegee intermediates.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Measurement of the near-threshold 𝐽/𝜓 photoproduction cross section with the CLAS12 experiment

We present measurements of the total and differential cross sections for near-threshold 𝐽/𝜓 photoproduction obtained with the CLAS12 detector at the Thomas Jefferson National Accelerator Facility. The results are based on data collected during the fall 2018 and spring 2019 running periods, using electron beams with energies of 10.6 and 10.2 GeV, respectively, scattered off a liquid-hydrogen target. Near-threshold 𝐽/𝜓 photoproduction offers a unique sensitivity to the strong interaction in the nonperturbative regime of quantum chromodynamics (QCD). The energy dependence of the cross section constrains the underlying 𝐽/𝜓 production mechanisms, including multigluon exchange and potential baryonic excitations. Additionally, the 𝑡 dependence of the differential cross section can be related to the transverse spatial distribution of gluons in the proton, providing critical input for theoretical descriptions of the gluonic structure of the proton. An interpretation of the results in terms of the gluon content of the proton is presented, providing new experimental constraints on QCD-inspired models of the proton structure and the role of gluonic degrees of freedom in hadronic mass generation.

form factors↗

Triaxiality and the nature of low-energy excitations in Ge 76

The deformation properties of the low-lying states in 76 Ge have been investigated following a safe energy Coulomb excitation measurement with the GRETINA tracking array and CHICO2 heavy-ion counter at the ATLAS accelerator facility at Argonne National Laboratory. A comprehensive set of transition and static E2 matrix elements were extracted from the measured differential Coulomb cross-sections, and compared with results of configuration interaction shell-model calculations and computations carried out within the framework of the generalized triaxial rotor model. The remarkable agreement between the calculated and experimental data supports a near-maximum triaxial deformation for the ground state of 76 Ge. Additionally, the degree of softness of the asymmetry in 76 Ge and 76 Se was investigated using rotational invariants generated from configuration interaction shell-model wave functions computed with the jj44b and JUN45 effective interactions. The resulting invariants are shown to be consistent with a stiff triaxial deformation in 76 Ge and a predominantly soft triaxial potential for 76 Se, in agreement with the conclusions of recent works by this collaboration.

59 ≤ A ≤ 89↗

Measurement of muon pairs produced via γ γ scattering in nonultraperipheral Pb + Pb collisions at s N N = 5.02 TeV with the ATLAS detector

Results of a measurement of dimuon photoproduction in nonultraperipheral Pb + Pb collisions at √ s NN = 5.02 TeV are presented. The measurement uses ATLAS data from the 2015 and 2018 Pb + Pb data-taking periods at the LHC with an integrated luminosity of 1.94 nb –1 . The γγ → μ + μ – pairs are identified via selections on pair momentum asymmetry and acoplanarity. Differential cross sections for dimuon production are measured in different centrality, average muon momentum, and pair rapidity intervals as functions of acoplanarity and k ⊥ , the transverse momentum kick of one muon relative to the other. Measurements are also made as a function of the rapidity separation of the muons and the angle of the muon pair relative to the second-order event plane to test whether magnetic fields generated in the quark-gluon plasma affect the measured muons. A prior observation of a centrality-dependent broadening of the acoplanarity distribution is confirmed. Furthermore, the improved precision of the measurement reveals a depletion in the number of pairs having small acoplanarity or k ⊥ values in more central collisions. The acoplanarity distributions in a given centrality interval are observed to vary with the mean p T of the muons in the pair, but the k ⊥ distributions do not. Comparisons with recent theoretical predictions are made. The predicted trends associated with effects of magnetic fields on the dimuons are not observed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

In Situ and Post-Mortem Characterizations of Ultrasonic Spot Welded AZ31B and Coated Dual Phase 590 Steel Joints

Ultrasonic spot welding using different welding conditions was applied to join dissimilar metals of galvanized DP590 steel and AZ31B magnesium sheets. In situ high-speed imaging, digital image correlation, and infrared thermography were utilized to quantitatively study the interfacial relative motion, surface indentation, and heat generation across the joint faying interface and the sheet/sonotrode interfaces under the welding condition of moderate welding power and short welding time. For welds made with high power and long welding time, lap shear tensile tests as well as fatigue tests were carried out. Different fracture modes were observed after the lap shear tensile tests and fatigue tests performed under different peak loads. Post-weld cross-sectional analysis with scanning electron microscopy coupled with energy dispersive X-Ray spectroscopy revealed the variation of morphology and chemical composition at the joint interface for welds made with different welding conditions.

36 MATERIALS SCIENCE↗

Acoustic systems containing curved duct sections

The analysis of waves in bends in acoustical ducting of rectangular cross section is extended to the study of motion near discontinuities. This includes determination of the characteristics of the tangential and radial components of the non-propagating modes. It is established that attenuation of the non-propagating modes strongly depends on frequency and that, in general, the sharper the bend, the less attenuation may be expected. Evaluation of a bend's impedance and of impedance-generated reflections is also presented in detail.

Rostafinski, W.↗

X-Ray Morphology of Cluster-Mass Haloes in Self-Interacting Dark Matter

We perform cosmological zoom-in simulations of 19 relaxed cluster-mass haloes with the inclusion of adiabatic gas in the cold dark matter (CDM) and self-interacting dark matter (SIDM) models. These clusters are selected as dynamically relaxed clusters from a parent simulation with M200(1-3) × 10 15 M. Both the dark matter and the intracluster gas distributions in SIDM appear more spherical than their CDM counterparts. Mock X-ray images are generated based on the simulations and are compared to the real X-ray images of 84 relaxed clusters selected from the Chandra and ROSAT archives. We perform ellipse fitting for the isophotes of mock and real X-ray images and obtain the ellipticities at cluster-centric radii of r0.1–0.2R 200 .The X-ray isophotes in SIDM models with increasing cross-sections are rounder than their CDM counterparts, which manifests as asystematic shift in the distribution function of ellipticities. Unexpectedly, the X-ray morphology of the observed non-cool-coreclusters agrees better with SIDM model swith cross-section (σ/m)=0.5–1cm2g−1 than CDM and SIDM with (σ/m)=0.1cm2g−1. Our statistical analysis indicates that the latter two models are disfavoured at the 68 percent confidence level (as conservative estimates). This conclusion is not altered by shifting the radial range of measurements or applying a temperature selection criterion. However, the primary uncertainty originates from the lack of baryonic physics in the adiabatic model, such as cooling, star formation and feedback effects, which still have the potential to reconcile CDM simulations with observations.

dark matter – cosmology↗

Comparison of Ring Diagrams Based on the Doppler Shifts of Synthetic Data Obtained with Bisector Method and SDO/HMI Pipeline

Ring diagrams are cross-sections of three-dimensional spatiotemporal power spectra of solar oscillations. The rings reveal information about sub-surface flows and represent an important tool for helioseismology. Ring diagrams can be constructed using Doppler velocity or intensity maps of spectral lines. How the velocities are computed is an important factor for accuracy of information we can retrieve on subsurface flows. In our work, the ring diagrams are generated from Doppler shift data of synthesized Fe I 6173 Å line. We compare ring diagrams computed by two methods–HMI line-of-sight pipeline and the bisector of Fe line. Fe I line is synthesized for StellarBox 3D Radiative hydrodynamic simulations under LTE assumption. We aim to answer the following questions: 1.How do power spectra obtained from velocities computed with the HMI pipeline and bisector of the Fe I 6173Å compare? 2.How do the power spectral density retrieved with each method vary with heliocentric angle? 3.What is the effect of changing resolution on the power spectral density in ring diagrams obtained with the two methods?

SMD↗

The NuMI Flux Prediction at ICARUS

The Deep Underground Neutrino Experiment (DUNE) is a next-generation long-baseline neutrino oscillation experiment seeking to probe fundamental symmetries within the structure of the Pontecorvo-Maki-Nakagawa-Sakata (PMNS) mixing matrix, and perform precision measurements its parameters including the neutrino mass ordering via the sign of $\Delta m^2_{31}$, and the charge-parity violating phase, $\delta_{CP}$. To make these measurements with high precision, DUNE will require external $\nu$-Ar scattering cross section data as a crucial input to the oscillation fit. Imaging Cosmic And Rare Underground Signals (ICARUS) is a 476 t liquid argon neutrino detector located at Fermi National Accelerator Laboratory (FNAL) where it is serving as the far detector for the Short-Baseline Neutrino (SBN) program along the Booster Neutrino Beam (BNB) axis. ICARUS additionally lies 795 m downstream and 100.1 mrad off-axis of the Neutrinos at the Main Injector (NuMI) neutrino beam. From this position, ICARUS is exposed to a large flux of NuMI (anti-)electron and (anti-)muon neutrinos, and poses a unique opportunity to provide high-statistics measurements of quasi-elastic and single pion-production cross sections for four neutrino flavors ($\nu_{\mu}$, $\nu_{e}$, $\bar{\nu}_{\mu}$, $\bar{\nu}_{e}$). This dissertation is centered around accurately characterizing the models and estimating their precision for use in making these measurements. This includes identifying major sources of uncertainty in the models such that they can be properly propagated to the cross section measurements. Specifically, this work focused on the model of the NuMI beamline and its impact on the neutrino fluxes, but also delved into the detector response model and its impact on reconstructed observables in the detector. Significant efforts were made to improve the characterization to enhance precision and thus reduce the level of propagated uncertainty. In particular, the NuMI flux was determined to be composed of 57% $\nu_{\mu}$, 38% $\bar{\nu}_{\mu}$, 3% $\nu_{e}$, and 2% $\bar{\nu}_{e}$ while the horns are operating in the positive-particle focusing configuration. The total uncertainty on the $\nu_{\mu} + \bar{\nu}_{\mu}$ ($\nu_{e} + \bar{\nu}_{e}$) flux while operating in the forward horn operating mode was determined to be 10.84% (9.04%). Compared to the on-axis flux, mesons that eventually decay to neutrinos more frequently reinteract within the NuMI structure, resulting in elevated uncertainty as these processes are not well-constrained by existing hadron interaction cross section measurements. Covariance matrices were calculated to propagate the flux uncertainty characterization to NuMI analyses.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗