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At least 919 records · Page 51
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Carbon accumulation rate peaks at 1,000-m elevation in tropical planted and regrowth forests

Tropical planted and regrowth forests (TPRFs) are one of the most low-cost components for recovering biomass-stored carbon in the tropics. Nevertheless, challenges persist in pinpointing which elevational ranges exhibit the largest carbon accumulation rate ($γ$ rapid ) due to the highly inconsistent previous assessments. This prevents the selection of optimal locations for implementing large-scale reforestation in the tropics. Here, in this study, we proposed a refined approach that used a carbon accumulation threshold (<80% of the maximum value) to quantify $γ$ rapid in TPRFs at various elevations. We find that $γ$ rapid increases with elevations from 300 to 1,000 m and declines at elevations >1,000 m. TPRFs at elevations ~1,000 m exhibit three times more $γ$ rapid than lowland TPRFs. This optimal elevation, highly dependent on background temperatures, varies slightly but significantly across different mountains. These findings provide guidelines for policymakers to determine the optimal elevations from regional to continental scales when implementing reforestation initiatives in the tropics.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Reproducible emission from nonlinear random lasers

Multiple scattering of light serves as a mechanism for feedback in random lasers. Consequently, internal spatial mode patterns, lasing wavelengths, and output directionality can all be random. Strong mode interaction can occur in such devices due to spatially overlapping modes resulting in nonlinearity with respect to the pump input power. Nevertheless, temporal coherence and lasing mode amplitude can be fixed at a constant pumping rate. This is a property desirable for applications where unique randomness is exploited but expected to be reliable over time, such as physical unclonable functions. Random lasers can also be cheaply and easily fabricated, exhibit relatively low lasing thresholds and high emission intensity. However, the precise scattering properties of such structures and fluctuations in the pump field can make device emission irreproducible, thereby limiting random laser applications. Here, in this work, we directly compare the random lasing spectra from zinc oxide samples fabricated in four distinct ways: spin-coating, sputtering, solgel deposition, and atomic layer deposition. The particular method of fabrication has a strong impact. Samples made through atomic layer deposition here exhibit both reproducibility and strong nonlinearity desirable for applications. Randomness in emission spectra persists across hundreds of repeated and averaged measurements irrespective of spatial location and is demonstrably nonlinear with respect to input signal intensity.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

The evidence of N = 16 shell closure and β -delayed neutron emission from 25 F

We measured the β -delayed neutron emission from 25 F for the first time at the Facility for Rare Isotope Beams (FRIB). Using combined neutron and γ -ray detector systems of the FRIB Decay Station Initiator (FDSi), we observed β -decay transitions populating neutron unbound states between 4.2 and 8 MeV in 25 Ne. The experimental results led to the revision of the β -decay half-life and β -delayed neutron-emission probability of 25 F. The β -decay strength distribution of 25 F extracted from the data agrees with the shell-model predictions using the USDB and SDPF-M effective interactions. This result indicates that the spherical neutron shell gap persists in 25 F and 25 Ne.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Shell effects in quasi-fission for calcium induced reactions forming thorium isotopes

Quantum shell effects induce an asymmetric fission mode in actinides, which disappears in neutron deficient isotopes. Quasi-fission, characterized by a significant mass transfer in heavy ion collisions at low-energies, is expected to be affected by similar shell effects. This is studied in 40−56 Ca+176 reactions with the time-dependent Hartree-Fock approach. All reactions exhibit a mass equilibration process that stops when a heavy fragment with 𝑍 ≃ 54 protons is formed. Unlike the fission of thorium compound nuclei, quasi-fission does not exhibit a transition to symmetric modes in neutron deficient systems. This observation is interpreted in terms of potential energy surfaces that show a persistence of an asymmetric valley with an increasing barrier preventing its population in fission of the most neutron deficient thorium isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

No evidence of a reduction in the dipole polarisability at shell closures

Photoabsorption reactions have a long and productive history as probes of the response of nuclei to electromagnetic fields. In recent years, there has been a suggestion that the dipole polarisability may be reduced at shell closures, potentially due to the reduced level density. In the current paper, more recent photoabsorption strengths are reanalysed including nuclei on closed proton shells to search for a similar reduction. The previously reported reduction is not reproduced. We conclude that the previously observed reduction may be due to incomplete evaluations of the photoabsorption due to missing cross section contributions and experimental artefacts. More experimental data are necessary to draw a firm conclusion about whether shell effects persist into high excitation energies, especially data which can obviate any systematic effects and look at relative photoabsorption strengths between nuclei.

Giant dipole response↗
DOE OSTI2026

Multiplicity dependence of K*(892) ± production in pp collisions at $\sqrt{s}$ = 13 TeV

The first results of K*(892) ± production at midrapidity (|y| < 0.5) in pp collisions at $\sqrt{s}$= 13 TeV as a function of the event multiplicity are presented. The K*(892) ± has been reconstructed via its hadronic decay channel K*(892) ± → π ± + K$^0_{\textrm{S}}$ using the ALICE detector at the LHC. For each multiplicity class, the differential transverse momentum (p T ) spectrum, the mean transverse momentum ⟨p T ⟩, the p T -integrated yield (dN/dy), and the ratio of the K*(892) ± to K$^0_{\textrm{S}}$ yields are reported. These are consistent with previous K*(892) 0 resonance results with a higher level of precision. Comparisons with phenomenological models such as PYTHIA6, PYTHIA8, EPOS-LHC, and DIPSY are also discussed. For the first time, a significant K*(892) ± /K$^0_{\textrm{S}}$ suppression in pp collisions is observed at a 7σ level passing from low to high multiplicity events. The ratios of the p T -differential yields of K*(892) ± and K$^0_{\textrm{S}}$ in high and low multiplicity events are also presented along with their double ratio. For p T ≲ 2 GeV/c this double ratio persists below unity by more than 3σ suggesting that the suppression affects mainly low p T resonances. The measured decreasing trend of the K*(892) ± /K$^0_{\textrm{S}}$ ratio with increasing multiplicity, which in heavy-ion collisions is typically attributed to the rescattering of decay particles of the short-lived resonances, is reproduced by the EPOS-LHC model without the use of hadronic afterburners.

Hadronic resonance production↗
DOE OSTI2020

A data analytical approach for assessing the efficacy of Operational Technology active defenses against insider threats

In recent years, the need for Operational Technology (OT) defenses has been recognized, serving as an additional line of defense when Information Technology (IT) defenses are bypassed. This is no longer considered an uncommon possibility when dealing with advanced persistent threat (APT) actors expected to be state-sponsored and receiving insider assistance. In these extreme adversarial situations, OT defenses aim to provide another layer of defense for the system, introduced directly at the physical process level, as described by the sensors data, the system model, and control actions. Just like IT defenses, two schools of thought, i.e., passive and active defenses, have emerged to address this challenge. In active defenses, representing the focus of this paper, known signatures, synthesized based on the system's unique characteristics, are inserted into the system. In contradistinction, passive methods rely solely on observing system behavior in search of patterns of normal behavior with deviations thereof representing abnormal behavior. In their most sophisticated implementations, both passive and active defenses rely on the use of data analytics to identify the patterns and synthesize the observed and/or inserted signatures. Past research has shown that passive defenses may be bypassed by APT actors relying on data analytics and their intimate knowledge of the system to evade detection by respecting the patterns identified by the defenders. Here this manuscript explores the use of active defenses under the assumption that the attacker has privileged access to the system, including access to the system's model and sensors data. Specifically, this manuscript assesses the ability of active defenses to remain invisible to the attackers, and discusses the associated challenges that must be addressed to ensure their resiliency against APT actors.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2020

Chain flexibility and glass transition temperatures of poly(n-alkyl (meth)acrylate)s: Implications of tacticity and chain dynamics

The relationship between chain microstructure and glass transition temperature (T g ) is complicated for poly(alkyl methacrylate)s and poly(alkyl acrylate)s. Despite intensive studies, relationships between the structures of these polymers and their properties, including solution characteristics and T g , are still controversial. Solution properties, chain conformations, including Flory's characteristic ratio (C ∞ ), persistence length (l p ), and chain diameters, and T g are reported for series of poly(n-alkyl acrylate)s and poly(n-alkyl methacrylate)s having alkyl side chain lengths (n) ranging from 1 to 10 carbons in length, with uniform and well-characterized tacticities. Chain flexibilities of both series of polymers decrease as n increases, reflecting increased hindrances to rotation about backbone bonds as side chains become longer. Conversely, the T g s for both series of polymers decrease substantially as n increases, reflecting the greater side chain mobilities of long alkyl substituents. For shorter alkyl chain lengths, T g s for the poly(n-alkyl acrylate)s are much lower than for the corresponding poly(n-alkyl methacrylate)s, a difference which has been attributed in the past to the presumed reduced chain flexibility of polymethacrylates due to the presence of the α-methyl substituent. However, contrary to such expectations, C ∞ and l p values for these two series of polymers are nearly identical at a given n value, except for the longest n-alkyl substituents. Instead, the differences in T g may be attributed to the differences in tacticity of the two series – almost ideally atactic for the poly(n-alkyl acrylate)s but high in syndiotacticity for the poly(n-alkyl methacrylate)s. The T g s for the two series of polymers approach that of polyethylene at longer alkyl chain lengths. In addition, the effects of tacticity and chain dynamics on C ∞ , l p , and T g of poly(methyl methacrylate) is discussed.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Effect of Microstructure on Chain Flexibility and Glass Transition Temperature of Polybenzofulvene

Polybenzofulvene (PBF) is a polydiene with a very high glass transition temperature (T g ), which makes it a potential candidate for use as the hard block for high-temperature thermoplastic elastomer applications. The T g s of polydienes are known to be related to chain flexibility. However, no studies have been reported that correlate the chain flexibility to the microstructure of PBF. Herein, we present a study of solution properties of linear PBFs with narrow molecular weight dispersity and having 1,2-addition ranging from 23% to 99%. The materials were prepared by living anionic polymerization under different conditions. Specifically, the chain flexibility as defined by the Flory's characteristic ratio, , and dependence of chain flexibility on microstructure by combined measurements of intrinsic viscosity and molecular weight using triple-detector size exclusion chromatography (SEC) is studied. The persistence lengths (l p ) and chain diameters (d B ) were also estimated using the touched-bead wormlike chain model. To the best of our knowledge, the characteristic ratio of PBF is found to be the highest of all polydienes that have been reported so far.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Fluorescent aggregate structure revealed in bisphenol F epoxy thermoset

Bisphenol F (BPF) epoxy resin is a prepolymer component of thermosets used in construction of reinforced carbon fiber composites (RCFC). The fluorescence of this resin can provide information about chemical and structural alterations of the thermoset from thermal or mechanical damage. While some work has investigated the fluorescence spectra of bisphenol A epoxy resin, a structural analog of BPF, none have studied BPF. The purpose of this study is to investigate the baseline fluorescence spectra of the BPF epoxy resin for features that could be utilized for monitoring damage and structural alterations. Bisphenol F epoxy resin was found to have two emission peaks with a broad peak centered at 410 nm and a sharp peak centered at 550 nm. The broad emission peak was identified as the fluorescence from BPF epoxy monomer while the sharp emission peak was found to be from an aggregate structure present in the epoxy resin. It is hypothesized that this structure is an H-aggregate based on the emission features and structural stability of the aggregate compared to the alternative J-aggregate which was determined via density functional theory calculations. The H-aggregate was found to persist into one of the cured thermoset formulations evaluated but was lost when exposed to elevated temperatures below thermal degradation of the thermoset. This loss of aggregate structure was due to polymer network rearrangement. This new fluorescence signature can be used as an indicator of polymer network rearrangement from thermal exposure which may alter the expected material performance and precede thermal degradation.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Foundational insights into the mechanical and molecular evolution of porcine skin gelatin during gelation

Gelatin is a widely used material in biomedical fields, particularly in regenerative medicine and tissue engineering, due to its biocompatibility and versatile properties. While prior research has explored methods to enhance gelatin's mechanical strength and stability, fundamental studies on gelatin, specifically its curing process, mechanical stiffness, and chemical evolution during gelation, remain limited. This study uses ultrasonic testing and Fourier Transform Infrared Spectroscopy (FTIR) to examine gelatin's stiffness and molecular changes during gelation. Samples of 175 and 300 Porcine Skin Bloom Strength Gelatin at concentrations of 2% and 6% (w/v) were analyzed. Through transmission ultrasonic testing helped identify key transition points in gelation, with higher concentrations exhibiting delayed transitions. FTIR revealed that C-N bond formation peaks early while N-H bond deformation persists. A correlation emerged between sound speed and peak absorbance, suggesting that changes in molecular mobility may contribute to the observed sound speed behavior during periods of active bond formation. However, as gelation continues, fewer bonding components may be available, potentially decreasing molecular movement and contributing to the observed increase in sound speed. These findings provide insights into gelatin's mechanical and chemical evolution, offering a framework for improved control over its gelation kinetics. Swept-Frequency Acoustic Interferometry (SFAI) was performed at the end of the curing process to measure the sound speed, enabling the calculation of the bulk moduli of the gelatin samples. The combined use of ultrasonic and FTIR testing provides a non-destructive method for characterizing gelatin and other biomaterials. This approach advances understanding of gelatin curing behavior and supports the development of safer biomaterials with tailored mechanical properties for various applications such as tissue engineering and regenerative medicine.

Biomaterials↗
DOE OSTI2025

Paleoclimatic implications of glacial fluctuations in the Sierra Nevada del Cocuy, northern Andes, Colombia, during the Lateglacial and Holocene

The reconstruction of former mountain glaciers from geomorphic mapping and cosmogenic-nuclide surface-exposure dating provides a unique opportunity to infer patterns of past terrestrial climate variability. Tropical mountain glaciers are particularly valuable as there are comparatively few terrestrial climate proxies at equatorial latitudes relative to higher latitudes. As the single largest climate zone on Earth, the tropics play an outsized role in mediating global climate via the ocean-atmosphere transfer of latent heat and water vapor. Nonetheless, there remains a persistent gap in our understanding of how the tropics influenced – or were influenced by – the high-magnitude climate shifts of the Late Pleistocene, and whether this high-energy region simply responded to extratropical forcing or was itself a driver of global climatic change. To help address this knowledge gap, we analyzed geologic evidence for past glacial fluctuations in three adjacent valleys in the Sierra Nevada del Cocuy, the highest subrange of the Eastern Cordillera in the Colombian Andes, to provide a terrestrial record of atmospheric temperature during the latter part of Termination 1. Coupled with geomorphic mapping and paleo-snowline reconstructions, our beryllium-10 glacial chronology indicates that glaciers in the humid inner tropics underwent pronounced growth and gradual decay during the Antarctic Cold Reversal (14.5–12.8 ka) and Younger Dryas (12.8–11.7 ka) periods, respectively, following a trend that, according to directly dated moraine records from throughout both polar hemispheres, appears to have been global. While the specific mechanism(s) behind this large-scale behavior remains to be corroborated, we revisit the hypothesis that ocean-atmosphere heat transfer and water vapor flux are key drivers of abrupt Lateglacial temperature fluctuations. Subsequent to the Lateglacial, deglaciation of the Sierra Nevada del Cocuy accelerated during the Early Holocene, a pattern also observed in other tropical glacier records. More recently, the magnitude of snowline rise and glacier retreat over the last two centuries supports the view that modern tropospheric warming is anomalously strong at least relative to the last ∼16,000 years.

Andes↗
DOE OSTI2023

Influence of the irradiated pulmonary microenvironment on macrophage and T cell dynamics

The lung is sensitive to radiation, which increases the risk of normal tissue toxicity following radiation therapy. Adverse outcomes include pneumonitis and pulmonary fibrosis, which are thought to result from dysregulated intercellular communication within the pulmonary microenvironment. Macrophage accumulation in the lung following radiation exposure is implicated in these pathogenic outcomes. Here we investigate the role of the microenvironment in macrophage and T cell dynamics. Materials and methods C57Bl/6 mice received 6Gyx5 x-ray irradiation to the right lung. Macrophage and T cell dynamics were investigated in ipsilateral right lungs, contralateral left lungs and compared to those from non-irradiated control subjects at 4-26wk post exposure. Lungs were evaluated by flow cytometry, histology and proteomics. Results In uni-lung irradiated subjects, focal regions of macrophage accumulation were noted in both lungs by 8wk, however fibrotic lesions were observed only in ipsilateral lungs by 26wk. Both infiltrating and alveolar macrophages populations transiently expanded in both lungs, however a transitional CD11b+ alveolar macrophage population persisted only in ipsilateral lungs and expressed lower CD206. Concurrently, arginase-1+ macrophages were noted within areas of macrophage accumulation in ipsilateral but not contralateral lungs at 8 and 26wk post exposure, while CD206+ macrophages were absent from these accumulations. While CD8+ T cells were present in both lungs of irradiated subjects, T regulatory cells were only increased in ipsilateral lungs. Unbiased proteomics analysis of immune cells revealed a substantial number of differentially expressed proteins in ipsilateral lungs when compared to either contralateral or non-irradiated lungs, as well as between contralateral lungs from irradiated subjects and non-irradiated controls. Conclusions Pulmonary macrophage and T cell dynamics are impacted by the microenvironmental conditions that develop in the lung following radiation exposure, both locally and systemically. Our findings demonstrate that while macrophages and T cells infiltrate and expand in both lungs, they diverge phenotypically depending on their environment.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2021

Is a Prescribed Fire Sufficient to Slow the Spread of Woody Plants in an Infrequently Burned Grassland? A Case Study in Tallgrass Prairie

In many mesic grasslands, such as the central Great Plains in North America, frequent fire is a key regulator of ecological processes. Long periods of infrequent fire facilitate the conversion of herbaceous-dominated grassland to woody-dominated shrubland or woodland. At the Konza Prairie Biological Station in northeast Kansas, one infrequently burned portion of the landscape has undergone transformation from grassland to woodland after nearly 30 yr without fire. In Spring 2017, a prescribed burn was implemented to assess fire effectiveness on woody plant mortality. A postfire census of 3 000+ individual woody plants identified the distribution of species by size (height), topographic position, and slope on the landscape. Mortality and canopy fire damage were calculated for each individual. In lowland locations with near-continuous shrub cover (30.7% of the landscape), woody plants were unaffected by fire. However, in upland and slope locations, where shrubs and trees were sparser, survival probability varied by topographic position and species. In these locations 68% of all woody individuals experienced 90% or greater fire damage to the canopy, with 56% of these individuals exhibiting new canopy regrowth within 2 mo after the fire. Here, the two most abundant woody shrubs, Cornus drummondii and Rhus aromatica, showed high survival at all height classes and landscape positions. The two abundant tree species, Gleditsia triacanthos and Juniperus virginiana, showed increased survival probability with tree height that varied by landscape position. Survival of J. virginiana also varied according to proximity and size of neighboring clonal shrubs, providing a mechanism for persistence of this fire-sensitive tree species even at small height classes. The probability survival curves developed here are useful for managers assessing when to prescribe fire to maximize mortality for J. virginiana and provide insight relevant for broader ecological understanding of woody encroachment within grasslands throughout the world.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

OC6 phase I: Improvements to the OpenFAST predictions of nonlinear, low-frequency responses of a floating offshore wind turbine platform

We report in the OC5 and OC6 projects, the authors observed a persistent underprediction of the nonlinear, low-frequency responses of an offshore wind semisubmersible with many mid-fidelity engineering models, including the OpenFAST tool developed by the National Renewable Energy Laboratory. Both the low-frequency wave excitation in surge and pitch and the resulting resonance motions were severely underpredicted. In response, we developed several modifications to the OpenFAST model from the OC5/6 projects to improve the predictions of the low-frequency wave loads and responses. All modifications are in the modeling of the viscous drag forces. Efforts were made to provide physical justifications to the changes and to limit the number of additional parameters requiring tuning, so that the modified model can be applied to other floating wind systems. With the proposed modifications, the predictions of the low-frequency surge and pitch wave loads on a fixed floater and the resonance responses of a floating structure are both significantly improved with a single set of model coefficients, which leads to good agreement with the measurements from the OC6 wave-basin experimental campaign.

17 WIND ENERGY↗
DOE OSTI2023

A comparison of the power potential for surface- and seabed-deployed tidal turbines in the San Juan Archipelago, Salish Sea, WA

The San Juan archipelago lies along the axis of tidal movement between Straits of Juan de Fuca and Strait of Georgia in the Salish Sea. The amplitude of the tidal exchange produces significant tidal currents between the islands, as well as in Rosario and Haro Straits. These are of interest as a future source of electrical power generation, given the islands’ dependence on electricity supply by a subsea cable from the mainland. Here, we evaluate the tidal current energy potential in this region through a re-analysis of measurements collected by the National Ocean Service (NOS) and a high-resolution numerical model. Given the considerable variations in water depth and vertical velocity profiles across candidate tidal energy sites, we consider the trade-offs between tidal turbines deployed from a floating platform and those anchored to the seabed. Measurement re-analysis indicates several locations that could support tidal current power generation by MW-scale turbines with an acceptable balance between turbine size, rated power, and capacity factor. Even for relatively large (30 m) turbine diameters, surface-deployed turbines would be expected to produce up to 30 % more electricity than the same turbine deployed near the seabed due to vertical shear, with this difference increasing for smaller diameter turbines. A benchmark comparison at the measurement locations with the highest power generation potential shows relatively good model fidelity, though, even with relatively high resolution, time-average power density disagreements of ± 50 % persist throughout the water column. Nonetheless, the simulation identifies several locations with power generation potential more than twice as high as locations in the measurement re-analysis. These sites were either not surveyed by NOS or excluded due to data quality issues. Altogether, these results demonstrate the complimentary of models and measurements for tidal energy site assessment and suggest that tidal currents could be an important source of electricity generation in the San Juan archipelago.

16 TIDAL AND WAVE POWER↗
DOE OSTI2024

Control-inspired design and power optimization of an active mechanical motion rectifier based power takeoff for wave energy converters

Ocean waves have high energy density and are persistent and predictable. Yet, converting wave energy to a useable form remains challenging. A significant hurdle is the oscillatory nature of waves resulting in the alternating loads, which necessitate the use of rectification at some stage of the energy conversion. This research effort presents a novel design of active mechanical motion rectifier (AMMR) for the power takeoff (PTO), which provides enhanced controllability and better power performance when compared to passive mechanical motion rectifiers (MMR). Inspired by transistors used in synchronous electrical rectifiers, the proposed design uses controllable electromagnetic clutches in the mechanical transmission to allow active engagement-disengagement control; thus, rectifying the oscillatory motion into a unidirectional rotation for high energy conversion efficiency and allowing the generator in unidirectional rotation to control the bidirectional wave capture structure for maximizing the power output. A semi-analytical computational approach is developed to efficiently evaluate the optimal power achieved using the proposed AMMR-based PTO and active control. It is found that the AMMR-based PTO design yields a higher optimal power than the previous passive MMR design across the wave spectrum. The influences of generator inertia and reactive power are discussed. Furthermore, the effects of control parameters on the power output and the optimal trajectories are analyzed. Wave tank tests with the AMMR prototype demonstrated the effectiveness of AMMR based PTO design and validated the numerical analysis.

16 TIDAL AND WAVE POWER↗