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NASA NTRS2013

Real-Tme Boron Nitride Erosion Measurements of the HiVHAc Thruster via Cavity Ring-Down Spectroscopy

Cavity ring-down spectroscopy was used to make real-time erosion measurements from the NASA High Voltage Hall Accelerator thruster. The optical sensor uses 250 nm light to measure absorption of atomic boron in the plume of an operating Hall thruster. Theerosion rate of the High Voltage Hall Accelerator thruster was measured for discharge voltages ranging from 330 to 600 V and discharge powers ranging from 1 to 3 kW. Boron densities as high as 6.5 x 10(exp 15) per cubic meter were found within the channel. Using a very simple boronvelocity model, approximate volumetric erosion rates between 5.0 x 10(exp -12) and 8.2 x 10(exp -12) cubic meter per second were found.

Hall thruster↗

NASA NTRS2013

Effects of the LBV Primary's Mass-loss Rate on the 3D Hydrodynamics of eta Carinae's Colliding Winds

At the heart of eta Carinae's spectacular "Homunculus" nebula lies an extremely luminous (L(sub Total) greater than approximately 5 × 10(exp 6) solar luminosity) colliding wind binary with a highly eccentric (e approximately 0.9), 5.54-year orbit (Figure 1). The primary of the system, a Luminous Blue Variable (LBV), is our closest (D approximately 2.3 kpc) and best example of a pre-hypernova or pre-gamma ray burst environment. The remarkably consistent and periodic RXTE X-ray light curve surprisingly showed a major change during the system's last periastron in 2009, with the X-ray minimum being approximately 50% shorter than the minima of the previous two cycles1. Between 1998 and 2011, the strengths of various broad stellar wind emission lines (e.g. Halpha, Fe II) in line-of-sight (l.o.s.) also decreased by factors of 1.5 - 3 relative to the continuum2. The current interpretation for these changes is that they are due to a gradual factor of 2 - 4 drop in the primary's mass-loss rate over the last approximately 15 years1, 2. However, while a secular change is seen for a direct view of the central source, little to no change is seen in profiles at high stellar latitudes or reflected off of the dense, circumbinary material known as the "Weigelt blobs"2, 3. Moreover, model spectra generated with CMFGEN predict that a factor of 2 - 4 drop in the primary's mass-loss rate should lead to huge changes in the observed spectrum, which thus far have not been seen. Here we present results from large- (plus or minus 1620 AU) and small- (plus or minus 162 AU) domain, full 3D smoothed particle hydrodynamics (SPH) simulations of eta Car's massive binary colliding winds for three different primary-star mass-loss rates (2.4, 4.8, and 8.5 × 10(exp -4) solar mass/yr). The goal is to investigate how the mass-loss rate affects the 3D geometry and dynamics of eta Car's optically-thick wind and spatially-extended wind-wind collision (WWC) regions, both of which are known sources of observed X-ray, optical, UV, and near-IR emission and absorption. We use two domain sizes in order to better understand how the primary's mass-loss rate influences the various observables that form at different length scales. The 3D simulations provide information important for helping constrain η Car's recent mass-loss history and future state.

lavestigate↗

NASA NTRS2016

Airborne Lidar for Simultaneous Measurement of Column CO2 and Water Vapor in the Atmosphere

The 2-micron wavelength region is suitable for atmospheric carbon dioxide (CO2) measurements due to the existence of distinct absorption feathers for the gas at this particular wavelength. For more than 20 years, researchers at NASA Langley Research Center (LaRC) have developed several high-energy and high repetition rate 2-micron pulsed lasers. This paper will provide status and details of an airborne 2-micron triple-pulse integrated path differential absorption (IPDA) lidar. The development of this active optical remote sensing IPDA instrument is targeted for measuring both CO2 and water vapor (H2O) in the atmosphere from an airborne platform. This presentation will focus on the advancement of the 2-micron triple-pulse IPDA lidar development. Updates on the state-of-the-art triple-pulse laser transmitter will be presented including the status of seed laser locking, wavelength control, receiver telescope, detection system and data acquisition. Future plans for the IPDA lidar system for ground integration, testing and flight validation will also be presented.

Singh, Upendra N.↗

NASA NTRS2017

A Methane Lidar for Greenhouse Gas Measurements

Atmospheric methane is the second most important greenhouse gas with 25 times the radiativeforcing of carbon dioxide. We will present results from an airborne campaign using a lidar at1.65m using optical parametric generation. OCIS codes: ((280.1910) DIAL, differential absorption lidar; (120.0280) Remote sensing and sensors; (010.1280) Atmospheric composition.

Remote Sensin↗

NASA NTRS2019

Atmospheric Correction for Coastal Waters Based on Multi-Angle Polarimetric Observations

Atmospheric correction is an essential procedure of ocean color remote sensing, which obtains water-leaving signals from satellite or airborne sensors. Due to the small percentage of the water leaving signals in the total measurement, atmospheric correction requires precise evaluation of the radiometric contributions from the aerosol and ocean surface. It is often challenging over coastal waters when absorbing aerosols are present and when water leaving signals in the near infrared spectral region are non-negligible. In this work, we report on a joint retrieval algorithm that determines aerosol and ocean optical properties using the polarimetric measurements based on a coupled atmosphere and ocean radiative transfer model. Two bio-optical models are designed for ocean water properties. One model parameterizes the open ocean optical properties in terms of the concentration of chlorophyll a. The other is a generalized bio-optical model for coastal waters that describes the absorption and scattering by phytoplankton, colored dissolved organic matter and non-algal particles using multiple parameters. We applied the algorithm to the airborne Research Scanning Polarimeter (RSP) measurements acquired over both open and coastal ocean waters. Through the comparisons with in situ ocean color measurements, the flexibility and accuracy of the retrieval algorithm in retrieving aerosol and water leaving radiance properties are demonstrated under various aerosol and ocean water conditions.

Gao, Meng↗

NASA NTRS2022

Global Dust Cycle and Direct Radiative Effect in E3SM Version 1: Impact of Increasing Model Resolution

Quantification of dust aerosols in Earth System Models (ESMs) has important implications for water cycle and biogeochemistry studies. This study examines the global life cycle and direct radiative effects (DREs) of dust in the U.S. Department of Energy's Energy Exascale Earth System Model version 1 (E3SMv1), and the impact of increasing model resolution both horizontally and vertically. The default 1° E3SMv1 captures the spatial and temporal variability in the observed dust aerosol optical depth (DAOD) reasonably well, but overpredicts dust absorption in the shortwave (SW). Simulations underestimate the dust vertical and long-range transport, compared with the satellite dust extinction profiles. After updating dust refractive indices and correcting for a bias in partitioning size-segregated emissions, both SW cooling and longwave (LW) warming of dust simulated by E3SMv1 are increased and agree better with other recent studies. The estimated net dust DRE of −0.42 Wm−2 represents a stronger cooling effect than the observationally based estimate −0.2 Wm−2 (−0.48 to +0.2), due to a smaller LW warming. Constrained by a global mean DAOD, model sensitivity studies of increasing horizontal and vertical resolution show strong influences on the simulated global dust burden and lifetime primarily through the change of dust dry deposition rate; there are also remarkable differences in simulated spatial distributions of DAOD, DRE, and deposition fluxes. Thus, constraining the global DAOD is insufficient for accurate representation of dust climate effects, especially in transitioning to higher- or variable-resolution ESMs. Better observational constraints of dust vertical profiles, dry deposition, size, and LW properties are needed.

dust aerosol↗

NASA NTRS2024

Analyses of the MISSE 9-15 Polymers and Composites Experiment 1-4 (PCE 1-4) Contamination Samples

Spacecraft in low Earth orbit (LEO) are subjected to harsh environmental conditions, including radiation (cosmic rays, ultraviolet (UV), x-ray and charged particle radiation), micrometeoroids and orbital debris, temperature extremes, thermal cycling, and atomic oxygen (AO). These environmental exposures can result in erosion, embrittlement and optical property degradation of susceptible materials threatening spacecraft performance and durability. To increase our understanding of environmental effects such as AO erosion and radiation induced embrittlement of spacecraft materials, NASA Glenn Research Center developed a series of experiments that were flown as part of the Materials International Space Station Experiment (MISSE) missions on the exterior of the International Space Station (ISS). Recently, four Glenn experiments with 365 flight samples were flown on ISS’s MISSE-Flight Facility (MISSE-FF). These experiments are the Polymers and Composites Experiment-1 (PCE-1) flown as part of the MISSE-9 mission, the PCE-2 flown as part of the MISSE-10 mission, the PCE-3 flown as part of the MISSE-12 and MISSE-15 missions, and the PCE-4 flown as part of the MISSE-13 mission. Each of these experiments included passive contamination witness samples in each flight direction for post-flight molecular contamination analyses. A total of 13 contamination flight samples were flown. The post-flight analyses of the PCE 1-4 contamination samples include X-ray Photoelectron Spectroscopy (XPS) analyses (surface and ion sputter depth analyses) and optical properties (total reflectance, total transmittance and solar absorptance). This paper provides results of post-flight analyses of the PCE 1-4 contamination samples and their corresponding control samples. Knowledge of on-orbit contamination is important for the PCE 1-4 flight data interpretation.

Atomic Oxygen↗

NASA NTRSDate not supplied

Manufacturing, Characterization and Terrestrial Passive Radiative Cooling Performance of Nanofibrous PTFR-PEO Composite Thermal Coatings

Passive heat management is desirable in many applications since it can reduce the energy expended for cooling, for example, in buildings and automobiles. Specifically, materials with wavelength-dependent reflectance and emittance can manage incident solar fluxes while enabling passive radiative cooling by thermal emission. This study demonstrates the use of polymeric nanofibers, specifically polytetrafluoroethylene (PTFE) and polyethylene oxide (PEO) composite, as thermal coatings for passive temperature control. Employing the electrospinning fabrication process, we engineer nano and micro-scale fibrous structures, studying the influence of fabrication parameters, such as precursor material concentration and rotating collector speed, on fiber geometry and optical properties. To understand the role of material and fiber geometry on optical performance, we characterize various samples' spectral reflectance, absorptance, and transmittance using spectrophotometers interfaced with integrating spheres. The results show the potential of nanofabricated PTFE-PEO coatings as promising candidates for passive thermal control. We highlight their competitive edge by comparing their solar reflectance and emittance values to existing passive radiative thermal control materials. In essence, this study contributes to advancing passive heat management technologies, offering insights into optimizing material composition and fabrication techniques for enhanced performance in various applications.

Chieloka Ibekwe↗

NASA NTRS1994

Physical processes in eclipsing pulsars: Eclipse mechanisms and diagnostics

We investigate how the radio emission of a pulsar interacts with plasma derived from a stellar companion. Various physical mechanisms that can cause radio pulse eclipse are discussed, and predictions are made for the polarization properties of the emergent radio wave. We consider eclipses by a wind from the stellar companion, by a stellar magnetosphere, or by material entrained in the pulsar wind. Eclipses due to refraction require either a relatively high plasma density or a sharp edge to the plasma distribution. The conditions that must prevail for free-free absorption to be effective in eclipsing a radio beam are also outlined. Pulse smearing may be important at higher frequencies; related eclipse mechanisms include pulse spreading due to a rapidly changing electron column, and scattering by Langmuir turbulence. The high brightness temperature radio beam can generate its own plasma turbulence via a number of nonlinear parametric instabilities, such as the instability associated with stimulated Raman scattering. When the plasma turbulence is heavily damped, the radio bean can still undergo induced Compton scattering. Stimulated scattering effects such as these are very sensitive to the presence of narrow-band substructure in the pulsar radio emission. Finally, we consider the possibility that plasma derived from a stellar companion may mix with the relativistic pulsar wind and cause cyclotron absorption at low radio frequencies. Even if the cyclotron optical depth is small, fluctuations in the emergent polarization of the radio beam on the timescale of a few seconds are a very sensitive probe of the spatial structure of the magnetic field in the pulsar wind. The current observational properties of two known eclipsing pulsar systems, PSR 1957+20 and PSR 1744-24A, are used to construct tentative eclipse models. The favored model for PSR 1957+20 is cyclotron or synchrotron absorption by plasma embedded in the pulsar wind combined with pulse smearing at high frequency, and the favored model for PSR 1744-24A is backscattering off plasma turbulence generated by the stimulated Raman scattering parametric instability. Pulsar eclipses promise to provide a good diagnostic of pulsar winds and possible of the pulse emission mechanism.

Thompson, C.↗

NASA NTRS1994

Modeling the double-trough structure observed in broad absorption line QSOs using radiative acceleration

We present a model explaining the double trough, separated by delta v approximately = 5900 km/s, observed in the C IV lambda-1549 broad absorption line (BAL) in a number of BALQSOs. The model is based on radiative acceleration of the BAL outflow, and the troughs result from modulations in the radiative force. Specifically, where the strong flux from the Lyman-alpha lambda-1215 broad emission line is redshifted to the frequency of the N V lambda-1240 resonance line, in the rest frame of the accelerating N V ions, the acceleration increases and the absorption is reduced. At higher velocities the Lyman-alpha emission is redshifted out of the resonance and the N V ions experience a declining flux which causes the second absorption trough. A strongly nonlinear relationship between changes in the flux and the optical depth in the lines is shown to amplify the expected effect. This model produces double troughs for which the shallowest absorption between the two troughs occurs at v approximately = 5900 km/s. Indeed, we find that a substantial number of the observed objects show this feature. A prediction of the model is that all BALQSOs that show a double-trough signature will be found to have an intrinsic sharp drop in their spectra shortward of approximately 1200 A.

Arav, Nahum↗

NASA NTRS1995

CO and OH absorption toward the low-latitude radio source 2023+336

We report interferometric observations of (12)CO (0 to 1) 115 GHz and OH 1667 MHz absorption toward the extragalactic radio continuum source 2023+336. Our data show two partially blended absorption features near +2 km/s LSR which probably originate in local molecular clouds in the Cygnus rift, approximately 0.7 kpc away. The CO lines are optically thin, with tau(sub CO) = 0.5 +/- 0.1, while tau(sub OH) = 0.030 +/- 0.004. The detected absorption features have a combined velocity width of 3.0 km/s FWHM, greater than the width of the corresponding (12)CO emission features, Full Width of Half Maximum (FWHM) = 2.3 km/s, indicating that the absorbing gas in a approximately 1 AU diameter column shows a greater velocity range than the gas in the 0.2 pc diameter emission beam. CO excitation temperatures T(sub ex), range from 2.7 to 7.0 K across the line profile, implying that the gas along this line of sight is rotationally quite cold. By measuring the (12)CO excitation temperature and optical depth, we derive an abundance ratio, (CO)/(H2), of 6 x 10(exp -6), which is more than an order of magnitude lower than is seen elsewhere. Our low observed CO optical depth is inconsistent with the ratio of (12)CO to (13)CO emission line integrals, 16:1, which implies that the (12)CO is optically thick. As a solution to these anomalies, we propose that the CO absorption and emission arise from preferentially different parts of the molecular medium. Other solutions would require an anomalous (12)CO/(13)CO abundance ratio and an anomalous CO/H2 abundance ratio, or much lower excitation temperatures. Since we find no absorption at negative velocities with tau greater than 0.23 (2.5 sigma), there is no compelling evidence for the existence of an extensive population of cold molecular gas in the outer Galaxy along this line of sight.

Kobulnicky, Henry A.↗

NASA NTRS1981

Optical properties of the crustal aerosol - Relation to chemical and physical characteristics

Crustal aerosol absorption, expressed as a wavelength dependent imaginary index of refraction, n(im), was measured at both visible and infrared wavelengths. Measurements at visible wavelengths show values of n(im) that range from 0.02 at 300 nm to 0.004 to 700 nm. Infrared measurements show an absorption that is dominated by a silicate absorption with a maximum value of n(im) of about 1 near 10 microns. Comparisons of the present measurements with other reported measurements of well-documented crustal aerosols show a great deal of similarity among the measured values. It is shown that these measured optical properties, and the similarities and differences in the measured values, can be understood in terms of mineralogical characteristics of the aerosol and fractionation processes that occur in the generation and transport of these aerosols.

Patterson, E. M.↗

NASA NTRS2005

Bio-Optics of the Chesapeake Bay from Measurements and Radiative Transfer Calculations

We combined detailed bio-optical measurements and radiative transfer (RT) modeling to perform an optical closure experiment for optically complex and biologically productive Chesapeake Bay waters. We used this experiment to evaluate certain assumptions commonly used when modeling bio-optical processes, and to investigate the relative importance of several optical characteristics needed to accurately model and interpret remote sensing ocean-color observations in these Case 2 waters. Direct measurements were made of the magnitude, variability, and spectral characteristics of backscattering and absorption that are critical for accurate parameterizations in satellite bio-optical algorithms and underwater RT simulations. We found that the ratio of backscattering to total scattering in the mid-mesohaline Chesapeake Bay varied considerably depending on particulate loading, distance from land, and mixing processes, and had an average value of 0.0128 at 530 nm. Incorporating information on the magnitude, variability, and spectral characteristics of particulate backscattering into the RT model, rather than using a volume scattering function commonly assumed for turbid waters, was critical to obtaining agreement between RT calculations and measured radiometric quantities. In situ measurements of absorption coefficients need to be corrected for systematic overestimation due to scattering errors, and this correction commonly employs the assumption that absorption by particulate matter at near infrared wavelengths is zero.

Tzortziou, Maria↗

NASA NTRS1993

Optical properties of marine stratocumulus clouds modified by ships

Results are presented of an application of the diffusion domain method to multispectral solar radiation measurements obtained deep within a marine stratocumulus cloud layer modified by pollution from ships. In situ airborne measurements of the relative angular distribution of scattered radiation are compared to known asymptotic expressions for the intensity field deep within an optically thick cloud layer. Analytical expressions relating the ratio of the nadir-to-zenith intensities to surface reflectance, similarity parameter, and scaled optical depth beneath the aircraft flight level are used to analyze measurements obtained with the cloud absorption radiometer mounted on the University of Washington's C-131A research aircraft. It is shown that the total optical thickness of the cloud layer increased in the ship tracks, in contrast to the similarity parameter, which decreased. The decrease in absorption was a direct consequence of the reduction in cloud droplet size that occurred within the ship tracks.

King, Michael D.↗

NASA NTRS2006

Evaluation of Daytime Measurements of Aerosols and Water Vapor made by an Operational Raman Lidar over the Southern Great Plains

Raman lidar water vapor and aerosol extinction profiles acquired during the daytime over the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site in northern Oklahoma (36.606 N, 97.50 W, 315 m) are evaluated using profiles measured by in situ and remote sensing instruments deployed during the May 2003 Aerosol Intensive Operations Period (IOP). The automated algorithms used to derive these profiles from the Raman lidar data were first modified to reduce the adverse effects associated with a general loss of sensitivity of the Raman lidar since early 2002. The Raman lidar water vapor measurements, which are calibrated to match precipitable water vapor (PWV) derived from coincident microwave radiometer (MWR) measurements were, on average, 5-10% (0.3-0.6 g/m(exp 3) higher than the other measurements. Some of this difference is due to out-of-date line parameters that were subsequently updated in the MWR PWV retrievals. The Raman lidar aerosol extinction measurements were, on average, about 0.03 km(exp -1) higher than aerosol measurements derived from airborne Sun photometer measurements of aerosol optical thickness and in situ measurements of aerosol scattering and absorption. This bias, which was about 50% of the mean aerosol extinction measured during this IOP, decreased to about 10% when aerosol extinction comparisons were restricted to aerosol extinction values larger than 0.15 km(exp -1). The lidar measurements of the aerosol extinction/backscatter ratio and airborne Sun photometer measurements of the aerosol optical thickness were used along with in situ measurements of the aerosol size distribution to retrieve estimates of the aerosol single scattering albedo (omega(sub o)) and the effective complex refractive index. Retrieved values of omega(sub o) ranged from (0.91-0.98) and were in generally good agreement with omega(sub o) derived from airborne in situ measurements of scattering and absorption. Elevated aerosol layers located between about 2.6 and 3.6 km were observed by the Raman lidar on May 25 and May 27. The airborne measurements and lidar retrievals indicated that these layers, which were likely smoke produced by Siberian forest fires, were primarily composed of relatively large particles (r(sub eff) approximately 0.23 micrometers), and that the layers were relatively nonabsorbing (omega(sub o) approximately 0.96-0.98). Preliminary results show that major modifications that were made to the Raman lidar system during 2004 have dramatically improved the sensitivity in the aerosol and water vapor channels and reduced random errors in the aerosol scattering ratio and water vapor retrievals by an order of magnitude.

Ferrare, Richard↗

NASA NTRS1991

The composition of Phobos: Meteorite analogs based on KRFM and VSK spectral data from the Phobos 2 spacecraft

In 1989 the Phobos 2 spacecraft obtained 8-channel 0.3 to 0.6 mm KRFM spectra and two-channel wide-angel TV VSK images in bandpasses of 0.40 to 0.56 mm and 0.78 to 1.10 mm. The TV data were used to map four color ratio units on disk-resolved images of Phobos, and were combined with the KRFM spectra to analyze possible meteorite analogs for the mapped units. A total of 58 spectra of 39 meteorites were studied for similarities with Phobos data in spectral shape, absorption features, and visible near-IR color ratio. Analysis of the spectral data show that, among the meteorites studied, there are no unique spectral analogs for Phobos surface material. Currently, the closest spectral analogs are the optically altered black chondrite meteorites Gorlovka and Pervomaisky. The weak UV absorption bands in some KRFM spectra and the red slope in VSK color-ratio data indicate that carbonaceous chondrite-like material may also be a component of Phobos surface material. However, the lack of close carbonaceous chondrite spectral analogs and the existence of apparent absorption bands in KRFM spectra that are not seen in meteorite spectra suggest that there are processes and/or materials on the surface of Phobos that are not represented in the meteorite collections. The similarities between KRFM spectra of Phobos and the spectra of black chondrites suggest that optically altered mafic silicates may constitute a component of the surface material of Phobos, and that optical alteration and mixing by regolith processes may be an important factor in the evolution of Phobos surface material.

Britt, D. T.↗

NASA NTRS2006

Remote Sensing Reflectance and Inherent Optical Properties in the Mid-mesohaline Chesapeake Bay

We used an extensive set of bio-optical data and radiative transfer (RT) model simulations of radiation fields to investigate relationships between inherent optical properties and remotely sensed quantities in the optically complex, mid-mesohaline Chesapeake Bay waters. Field observations showed that the chlorophyll algorithms used by the MODIS (MODerate resolution Imaging Spectroradiometer) ocean color sensor (i.e. Chlor_a, chlor_MODIS, chlor_a_3 products) do not perform accurately in these Case 2 waters. This is because, when applied to waters with high concentrations of chlorophyll, all MODIS algorithms are based on empirical relationships between chlorophyll concentration and blue-green wavelength remote sensing reflectance (Rrs) ratios that do not account for the typically strong blue-wavelength absorption by non-covarying, dissolved and non-algal particulate components. Stronger correlation was observed between chlorophyll concentration and Rrs ratios in the red (i.e. Rrs(677)/Rrs(554)) where dissolved and non-algal particulate absorption become exponentially smaller. Regionally-specific algorithms that are based on the phytoplankton optical properties in the red wavelength region provide a better basis for satellite monitoring of phytoplankton blooms in these Case 2 waters. Good optical closure was obtained between independently measured Rrs spectra and the optical properties of backscattering, b(sub b), and absorption, a, over the wide range of in-water conditions observed in the Chesapeake Bay. Observed variability in the quantity f/Q (proportionality factor in the relationship between Rrs and the water inherent optical properties ratio b(sub b)/(a+b(sub b)) was consistent with RT model calculations for the specific measurement geometry and water bio-optical characteristics. Data and model results showed that f/Q values in these Case 2 coastal waters are not considerably different from those estimated in previous studies for Case 1 waters. Variation in surface backscattering significantly affected Rrs magnitude across the visible spectrum and was most strongly correlated (R(sup 2)=0.88) with observed variability in Rrs at 670 nm. Surface values of particulate backscattering were strongly correlated with non-algal particulate absorption, a(sub nap), in the blue wavelengths (R(sup 2)=0.83). These results, along with the measured values of backscattering fraction magnitude and non-algal particulate absorption spectral slope, suggest that suspended non-algal particles with high inorganic content are the major water constituents regulating b(sub b) variability in the mid-mesohaline Chesapeake Bay. Remote retrieval of surface b(sub b) and (a(sub nap), from Rrs(670) can be used in regionally-specific satellite algorithms to separate contribution by non-algal particles and dissolved organic matter to total light absorption in the blue, and monitor non-algal suspended particle concentration and distribution in these Case 2 waters.

Tzortziou, Maria↗

NASA NTRS1983

A survey of laser and selected optical systems for remote measurement of pollutant gas concentrations

Applications of the Differential Absorption Lidar (DIAL) technique to the remote sensing of pollutant gases are surveyed. In the DIAl technique, the differential absorption of two laser beams reflected back to a receiver from a target determines the concentration of the gas being studied. The types of instruments available are considered in detail: dye lidar (to measure nitrogen dioxide, sulfur dioxide, and ozone); carbon dioxide laser (for ozone, ethylene, ammonia, and hydrazine), helium-neon laser (for methane); hydrogen fluoride laser (for HF); and tunable diode laser (for nitric oxide and carbon monoxide). DIAL instruments are compared with other optical remote sensors such as Fourier-transform infrared spectrometers, correlation spectrometers (COSPEC and GASPEC), and grating spectrometers; and criteria for the selection of an appropriate gas measuring system are suggested. Laser and other optical remote sensors are found to be cost effective in many cases, despite the fact that they are more costly than point-monitoring systems.

Grant, W. B.↗