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At least 919 records · Page 51

Energy transfer mechanisms between molecules

Reliable rate coefficients for energy transfer and relaxation phenomena are needed in order to do the theoretical modeling which is necessary for accomplishing the following objectives: understanding and justifying proposed laser systems, determining limitations, identifying control parameters, and scaling to space-power requirements. Modeling also establishes the criteria to be followed for lasant selection. Lack of knowledge of rate coefficients is invariably the biggest obstacle to successful modeling. Existing theoretical methods are discussed, sources of error are identified, and transfer laser criteria suggested by the theory are listed. The emphasis is on vibrational-vibrational (V-V) energy transfer caused by both short range and long range interactions between molecules. Special attention is given to the importance of near-resonant collisional and dipole-dipole transfer. A technique is proposed for significantly improving the theoretical predictions of rate coefficients.

Meador, W. E.↗

Space-and Ground-Based Non-Accelerated Long Lifetime Data for Ruggedized Commercial Non-Planar Ring Oscillator (NPRO) Lasers

Lifetime data is presented for ruggedized commercial NPRO lasers used in the Tropospheric Emission Spectrometer (TES) Instrument on NASA’s Aura Earth-orbiting spacecraft, including 20 years of data from two life test units on the ground, 12 years of on-orbit data from TES Laser A, and 2 years of on-orbit data from TES Laser B. The TES lasers are diode-pumped Non-Planar Ring Oscillator (NPRO) lasers using Nd:YAG crystals. Since accelerated life testing was not possible on the complete laser, early prototype lasers that had gone through thermal cycling and vibration testing were placed on non-accelerated life tests with the hope of gathering at least a couple of years of data before launch. Long-term lifetime data for hybrid laser systems in space applications is not abundant, and out of necessity, accelerated reliability testing is usually done over a relatively short time with a large number of devices. The data presented in this paper is unique as it tracks the optical power output over time of a total of four lasers on the order of decades rather than months or years. Two of the lasers have each been on life test for over 20 years on the ground and are still operating, and the other two lasers have been on-orbit for 14 years. TES Laser A was still operating when the TES Instrument was decommissioned in January 2018. Therefore, the data presented covers over 450,000 non-accelerated device-hours, with 23% of those hours being in space.

Kane, T.J.↗

Laser-Based Means for Accelerating Nuclear Decay Rate

This project aims to replicate and build upon a reported series of results whereby nuclear decay of unstable species has been accelerated under laser irradiation in the presence of resonantly excited plasmonic nanoparticles. We are currently utilizing a laser system similar to that used within these reports as well as optimizing nanoparticle solution environments in an attempt to replicate reported results or provide alternative pathways that may explain some perceived discrepancies. The current work is being performed with equipment and techniques currently available at SRNL, including nanoparticle synthesis and pulsed lasers for plasmon excitation. The results of these experiments could provide quantitative data that can be used to resolve the discrepancies in the calculations and better estimate the ultimate utility of the process. If verified, this would represent a pathway for using readily available and scalable technology to reduce the long-term radiological storage requirements of certain forms of nuclear waste.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

LaserNetUS. Final report

In this proposal we have formed a consortium in response to a request from the DoE Office of Fusion Energy Sciences to establish a national network of Petawatt-class laser systems to act as domestic user facilities that can enable a broad range of frontier scientific research. This new entity is called LaserNet US. The network formed here is directly responsive to recommendations made in a recently released National Academy of Sciences Report with regard to US strategy for high intensity laser research, “Opportunities in Intense Ultrafast Lasers: Reaching for the Brightest Light”. As detailed in this report, the research in this area has the potential to transform science in a number of research fields and to open up new areas of fundamental research. High field science was initiated in the US in the 1990’s, and subsequently Europe and Asia have embraced this research field, investing more than a billion dollars in this area over the past several years. Our network includes five academic and two national lab-based high intensity laser facilities. These facilities are distributed geographically throughout the US and the network provides access to complementary facilities which have unique world-class laser and experimental capabilities. LaserNet US will make these existing Petawatt-class laser facilities available to users from around the country who until now have not had regular access to such machines. Consequently, the network, which will develop over time, will also become a key element in driving forward national research in high field and high energy density plasma science. In particular, the University of Michigan provides access to the Hercules laser facility and the T-cubed laser facility for collaborative experiments as part of the first year operation. In the second year - to begin in summer 2019 - the experiments will be chosen via proposal submission and review by an outside panel formed by DOE.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Lamp pumped Nd:YAG laser. Space-qualifiable Nd:YAG laser for optical communications

Results are given of a program concerned with the design, fabrication, and evaluation of alkali pump lamps for eventual use in a space qualified Nd:YAG laser system. The study included evaluation of 2mm through 6mm bore devices. Primary emphasis was placed upon the optimization of the 4mm bore lamp and later on the 6mm bore lamp. As part of this effort, reference was made to the Sylvania work concerned with the theoretical modeling of the Nd:YAG laser. With the knowledge gained, a projection of laser performance was made based upon realistic lamp parameters which should easily be achieved during following developmental efforts. Measurements were made on the lamp performance both in and out of the cavity configuration. One significant observation was that for a constant vapor pressure device, the spectral and fluorescent output did not vary for vacuum or argon environment. Therefore, the laser can be operated in an inert environment (eg. argon) with no degradation in output. Laser output of 3.26 watts at 430 watts input was obtained for an optimized 4mm bore lamp.

Ward, K. B.↗

Single event effects and laser simulation studies

The single event upset (SEU) linear energy transfer threshold (LETTH) of radiation hardened 64K Static Random Access Memories (SRAM's) was measured with a picosecond pulsed dye laser system. These results were compared with standard heavy ion accelerator (Brookhaven National Laboratory (BNL)) measurements of the same SRAM's. With heavy ions, the LETTH of the Honeywell HC6364 was 27 MeV-sq cm/mg at 125 C compared with a value of 24 MeV-sq cm/mg obtained with the laser. In the case of the second type of 64K SRAM, the IBM640lCRH no upsets were observed at 125 C with the highest LET ions used at BNL. In contrast, the pulsed dye laser tests indicated a value of 90 MeV-sq cm/mg at room temperature for the SEU-hardened IBM SRAM. No latchups or multiple SEU's were observed on any of the SRAM's even under worst case conditions. The results of this study suggest that the laser can be used as an inexpensive laboratory SEU prescreen tool in certain cases.

Kim, Q.↗

Geometric bias and time coincidence in 3-dimensional laser Doppler velocimeter systems

The measurement by a three-dimensional laser Doppler velocimeter of a turbulent flow has been numerically simulated. Errors associated with the probe volume geometry and the coincidence time window concept are revealed. One type of error occurs for high system data rates when multiple particles lead to system realizations. Another error occurs associated with a geometric bias discovered in the present study. This three-dimensional ldv geometric bias exists even for single-particle realizations and regardless of the system data rate. A technique for the elimination of the geometric bias is presented.

Brown, J. L.↗

Tracking and data acquisition system for the 1990's. Volume 8: TDAS frequency planning

Current planning calls for the TDAS to support new user and crosslink services, in addition to TDRSS-compatible services. TDRSS-compatible services would operate in current S-band and K-band channels used by TDRSS. New services, however, can take advantage of technology advances at microwave and optical frequencies. For augmented space-to-space services, 60 GHz and GaAs laser systems offer technical advantages, relative freedom from RFI, and a benign regulatory environment (i.e., minimal congestion and, in the case of 60 GHz, maximum regulatory support for TDAS-type services). For TDAS Earth-to-space and space-to-Earth services, the 30/20 GHz band offers the best mix of technical and regulatory advantages. But use of these bands would have to be coordinated with the U.S. military.

Heppe, S. B.↗

Performance Improvements to the Lidar Atmospheric Sensing Experiment (LASE)

Lidar Atmospheric Sensing Experiment (LASE) is the first fully-engineered, modular, tunable, autonomous Differential Absorption Lidar (DIAL) system for the remote measurement of water vapor, aerosols and clouds across the troposphere. It was designed, built and environmentally tested at LARC. LASE was designed to fly aboard a NASA/Ames ER-2 aircraft (NASA's high altitude aircraft) and operate at altitudes from 58,000 to 70,000 feet. Since its first flight on May 11, 1994, it has flown 28 total missions on board the ER-2. LASE has been validated with results showing an accuracy better than the initial requirement for vertical profiles of water vapor in the troposphere. LASE can also deploy on several other aircraft including the NASA P-3 and will fly aboard the NASA DC-8 during the Convection And Moisture EXperiment (CAMEX) in July-September 1998. The tunable laser system of LASE was designed to operate in a double-pulse mode at 5Hz, with energy outputs of up to 15OmJ per pulse in the 813 to 819nm wavelength region and with 99% of the output energy within a spectral interval of 1.06 pm. Sixteen wavelengths were selected to cover the various water vapor absorption cross sections needed for the DIAL measurement. The Ti:Sapphire laser was constructed using a frequency-doubled Nd:YAG laser as the pump source and a single mode diode laser as a injection seeder for the Ti:Al2O3 laser. We have improved the LASE instrument in several important ways. Improvements to the seed source have demonstrated that DFB laser diodes can be used as reliable seed sources on airborne DIAL instruments. The DFB diode has enabled LASE to gather more data and significantly reduced the maintenance required to insure that the system performance requirements are met. The multiwavelength sequential seeding technique is the current method of data collection for LASE. It has the advantages of providing an entire atmospheric coverage of H2O(v) from the ground to the aircraft altitude along a single ground track. The development of a flight deployable system to measure spectral purity will insure that the LASE instrument or any future flight based DIAL system can meet the performance specifications to insure data accuracy.

Edwards, W. C.↗

Longitudinal tapering in gas jets for increased efficiency of 10-GeV class laser plasma accelerators

Modern laser plasma accelerators often require plasma waveguides tens of centimeters long to propagate a high-intensity drive laser pulse. Tapering the longitudinal gas density profile in 10 cm scale gas jets could allow for single stage laser plasma acceleration well beyond 10 GeV with current petawatt-class laser systems. Via simulation and interferometry measurements, we show density control by longitudinally adjusting the throat width and jet angle. Density profiles appropriate for tapering were calculated analytically and via particle-in-cell simulations and were matched experimentally. Further, these simulations show that tapering can increase electron beam energy using 19 J laser energy from ∼9 GeV to > 12 GeV in a 30 cm plasma and the accelerated charge by an order of magnitude.

43 PARTICLE ACCELERATORS↗

Polar motion

Tracking of the Beacon Explorer-C satellite by a precision laser system was used to measure the polar motion and solid earth tide. The tidal perturbation of satellite latitude is plotted as variation in maximum latitude in seconds of arc on earth's surface as a function of the date, and polar motion is shown by plotting the variation in latitude of the laser in seconds of arc along the earth's surface as a function of date

Kolenkiewicz, R.↗

Understanding spectral dependance of laser-induced damage precursors in dielectric materials (Abbreviated report_23-ERD-006)

High peak and average power laser systems are typically limited by the handling fluence of the optical components. In particular, the multilayer dielectric coatings are known to be much lower operational fluence than the more ideal bulk materials. In this project we proposed and succeeded in probing different established classes of damage prone precursors at different wavelengths to understand their fundamental laser damage response as a function of wavelength. This study helped to shed light on the fundamental physics of the non-linear precursors that govern laser damage phenomena for ns-regime pulsed laser damage. In this study, we utilized the onsite coating capabilities (VPL, IBS coating lab) to purposefully generate laser damage-prone precursors in hafnia-based coatings (both single and multi-layer coatings). Specifically, we engineered coatings with craze lines initiated by nodules, generated coatings with our xenon-based coating process to suppress nanobubble formation and generated hafnia coatings under controlled oxygen flow conditions to study hafnia sub-oxides and oxygen flow dependance. In these studies we found that craze lines are rife with precursors that are sensitive to ultra-violet light but not to infrared light; we found that the removal of nanobubbles helps with all wavelengths tested, but is most impactful for ultra-violet light; we also found that ultra-violet laser damage performance of hafnia is closely matched to oxygen flow rate, while the infrared performance may be slightly better at lower flow rates. During this LDRD we also successfully stood up a new laser damage testing capability, namely a wavelength agile damage test station to study the spectral response of known laser-induced damage precursors. This is a unique and important capability for Lawrence Livermore National Lab, allowing us to understand the spectral response of materials under high intensity irradiation and damage. This is a vital tool to understand non-linear optical response at wavelengths that we have previously been unable to test at.

36 MATERIALS SCIENCE↗

Optimization of the catalytic oxidation of CO for closed-cycle CO2 laser applications

This report develops a basis for the design of a catalyst bed for the recombination of CO and O2 in a closed-cycle CO2 laser system. The catalyst is 1% Pt on SnO2 having a BET surface area of 6.7 sq m/g and a specific void volume of 0.374 cu cm/g. The design conditions are: a catalyst bed temperature of 100 C and a circulating flow rate of 10 lambda/min. Under these conditions, the required quantity of catalyst for prolonged laser operation of 668g. The rat law for the reaction of a stoichiometric mixture of 1% CO + 1/2% O2 in helium was determined to be overall first order; however, additional experiments with non-stoichiometric gas mixtures of CO and O2 are needed to determine the order of the CO concentration and the order of the O2 concentration in the rate law.

Miller, I. M.↗

Toward direct spatial and intensity characterization of ultra-high-intensity laser pulses using ponderomotive scattering of free electrons

Spatial distributions of electrons ionized and scattered from ultra-low-pressure gases are proposed and experimentally demonstrated as a method to directly measure the intensity of an ultra-high-intensity laser pulse. Analytic models relating the peak scattered electron energy to the peak laser intensity are derived and compared to paraxial Runge–Kutta simulations highlighting two models suitable for describing electrons scattered from weakly paraxial beams (f#>5) for intensities in the range of 1018−1021 W cm−2. Scattering energies are shown to be dependent on gas species, emphasizing the need for specific gases for given intensity ranges. Direct measurements of the laser intensity at full power of two laser systems are demonstrated, both showing a good agreement between indirect methods of intensity measurement and the proposed method. One experiment exhibited the role of spatial aberrations in the scattered electron distribution, motivating a qualitative study on the effect. We propose the use of convolutional neural networks as a method for extracting quantitative information on the spatial structure of the laser at full power. We believe the presented technique to be a powerful tool that can be immediately implemented in many high-power laser facilities worldwide.

47 OTHER INSTRUMENTATION↗

Performance of the Linear Ion Trap Mass Spectrometer for the Mars Organic Molecule Analyzer (MOMA) Investigation on the 2018 Exomars Rover

The 2018 ExoMars rover mission includes the Mars Organic Molecule Analyzer (MOMA) investigation. MOMA will examine the chemical composition of samples acquired from depths of up to two meters below the martian surface, where organics may be protected from degradation derived from cosmic radiation and/or oxidative chemical reactions. When combined with the complement of instruments in the rover's Pasteur Payload, MOMA has the potential to reveal the presence of a wide range of organics preserved in a variety of mineralogical environments, and to begin to understand the structural character and potential origin of those compounds. The MOMA investigation is led by the Max Planck Institute for Solar System Research (MPS) with the mass spectrometer subsystem provided by NASA GSFC. MOMA's linear ion trap mass spectrometer (ITMS) is designed to analyze molecular composition of: (i) gas evolved from pyrolyzed powder samples and separated in a gas chromatograph; and, (ii) ions directly desorbed from crushed solid samples at Mars ambient pressure, as enabled by a pulsed UV laser system, fast-actuating aperture valve and capillary ion inlet. Breadboard ITMS and associated electronics have been advanced to high end-to-end fidelity in preparation for flight hardware delivery to Germany in 2015.

linear ion trap mass spectrometer↗

Tunable Laser-Plasma Amplifier (Final Report)

Exploration at the laser intensity frontier has always offered new avenues for physics and reaching beyond this frontier is a grand challenge. Present-day petawatt-class lasers provide focused intensities on target of 10 22 W/cm 2 , corresponding to electric fields of 200 TV/m, while laser-plasma amplification opens a route for focused intensities well above 10 23 W/cm 2 . Intensities in this range provide the ability to test quantum electrodynamics in the unexplored low-energy, strong-field regime where signatures for new physics may arise. The behavior of matter under such extraordinary conditions is a rich and fascinating subject, not only in its own right in fundamental plasma physics, but for the many potential applications that promise to enrich the natural sciences in the future, including compact electron-beam, ion-beam particle accelerators, and ultra-bright X-ray sources. Although laser systems are now under construction internationally to access intensities of 10 23 W/cm 2 , the current technologies used appear to be fundamentally limited to these intensities. The realization of intensities beyond 10 23 W/cm 2 using parametric amplification in plasmas promises a breakthrough in high-energy density physics. Parametric amplification using Raman scattering in a plasma could provide the enabling technology for the generation of ultra-high-power laser pulses, but a more complete understanding of the nonlinear optics of plasmas is required. There is a significant gap in well-diagnosed laser-plasma instability studies of nonlinear plasma-wave phenomena, which are critical to understand for future laser-plasma devices. To achieve an efficient laser-plasma amplifier, plasma waves must be driven to large amplitude where significant energy can be rapidly transferred from the pump to the seed over the pulse duration of the seed. Simulations suggest that this nonlinear pump depletion regime can be achieved in the “pi-pulse” amplification regime. While simulations show this optimal regime with efficient amplification, it has remained elusive in experiments and there is a growing consensus within the community that thermal effects and pump beam limitations prevent laser-plasma amplifiers from progressing through the linear regime into the nonlinear pump depletion regime. Previous experiments have been significantly limited by the laser power available at the necessary wavelengths for the seed laser; therefore, the amplification is required to start in the linear regime where it is sensitive to many deleterious effects. The enabling technology (currently unique to plasma-wave amplification in the world) at the University of Rochester is the ability to provide a seed pulse with sufficient power (4 mJ/100 fs seed) to immediately drive nonlinear plasma waves into the pi-pulse regime and to tune its wavelength to optimize the efficiency of energy transfer. This in combination with the state-of-the-art OMEGA heater beams providing multiple kilojoules in a nanosecond to sufficiently heat the plasma make this system distinct from previous studies. These heater beams will provide, for the first time in Raman amplification studies, a homogeneous electron temperature high enough to prevent pump beam propagation issues that have plagued previous experiments. These systems will provide a platform for driving electron-plasma waves into the nonlinear regime where pump depletion and pulse shortening are predicted to lead to high amplification efficiencies (>30%). The Team has made significant progress through prior support from DOE Fusion Energy Sciences [DOE Office of Science Award Number DE-SC0016253 (2016-2022)]. This includes twenty-two peer-reviewed manuscripts, one patent, ten contributed talks presented at international conferences, and research that was highlighted as invited talks at fifteen international conferences. The broader impacts of this research are evident in the support of early career scientists, two Ph.D. theses, four current graduate students, a Masters Project, two undergraduate researchers, and an underrepresented minority student hired through the California Alliance for Minority Participation who now works as a Research Engineer in the group. This research met all of the funded research objectives and the highlights from primary Raman amplification thrust of this work are discussed below and form the foundation for the proposed research.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Simulation of Direct-Drive Hybrid Using Two Opposed Beams for Inertial Fusion Energy

Xcimer Energy is working to deliver high levels of laser light at the costs required for applications in fusion energy. The architecture of their integrated laser system is unique, in that it naturally supports a target which is illuminated by two opposed beams, and in a manner that can readily complement a reactor. This INFUSE proposal was submitted to investigate a target concept termed the Direct-Drive Hybrid or DDH, and make special use of radiation hydrodynamic simulations and expertise available to the Laboratory for Laser Energetics. The associated capabilities are unique to the field, and take great advantage of investments and advances made by the DOE and DOD over many decades. The primary goals were to stand up the DDH design in calculations for the first time, study and refine the concept, and provide the scientific basis for understanding and projecting proposals by Xcimer Energy. The main accomplishments have been summarized below.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Advanced laser stratospheric monitoring systems analyses

This report describes the software support supplied by Systems and Applied Sciences Corporation for the study of Advanced Laser Stratospheric Monitoring Systems Analyses under contract No. NAS1-15806. This report discusses improvements to the Langley spectroscopic data base, development of LHS instrument control software and data analyses and validation software. The effect of diurnal variations on the retrieved concentrations of NO, NO2 and C L O from a space and balloon borne measurement platform are discussed along with the selection of optimum IF channels for sensing stratospheric species from space.

Larsen, J. C.↗