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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 919 records · Page 51
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Tune compensation in nearly scaling fixed field alternating gradient accelerators

In this paper, we investigate the stability of the particle trajectories in fixed field alternating gradient accelerators (FFAs) in the presence of field errors. The emphasis is on the scaling radial sector FFA type: A collaboration work is ongoing in view of better understanding the properties of the 150 MeV scaling FFA at Kyoto University Institute for Integrated Radiation and Nuclear Science in Japan and progress toward high-intensity operation. Analysis of certain types of field imperfections revealed some interesting features that required the development of an analytical model based on the scalloping angle of the orbits. This helped explain some of the experimental results as well as generalize the concept of a scaling FFA to a nonscaling one for which the tune variations obey a well-defined law. Based on this, a compensation scheme of tune variations in imperfect scaling FFAs is presented. This is the cornerstone of a novel concept of a fixed tune FFA in which the scaling is not achieved at every azimuthal position of the ring but rather in an average sense.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Improved determination of the 𝛽−‾‾𝜈𝑒 angular correlation coefficient 𝑎 in free neutron decay with the 𝑎⁢SPECT spectrometer

We report on a precise measurement of the electron-antineutrino angular correlation (𝑎 coefficient) in free neutron beta decay from the 𝑎⁢SPECT experiment. The 𝑎 coefficient is inferred from the recoil energy spectrum of the protons which are detected in 4⁢𝜋 by the 𝑎⁢SPECT spectrometer using magnetic adiabatic collimation with an electrostatic filter. Data are presented from a 100-day run at the Institut Laue Langevin in 2013. The sources of systematic errors are considered and included in the final result. We obtain 𝑎=−0.10430⁢(84) which is the most precise measurement of the neutron 𝑎 coefficient to date. From this, the ratio of axial vector to vector coupling constants is derived giving |𝜆|=1.2677⁢(28).

Beck, Marcus↗
DOE OSTI2020

Constraining the destruction rate of K 40 in stellar nucleosynthesis through the study of the Ar 40 ( p , n ) K 40 reaction

Background: We present that K 40 plays a significant role in the radiogenic heating of Earth-like exoplanets, which can affect the development of a habitable environment on their surfaces. The initial amount of K 40 in the interior of these planets depends on the composition of the interstellar clouds from which they formed. Within this context, nuclear reactions that regulate the production of K 40 during stellar evolution can play a critical role. Purpose: In this study, we constrain for the first time the astrophysical reaction rate of K 40 ( n , p ) Ar 40 , which is responsible for the destruction of K 40 during stellar nucleosynthesis. We provide to the nuclear physics community high-resolution data on the cross section and angular distribution of the Ar 40 ( p , n ) K 40 reaction. These are important to various applications involving Ar 40 . The associated reaction rate of the Ar 40 ( p , n ) K 40 process addresses a reaction rate gap in the Joint Institute for Nuclear Astrophysics REACLIB database in the region of intermediate-mass isotopes. Methods: We performed differential cross-section measurements on the Ar 40 ( p , n ) K 40 reaction, for six energies in the center-of-mass system between 3.2 and 4.0 MeV and various angles between 0 ° and 135 ° . The experiment took place at the Edwards Accelerator Laboratory at Ohio University using the beam swinger target location and a standard neutron time-of-flight technique. We extracted total and partial cross sections by integrating the double differential cross sections we measured. Results: The total and partial cross sections varied with energy due to the contribution from isobaric analog states and Ericson type fluctuations. The energy-averaged neutron angular distributions were symmetrical relative to 90 ° . Based on the experimental data, local transmission coefficients were extracted and were used to calculate the astrophysical reaction rates of Ar 40 ( p , n ) K 40 and K 40 ( n , p ) Ar 40 reactions. The new rates were found to vary significantly from the theoretical rates in the REACLIB library. We implemented the new rates in network calculations to study nucleosynthesis via the slow neutron capture process, and we found that the produced abundance of K 40 is reduced by up to 10% compared to calculations with the library rates. At the same time, the above result removes a significant portion of the previous theoretical uncertainty on the K 40 yields from stellar evolution calculations. Conclusions: Our results support a destruction rate of K 40 in massive stars via the K 40 ( n , p ) Ar 40 reaction that is larger compared to previous estimates. The rate of K 40 destruction via the K 40 ( n , p ) Ar 40 reaction now has a dramatically reduced uncertainty based on our measurement. Lastly, this result directly affects the predicted stellar yields of K 40 from nucleosynthesis, which is a critical input parameter for the galactic chemical evolution models that are currently employed for the study of significant properties of exoplanets.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Consistency of nucleon-transfer sum rules in well-deformed nuclei

Here, nucleon-transfer sum rules have been assessed via a consistent reanalysis of cross-section data from neutron-adding (d, p) and -removing (d, t) reactions on well-deformed isotopes of Gd, Dy, Er, Yb, and W, with 92 ≤ N ≤ 108 , studied at the Niels Bohr Institute in the 1960s and 1970s. These are complemented by new measurements of cross sections using the (d, p), (d, t), and (p, d) reactions on a subset of these nuclei. The sum rules, defined in a Nilsson-model framework, are remarkably consistent. A single overall normalization is used in the analysis, which appears to be sensitive to assumptions about the reaction mechanism, and in the case of sums using the (d, t) reaction, differs from values determined from reactions on spherical systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Structure of even-even Sr isotopes with 50 ≤ N ≤ 58 neutrons

Excited levels in Sr 90 , Sr 92 , Sr 94 , and Sr 96 nuclei were reinvestigated using high-statistics multiple- γ coincidence data from neutron-induced fission of U 235 and spontaneous fission of Cf 252 , measured using Exogam at Institut Laue Langevin and Gammasphere arrays, respectively. The experimental goal was the search for new excited levels and firm spin-parity assignments to known levels. A total of 23 new levels with 30 new or corrected decays and 39 new or improved spin-parity assignments were obtained in the four nuclei. Negative-parity structures on top of 3 - excitation were firmly identified and extended to higher spins. New positive-parity structures in Sr 94 and Sr 96 were observed with 3 + excitations characteristic of γ collectivity. The 277.7-keV, E 2 decay from the 1507.0-keV level to the second 0 + level in Sr 96 , found in this paper, completes the coexisting deformed band in this nucleus. To learn about the microscopic structure of levels in the Sr 88 - 96 nuclei, we performed large-scale shell-model calculations. The calculations compared to the experiment, helped the discussion of the evolution of collectivity in strontium isotopes, highlighting the important role of various single-particle excitations in phase transitions and shape coexistence in the region. The special role of the neutron 9 / 2 + [ 404 ] extruder as a catalyst of the deformation change in the region is highlighted.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Developing the S 32 ( p , d ) S * 31 ( p ) ( γ ) reaction to probe the P 30 ( p , γ ) S 31 reaction rate in classical novae

Background: The 30 P(p,γ) 31 S reaction rate is one of the largest remaining sources of uncertainty in the final abundances of nuclei created in a classical nova involving a ONe white dwarf. The reaction rate directly influences silicon isotopic ratios, which are used as identifiers of presolar grains with nova origins. Additionally, the uncertainty in the 30 P(p,γ) 31 S reaction rate has been found to limit the use of nova nuclear thermometers based on observations of elemental ratios in nova ejecta. Purpose: Reduce uncertainties in the nuclear data for proton-unbound states in 31 S, which act as resonances for the 30 P(p,γ) 31 S reaction at classical nova temperatures, and develop a technique for high efficiency, high-resolution reaction-decay coincidence measurements. Methods: Here, the 32 S(p,d) 31 S reaction was used to populate the states of interest in 31 S. The experiment was performed at the Texas A&M Cyclotron Institute using the LLNL Hyperion array for the detection of charged particles and γ rays. A downstream silicon telescope was used to select reaction deuterons, and a single upstream silicon detector was used to measure protons emitted in the decay of unbound 31 S levels. Results: Several states in 31 S above the proton separation energy were observed to have been populated. Decay protons from the resonant states in 31 S were identified as events in the upstream silicon detectors that came in coincidence with deuterons in the downstream telescope. Protons emitted from these states were measured and branching ratios extracted. Conclusions: While no new reaction rate is derived, spin-parity assignments for several higher-lying proton unbound states have been confirmed. Measured p 0 branching ratios for these levels have been compared to previous measurements with good agreement, and in some cases provided a reduction in uncertainty. The previously identified T = 3/2 state may have been incorrectly assigned a large p 0 branching ratio in a previous measurement. The technique of measuring reaction-decay coincidences with a particle-gamma setup appears promising.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

β -delayed charged-particle decay of Si 22 , 23

The β decay of 22,23 Si by emission of delayed charged particles was investigated in an experiment at the Cyclotron Institute of Texas A&M University by means of an optical-readout time-projection chamber. The previously-known decay of the two isotopes by β-delayed one- and two-proton emission was confirmed. Here for the first time, a new, rare, decay mode for 23 Si, β-delayed three-proton emission, was observed and β-delayed proton-α emission tentatively identified. Moreover, the β-decay pattern for the ground state of 23 Si was studied by means of multireference density-functional-rooted calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Investigating the time dependence of neutron-proton equilibration using molecular dynamics simulations

Neutron-proton equilibration has previously been studied experimentally in dynamically deformed nuclei in heavy ion collisions [Phys. Rev. Lett. 118, 062501 (2017); Phys. Rev. C 95, 044604 (2017)] using the NIMROD detector array at the Cyclotron Institute at Texas A&M University. Results indicated the composition of the two heaviest fragments originating from the excited projectile-like fragment evolved exponential with respect to their orientation angle to be more similar. Constrained Molecular Dynamics and Antisymmetrized Molecular Dynamics simulations were performed for different formulations of the density dependence of the asymmetry energy term of the nuclear equation of state. The simulations are compared to experimental results, which indicate a better agreement with a softer interaction in the nuclear equation of state.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Examination of decay heat measurements and their relevance for understanding the origin of the reactor antineutrino anomaly

Measurements of the decay energy released as a function of time following the thermal neutron induced fission of 235 U and 239,241 Pu were performed in the 1970s at Oak Ridge National Laboratory with the purpose of quantifying possible loss of coolant accident scenarios. The derivative of this decay energy with respect to time, known in technical parlance as decay heat, is mainly composed of two terms, that of the electrons produced together with antineutrinos in the $β$-minus decay of the neutron-rich fission products, and that of the $γ$ rays produced in the subsequent decay of excited nuclear levels. In this work we study if this extensive set of decay energy measurements can be used to assess the reactor antineutrino anomaly, that is, the approximately 5% deficit of electron antineutrinos produced by nuclear reactors, first deduced by Mention and collaborators in 2011, and observed by the major reactor antineutrino experiments since. Furthermore, with the assistance of nuclear databases, we are able to obtain the ratio of electron spectra under equilibrium conditions for 235 U to 239 Pu, in better agreement with the lower trend recently reported by Kopeikin and collaborators, as well as those for 235 U to 241 Pu and 241 Pu to 239 Pu, which do not agree well with those measured at the Institut Laue-Langevin in the 1980s. We conclude that a new experimental campaign is needed to measure the electron spectra utilizing a high resolution and signal-to-noise-ratio electron spectrometer and a highly precise fission normalization procedure.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Elastic scattering in the 12 N + 197 Au system at 𝐸 lab = 70 MeV

Halo structure is an interesting exotic configuration developed in some light weakly bound nuclei, where a valence particle orbits a nuclear core. Signatures of halo structure can be observed in the angular distributions of the elastic scattering induced by these nuclei at energies around the Coulomb barrier. There are some well-studied reactions with neutron-rich halo nuclei, such as 6 He and 11 Li . However, the information is scarce on the proton-rich side. Recent works confirm the halo structure in the 8B nuclei but still lack more experimental studies for other proton-halo candidates, such as 12 N and 17 F. In this work, we report experimental data for the elastic scattering of 12 N on 197 Au target at 𝐸 lab = 70 MeV. The 12 N is a proton-rich nucleus with proton separation energy 𝑆 𝑝 = 600 keV, which is higher than the 8 B (𝑆 𝑝 = 137 keV) and almost the same as the 17 F (𝑆 𝑝 = 601 keV). Data were obtained at the Cyclotron Institute of Texas A&M University where the 12 N radioactive beam was produced by the momentum achromatic recoil spectrometer. The calculation of the optical model was used to fit the measured angular distribution for the elastic scattering and to obtain the reaction cross section 𝜎 𝑅 . We also performed continuum discretized coupled-channel calculations to compare with the experimental data. The angular distribution of the elastic cross sections exhibits a suppression of the Fresnel peak. From the fitting of the optical model, we obtain the total reaction cross section, 𝜎 𝑅 = 1269 ± 41 mb. The agreement between the CDCC calculation and the experimental elastic scattering data is limited and the breakdown does not exhaust the measured 𝜎 𝑅 . The resulting reduced reaction cross section 𝜎 Red for 12 N + 197 Au is large and comparable to the one obtained for the 8 B + 208 Pb system. This suggests a strong decoupling of the valence proton from the core because of the low binding energy and a dynamic polarization effect. Here, more research is required to estimate the contribution of core excitation.

Elastic scattering reactions↗
DOE OSTI2021

Azimuthal magnetic field distribution in gas-puff Z -pinch implosions with and without external magnetic stabilization

An experimental study of the magnetic field distribution in gas-puff Z pinches with and without a preembedded axial magnetic field (B z0 ) is presented. Spatially resolved, time-gated spectroscopic measurements were made at the Weizmann Institute of Science on a 300 kA, 1.6 μs rise time pulsed-power driver. The radial distribution of the azimuthal magnetic field, B θ , during the implosion, with and without a preembedded axial magnetic field of B z0 = 0.26 T, was measured using Zeeman polarization spectroscopy. The spectroscopic measurements of B θ were consistent with the corresponding values of B θ inferred from current measurements made with a B-dot probe. One-dimensional magnetohydrodynamic simulations, performed with the code TRAC-II, showed agreement with the experimentally measured implosion trajectory, and qualitatively reproduced the experimentally measured radial B θ profiles during the implosion when B z0 = 0.26 T was applied. Simulation results of the radial profile of B θ without a preembedded axial magnetic field did not qualitatively match experimental results due to magneto-Rayleigh-Taylor (MRT) instabilities. Furthermore, our analysis emphasizes the importance of MRT instability mitigation when studying the magnetic field and current distributions in Z pinches. Discrepancies of the simulation results with experiment are discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Experimental Search for Neutron to Mirror Neutron Oscillations as an Explanation of the Neutron Lifetime Anomaly

We report an unexplained >4σ discrepancy persists between “beam” and “bottle” measurements of the neutron lifetime. A new model proposed that conversions of neutrons n into mirror neutrons n', part of a dark mirror sector, can increase the apparent neutron lifetime by 1% via a small mass splitting Δm between n and n' inside the 4.6 T magnetic field of the National Institute of Standards and Technology Beam Lifetime experiment. A search for neutron conversions in a 6.6 T magnetic field was performed at the Spallation Neutron Source which excludes this explanation for the neutron lifetime discrepancy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

First Observation of the β3αp Decay of 13 O via β-Delayed Charged-Particle Spectroscopy

The β-delayed proton decay of 13 O has previously been studied, but the direct observation of β-delayed 3⁢α⁢p decay has not been reported. Rare 3⁢α⁢p events from the decay of excited states in 13 N* provide a sensitive probe of cluster configurations in 13 N*. To measure the low-energy products following β-delayed 3⁢αp decay, the Texas Active Target (TexAT) time projection chamber was employed using the one-at-a-time β-delayed charged-particle spectroscopy technique at the Cyclotron Institute, Texas A&M University. A total of 1.9 × 10 5 13 O implantations were made inside the TexAT time projection chamber. Furthermore, a total of 149 3⁢αp events were observed, yielding a β-delayed 3⁢αp branching ratio of 0.078(6)%. Four previously unknown α-decaying excited states were observed in 13 N at 11.3, 12.4, 13.1, and 13.7 MeV decaying via the 3⁢α + p channel.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Towards time-resolved MicroED grid preparation using mix-and-inject gas dynamic virtual nozzles

Recent progress in gas dynamic virtual nozzle (GDVN) technologies in combination with high-brilliance synchrotron and X-ray free-electron lasers (XFELs) has allowed the visualization of protein dynamics in crystallo by mixing macromolecular protein crystals with a substrate using tunable mixing times on the order of milliseconds to seconds prior to serial X-ray diffraction data collection. This has become the method of choice for high-resolution structure determination of intermediate states. However, such experiments require large counts of crystals of proper sizes for high-resolution data collection, and premium beam times for screening efforts. Cryogenic microcrystal electron diffraction (MicroED) represents a complementary technique that may be a more accessible avenue for time-resolved nanocrystallography compared with serial X-ray diffraction experiments. MicroED can produce full diffraction datasets from just a few submicrometre-thick crystals, and the approach is more readily accessible, requiring standard cryogenic transmission electron microscopy (TEM) equipment available at many universities and institutes. Cryogenic MicroED, like other forms of cryo-EM, begins with rapidly freezing biological material on electron microscopy grids. In the case of MicroED, micro- to nano-crystals (<500 nm thick) are deposited onto electron microscopy grids and plunge-frozen for subsequent electron diffraction data collection. Here, we have incorporated GDVN technology developed originally for XFEL experiments into the freezing process as a first step towards time-resolved studies. We describe the limited deposition efficiency of the model MicroED protein proteinase K on TEM grids using GDVNs, preceding sample vitrification and successful MicroED data collection. We discuss both the initial results from such experiments and the methodological challenges in developing this approach into a reliable workflow for millisecond-to-second time-resolved structural studies of macromolecules. Our results promise a strategy to deposit crystals on grids using GDVNs and determine high-resolution structures by MicroED, constituting a first step towards development of time-resolved MicroED experiments.

MicroED↗
DOE OSTI2021

Enabling discovery data science through cross-facility workflows

Experimental and observational instruments for scientific research (such as light sources, genome sequencers, accelerators, telescopes and electron microscopes) increasingly require High Performance Computing (HPC) scale capabilities for data analysis and workflow processing. Next-generation instruments are being deployed with higher resolutions and faster data capture rates, creating a big data crunch that cannot be handled by modest institutional computing resources. Often these big data analysis pipelines also require near real-time computing and have higher resilience requirements than the simulation and modeling workloads more traditionally seen at HPC centers. While some facilities have enabled workflows to run at a single HPC facility, there is a growing need to integrate capabilities across HPC facilities to enable cross-facility workflows, either to provide resilience to an experiment, increase analysis throughput capabilities, or to better match a workflow to a particular architecture. In this paper we describe the barriers to executing complex data analysis workflows across HPC facilities and propose an architectural design pattern for enabling scientific discovery using cross-facility workflows that includes orchestration services, application programming interfaces (APIs), data access and co-scheduling.

Antypas, Katerina B.↗
DOE OSTI2024

Enhancing Discoverability and Management of Atmospheric Data at Scale: Solutions from the ARM Data Center

The Atmospheric Radiation Measurement (ARM) is a multi-laboratory and multi-institutional U.S. Department of Energy (DOE) Office of Science National User Facility. The ARM Data Center (ADC), located at Oak Ridge National Laboratory, collects, archives, and shares vast atmospheric data crucial for climate research. The ADC manages over 7 PB of data from 460 instruments worldwide, processing it into more than 11,000 diverse data products using the Network Common Data Form (NetCDF) for machine-independent accessibility. The primary challenge addressed in this paper is the efficient management and distribution of vast and diverse datasets essential for the climate research community, enhancing accessibility through advanced tools like Data Discovery. The ADC has developed advanced infrastructure and software architecture to handle the continuous influx of heterogeneous data to enhance data discoverability, resulting in increased scientific collaboration. In 2023, users from over 34 countries downloaded and utilized ARM data, resulting in 1,455 publications. The ADC’s efforts have significantly improved the discoverability and usability of atmospheric data, fostering extensive scientific research and collaboration. This paper details the solutions implemented by the ADC team for efficient data discovery and distribution, and it demonstrates ARM’s capability of staging processed data for scientific analysis.

Shah, Chirag [ORNL] (ORCID:0000000203145737)↗
DOE OSTI2021

Educating HPC Users in the use of advanced computing technology

We examine a multi-modal approach to educating and training users of an advanced computing technology testbed at the Institute for Advanced Computational Science at Stony Brook University. Ookami provides researchers worldwide with access to 176 Fujitsu A64FX compute nodes, this being the same processor technology powering the Japanese Fugaku supercomputer, the fastest computer in the world since June 2020. However, achieving high-performance on this Arm-based, leadership computing technology requires that users be familiar with details of computer architecture, performance analysis and modeling, and high-performance programming models that are commonly omitted in introductory programming courses. Indeed, regardless of their seniority, many of the testbed users are surprisingly unfamiliar with basic concepts such as vectorization, pipelining, latency/bandwidth, roofline models, computing energy/power, threads, and non-uniform memory access. These same concepts also pervade mainstream x86 technologies, so this is of widespread concern. Due to the national/global nature of our user community that is also very diverse in both discipline and experience, the inability to offer formal classes, and our experience that most people do not tend to read online documentation or training materials in sufficient depth, we have consciously employed multiple approaches that heavily emphasize (online) personal interactions and transfer of skills. Online documentation has been organized around best-practices and FAQs; twice-weekly hackathons and office hours via Zoom enable deep dives by both the team and the user community with multiple broad benefits; a Slack channel provides both real time and archived answers and discussions; and workshops, training and webinars target community needs as they arise. Furthermore, the perspective that these tools are being used in an educational setting rather than just for project communication makes them more effective and contributes to community success.

A64FX↗
DOE OSTI2021

Electrical Measurement and Verification of Energy in DC Buildings

Today's selection of DC buildings features a diverse set of electrical topologies and turnkey solutions, and each has specific design trade-offs and optimizations. Designers desperately need standardized metrics and procedures for measurement and verification (M&V) to analyze and compare the advantages of each DC solution to traditional AC building networks. This work develops the Measurement-Informed Modeling (MIM) method, which can be used to determine full-building efficiency and energy savings. The MIM M&V procedure develops a building model, and refines the model with metered data. This work demonstrates the MIM method by measuring the full-building efficiency of two DC buildings operated by the Institute of Building Research in Shenzhen, China. The MIM procedure can ultimately be used to compare and improve the efficiency of various DC topologies.

buildings↗