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At least 919 records · Page 51

Birefringent Glass‐Engraved Quasi‐Linear Nanograting Metasurface Based on Self‐Organizing Process for Large Aperture High Power Laser Applications

All-glass metasurface “nanograting” structures that exhibit birefringence in the formed layer are reported. The key enabler of this work is ion beam processing at an angle sufficiently off-normal incidence, inducing self-assembly of a deposited metal layer into quasi-linear metallic features that can function as an etching mask. As a result, a fused silica metasurface, monolithic to the underlying substrate, is demonstrated at 375 nm wavelength to exhibit a phase delay angle of 30° between the principal axes. The capability of an angled etch mask replenishment process is also demonstrated for achieving deeper etch depth and for increasing the grating period, another first – to the best of the knowledge. This is the first display of a technology capable of fabricating glass-engraved near-linear grating structure with a feature-to-feature period as small as 118.6 nm. Furthermore, this technology has the potential to generate grating-like structures with periods as small as 12.4 nm, as demonstrated here with reactive ion beam processing assisted mask assembly. Furthermore, these structures are shown to have reflectivity < 0.4% across the wavelength band 350 nm – 1000 nm. Such a technology can enable laser-durable grating structures for the deep-UV and even down to soft X-ray wavelengths.

Ray, Nathan J. [Lawrence Livermore National Labora↗

Atom Probe Tomography for understanding microstructural and chemical changes in nuclear materials

Atom Probe Tomography (APT) is routinely employed to determine 3D microstructure and chemistry changes in structural materials used in reactor to understand irradiation effect. These findings help to correlate changes to mechanical and physical properties of nuclear materials which are subjected to extreme reactor conditions. With safety and economics of a reactor in mind, it is essential to be able to predict the changes in the fuel composition and microstructure as a function of burnup. Also, there is current need to develop advanced fuels with improved properties and performance which requires the experimental data on changes in microstructure, physical and chemical properties after irradiation for feedback process. A novel approach is presented to determine the local burnup in irradiated fuels using isotopic quantification obtained by Atom Probe Tomography (APT). Considering the volume of sample used (<100?µm3) for APT experiments using the lift-out process in a scanning electron microscope equipped with a Focused Ion Beam (FIB), the presented method determines the local burnup from a nuclear fuel, where a minimal amount of waste is produced. In this work, three samples were analyzed with different burnup conditions to quantify the isotopes of 235U, 236U, and 238U for burnup calculation in the irradiated metallic U–7Mo dispersion fuel. The calculated values were found in excellent agreement with MCNP calculations. With regard to structural materials, one of the primary factors limiting the utilization of fuel rods of Zr alloys is hydrogen pick up during oxidation. Past experimental studies have shown that the hydrogen pickup in Zirconium alloys is influenced by the alloy composition as well by irradiation temperature and neutron dose. Oftentimes, it is not feasible to carry out comprehensive studies on understanding the microstructural evolution in neutron irradiated materials since in reactor irradiation programs are extremely costly, lengthy and logistically complicated. The use of ion irradiation as a substitute has grown in recent years for several reasons including less radioactivity, faster irradiations and lower costs. In the framework of the MUZIC 3 project, samples of Zircaloy-4 have been proton and Zr2+ irradiated at the Michigan Ion Beam Lab (MIBL) facility with aim to create a microstructure that is similar to that observed after in-reactor service. The temperature of the environment is adjusted to compensate for the higher dose rate, as has been done previously. As a first step in this project the irradiated microstructures have been characterized using Transmission Electron Microscopy and Atom Probe Tomography to elucidate the microstructural changes, including precipitate amorphization and dissolution and the formation of dislocation loops. This presentation plans to highlight initial finding of this project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Generation, saturation, and convection of electrostatic waves in Jupiter's shock foot

In this paper, a model is developed for the analysis of the electrostatic waves produced in the shock foot at Jupiter. It is shown that an ion beam instability involving the ions reflected at the shock ramp and the incoming solar-wind electrons produces waves at the observed frequencies and that saturation via orbit diffusion limits the waves to amplitudes near to what is observed. Results from a two-dimensional model of the reflected beam in the foot indicate that the waves propagate against the solar wind away from the shock ramp and are amplified up to their saturation amplitudes. The saturation results, combined with the electron temperature profile due to wave-particle interactions predicted by quasi-linear theory, reproduce a wave amplitude profile for the shock foot that is in reasonable agreement with the observations.

Moses, S. L.↗

Transmission electron microscopy with in-situ ion irradiation: Facilities and community

Whilst there is a clear scientific and technological need for the technical capabilities of transmission electron microscopes with in-situ ion irradiation, it also requires a collaborative community of international researchers to support such facilities in successfully meeting this demand. Instruments of this type serve to provide fundamental understanding of the mechanisms which drive changes in materials important to nuclear fission and fusion energy, the semiconductor industry, quantum information systems, space travel, astronomy, geology and many more applications. As these areas continue to evolve and the instrumentation possibilities expand, the capacity of in-situ ion irradiation facilities must also develop hand-in-hand with the user community to deliver an ever-greater diversity of high-fidelity extreme-environment experimentation. Future directions for the field, such as miniaturization from MEMS/microfluidic devices and advanced controls with ML-based analysis, continuously emerge to advance both the hardware and software which support the coupling of TEMs with ion beams. This review sets out to provide up-to-date insights into the community and advancement of current, and development of future, facilities which have the potential to further unlock access to the nanoscale exploration of coupled extreme environments crucial to many of the important science and engineering challenges we face today.

In-situ irradiation↗

Features of ion generation by a picosecond laser in the range of 10 11 –10 13 W cm -2 power densities

Picosecond lasers (ps-lasers) have significant advantages for the generation of low charge state ions compared to nanosecond lasers because the influence of heat conductivity on a solid target is almost negligible in the case of ps-laser ablation for laser pulse durations less than 10 ps. However, there is no comprehensive data on ion yields for different elements and target irradiation conditions for laser power densities at the target surface around and below 10 13 W cm –2 , which is of interest to our study of such plasmas as a source of low charge state ions for various applications, particularly for external injection of those ions into an Electron Beam Ion Source (EBIS). We investigated ion generation from Al, Ti, Cu, Nb and Ta target elements by a ps-laser with power densities in the range of 10 11 –10 13 W cm –2 at the target surface. A ps-laser with 1.27 mJ maximum energy within an 8 ps pulse and repetition rate up to 400 Hz has been used to generate a laser-ablated plasma. Dependencies of ion current versus time, total charge of registered ions as well as ion kinetic energy distributions are characterized using a Faraday cup. Significant difference in ion current dynamics between first, second and following shots onto the same target spot was found for all five target elements. The total charge of ions registered by the Faraday cup increases linearly with increasing laser pulse energy and is almost independent of the target element and number of shots onto the same target spot for all five target elements studied. The results obtained give us a basis for specification and design of the source of low charge state ions for external injection into EBIS.

43 PARTICLE ACCELERATORS↗

Mathematical model of the current density for the 30-cm engineering model thruster

Mathematical models are presented for both the singly and doubly charged ion current densities downstream of the 30-cm engineering model thruster with 0.5% compensated dished grids. These models are based on the experimental measurements of Vahrenkamp at a 2-amp ion beam operating condition. The cylindrically symmetric beam of constant velocity ions is modeled with continuous radial source and focusing functions across 'plane' grids with similar angular distribution functions. A computer program is used to evaluate the double integral for current densities in the near field and to obtain a far field approximation beyond 10 grid radii. The utility of the model is demonstrated for (1) calculating the directed thrust and (2) determining the impingement levels on various spacecraft surfaces from a two-axis gimballed, 2 x 3 thruster array.

Cuffel, R. F.↗

Ion plating studies for high temperature applications

An experimental project was undertaken to ion plate, by electron beam evaporation, Al films onto 4340 steel substrates using (and at the time troubleshooting) the custom built V.T.A. 7375 electron beam ion plating system. A careful recent literature and commercial vendor survey indicates possible means of improving the trouble plagued V.T.A. system.

Davis, J. H.↗

Passivation of carbon steel through mercury implantation

An experiment, in which carbon steel samples were implanted with mercury ions from a broad beam ion source and their corrosion characteristics in air were evaluated, is described. Mercury doses of a few mA min/square cm at energies of a few hundred electron volts are shown to effect significant improvements in the corrosion resistance of the treated surfaces. In a warm moist environment the onset of rusting was extended from 15 min. for an untreated sample to approximately 30 hrs. for one implanted at a dose of 33 mA min/square cm with 1000 eV mercury ions.

Wilbur, P. J.↗

Diamondlike flake composites

A carbon coating is vacuum arc deposited on a smooth surface of a target which is simultaneously ion beam sputtered. The bombarding ions have sufficient energy to create diamond bonds. Spalling occurs as the carbon deposit thickens. The resulting diamond-like carbon flakes are mixed with a binder or matrix material to form a composite material having improved thermal, electrical, mechanical, and tribological properties when used in aerospace structures and components.

Banks, B. A.↗

Diamondlike flakes

A carbon coating was vacuum arc deposited on a smooth surface of a target which was simultaneously ion beam sputtered. The bombarding ions have sufficient energy to create diamond bonds. Spalling occurs as the carbon deposit thickens. The resulting diamond like carbon flakes improve thermal, electrical, mechanical, and tribological properties when used in aerospace structures and components.

Banks, B. A.↗

Superthermal ionospheric outflows

In recent years observations have shown that the terrestrial ionosphere serves as a significant source of the hot plasma in the magnetosphere. These findings imply that cold plasma flows upward to great altitudes and at some point along the way gains energies much larger than typical ionospheric values. The present investigation is mainly concerned with observations of ionospheric outflows at energies higher than those predicted by ambipolar wind models but lower than those associated with keV auroral ion acceleration, giving particular attention to the energy range from a few to a few hundred electron volts. The ion flows in the energy range intermediate between polar wind and keV auroral ion beams are called superthermal ion outflows. It is shown that recent observations of superthermal ion outflows from the terrestrial ionosphere are related to theoretical models of the topside ionosphere.

Moore, T. E.↗

Thermalization of neutral-beam-injected ions by lower hybrid waves in Jupiter's magnetosphere

A theoretical analysis of lower-hybrid wave generation by a ring distribution of superthermal ions is presented. A kinetic instability of waves traveling across the magnetic field occurs when fast neutrals escaping from the Io plasma torus are reionized and accelerated to corotation speed in Jupiter's magnetosphere. Instability is possible for modest threshold values of V/a0 = 3 - 7 where V is the pickup gyrospeed and a0 is the background-ion thermal speed. Consequent effects include the relaxation of the pickup-ion distribution and the acceleration of superthermal electrons.

Barbosa, D. D.↗

Pseudomorphic In(y)Ga(1-y)As/GaAs/Al(x)Ga(1-x)As single quantum well surface-emitting lasers with integrated 45 deg beam deflectors

The paper reports on the first demonstration of pseudomorphic InGaAs single quantum well surface-emitting lasers (SELs), with etched vertical mirrors and integrated 45-deg beam deflectors fabricated by ion beam etching. 100-micron-wide broad-area SELs exhibited a threshold current of 320 mA, a total power of 126 mW, and a total external differential quantum efficiency of 0.09 W/A for a 500-micron-long cavity. The perpendicular far-field pattern of broad-area SELs showed a full width at half maximum of about 20 deg. Lasers with various types of cavities fabricated from the same wafer were compared. Broad-area edge-emitting lasers had a threshold current of 200 mA, a total power of 700 mW, and a total external differential quantum efficiency of 0.52 W/A.

Kim, Jae-Hoon↗

Testing and management of flight instruments and their data

Hardware activities were concentrated on the Low Energy Ion Facility (LEIF), which is used for testing and calibration of most of the flight instruments for near-Earth observations. The ion beam generated by the ion source in the LEIF has been required for the proper testing and calibration of the primary components of the Thermal Ion Dynamics Experiment (TIDE) to be flown on the POLAR spacecraft of the Global Geospace Science (GGS) flight program. Additional work has been done on equipment and techniques for diagnosing and testing microchannel plates. These plates are used in the imager as well as the flight instruments.

Comfort, Richard H.↗

A survey of low frequency waves at Jupiter: The Ulysses encounter

We report the results of a survey of low-frequency (LF) plasma waves detected during the Ulysses Jupiter flyby. In the Jovian foreshock, two predominant wave periods are detected: 10(exp 2)-s and 5-s, as measured in the spacecraft frame. The 10(exp 2)-s waves are highly nonlinear propagate at large angles to vector-B(sub 0) (typically 50 deg), are steepened, and sometimes have attached whistler packets. For the interval analyzed the 10(exp 2)-s waves had mixed right-and left-hand polarizations. We argue that these are all consistent with being right-hand magnetosonic waves in the solar wind frame. The 10(exp 2)-s waves with attached whistler are similar to cometary waves. The trailing portions are linearly polaraized and the whistler portions circularly polarized with amplitudes decreasing linearly with time. The emissions are generated by approximately 2-keV protons flowing from the Jovian bow shock/magnetosheath into the upstream region. The instability is the ion beam instability. Higher Z ions were considered as a source of the waves but have been ruled out because of the low sunward velocities needed for their resonance. The 5-s waves have delta vector-B/B(sub 0 approximately = 0.5, are compressive and are left-hand polarized in the spacecraft frame. Local generation by three different resonant interactions were considered and have been ruled out. One possibility is that these waves are whistler mode by-products of the steepened lower-frequency magnetosonic waves. Mirror mode structures were detected throughout the outbound magnetosheath passes. For these structures, the theta(sub kB) values were consistently in the range of 80 deg to 90 deg, exceptionally high values.

Tsurutani, Bruce T.↗