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DOE OSTI2023

Ablation loading of barium ions into a surface-electrode trap

Trapped-ion quantum information processing may benefit from qubits encoded in isotopes that are practically available in only small quantities, e.g., due to low natural abundance or radioactivity. Laser ablation provides a method of controllably liberating neutral atoms or ions from low-volume targets, but energetic ablation products can be difficult to confine in the small ion-electrode distance, micron-scale microfabricated traps amenable to high-speed, high-fidelity manipulation of ion arrays. Here, we investigate ablation-based ion loading into surface-electrode traps of different sizes to test a model describing ion loading probability as a function of effective trap volume and other trap parameters. We characterize loading of ablated barium from a metallic source in two cryogenic surface-electrode traps with 730 and 50 μm ion-electrode distances. Furthermore, our loading rate agrees with a predictive analytical model, providing insight for the confinement of limited-quantity species of interest for quantum computing, simulation, and sensing.

74 ATOMIC AND MOLECULAR PHYSICS↗

NASA NTRS1993

Decay of equatorial ring current ions and associated aeronomical consequences

The decay of the major ion species which constitute the ring current is studied by solving the time evolution of their distribution functions during the recovery phase of a moderate geomagnetic storm. In this work, only equatorially mirroring particles are considered. Particles are assumed to move subject to E x B and gradient drifts. They also experience loses along their drift paths. Two loss mechanisms are considered: charge exchange with neutral hydrogen atoms and Coulomb collisions with thermal plasma in the plasmasphere. Thermal plasma densities are calculated with a plasmaspheric model employing a time-dependent convection electric field model. The drift-loss model successfully reproduces a number of important and observable features in the distribution function. Charge exchange is found to be the major loss mechanism for the ring current ions; however the important effects of Coulomb collisions on both the ring current and thermal populations are also presented. The model predicts the formation of a low-energy (less than 500 eV) ion population as a result of energy degradation caused by Coulomb collision of the ring current ions with the plasmaspheric electrons; this population may be one source of the low-energy ions observed during active and quiet periods in the inner magnetosphere. The energy transferred to plasmaspheric electrons through Coulomb collisions with ring current ions is believed to be the energy source for the electron temperature enhancement and the associated 6300 A (stable auroral red (SAR) arc) emission in the subauroral region. The calculated energy deposition rate is sufficient to produce a subauroral electron temperature enhancement and SAR arc emissions that are consistent with observations of these quantities during moderate magnetic activity levels.

Fok, M.-C.↗

NASA NTRS1985

Supersonic ion outflows in the polar magnetosphere via the geomagnetic spectrometer

Observations of 'supersonic' O(+) outflows by DE-1 in the polar magnetosphere are interpreted as a velocity-filter effect resulting from the transport of these low energy ions from a horizontally narrow source associated with the polar cleft topside ionosphere into the polar cap magnetosphere. Under certain simplifying circumstances, it is shown that the 'Mach number' for the flow is essentially a geometrically determined quantity, approximately the ratio of the horizontal distance of the observation location to the source over the horizontal width of the source. A recently developed two-dimensional kinetic model of ion transport in the polar magnetosphere is used to calculate distribution functions and the associated bulk flow parameters, and these calculated quantities are compared with measured flow parameters from DE-1.

Horwitz, J. L.↗

NASA NTRS1997

Multi-Species Test of Ion Cyclotron Resonance Heating at High Altitudes

Observations of ion distributions and plasma waves obtained by the Dynamics Explorer 1 satellite in the high-altitude, nightside auroral zone are used to study ion energization for three ion species. A number of theoretical models have been proposed to account for the transverse heating of these ion populations. One of these, the ion cyclotron resonance heating (ICRH) mechanism, explains ion conic formation through ion cyclotron resonance with broadband electromagnetic wave turbulence in the vicinity of the characteristic ion cyclotron frequency. The cyclotron resonant heating of the ions by low- frequency electromagnetic waves is an important energy source for the transport of ions from the ionosphere to the magnetosphere. In this paper we test the applicability of the ICRH mechanism to three simultaneously heated and accelerated ion species by modelling the ion conic formation in terms of a resonant wave-particle interaction in which the ions extract energy from the portion of the broadband electromagnetic wave spectrum which includes the ion cyclotron frequency. Using a Monte Carlo technique we evaluate the ion heating produced by the electromagnetic turbulence at low frequencies and find that the wave amplitudes near the ion cyclotron frequencies are sufficient to explain the observed ion energies.

Persoon, A. M.↗

NASA NTRS2003

Two-Dimensional Transport Studies for the Composition and Structure of the Io Plasma Torus

The overall objective of this project is to investigate the roles of local and spatially extended plasma sources created by Io, plasma torus chemistry, and plasma convective and diffusive transport in producing the long-lived S(+), S(++) and O(+) radial ribbon structures of the plasma torus, their System III longitude and local-time asymmetries, their energy sources and their possible time variability. To accomplish this objective, two-dimensional [radial (L) and System III longitude] plasma transport equations for the flux-tube plasma content and energy content will be solved that include the convective motions for both the east-west electric field and co-rotational velocity-lag profile near Io s orbit, radial diffusion, and the spacetime dependent flux-tube production and loss created by both neutral-plasma and plasma-ion reaction chemistry in the plasma torus. For neutral-plasma chemistry, the project will for the first time undertake the calculation of realistic three-dimensional, spatially-extended, and time-varying contributions to the flux-tube ion-production and loss that are produced by Io's corona and extended neutral clouds. The unknown two-dimensional spatial nature of diffusion in the plasma transport will be isolated and better defined in the investigation by the collective consideration of the foregoing different physical processes. For energy transport, the energy flow from hot pickup ions (and a new electron source) to thermal ions and electrons will be included in investigating the System III longitude and local-time temperature asymmetries in the plasma torus. The research is central to the scope of the NASA Sun-Earth Connection Roadmap in Quest II Campaign 4 "Comparative Planetary Space Environments" by addressing key questions for understanding the magnetosphere of planets with high rotation rates and large internal plasma sources and, in addition, is of considerable importance to the NASA Solar System Exploration Science Theme. In this regard, Jupiter is the most extreme example with its rapid rotation and with its inner Galilean satellite Io providing the dominant plasma source for the magnetosphere.

Smyth, William H.↗

NASA NTRS1982

Theory of the fine structure of auroral kilometric radiation

Recent data from ISEE 1 show auroral kilometric radiation (AKR) with finely separated bands in frequency. The observation that the AKR fine structure frequency separation is about equal to the ion cyclotron frequency at the AKR source is strong evidence for the interaction of AKR and electrostatic ion cyclotron (EIC) waves in the source, as proposed by Grabbe et al. (1980) to explain the origin of AKR. It is pointed out that no other wave of frequency close to the band separation is known to exist in the auroral source region. The fine structure observed in the source region AKR is the first evidence for EIC waves in the lower source region (3000 - 5000 km attitude), as required in the theory of Grabbe et al.

Grabbe, C. L.↗

NASA NTRS1976

Heavy ions from the Galilean satellites and the centrifugal distortion of the Jovian magnetosphere

The Galilean satellites constitute a potentially significant source of plasma to the Jovian atmosphere. The paper examines the distortion of the Jovian magnetosphere that would result from injection of ions at the Galilean satellites. The magnetic distortion produced is a localized perturbation near the equatorial plane, in contrast to the large-scale distortion produced by Jovian atmospheric ions. The study estimates the relative perturbation currents resulting from the two sources in terms of the unknown ion production rate at the satellites. It is found that the two perturbations would be of comparable magnitudes if the ion source flux at all of the Galilean satellites were comparable to the photo-ion escape flux from Jupiter's atmosphere. More specifically, ions produced by the Galilean satellites should be confined near the equatorial plane of Jupiter's magnetosphere in a sheet whose thickness is determined by a centrifugal scale height given essentially by the ion thermal speed divided by the corotation frequency.

Hill, T. W.↗

DOE OSTI2024

Europa modifies Jupiter’s 1 plasma sheet

Jupiter's plasma sheet has been understood to be primarily composed of Io-genic sulfur and oxygen, along with protons at lower mass density. These ions move radially away from Jupiter, filling its magnetosphere. The material in the plasma sheet interacts with Europa, which is also a source of magnetospheric pickup ions, primarily hydrogen and oxygen. Juno's thermal plasma instrument JADE, the Jovian Auroral Distributions Experiment, has provided comprehensive in situ observations of the composition of Jupiter's plasma sheet ions with its Time-of-Flight mass-spectrometry capabilities. Here, we present observations of the magnetospheric composition in the Europa-Ganymede region of Jupiter's magnetosphere. We find material from Europa is intermittently present at comparable densities to Io-genic plasma. The intermittency of Europa-genic signatures suggests Europa's neutral oxygen toroidal cloud is more localized to Europa's vicinity than its hydrogen cloud. These observations reveal a more complex and compositionally diverse magnetosphere than previously thought.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Europa Modifies Jupiter's Plasma Sheet

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1983

Field-aligned ion beams upstream of the earth's bow shock Evidence for a magnetosheath source

High time resolution ISEE-1 and -2 observations of upstream field-aligned ion beams at several crossings of the earth's bow shock indicate that some beams are due to high energy magnetosheath particles leaking through the shock into the upstream region. The distribution immediately downstream of these oblique shocks consists of a 'core' of directly transmitted, slightly heated ions, plus a crescent-shaped, high-velocity distribution, centered roughly on the magnetic field in the direction toward the upstream region, with a fairly well defined low velocity cutoff.

Thomsen, M. F.↗

NASA NTRS1993

Local time occurrence frequency of energetic ions in the earth's magnetosheath

The occurrence frequency of energetic ions in the energy range from 8 to 40 keV/e as a function of local time in the magnetosheath is presented. Energetic ions are observed in the magnetosheath with a minimum probability of 25 percent for all local times. The occurrence frequency for the energetic ions is higher on the dawnside than on the duskside but shows a relative maximum postnoon in the local time range from 12 to 15 hours. The postnoon relative maximum is attributed to a magnetospheric source for the energetic ions while the dawn-dusk asymmetry is attributed to a quasi-parallel bow shock source.

Fuselier, S. A.↗

DOE OSTI2020

Single-ion addressing via trap potential modulation in global optical fields

To date, individual addressing of ion qubits has relied primarily on local Rabi or transition frequency differences between ions created via electromagnetic field spatial gradients or via ion transport operations. Alternatively, it is possible to synthesize arbitrary local one-qubit gates by leveraging local phase differences in a global driving field. Here we report individual addressing of 40 Ca + ions in a two-ion crystal using axial potential modulation in a global gate laser field. We characterize the resulting gate performance via one-qubit randomized benchmarking, applying different random sequences to each co-trapped ion. We identify the primary error sources and compare the results with single-ion experiments to better understand our experimental limitations. These experiments form a foundation for the universal control of two ions, confined in the same potential well, with a single gate laser beam.

quantum computing↗

NASA NTRS1989

High-current plasma contactor neutralizer system

A plasma-contactor neutralizer system is described, for the stabilizing the Orbiter's potential during flights of the Atmospheric Laboratory for Applications and Science missions. The plasma contactor neutralizer will include a Xe plasma source that can provide steady-state ion-emission currents of up to 1.5 A. The Orbiter's potential will be maintained near that of the surrounding space plasma during electron-beam accelerator firings through a combination of ion emission from the Xe plasma source and electron collection from the ambient space plasma. Configuration diagrams and block diagrams are presented along with the performance characteristics of the system.

Beattie, J. R.↗

NASA NTRS1997

Multi-Species Test of Ion Cyclotron Resonance Heating at High Altitudes

Observations of ion distributions and plasma waves obtained by the Dynamics Explorer 1 satellite in the high-altitude, nightside auroral zone are used to study ion energization for three ion species. A number of theoretical models have been proposed to account for the transverse heating of these ion populations. One of these, the ion cyclotron resonance heating (ICRH) mechanism, explains ion conic formation through ion cyclotron resonance with broadband electromagnetic wave turbulence in the vicinity of the characteristic ion cyclotron frequency. The cyclotron resonant heating of the ions by low-frequency electromagnetic waves is an important energy source for the transport of ions from the ionosphere to the magnetosphere. In this paper we test the applicability of the ICRH mechanism to three simultaneously heated and accelerated ion species by modelling the ion conic formation in terms of a resonant wave-particle interaction in which the ions extract energy from the portion of the broadband electromagnetic wave spectrum which includes the ion cyclotron frequency. Using a Monte Carlo technique we evaluate the ion heating produced by the electromagnetic turbulence at low frequencies and find that the wave amplitudes near the ion cyclotron frequencies are sufficient to explain the observed ion energies.

Persoon, A. M.↗

NASA NTRS1982

The Venus ionosphere at grazing incidence of solar radiation - Transport of plasma to the night ionosphere

A quasi-two-dimensional model of the Venusian ionosphere is used to calculate the ion number densities and horizontal ion bulk velocities expected for a range of solar zenith angles near the terminator (80-100 deg). These results are compared with data from the Pioneer Venus Orbiter retarding potential analyzer. It is shown that antisunward horizontal plasma fluxes produced by solar EUV-induced pressure gradients are sufficient to maintain the nighttime ionosphere. While photoionization is the dominant source of ionospheric plasma for solar zenith angles less than 92 deg, plasma transport from the dayside is the dominant plasma source for solar zenith angles greater than 95 deg. It is also shown that the main nightside plasma peak at a height of 140 km is of the F2 type; its height and shape are therefore quite insensitive to the height of the ion source.

Whitten, R. C.↗

NASA NTRS1983

Initial hot plasma composition results from the Dynamics Explorer

Initial observations from the energetic ion composition spectrometer on the DE-1 spacecraft have found mass or charge dependent processes to be operating in the vicinity of an inverted-V event in the auroral acceleration region, above the polar cap ionosphere, and in the mid-altitude dayside cusp. Separate color spectrograms for the different ion species provide a synoptic picture of these processes that can contribute significantly to our understanding of both the solar wind and the ionosphere as sources of energetic magnetospheric ions.

Shelley, E. G.↗

NASA NTRS1972

Location of the electron acceleration region in solar flares.

Observations of impulsive solar flare X rays (energy greater than 10 keV) by the OGO-5 satellite and the measurements of energetic solar electrons made with the Explorer-35 and Explorer-41 (IMP-5) satellites during the period March 1968-September 1969 have been analyzed in order to determine the ion density in the X-ray source region as well as the location of the electron acceleration region in the solar atmosphere. The ion density in the X-ray source region varies from event to event and lies between 1 and 100 billion ions per cu cm for those events in which the impulsive X-ray emission could be detected; for those events in which no impulsive emission was detected above threshold, the ion density in the X-ray source was less than one billion ions per cu cm. At least in some small solar flares, the region where the electrons are accelerated during the flash phase is located in the lower corona.

Kane, S. R.↗

DOE OSTI2022

Efficient conversion of low-concentration nitrate sources into ammonia on a Ru-dispersed Cu nanowire electrocatalyst

We report electrochemically converting nitrate ions, a widely distributed nitrogen source in industrial wastewater and polluted groundwater, into ammonia represents a sustainable route for both wastewater treatment and ammonia generation. However, it is currently hindered by low catalytic activities, especially under low nitrate concentrations. Here we report a high-performance Ru-dispersed Cu nanowire catalyst that delivers an industrial-relevant nitrate reduction current of 1 A cm –2 while maintaining a high NH 3 Faradaic efficiency of 93%. More importantly, this high nitrate-reduction catalytic activity enables over a 99% nitrate conversion into ammonia, from an industrial wastewater level of 2,000 ppm to a drinkable water level <50 ppm, while still maintaining an over 90% Faradaic efficiency. Coupling the nitrate reduction effluent stream with an air stripping process, we successfully obtained high purity solid NH 4 Cl and liquid NH 3 solution products, which suggests a practical approach to convert wastewater nitrate into valuable ammonia products. Density functional theory calculations reveal that the highly dispersed Ru atoms provide active nitrate reduction sites and the surrounding Cu sites can suppress the main side reaction, the hydrogen evolution reaction.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗