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NASA NTRS1991

Isotopic constraints on the origin of meteoritic organic matter

Salient features of the isotopic distribution of H, C and N in the organic material found in carbonaceous meteorites are noted. Most organic fractions are strongly enriched in D with respect to the D/H ratio characteristic of H2 in the protosolar system; substantial variations in C-13/C-12 ratio are found among different molecular species, with oxidised species tending to be C-13 enriched relative to reduced species; some homologous series reveal systematic decrease in C-13/C-12 with increasing C number; considerable variation in N-15/N-14 ratio is observed within organic matter, though no systematic pattern to its distribution has yet emerged; no interelement correlations have been observed between isotope enrichments for the different biogenic elements. The isotopic complexity echoes the molecular diversity observed in meteoritic organic matter and suggests that the organic matter was formed by multiple processes and/or from multiple sources. However, existence of a few systematic patterns points towards survival of isotopic signatures characteristic of one or more specific processes. The widespread D enrichment implies either survival of many species of interstellar molecule or synthesis from a reservoir containing a significant interstellar component. Several of the questions raised above can be addressed by more detailed determination of the distribution of the H, C and N isotopes among different well-characterized molecular fractions. Thus, the present study is aimed at discovering whether the different amino acids have comparable D enrichments, which would imply local synthesis from a D-enriched reservoir, or very viable D enrichments, which would imply survival of some interstellar amino acids. The same approach is also being applied to polycyclic aromatic hydrocarbons. Because the analytical technique employed (secondary ion mass spectrometry) can acquire data for all three isotopic systems from each molecular fraction, any presently obscured interelement isotopic correlation should also be revealed, which will aid in identifying pertinent synthetic processes.

Kerridge, J. F.↗
NASA NTRS1992

Time variation of the meteoritic contribution to the atmosphere of Mars

The meteoritic contribution to the planets of the inner solar system varies significantly with time. During the first billion years, the flux of meteoritic material was significantly greater than present. Over the past 3.6 billion years, the background flux has been relatively constant, but shorter periods of significantly enhanced flux are associated with discrete events such as major impacts of large bodies onto the planets or their moons and passage through cometary debris streams. The topics covered include the following (1) the last 3.6 billion years; (2) large impacts; (3) passage through comet tail; and (4) major collision in the main-belt.

Flynn, G. J.↗
NASA NTRS1992

An ejection model for SNC meteorites: An indication for recent volcanism on Mars

When compared to other achondrites, Shergotty-Nakhla-Chassigny (SNC) meteorites are viewed as anomalous objects. This conclusion is based mainly on their extremely young crystallization ages and their short cosmic ray exposure times. Further, SNC's noble gas and nitrogen components indicate a martian origin for these objects. If these meteorites are from Mars, then the most confounding question facing the planetary science community is how were they ejected from the planet's surface. The following is an investigation of that question.

Manker, J. P.↗
NASA NTRS1992

Presolar (?) corundum in the Orgueil meteorite

The discovery in chondritic meteorites of diamond, SiC, and poorly crystallized graphite that formed around other stars demonstrated conclusively that presolar dust survived the formation of the solar system to be incorporated into meteorites. The presolar nature of these grains is shown by the highly unusual isotopic compositions of their constituent elements. To date, all recognized types of presolar grains have been carbon rich and apparently formed around carbon stars, those with C/O greater than 1. The discovery of the first oxygen-rich grain with isotopic characteristics consistent with a presolar origin is reported. Oxygen-rich grains presumably form only around stars with C/O less than 1.

Huss, G. R.↗
NASA NTRS1991

Exposure histories of lunar meteorites - ALHA81005, MAC88104, MAC88105, and Y791197

The cosmogenic radionuclides Ca-41, Cl-36, Al-26, and Be-10 in the Allan Hills 81005, MacAlpine Hills 88104, MacAlpine Hills 88105, and Yamato 791197 meteorites were measured by accelerator mass spectrometry. Mn-53 in Allan Hills 81005 and Yamato 791197 was measured by neutron activation. These four lunar meteorites experienced similar histories. They were ejected from near the surface of the moon ranging in depth down to 400 g/sq cm and had very short transition times (less than 0.1 Ma) from the moon to the earth. A comparison of the cosmogenic nuclide concentrations in MacAlpine Hills 88104 and MacAlpine Hills 88105 clearly indicates that they are a pair from the same fall.

Nishiizumi, K.↗
NASA NTRS1991

Exposure histories of the lunar meteorites - MAC88104, MAC88105, Y791197, and Y86032

Four lunar meteorites were analyzed for the cosmogenic radionuclides Be-10, Al-26, Cl-36, and Ca-41. Histories of exposure to cosmic rays were modelled in terms of two-stage irradiations, each with a long first stage on the moon, lasting a time T sub 2pi greater than 5 Ma at a burial depth d sub 2pi(g/sq cm), followed by a second stage in space, i.e., the transit time between the moon and the earth, lasting a time T sub 4pi (Ma) in a body of typical metereological size. It is inferred that the production rate is of the order of 5/Ma and the arrival rate worldwide is about 3,000,000 meteorites/Ma. It is concluded that each impact event large enough to produce lunar meteorites sends a large number of them to the earth.

Vogt, S.↗
NASA NTRS1991

Thermoluminescence constraints on the metamorphic, shock, and brecciation history of basaltic meteorites

The metamorphic, shock, and brecciation history of 18 eucrites, 13 howardites, 6 diogenites, and 15 mesosiderites is investigated via induced thermoluminescence measurements performed on them. The eucrites show a 15-fold range of TL sensitivities, which correlate with petrographic indicators of metamorphic intensity. The temperature of the dominant TL peak observed for basaltic meteorites, and experiments in which four eucrites with diverse petrographic properties were annealed at various temperatures in the laboratory, suggests that the metamorphic equilibration temperatures for most basaltic meteorites were not more than 800 C. Assuming this temperature was typical of conditions during metamorphism, then burial depths for type-above-5 eucrites were greater than 350 m and less than 50 m for type-2 eucrites. Since TL peak temperatures are related to the degree of disorder in the Al, Si chain in feldspar, the present data provide independent evidence for very slow cooling rates for mesosiderites and for the slower cooling rates for some cumulate eucrites relative to equilibrated noncumulate eucrites.

Batchelor, J. D.↗
NASA NTRS1992

Fall days of the SNC meteorites - Evidence for an SNC meteoroid stream, and a common site of origin

Four of the SNC meteorites of putative Martian origin are falls. Two of these fell on October 3: Chassigny in 1815 and Zagami in 1962. The probability of this coincidence arising from random fall days is approximately 1 in 60. If this coincidence is not the result of chance, it suggests that some of the SNC meteorites are derived from a meteoroid stream. In that Chassigny and Zagami span nearly the full range of SNC lithologies and histories, the coincidence of fall days is consistent with suggestions that all of the SNCs came from a single site (impact crater) on their parent planet.

Treiman, Allan H.↗
NASA NTRS1992

Petrogenesis of the nakhlite meteorites - Evidence from cumulate mineral zoning

Attention is given to a simple igneous petrogenesis for the meteorite Nakhla, which was previously called into question because Mg/Fe ratios in olivine indicate substantial disequilibrium between the predominant cumulus minerals (olivine and augite). Comparative analyses of simulated diffusive zoning and the observed cumulus mineral zoning for all three nakhlites (Nakhla, Governador Valadares, and Lafayette) show that their current compositions do not necessarily reflect parental magma compositions. Diffusion has altered primary cumulus compositions to varying degrees, Nakhla being the least affected, and Lafayette being almost completely reequilibrated. Since mineral zoning in each meteorite is strongly concentric around mesostasis areas, it is inferred that reaction with intercumulus liquid has controlled the observed zoning. It is argued that the nakhlites appear to be a series of relatively simple cumulate rocks which have undergone various amounts of late-magmatic and subsolidus diffusion, possibly reflecting their relative positions in a cooling cumulate pile.

Harvey, Ralph P.↗
NASA NTRS1979

Some unique meteorites found in Antarctica and their relation to asteroids

Two unique meteorites were identified by means of a mineralogical examination of the smaller-sized Yamato achondrites. Yamato-74130 is the most iron-rich ureilite with Na, Cr-rich augite instead of pigeonite. Yamato-74160 was extensively recrystallized, but the composition and proportion of olivine, orthopyroxene, augite, and plagioclase is consistent with LL7 chondrites. ALHA77005 is a unique achondrite with olivine, possibly three pyroxene assemblages, and maskelynite. These meteorites provide evidence that there may be other 'thermalized' asteroids than the howardite parent body. Detailed petrologic descriptions of the unique achondrites, recrystallized diogenite Yamato-74013, and the rapidly cooled eucrite Yamato-74450 with pyroxene phenocrysts are given. It is inferred from the bulk chemistry and the mineralogical reexamination of Yamato-75028 that it is composed of the H5-type clasts and chondrule-rich H(L)3-like matrix with the H5 fragments. A close relationship in the collisional evolution of some asteroids with these materials is inferred.

Takeda, Hiroshi↗
NASA NTRS1992

Martian parent craters for the SNC meteorites

Information on the petrology and ages of the SNC meteorites, together with geological data derived from Viking Orbiter images, are used to identify 25 candidate impact craters in the Tharsis region of Mars that could possibly be the source craters for these meteorites. The craters chosen as candidate source craters had diameters greater than 10 km, morphologies indicative of young craters, and satisfied both the petrological criteria of the SNCs and the proposed 1.3 Ga crystallization ages. On the basis of the constraints implied by the identification of the candidate source craters, interpretations of the absolute chronology of Mars are proposed.

Mouginis-Mark, P. J.↗
NASA NTRS1992

Simulated meteorite impacts and volcanic explosions: Ejecta analyses and planetary implications

Past cratering studies have focused primarily on crater morphology. However, important questions remain about the nature of crater deposits. Phenomena that need to be studied include the distribution of shock effects in crater deposits and crater walls; the origin of mono- and polymict breccia; differences between local and distal ejecta; deformation induced by explosive volcanism; and the production of unshocked, high-speed ejecta that could form the lunar and martian meteorites found on the Earth. To study these phenomena, one must characterize ejecta and crater wall materials from impacts produced under controlled conditions. New efforts at LLNL simulate impacts and volcanism and study resultant deformation. All experiments use the two-stage light-gas gun facility at LLNL to accelerate projectiles to velocities of 0.2 to 4.3 km/s, including shock pressures of 0.9 to 50 GPa. We use granite targets and novel experimental geometries to unravel cratering processes in crystalline rocks. We have thus far conducted three types of simulations: soft recovery of ejecta, 'frozen crater' experiments, and an 'artificial volcano. Our ejecta recovery experiments produced a useful separation of impactites. Material originally below the projectile remained trapped there, embedded in the soft metal of the flyer plate. In contrast, material directly adjacent to the projectile was jetted away from the impact, producing an ejecta cone that was trapped in the foam recovery fixture. We find that a significant component of crater ejecta shows no signs of strong shock; this material comes from the near-surface 'interference zone' surrounding the impact site. This phenomenon explains the existence of unshocked meteorites on the Earth of lunar and martian origin. Impact of a large bolide on neighboring planets will produce high-speed, weakly shocked ejecta, which may be trapped by the Earth's gravitational field. 'Frozen crater' experiments show that the interference zone is highly localized; indeed, disaggregation does not extend beyond approx. 1.5 crater radii. A cone-shaped region extending downward from the impact site is completely disaggregated, including powdered rock that escaped into the projectile tube. Petrographic analysis of crater ejecta and wall material will be presented. Finally, study of ejecta from 0.9- and 1.3-GPa simulations of volcanic explosions reveal a complete lack of shock metamorphism. The ejecta shows no evidence of PDF's, amorphization, high-pressure phases, or mosaicism. Instead, all deformation was brittle, with fractures irregular (not planar) and most intergranular. The extent of fracturing was remarkable, with the entire sample reduced to fragments of gravel size and smaller.

Gratz, A. J.↗
NASA NTRS1992

Classification of four ordinary chondrites from the Monnig Meteorite Collection

We classified four ordinary chondrites from the Monnig Meteorite Collection into compositional groups, petrologic types and shock stages, based on optical microscopy in transmitted and reflected light, and electron microprobe and modal analyses. These meteorites are Allen, Texas, H4(S2): May Day, Kansas, H4(S2); Pony Creek, Texas, H4(S3); and Springer, Oklahoma, H5(S3).

Ehlmann, Arthur J.↗
NASA NTRS1992

Isotopic and molecular analyses of hydrocarbons and monocarboxylic acids of the Murchison meteorite

The monocarboxylic acids and hydrocarbons of the Murchison meteorite (CM2) were isolated for isotropic analysis. The nonvolatile hydrocarbons were analyzed as crude methanol and benzene-methanol extracts and also after separation by silica gel chromatography into predominantly aliphatic, aromatic, and polar hydrocarbon fractions. The volatile hydrocarbons were obtained after progressive decomposition of the meteorite matrix by freeze-thaw, hot water, and acid treatment. Molecular analyses of the aromatic hydrocarbons showed them to comprise a complex suite of compounds in which pyrene, fluoranthene, phenanthrene, and acenaphthene were the most abundant components, a result similar to earlier analyses. The polar hydrocarbons also comprise a very complex mixture in which aromatic ketones, nitrogen, and sulfur heterocycles were identified. The monocarboxylic acids, aliphatic, aromatic, and polar hydrocarbons, and the indigenous volatile hydrocarbons were found to be D-rich. The deuterium enrichment observed in these compounds is suggestive. In two separate analyses, the delta-D values of the nonvolatile hydrocarbons were observed to increase in the following order: aliphatic-aromatic-polar. This finding is consistent with an early solar system or parent body conversion of aromatic to aliphatic compounds as well as the suggestion of pyrolytic formation of aromatic from aliphatic compounds.

Krishnamurthy, R. V.↗
NASA NTRS1993

Experimental partitioning studies near the Fe-FeS eutectic, with an emphasis on elements important to iron meteorite chronologies (Pb, Ag, Pd, and Tl)

Partitioning coefficients for metal/sulfide liquid, troilite/sulfide liquid, and schreibersite/sulfide liquid were determined for Ag, Au, Mo, Ni, Pd, and Tl (using EMPA and proton-induced X-ray microprobe and ion microprobe analyses) in order to understand the chronometer systems of iron meteorites. In general, the obtained schreibersite/metal and troilite/metal partition coefficients for 'compatible' elements were quite similar to those inferred from natural assemblages, reinforcing an earlier made conclusion that there is a class of elements for which experimental troilite/metal and schreibersite/metal partition coefficients approximate those inferred from natural samples. The consistency between experimental and natural assemblages, however, was not observed for Ag, Pb, and Tl, indicating that the abundances of these elements determined in 'metal' and 'troilite' separates from iron meteorites are influenced by trace minerals that concentrate incompatible elements.

Jones, J. H.↗
NASA NTRS1993

An improbable concentration of basaltic meteorite falls (HED and mesosiderite) in the mid-20th century

The present examination of the historical record of HED and mesosiderite basaltic meteorite falls attempts to determine whether that record is consistent with completely random fall times. Strong evidence for nonrandomness emerges, in view of a significant cluster of falls for the 1924-1939 period. The causes of the cluster appear to have acted only on basaltic meteorites, and in a way that was of only 15-year-duration.

Treiman, Allan H.↗
NASA NTRS1990

Lunar meteorite Yamato-86032 - Mineralogical, petrological, and geochemical studies

Yamato-86032 is a shock-lithified anorthositic fragmental breccia. It consists mainly of highly feldspathic meta-breccias and meta-meltrocks and possibly contains a small contribution from mare lithologies, but there is no indication of a KREEP component. In many respects Y-86032 is similar to the previously described lunar meteorites Y-82192/3, but there are some notable differences. We have analyzed about 40 major and trace elements in bulk matrix, impact melt, and clast samples from two chips of Y-86032. The abundances of most lithophile and incompatible elements are lower in Y-86032 than in Y-82192 (which contains very low abundances compared to normal lunar highland rocks). The REE abundances are comparable to those of Y-82192. The elements Sc, Cr, Mn, Fe and Co have significantly lower abundances than in Y-82192, and the siderophile element pattern is also different. Since cosmic ray exposure data indicate pairing of Y-86032 with Y-82192/3, the source region for these meteorites on the moon must have been fairly heterogeneous.

Koeberl, Christian↗
NASA NTRS1993

Exposure history of the lunar meteorite, Elephant Moraine 87521

We report the noble gas concentrations and the Al-26, Be-10, Cl-36, and Ca-41 activities of the Antarctic lunar meteorite Elephant Moraine 87521. Although the actual exposure history of the meteorite may have been more complex, the following model history accounts satisfactorily for the cosmogenic nuclide data: A first stage of lunar irradiation for about 1 Ma at a depth of 1-5 g/sq cm followed, not necessarily directly, by a second one for 26 Ma at about 565 g/sq cm; launch from the moon less than 0.1 Ma ago; and arrival on earth 15-50 ka ago. The small concentration of trapped gases shows that except for some material that may have been introduced at the moment of launch, EET 87521 spent less than 1 Ma at a lunar depth less than 1 g/sq cm. EET 87521 has a K/Ar age in the range 3.0-3.4 Ga, which is typical for lunar mare basalts.

Vogt, S.↗