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At least 901 records · Page 50

Magnetic field impact on the laser heating in MagLIF

Prior to implosion in Magnetized Liner Inertial Fusion (MagLIF), the fuel is heated to temperatures on the order of several hundred eV with a multi-kJ, multi-ns laser pulse. In this paper, we present two laser heated plasma experiments, relevant to the MagLIF preheat stage, performed at Z with beryllium liners filled with deuterium and a trace amount of argon. In one experiment, there is no magnetic field and, in the other, the liner and fuel are magnetized with an 8.5 T axial magnetic field. The recorded time integrated, spatially resolved spectra of the Ar K-shell emission are sensitive to electron temperature T e . Individual analysis of the spatially resolved spectra produces electron temperature distributions T e (z) that are resolved along the axis of laser propagation. In the experiment with magnetic field, the plasma reaches higher temperatures and the heated region extends deeper within the liner than in the unmagnetized case. Radiation magnetohydrodynamics simulations of the experiments are presented and post-processed. A comparison of the results from experimental and simulated data reveals that the simulations underpredict T e in both cases but the differences are larger in the case with magnetic field.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Non-uniform longitudinal current density induced power saturation in GaAs-based high power diode lasers

The output power of modern 975 nm GaAs-based broad area diode lasers is limited by increasing carrier and photon losses at high bias. Here, we use experiment and one-dimensional calculations on these devices to reveal that higher current densities (and hence higher local recombination rates and higher losses) arise near the front facet due to spatial hole burning and that the non-uniformity is strongly affected by laser geometry, which is more severe for longer resonators and less severe for higher front facet reflectivity. Specifically, we use devices with a segmented p-contact to directly measure the current distribution along the resonator and compare this with laser simulation. Devices with a 6 mm resonator show 29% more current at the front than back, twice as large as the 15% current non-uniformity in devices with a 3 mm resonator. In contrast, increased front facet reflectivity (20% rather than 0.8%) is shown to almost halve the current non-uniformity from 29% to 18% in devices with a 6 mm resonator and reduces power saturation. Although the magnitude of current non-uniformity in experiment and theory is broadly consistent, in experiment, an additional divergence is seen in current flow (and hence recombination rate) near the facets, and earlier power saturation occurs. Finally, we discuss the possible saturation mechanisms that are not included in the simulation.

47 OTHER INSTRUMENTATION↗

Using extended MHD to explore lasers as a trigger for x-pinches

X-pinches have been shown to be a source of extremely intense x-ray emissions useful for diagnosing plasma dynamics and imaging biological objects. The most striking feature of an x-pinch is the hotspot, the point source from where all the x rays come from. Unfortunately, the exact timing and location of the hotspot are still unpredictable. Since an x-pinch hotspot forms from instabilities (like an m = 0 mode), we will computationally explore whether we can use a high-power laser to control the timing and location of these instabilities. Our goal is to reduce the temporal and spatial jitter associated with the x-ray burst. Using an extended MHD (XMHD) code, we explore the non-relativistic instability generation using a current profile of a 250 kA linear transformer driver system and laser characteristics of SLAC's Matter in Extreme Conditions laboratory. Our results include both laser-penetration results using a boundary-defined electromagnetic (EM) wave and instability results from a power-deposition method.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Spatio-temporal ablation dynamics and plasma chemistry of aluminum induced by temporally modulated ytterbium fiber laser

Here, in this work, we studied single-pulse ablation dynamics of a temporally modulated continuous wave laser-material interaction with Al using in situ multimodal time-resolved diagnostics that describe in detail the associated physical and chemical processes. Time-resolved scattering, emission imaging, and optical emission spectroscopy unveiled a sequence of events spread out across three distinct phases: (i) early phase ablation process, associated with particle generation and liquid Al column formation (<20 μs), (ii) secondary detonation when sufficient ejected material is accumulated over the surface (20-50 μs), and (iii) molten liquid Al pool oscillation on the surface, followed by large droplet ejection from the liquid pool (100-500 μs). Atomic Al and AlO were observed with optical emission spectroscopy at different ratios during the entire lifetime of the event, verifying the formation of oxidized Al vapor upon its interaction with air. Morphological and compositional characterization confirmed surface oxidation and material re-solidification in the form of protrusions produced during the irradiation process. This work provides insights into the complex physical and chemical mechanisms of single-pulse ablation in the sub-millisecond laser pulse regime, which are critically important for parameter optimization in a variety of laser processing, microfabrication, and deposition applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Comparison of excitation temperature of a laser-produced plasma by combining emission and absorption spectroscopy

Measurement of the temporal evolution of laser-produced plasma temperature is very important for many of its applications, and several plasma diagnostic tools are routinely used by researchers. However, it is very challenging to measure the properties of the plasma at the early and late times of its evolution using a single diagnostic tool. In this study, we combined emission and laser absorption spectroscopy to compare the excitation temperatures of a laser-produced uranium plasma system. Several U I transitions in the near-infrared spectral range (775–800 nm) were considered, and the Boltzmann plot method was used to measure the excitation temperatures using both emission and absorption spectroscopy. Emission spectroscopy provided early-time temperature measurements of the plasma up to times 2–20 µs, while absorption spectroscopy provided temperature measurements at late times of plasma evolution (for times 5–80 µs). The emission and absorbance of U I transitions were found to follow the Boltzmann distribution, indicating the plasma is likely in the state of local thermodynamic equilibrium even at late times of its lifetime. The emission and absorption-based time-resolved excitation temperatures demonstrated good agreement at earlier times (≤15 µs) in the overlapped temporal region, while a deviation in the measured values was seen at times (≥15 µs), and potential reasons for such a disagreement are discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Soft X-ray and EUV emission spectra of beryllium plasma produced by neodymium-glass laser radiation with broad frequency and angular spectra

We present the results of an experimental study of soft X-ray (SXR) and extreme ultraviolet emission spectra of the plasma produced by exposing a plane solid beryllium target to laser radiation with broad frequency and angular spectra. SXR lines up to 1s – 9p of Be IV as well as the plasma continuum are recorded for a laser focal-spot intensity of 5.3 × 10{sup 13} W cm{sup −2}. To model the SXR beryllium plasma spectra, simulations are carried out using the INDHAUS programme and the FLYCHK code in the framework of local thermodynamic equilibrium model, which agree nicely with experimentally obtained results. (laser plasma)

36 MATERIALS SCIENCE↗

Control of the optical properties of gum and dentin tissue of a human tooth at laser spectral lines in the range of 200 – 800 nm

A change in the optical properties of the tissue of the gums and dentin of a human tooth is experimentally investigated in vitro with the application of a 99.5 % glycerol solution. The kinetics of the total transmittance in the spectral range of 200 – 800 nm on characteristic laser lines is studied. It is shown that the effectiveness of optical clearing, expressed as a relative increase in the total transmittance, for gum tissue in the laser radiation range of 200 – 800 nm can vary significantly (by an order of magnitude). In this case, the absolute values of optical transmittance in the UV region are relatively small due to the strong absorption by the endogenous chromophores of the studied tissues, and in the visible and NIR regions, on the contrary, they are significant, which is due to the absence of strongly absorbing chromophores. The effectiveness of dentin clearing in the entire visible and NIR spectral regions is on average 25 % for 300 minutes of immersion of the sample in a 99.5 % glycerol solution. The presented results are necessary for increasing the efficiency of laser therapy and methods for optical monitoring of morphological changes in biological tissues for the purpose of early diagnosis of diseases. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Self-compression of laser pulses in a discrete medium

Using the discrete nonlinear Schrödinger equation, we study the laser radiation self-action dynamics in a nanostructured waveguide system. It is shown that for a laser pulse energy exceeding the critical value, the nonlinear evolution of the wave field markedly differs from the corresponding process in a continuous medium. While the pulse propagates in a discrete medium, its length decreases to values comparable to the scale of the structure and the velocity decreases to zero. The system parameters are determined at which the wave field after the laser pulse termination begins to propagate in the opposite direction in a compressed form. The process of slowing down and stopping the pulse is accompanied by strong radiation losses, so that about a third of the energy of the initial field distribution remains in the final compressed state. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Synthesis of TiO{sub 2} nanoparticles decorated with gold nanoclusters using pulsed laser ablation in liquid

Amorphous spherical titanium dioxide (TiO{sub 2}) nanoparticles, decorated gold nanoparticles, are shown to be formed under irradiation of commercial TiO{sub 2} nanopowders dispersed in aqueous solution of hydrogen tetrachloroaurate (HAuCl{sub 4}) by second-harmonic nanosecond pulses of an Nd : YAG laser. It is found that these hybrid nanostructures are formed during laser-induced remelting of the initial nanoparticles, stimulated by gold nanoclusters (providing more efficient absorption of visible laser radiation by titanium dioxide) recovered on their surface. The morphology and chemical composition of the newly formed hybrid nanomaterials are investigated in detail by electron microscopy, Raman spectroscopy, and energy-dispersive analysis. It is shown that the average size and number of gold nanoparticles recovered on the TiO{sub 2} surface can be controlled by varying the concentration ratio of the initial nanomaterial and HAuCl{sub 4}. A spectroscopic analysis of light scattering by single hybrid nanoparticles and the results of numerical calculation of the structure of electromagnetic fields near their surface indicate good prospects of these hybrid nanomaterials for various applications in modern optics, optoelectronics, and nanophotonics; for example, for designing chemo- and biosensor platforms and new-generation solar cells. (nanoparticles)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Compact ultrastable laser system for spectroscopy of {sup 2}S{sub 1/2} → {sup 2}D{sub 3/2} quadrupole transition in {sup 171}Yb{sup +} ion

We report the results of studying a compact laser system designed for manipulating a quantum state of the optical qubit based on the {sup 2}S{sub 1/2} → {sup 2}D{sub 3/2} quadrupole transition in the {sup 171}Yb{sup +} ion at a wavelength of 435.5 nm. An emission power of the laser system reaches 500 μW at λ = 435.5 nm and the relative frequency instability of at most 3 × 10{sup −15} is achieved at averaging intervals from 0.5 to 50 s with a subtracted linear frequency drift. The compactness of the developed system makes it possible to employ it in transportable systems including optical clocks. (laser spectroscopy)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Acousto-optic modulators of high-power laser radiation on the basis of KGW and KYW crystals

Different modifications of acousto-optic modulators (AOMs) based on KG(WO{sub 4}){sub 2} (KGW) and KY(WO{sub 4}){sub 2} (KYW) crystals, designed for Q switching of high-power pulsed lasers, is developed and investigated. It is shown that AOMs based on these crystals are universal, can be combined with different lasers in the wavelength range of 1 – 3 μm, and have a high radiation resistance in the absence of antireflection coatings and light input at Brewster’s angle. The operation efficiency of KGW-based AOMs is experimentally demonstrated. Solid-state lasers based on Cr : Er : YSGG (λ = 2.78 μm), Cr : Yb : Ho : YSGG (λ = 2.87 μm), Cr : Tm : Ho : YSGG (λ = 2.09 μm), and Nd : YAG (λ = 1.064 μm) crystals with active acousto-optic Q switching, operating in the repetitively pulsed regime with a high beam quality and without surface destruction, are investigated. Lasing pulses (30 – 60)-ns long with energy up to 32 mJ at a repetition rate from 1 to 1000 Hz are obtained. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Thermal conductivity of a laser plasma

Here, we present a model of the electron thermal conductivity of a laser-produced plasma. The model, supported by Vlasov–Fokker–Planck simulations, predicts that laser absorption reduces conductivity by forcing electrons out of a Maxwell–Boltzmann equilibrium, which results in depletion of both low-velocity bulk electrons and high-velocity tail electrons. We show that both the bulk and tail electrons approximately follow super-Gaussian distributions, but with distinct exponents that each depend on the laser intensity and wavelength through the parameter a = Zv$^{2}_{E}$/v$^{2}_{T}$. For a value of a = 0.5, tail depletion reduces the thermal conductivity to half its zero-intensity value. We present our results as simple analytic fits that can be readily implemented in any radiation-hydrodynamics code or used to correct the local limit of non-local conduction models.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Single-Shot Reconstruction of Electron Beam Longitudinal Phase Space in a Laser Wakefield Accelerator

We report on a single-shot longitudinal phase-space reconstruction diagnostic for electron beams in a laser wakefield accelerator via the experimental observation of distinct periodic modulations in the angularly resolved spectra. Such modulated angular spectra arise as a result of the direct interaction between the ultrarelativistic electron beam and the laser driver in the presence of the wakefield. A constrained theoretical model for the coupled oscillator, assisted by a genetic algorithm, can recreate the experimental electron spectra and, thus, fully reconstructs the longitudinal phase-space distribution of the electron beam with a temporal resolution of approximately 1.3 fs. In particular, it reveals the slice energy spread of the electron beam, which is important to measure for applications such as x-ray free electron lasers. In our experiment, the root-mean-square energy spread retrieved is bounded at 9.9 MeV, corresponding to a 0.9%–3.0% relative spread, despite the overall GeV energy beam having approximately 100% relative energy spread.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Amplification of laser imprint in the presence of strong, externally imposed, target-normal magnetic fields

Here, an experiment was performed on the OMEGA EP Laser System to investigate the effects of magnetic fields on laser imprint. A 30 µ⁢m thick CH target was driven by a single beam delivering 3.0 kJ of UV energy in a 5 ns square pulse without smoothing by spectral dispersion. The Rayleigh-Taylor amplification of this beam's imprint on the target surface was monitored using face-on gated x-ray radiography from a Gd backlighter. Magnetic fields of up to 45 T were applied normal to the target surface. Analysis of the resulting radiographs shows a 60 ± 13% increase in the spectrally resolved surface perturbation amplitudes, consistent at all times and for all unsaturated frequencies. This consistency indicates that the increase in perturbation amplitudes was due to a change in the initial amplitudes rather than Rayleigh-Taylor growth. This is supported by the trajectory of individual modes and the inferred time-averaged perturbation growth rates. Laser imprint is therefore inferred to have increased due to strong magnetic fields that remain in the conduction zone of the target, suppressing off-axis electron motion and limiting the effects of thermal smoothing.

direct drive↗

Compact, All-PM Fiber Integrated and Alignment-Free Ultrafast Yb:Fiber NALM Laser With Sub-Femtosecond Timing Jitter

We report a simple and compact design of a dispersion compensated mode-locked Yb:fiber oscillator based on a nonlinear amplifying loop mirror (NALM). The fully polarization maintaining (PM) fiber integrated laser features a chirped fiber Bragg grating (CFBG) for dispersion compensation and a fiber integrated compact non-reciprocal phase bias device, which is alignment-free. The main design parameters were determined by numerically simulating the pulse evolution in the oscillator and by analyzing their impact on the laser performance. Experimentally, we achieved an 88 fs compressed pulse duration with sub-fs timing jitter at 54 MHz repetition rate and 51 mW of output power with 5.5×10 -5 [20 Hz, 1 MHz] integrated relative intensity noise (RIN). Furthermore, we demonstrate tight phase-locking of the laser's carrier-envelope offset frequency ( fceo ) to a stable radio frequency (RF) reference and of one frequency comb tooth to a stable optical reference at 291 THz.

47 OTHER INSTRUMENTATION↗

Novel Process for Screen-Printed Selective Area Front Polysilicon Contacts for TOPCon Cells Using Laser Oxidation

The efficiency potential of double-side tunnel oxide passivated contact (DS-TOPCon) solar cells is limited by parasitic absorption in the front poly-Si layer, despite excellent passivation and high V OC . The use of patterned poly-Si only under the front metal grid lines can significantly reduce the parasitic absorption loss without sacrificing voltage. In this work, we demonstrate a simple, manufacturing-friendly method of patterning the front poly-Si using a nanosecond UV (355 nm) laser. We found that with laser powers ≥3 W at a 400 mm/s scan speed, an estimated 1–4 nm thick stoichiometric SiO 2 layer was grown on TOPCon. This served as a mask for KOH-etching of 200 nm poly-Si, allowing for patterning of poly-Si fingers required for selective TOPCon. While laser powers above 3 W caused substantial deterioration in passivation quality, the resulting damage in J 0 was largely recovered by subsequent PECVD SiN x deposition. At 3 W, the full area J 0 was found to be 36.8 fA·cm –2 . Furthermore, this translates to 1.68 fA·cm –2 for 4.48% coverage from the wing area of the polyfinger lines (100 lines–100 μm wide and 30 μm metal) contributing to a total front J 0 of ~10 fA·cm –2 , well suited for 25% efficient solar cells

42 ENGINEERING↗

High-Resolution Thermal Profiling of a High-Power Diode Laser Facet During Aging

Here, we study the facet temperature distribution of a high-power diode laser over its lifetime using a noncontact, high spatial resolution CCD-based thermoreflectance technique. Based on the known correlation between non-radiative defects and heating, thermal maps can provide valuable information regarding the formation and evolution of small point defects that are at or near the facet during aging. In the laser under study in this work we measure the appearance of local hot spots on the facet, including concentrated hot spots that appear just before or just after COD and are correlated with loss of local light emission. The locations of these hot spots do not exhibit morphology changes in high-resolution SEM imaging of the facet, indicating that the related defects are too small to be observable in SEM or are located at some depth under the facet. Prior to COD, we measure a gradual facet temperature increase accompanied by a gradual optical power decrease and gradual facet optical absorption increase, indicating gradual degradation of the laser.

47 OTHER INSTRUMENTATION↗

Doping engineering: Next step toward room temperature performance of terahertz quantum cascade lasers

We hereby offer a comprehensive analysis of various factors that could potentially enable terahertz quantum cascade lasers (THz QCLs) to achieve room temperature performance. We thoroughly examine and integrate the latest findings from recent studies in the field. Our work goes beyond a mere analysis; it represents a nuanced and comprehensive exploration of the intricate factors influencing the performance of THz QCLs. Through a comprehensive and holistic approach, we propose novel insights that significantly contribute to advancing strategies for improving the temperature performance of THz QCLs. This all-encompassing perspective allows us not only to present a synthesis of existing knowledge but also to offer a fresh and nuanced strategy to improve the temperature performance of THz QCLs. We draw new conclusions from prior works, demonstrating that the key to enhancing THz QCL temperature performance involves not only optimizing interface quality but also strategically managing doping density, its spatial distribution, and profile. This is based on our results from different structures, such as two experimentally demonstrated devices: the spit-well resonant-phonon and the two-well injector direct-phonon schemes for THz QCLs, which allow efficient isolation of the laser levels from excited and continuum states. In these schemes, the doping profile has a setback that lessens the overlap of the doped region with the active laser states. Our work stands as a valuable resource for researchers seeking to gain a deeper understanding of the evolving landscape of THz technology. Furthermore, we present a novel strategy for future endeavors, providing an enhanced framework for continued exploration in this dynamic field. This strategy should pave the way to potentially reach higher temperatures than the latest records reached for T max of THz QCLs.

47 OTHER INSTRUMENTATION↗