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At least 901 records · Page 50

Free energy and specific heat near a quantum critical point of a metal

We analyze the free energy and the specific heat for fermions interacting with a gapless boson at a quantum-critical point (QCP) in a metal. We use the Luttinger-Ward-Eliashberg formula for the free energy in the normal state, which includes contributions from bosons, fermions, and their interaction, all expressed via fully dressed fermionic and bosonic propagators. The sum of the last two contributions is the free energy F γ of an effective low-energy model of fermions with boson-mediated dynamical 4-fermion interaction V(Ω m ) ∝ 1/|Ω m | γ (the γ model). This purely electronic model has been used to analyze the interplay between non-Fermi liquid behavior and pairing near a QCP, which are both independent of the upper energy cutoff Λ. However, the specific heat C γ (T), obtained from F γ , does depend on Λ. We argue that this dependence is spurious and cancels out, once we include the contribution from bosons. We further argue that the full C(T) is the sum of the contribution from free fermions and the one from a critical boson, with the fully dressed propagator, other terms cancel out. We compare the full C(T) with the C γ (T), obtained using recently proposed regularization of F γ . We argue that for γ < 1, the full C(T) and the regularized C γ (T) differ by a γ-dependent prefactor, while for γ > 1, the full C(T) and C γ (T) differ by the positive contribution from free massless fermions (a positive constant for the electron-phonon case γ = 2). For these γ, C γ (T) is negative, but the full C(T) is positive. We argue that only the full C(T) matters as the positive and the negative contributions originate from the term in C(T) which contains the fully dressed bosonic propagator. Here, we then argue that the normal state remains stable until the pairing instability develops.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Imaging a terahertz superfluid plasmon in a two-dimensional superconductor

The superconducting gap defines the fundamental energy scale for the emergence of dissipationless transport and collective phenomena in a superconductor. In layered high-temperature cuprate superconductors, in which the Cooper pairs are confined to weakly coupled two-dimensional (2D) copper–oxygen (CuO 2 ) planes, terahertz (THz) spectroscopy at subgap millielectronvolt (meV) energies has provided crucial insights into the collective superfluid response perpendicular to the superconducting layers. However, within the CuO 2 planes, the collective superfluid response manifests as plasmonic charge oscillations at energies far exceeding the superconducting gap, obscured by strong dissipation. Here, in this study, we present spectroscopic evidence of a below-gap, 2D superfluid plasmon in few-layer Bi 2 Sr 2 CaCu 2 O 8+x and spatially resolve its deeply subdiffractive THz electrodynamics. By placing the superconductor in the near field of a spintronic THz emitter, we reveal this distinct resonance—absent in bulk samples and observed only in the superconducting phase—and determine its plasmonic nature by mapping the geometric anisotropy and dispersion. Crucially, these measurements offer a direct view of the momentum-dependent and frequency-dependent superconducting transition in two dimensions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Semicomputational calculation of Bragg shift in stratified materials

The fiber Bragg grating (FBG) may be viewed as a one dimensional photonic band-gap crystal by virtue of the periodic spatial perturbation imposed on the fiber core dielectric material. Similar to media supporting Bloch waves, the engraved weak index modulation, presenting a periodic “potential” to an incoming guided mode photon of the fiber, yields useful spectral properties that have been the basis for sensing applications and emerging quantum squeezing and solitons. The response of an FBG sensor to arbitrary external stimuli represents a multiphysics problem without a known analytical solution despite the growing use of FBGs in classical and quantum sensing and metrology. Here, we study this problem by first presenting a solid mechanics model for the thermal and elastic states of a stratified material. Additionally, the model considers an embedded optical material domain that represents the Bragg grating, here in the form of an FBG. Using the output of this model, we then compute the optical modes and their temperature- and stress-induced behavior. The developed model is applicable to media of arbitrary shape and composition, including soft matter and materials with nonlinear elasticity and geometric nonlinearity. Finally, we employ the computed surface stress and temperature distributions along the grating to analytically calculate the Bragg shift, which is found to be in reasonable agreement with our experimental measurements.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Tunable electron–flexural phonon interaction in graphene heterostructures

Peculiar electron-phonon interaction characteristics underpin the ultrahigh mobility, electron hydrodynamics, superconductivity, and superfluidity observed in graphene heterostructures. Here, the Lorenz ratio (L) between the electronic thermal conductivity and the product of the electrical conductivity and temperature provides unique insight into electron-phonon interactions that is inaccessible to past graphene measurements. Here we show an unusual L peak in degenerate graphene near 60 Kelvin and decreased peak magnitude with increased mobility. When combined with ab initio calculations of the many-body electron-phonon self-energy and analytical models, this experimental observation reveals that broken reflection symmetry in graphene heterostructures can relax a restrictive selection rule to allow quasielastic electron coupling with an odd number of flexural phonons, contributing to the increase of L toward the Sommerfeld limit at an intermediate temperature sandwiched between the low-temperature hydrodynamic regime and the inelastic electron-phonon scattering regime above 120 Kelvin. In contrast to past practices of neglecting flexural phonon contributions to transport in two-dimensional materials, this work suggests that tunable electron-flexural phonon coupling can provide a handle to control quantum matter at the atomic scale, such as magic angle twisted bilayer graphene where low-energy excitations may mediate Cooper pairing of flat-band electrons.

36 MATERIALS SCIENCE↗

Institute for Quantum Matter

The mission of the Institute for Quantum Matter (IQM) Energy Frontier Research Center was to discover and understand emergent properties in material systems with the potential for transformative impacts on energy and information technologies.

36 MATERIALS SCIENCE↗

Calibrating the scintillation and ionization responses of xenon recoils for high-energy dark matter searches

We report liquid xenon-based direct detection dark matter experiments have recently expanded their searches to include high-energy nuclear recoil events as motivated by effective field theory dark matter and inelastic dark matter interaction models, but few xenon recoil calibrations above 100 keV are currently available. In this work, we measured the scintillation and ionization yields of xenon recoils up to 426 keV. The experiment uses 14.1 MeV neutrons to scatter off xenon in a compact liquid xenon time projection chamber and produce quasimonoenergetic xenon recoils between 39 and 426 keV. We report the xenon recoil responses and their electric field dependence for recoil energies up to 306 keV; due to the low event statistics and the relatively mild field dependence, the yield values at higher energies are reported as the average of xenon responses for electric fields between 0.2 and 2.0 kV/cm. This result will enable xenon-based dark matter experiments to significantly increase their high-energy dark matter sensitivities by including energy regions that were previously inaccessible due to lack of calibrations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Field-resolved observation of exciton coherence in a van der Waals magnet

The emergence of coherence among electronic quasiparticles underlies collective quantum phenomena from superconductivity to superradiance. In semiconductors, exciton coherence is generally thought to decay rapidly due to scattering and dephasing, limiting its persistence on ultrafast timescales. Here, in this work, we demonstrate a light-field-driven mechanism that creates and stabilizes exciton coherence in the layered antiferromagnet CrSBr. We directly record the coherent optical field emitted by excitons and track in real time how a deterministic phase, imprinted by the excitation laser, drives incoherent excitons to synchronize into a collective state. This ensemble remains phase coherent for more than 2 ps, whereas its resonance energy undergoes an ultrafast modulation mediated by spin and lattice interactions. The time-resolved field evolution indicates that the multiple peaks seen in conventional spectra originate from a single excitonic resonance subject to dynamic energy modulation. Our findings establish optical phase imprinting as a mechanism to control and sustain collective order in semiconducting magnets, bridging light-driven dynamics with excitonic and magnetic correlations in layered quantum materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Light-induced anomalous Hall conductivity in the massive three-dimensional Dirac semimetal Co 3 ⁢Sn 2 ⁢S 2

Weyl semimetals can emerge from Dirac semimetals when the time-reversal or spatial-inversion symmetries are broken. Recently, it has been proposed based on Floquet theory that Dirac semimetals can be converted into Weyl semimetals even by shining circularly polarized light (CPL). Here we have investigated the possibility of such a Dirac-Weyl conversion by measuring the CPL-induced anomalous Hall conductivity (AHC) in a massive 3D Dirac semimetal Co 3 ⁢Sn 2 ⁢S 2 in the paramagnetic phase using ultrafast midinfrared pump-terahertz Faraday rotation probe spectroscopy. We find that the field-strength and driving frequency dependence of the observed AHC is well accounted for by CPL-induced nonzero Berry curvature associated with the splitting of the Dirac bands as predicted by the Floquet theory. As a result, the estimated splitting of the Dirac bands reaches about 60% of the mass gap and the calculated CPL-induced AHC quantitatively reproduces the experimental observation, demonstrating a promising route toward the realization of Floquet-Weyl states from massive Dirac semimetals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DC electrical conductivity measurements of warm dense matter using ultrafast THz radiation

We describe measurements of the DC electrical conductivity of warm dense matter using ultrafast terahertz (THz) pulses. THz fields are sufficiently slowly varying that they behave like DC fields on the timescale of electron–electron and electron–ion interactions and hence probe DC-like responses. Using a novel single-shot electro-optic sampling technique, the electrical conductivity of the laser-generated warm dense matter was determined with <1 ps temporal resolution. We present the details of the single-shot THz detection methodology as well as considerations for warm dense matter experiments. We, then, provide proof-of-concept studies on aluminum driven to the warm dense matter regime through isochoric heating and shock compression. Our results indicate a decrease in the conductivity when driven to warm dense matter conditions and provide a platform for future warm dense matter studies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Extremely Weakly Interacting ΔS z = 0 and ΔS z = 1 Excitations and Evidence for Fractional Quantization in a Magnetization Plateau: CeSb

The plateau at 1/3 of the saturation magnetization $M_s$ in the metamagnet CeSb is accompanied by a state of ferromagnetic layers of spins in an up-up-down sequence. We measured M and the specific heat C in the plateau, spin wave analyses of which reveal two distinct branches of excitations. Those with $ΔS_z = 1$ as measured by M, coexist with a much larger population of $ΔS_z = 0$ excitations measured by C but invisible to M. The large density of $ΔS_z = 0$ excitations, their energy gap, and their seeming lack of interaction with $ΔS_z = 1$ excitations suggest an analogy with astrophysical dark matter. Furthermore, in the middle of the plateau three sharp jumps in M(H) are seen, the size of which, $0.15 \% M_s$, is consistent with fractional quantization of magnetization per site in the down-spin layers.

36 MATERIALS SCIENCE↗

Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy

We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.

47 OTHER INSTRUMENTATION↗

Superconductivity from energy fluctuations in dilute quantum critical polar metals

Abstract Superconductivity in low carrier density metals challenges the conventional electron-phonon theory due to the absence of retardation required to overcome Coulomb repulsion. Here we demonstrate that pairing mediated by energy fluctuations, ubiquitously present close to continuous phase transitions, occurs in dilute quantum critical polar metals and results in a dome-like dependence of the superconducting T c on carrier density, characteristic of non-BCS superconductors. In quantum critical polar metals, the Coulomb repulsion is heavily screened, while the critical transverse optical phonons decouple from the electron charge. In the resulting vacuum, long-range attractive interactions emerge from the energy fluctuations of the critical phonons, resembling the gravitational interactions of a chargeless dark matter universe. Our estimates show that this mechanism may explain the critical temperatures observed in doped SrTiO 3 . We provide predictions for the enhancement of superconductivity near polar quantum criticality in two- and three-dimensional materials that can be used to test our theory.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

EXPANSE: A time-of-flight EXPanded Angle Neutron Spin Echo spectrometer at the Second Target Station of the Spallation Neutron Source

EXPANSE, an EXPanded Angle Neutron Spin Echo instrument, has been proposed and selected as one of the first suite of instruments to be built at the Second Target Station of the Spallation Neutron Source at the Oak Ridge National Laboratory. This instrument is designed to address scientific problems that involve high-energy resolution (neV– μeV) of dynamic processes in a wide range of materials. The wide-angle detector banks of EXPANSE provide coverage of nearly two orders of magnitude in scattering wavenumbers, and the wide wavelength band affords approximately four orders of magnitude in Fourier times. This instrument will offer unique capabilities that are not available in the currently existing neutron scattering instruments in the United States. Specifically, EXPANSE will enable direct measurements of slow dynamics in the time domain over wide Q-ranges simultaneously and will also enable time-resolved spectroscopic studies. The instrument is expected to contribute to a diverse range of science areas, including soft matter, polymers, biological materials, liquids and glasses, energy materials, unconventional magnets, and quantum materials.

47 OTHER INSTRUMENTATION↗

Early-Universe Simulations of the Cosmological Axion

Ultracompact dark matter (DM) minihalos at masses at and below 10 –12 $M_⊙$ arise in axion DM models where the Peccei-Quinn (PQ) symmetry is broken after inflation. The minihalos arise from density perturbations that are generated from the nontrivial axion self-interactions during and shortly after the collapse of the axion-string and domain-wall network. We perform high-resolution simulations of this scenario starting at the epoch before the PQ phase transition and ending at matter-radiation equality. We characterize the spectrum of primordial perturbations that are generated and comment on implications for efforts to detect axion DM. In this work, we also measure the DM density at different simulated masses and argue that the correct DM density is obtained for $m_a$ = 25.2 ± 11.0 μ eV .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Topology control of human fibroblast cells monolayer by liquid crystal elastomer

Eukaryotic cells in living tissues form dynamic patterns with spatially varying orientational order that affects important physiological processes such as apoptosis and cell migration. The challenge is how to impart a predesigned map of orientational order onto a growing tissue. Here, we demonstrate an approach to produce cell monolayers of human dermal fibroblasts with predesigned orientational patterns and topological defects using a photoaligned liquid crystal elastomer (LCE) that swells anisotropically in an aqueous medium. The patterns inscribed into the LCE are replicated by the tissue monolayer and cause a strong spatial variation of cells phenotype, their surface density, and number density fluctuations. Unbinding dynamics of defect pairs intrinsic to active matter is suppressed by anisotropic surface anchoring allowing the estimation of the elastic characteristics of the tissues. The demonstrated patterned LCE approach has potential to control the collective behavior of cells in living tissues, cell differentiation, and tissue morphogenesis.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Nuclear Matter in 1 + 1 Dimensions

We review the solution of QCD in two spacetime dimensions. Following the analysis of Baluni, for a single flavor, the model can be analyzed using Abelian bosonization. The theory can be analyzed in strong coupling, when the quarks are much lighter than the gauge coupling. In this limit, the theory is given by a Luttinger liquid.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Quantum control of exciton wave functions in 2D semiconductors

Excitons—bound electron-hole pairs—play a central role in light-matter interaction phenomena and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing challenge in solid-state optics has been to achieve precise and scalable control over excitonic motion. We present a technique using nanostructured gate electrodes to create tailored potential landscapes for excitons in 2D semiconductors, enabling in situ wave function shaping at the nanoscale. Our approach forms electrostatic traps for excitons in various geometries, such as quantum dots, rings, and arrays thereof. We show independent spectral tuning of spatially separated quantum dots, achieving degeneracy despite material disorder. Owing to the strong light-matter coupling of excitons in 2D semiconductors, we observe unambiguous signatures of confined exciton wave functions in optical reflection and photoluminescence measurements. This work unlocks possibilities for engineering exciton dynamics and interactions at the nanometer scale, with implications for optoelectronic devices, topological photonics, and quantum nonlinear optics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗