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At least 91 records · Page 5

A Comparison of Measurements from ATMOS and Instruments Aboard the ER-2 Aircraft: Tracers of Atmospheric Transport and Halogenated Gases

We compare volume mixing ratio profiles of N2O, O3, NO(y), H2O, CH4, and CO in the mid-latitude lower stratosphere measured by the ATMOS Fourier transform spectrometer on the ATLAS-3 Space Shuttle Mission with in situ measurements acquired from the NASA ER-2 aircraft during Nov 1994. ATMOS and ER-2 observations of (N2O) show good agreement, as do measured correlations of (O3), (NO(y)), (H2O), and (CH4) with (N2O). Thus a consistent measure of the hydrogen (H2O, CH4) content of the lower stratosphere is provided by the two platforms. The similarity of (NO(y)) determined by detection of individual species by ATMOS and the total (NOy) measurement on the ER-2 provides strong corroboration for the accuracy of both techniques. A 25% discrepancy in lower stratospheric (CO) observed by ATMOS and the ER-2 remains unexplained. Otherwise, the agreement for measurements of long-lived tracers demonstrates the ability to combine ATMOS data with in situ observations for quantifying atmospheric transport.

Chang, A. Y.↗

A Comparison of Measurements from ATMOS and Instruments Aboard the ER-2 Aircraft: Tracers of Atmospheric Transport

We compare volume mixing ratio profiles of N2O, O3, NO(y) H2O, CH4, and CO in the mid-latitude lower stratosphere measured by the ATMOS Fourier transform spectrometer on the ATLAS-3 Space Shuttle Mission with in situ measurements acquired from the NASA ER-2 aircraft during Nov 1994. ATMOS and ER-2 observations of [N2O] show good agreement, as do measured correlations of [O3], [NO(y)], [H2O], and [CH4] with [N2O]. Thus a consistent measure of the hydrogen (H2O, CH4) content of the lower stratosphere is provided by the two platforms. The similarity of [NO(y)] determined by detection of individual species by ATMOS and the total [NO(y)] measurement on the ER-2 provides strong corroboration for the accuracy of both techniques. A 25% discrepancy in lower stratospheric [CO] observed by ATMOS and the ER-2 remains unexplained. Otherwise, the agreement for measurements of long-lived tracers demonstrates the ability to combine ATMOS data with in situ observations for quantifying atmospheric transport.

Chang, A. Y.↗

[Analysis of Multiplatform CO (Carbon Monoxide) Measurements During Trace-P Mission]

Carbon monoxide is considered mission critical (TRACE-P NRA) because it is one of the gases involved in controlling the oxidizing power of the atmosphere and, as a tracer gas, is valuable in interpreting mission data sets. Carbon monoxide exhibits interannual differences, suggesting relatively short-term imbalances in sources and sinks. Sources of CO are dominated by fossil fuel combustion, biomass burning, and the photochemical oxidation of CH4 and nonmethane hydrocarbons while reaction with OH is believed to be the major sink for atmospheric CO, with additional losses due to soil uptake. Uncertainties in the magnitude and distribution of both sources and sinks remain fairly large however, and additional data are required to refine the global budget. Seasonal changes and a northern hemispheric latitudinal gradient have been described for a variety of Pacific basin sites through long-term monitoring of surface background levels. Latitudinal variations have also recently been described at upper tropospheric altitudes over a multi-year period by. TRACE-P will provide an aircraft survey of CO over the northern Pacific in the northern spring when CO concentrations are at their seasonal maximum in the northern hemisphere (NH) and at their seasonal minimum in the southern hemisphere (SH). Previous GTE missions, Le., PEM West-B and PEM Tropics-B, ground-based, and satellite observations (MAPS, April 1994) give us a general picture of the distribution of CO over the northern Pacific during this season. Based on these measurements, background CO levels over remote ocean areas are anticipated to be in the range of 110 - 180 ppbv, while those closer to the Asian continent may rise as high as 600 ppbv. These measurements also reveal high spatial variability (both horizontal and vertical) as well as temporal variations in CO over the area planned for the TRACE-P mission. This variability is a result of multiple CO sources, the meteorological complexity of transport processes, and the photochemical aging of air masses. The influence of biomass burning in the southern Pacific should be relatively small since the mission coincides with the southern tropical wet season when agricultural burning is at its seasonal low. The proposed CO measurements taken during TRACE-P should therefore largely be a function of the impact of various NH sources, primarily Asian and predominantly fossil fuel combustion and biomass burning. These processes are also major sources of many other atmospheric pollutants, consequently making accurate and precise CO measurements is one of the highest TRACE-P priorities [TRACE-P NRA]. The TRACE-P mission emphasizes the dual objectives of assessing the magnitude of the transport of chemically and radiatively important gases such as CO from Asia to the western Pacific, and determining how emissions change and are modified during this transport.

Pougatchev, Nikita S.↗

Multi-Campaign Ship and Aircraft Observations of Marine Cloud Condensation Nuclei and Droplet Concentrations

In-situ marine cloud droplet number concentrations (CDNCs), cloud condensation nuclei (CCN), and CCN proxies, based on particle sizes and optical properties, are accumulated from seven field campaigns: ACTIVATE; NAAMES; CAMP2EX; ORACLES; SOCRATES; MARCUS; and CAPRICORN2. Each campaign involves aircraft measurements, ship-based measurements, or both. Measurements collected over the North and Central Atlantic, Indo-Pacific, and Southern Oceans, represent a range of clean to polluted conditions in various climate regimes. With the extensive range of environmental conditions sampled, this data collection is ideal for testing satellite remote detection methods of CDNC and CCN in marine environments. Remote measurement methods are vital to expanding the available data in these difficult-to-reach regions of the Earth and improving our understanding of aerosolcloud interactions. The data collection includes particle composition and continental tracers to identify potential contributing CCN sources. Several of these campaigns include High Spectral Resolution Lidar (HSRL) and polarimetric imaging measurements and retrievals that will be the basis for the next generation of space-based remote sensors and, thus, can be utilized as satellite surrogates.

Atmospheric chemistry↗

Applied Uses of MERRA Reanalyses: Current and Future Prospects

During the initial planning of the Modern Era Retrospective-analysis for Research and Applications (MERRA), the project was envisioned to become a tool for applied sciences and decision makers, as well as weather and climate research. MERRA was the first reanalysis to provide data at 1 hourly frequencies. After discussions with wind energy users, 50m above the surface winds were included in the data collection to begin to represent the environment at the turbine height. MERRA-2 was the first reanalysis to include interactive and assimilated aerosols. From these, PM 1, 2.5 and 10 records have been computed and contribute to the climate and health sector. The US Center for Disease Control is accessing MERRA-2 data for comparison along with their health data. MERRA-2 Extreme Indices have been computed from the high frequency data (e.g. precipitation maxima, heat waves and fire weather). These have been used to characterize the changing extremes in the United States and around the globe as well as the weather associated with the extremes. The next-generation, MERRA-21C, includes increased resolution (25km) and continues to provide innovative Earth system data. For example, a boundary layer collection will provide constant height level data starting at 100m, continuing up to 4000m. This will provide detailed information about the boundary layer processes that greatly affect the biosphere. Chemical tracers for constituents are included in the system. The ensemble data assimilation is run with 32 members, and the variance for critical variables are stored. We will explore the use of this variance as one measure of uncertainty relevant for applied uses, which has not been included in any MERRA reanalysis. We will discuss use case scenarios developed to engage with the energy and financial sectors, to better understand their needs for climate data. Prospects for further downscaling of reanalyses will also be explored.

Michael Bosilovich↗

Origins of Energetic Ions in the Earth's Magnetosheath

The analysis and interpretation of the combined scientific data from the Hot Plasma Composition Experiment (HPCE) and the Charge Energy Mass (CHEM) spectrometer on the Active Mesospheric Particle Tracer Experiment (AMPTE) Charge Composition Explorer (CCE) spacecraft are discussed. These combined data sets have and will be used to survey the energetic ion environment in the Earth's magnetosheath to determine the origins and relative strengths of the energetic ion populations found there. A computer code was developed to analyze and interpret the data sets. The focus of the first year was on the determination of the contribution of leaked magnetospheric protons to the total energetic proton population. Emphasis was placed on intervals when the AMPTE spacecraft was in the plasma depletion layer because it was argued that in this region, only the leaked population contributes to the energetic ion population. Manipulation of the CHEM data and comparison of the CHEM and HPCE data over their common energy range near the magnetopause also contributed directly to a second study of that region.

Fuselter, S. A.↗

Is stellar differential rotation observable?

Daily measures of the disk integral 2.8 GHz solar flux from the years 1947 through 1982 are analyzed to determine the detectability of stellar differential rotation using the tracer method. Autocorrelation and power spectral analyses of 1 yr data sets yield rotation periods whose scatter about the mean period is too large to permit detection of the expected differential rotation signal. The principal noise source is the random appearance of tracer regions on the solar surface, in time and longitude. Criteria are given for optimizing stellar observations and analyses to detect differential rotation.

Labonte, B. J.↗

Biogeochemical Protocols and Diagnostics for the CMIP6 Ocean Model Intercomparison Project (OMIP)

The Ocean Model Intercomparison Project (OMIP) focuses on the physics and biogeochemistry of the ocean component of Earth system models participating in the sixth phase of the Coupled Model Intercomparison Project (CMIP6). OMIP aims to provide standard protocols and diagnostics for ocean models, while offering a forum to promote their common assessment and improvement. It also offers to compare solutions of the same ocean models when forced with reanalysis data (OMIP simulations) vs. when integrated within fully coupled Earth system models (CMIP6). Here we detail simulation protocols and diagnostics for OMIP's biogeochemical and inert chemical tracers. These passive-tracer simulations will be coupled to ocean circulation models, initialized with observational data or output from a model spin-up, and forced by repeating the 1948-2009 surface fluxes of heat, fresh water, and momentum. These so-called OMIP-BGC simulations include three inert chemical tracers (CFC-11, CFC-12, SF [subscript] 6) and biogeochemical tracers (e.g., dissolved inorganic carbon, carbon isotopes, alkalinity, nutrients, and oxygen). Modelers will use their preferred prognostic BGC model but should follow common guidelines for gas exchange and carbonate chemistry. Simulations include both natural and total carbon tracers. The required forced simulation (omip1) will be initialized with gridded observational climatologies. An optional forced simulation (omip1-spunup) will be initialized instead with BGC fields from a long model spin-up, preferably for 2000 years or more, and forced by repeating the same 62-year meteorological forcing. That optional run will also include abiotic tracers of total dissolved inorganic carbon and radiocarbon, CTabio and 14CTabio, to assess deep-ocean ventilation and distinguish the role of physics vs. biology. These simulations will be forced by observed atmospheric histories of the three inert gases and CO2 as well as carbon isotope ratios of CO2. OMIP-BGC simulation protocols are founded on those from previous phases of the Ocean Carbon-Cycle Model Intercomparison Project. They have been merged and updated to reflect improvements concerning gas exchange, carbonate chemistry, and new data for initial conditions and atmospheric gas histories. Code is provided to facilitate their implementation.

Carbon↗

An investigation into the flow behavior of a single phase gas system and a two phase gas/liquid system in normal gravity with nonuniform heating from above

The fluid behavior in normal gravity of a single phase gas system and a two phase gas/liquid system in an enclosed circular cylinder heated suddenly and nonuniformly from above was investigated. Flow visualization was used to obtain qualitative data on both systems. The use of thermochromatic liquid crystal particles as liquid phase flow tracers was evaluated as a possible means of simultaneously gathering both flow pattern and temperature gradient data for the two phase system. The results of the flow visualization experiments performed on both systems can be used to gain a better understanding of the behavior of such systems in a reduced gravity environment and aid in the verification of a numerical model of the system.

Disimile, Peter J.↗

Simulation of Ozone and Long Lived Tracers in the GSFC Two-Dimensional Model

The GSFC two-dimensional transport and chemistry model has been used for a wide variety of scientific and assessment studies of stratospheric ozone. Transport is a key element in the ozone simulations, and we have recently upgraded our model transport formulation to include much of the information about atmospheric transport processes available from existing data sets. To properly evaluate the model transport, it is desirable to examine the effects of transport and photochemistry separately. Recently, high quality observations of several long lived stratospheric tracers have become available from aircraft, balloon, and satellite measurement systems. This data provides a means to do a detailed model transport evaluation, as has been done in the recent Models and Measurements Intercomparison Project II. In this paper, we will discuss the GSFC 2D model simulations of ozone together with model-data comparisons of long lived tracers such as methane and the age of air transport diagnostic. We will show that the model can reproduce many of the transport-sensitive features observed in the stratosphere, and can compare reasonably well with measurements of both total ozone and long lived tracers simultaneously. We will also discuss the model deficiencies in simulating some of the detailed aspects of the observations.

Fleming, Eric L.↗

Observations of SO in dark and molecular clouds

The 1(0)-0(1) transition of SO at 30 GHz has been observed in several sources, including the first detection of sulfur monoxide in cold dark clouds without apparent internal energy sources. The SO transition appears to be an excellent tracer of structure in dark clouds, and the data support suggestions that self-absorption is important in determining emission profiles in such regions for large line-strength transitions. Column densities estimated from a comparison of the results for the two isotopic species indicate a high fractional abundance of SO in dark clouds.

Rydbeck, O. E. H.↗

Designing Delta-DOR acquisition strategies to determine highly elliptical earth orbits

Delta-DOR acquisition strategies are designed for use in determining highly elliptical earth orbits. The requirements for a possible flight demonstration are evaluated for the Charged Composition Explorer spacecraft of the Active Magnetospheric Particle Tracer Explorers. The best-performing strategy uses data spanning the view periods of two orthogonal baselines near the same orbit periapse. The rapidly changing viewing geometry yields both angular position and velocity information, but each observation may require a different reference quasar. The Delta-DOR data noise is highly dependent on acquisition geometry, varying several orders of magnitude across the baseline view periods. Strategies are selected to minimize the measurement noise predicted by a theoretical model. Although the CCE transponder is limited by S-band and a small bandwidth, the addition of Delta-DOR to coherent Doppler and range improves the one-sigma apogee position accuracy by more than an order of magnitude. Additional Delta-DOR accuracy improvements possible using dual-frequency (S/X) calibration, increased spanned bandwidth, and water-vapor radiometry are presented for comparison. With these benefits, the residual Delta-DOR data noise is primarily due to quasar position uncertainties.

Frauenholz, R. B.↗

Venus O2 visible and IR nightglow: Implications for lower thermosphere dynamics and chemistry

The National Center for Atmospheric Research thermospheric general circulation model for the Venus thermosphere is modified to examine two observed night airglow features, both of which serve as sensitive tracers of the thermospheric circulation. New O2 nightglow data from the Pioneer Venus Orbiter (PVO) star tracker (O2 Herzberg II at 400-800 nm) and ground-based telescopes (O2 IR at 1.27 microns) yield additional model constraints for estimating Venus winds over 100-130 km. Atomic oxygen, produced by dayside CO2 photolysis peaking near 110 km, and transported to the nightside by the global wind system, is partially destroyed through three-body recombination, yielding the O2 Herzberg II visible nightglow. This emission is very sensitive to horizontal winds at altitudes between 100 and 130 km. Other trace species catalytic reactions also contribute to the production of the very strong nightside infrared (1.27 microns) emission. This paper examines the dynamical and chemical implications of these new data using the Venus thermospheric general circulation model (VTGCM) as an analysis tool. Three-dimensional calculations are presented for both solar maximum and solar medium conditions, corresponding to early PVO (1979-1981) and PVO entry (mid-1992) time periods. Very distinct periods are identified in which zonal winds are alternately weak and strong in the Venus lower thermosphere. VTGCM sensitivity studies are conducted to assess the impacts of potential changes in thermospheric zonal and day-to-night winds, and eddy diffusion on the corresponding nightglow intensities. It appears that cyclostrophic balance extends above 80 km periodically, owing to a reversal of the upper mesosphere latitudinal temperature gradient, and thereby producing strong zonal winds and correspondingly modified O2 nightglow distributions that are observed.

Bougher, S. W.↗

Quasi-horizontal transport and mixing in the Antarctic stratosphre

The quasi-horizontal transport and mixing properties of the Antarctic stratosphere are investigated with a simi-Lagrangian transport model and a 'contour advection' technique for the winter and spring of 1992 using analyzed winds from the United Kingdom Meteorological Office data assimiliation system. Transport calculations show that passive tracers are well mixed inside the polar vortex as well as in the midlatitude 'surf zone.' A the vortex edge, strong radial gradients in the tracer fields are well preserved, and their evolutions follow that of the potential vorticity until some time after the breakdown of the polar vortex. In the middle stratosphere there is little tracer exchange across the vortex edge in August and September. Some vortex air is eroded into the surf zone in filamentary form in October, and very strong exchange of air occurs between high and middle latitudes in November. In the lower stratosphere the vortex is not so isolated from the midlatitudes as in the middle stratosphere, and there is more mass exchange across the vortex edge. Calculations of the lengthening of material contours using the contour advection technique show that in the middle stratosphere, strong stirring (i.e., stretching and folding of material elements) occurs in the inner vortex, while the strongest stirring occurs in the midlatitude surf zone and the weakest occurs at the vortex edge. In the lower strtosphere, strong stirring occurs in the inner vortex. Stirring is moderate at the vortex edge and in the midlatitudes.

Chen, Ping↗

Radon as a tracer of biogenic gas equilibration and transport from methane-saturated sediments

Data on Rn-222 activity in methane-rich gas bubbles from anoxic coastal sediments of Cape Lookout Bight, North Carolina, were used to determine gas equilibration with pore waters and the rates of ebullitive stripping and transport of gases to overlying waters and the atmosphere. Results showed that, during summer months, the bubble ebullition process strips and transports 1.9-4.8 percent/day of the standing crop of radon (and, by inference, other gases equilibrated with gas bubbles) in surface sediments of Cape Lookout Bight to the troposphere. Thus, the ebullitive mode of gas transport represents an effective mechanism for delivering reduced biogenic gases directly to the atmosphere.

Martens, Christopher S.↗

An experimental method for measuring droplet impingement efficiency on two- and three-dimensional bodies

An efficient and accurate method is described for extracting water droplet impingement efficiency data from dye impregnated blotter paper samples obtained by employing a dye-tracer technique in wind tunnel spray tests. The method is based on laser reflectance spectroscopy. A brief description of the test method, instrumentation, and data reduction system is also presented. Preliminary test results and analyses are included for a cylinder and a 65(2)015 airfoil.

Papadakis, M.↗

Stereo Imaging Velocimetry

Stereo imaging velocimetry (SIV) will permit the collection of quantitative, three-dimensional flow data from any optically transparent fluid that can be seeded with tracer particles. This includes such diverse experiments as the study of multiphase flow, bubble nucleation and migration, pool combustion, and crystal growth. This technique will be useful to the microgravity science community as our investigations of fluid behavior in reduced-gravity environments enhance our knowledge of heat transfer, surface tension, concentration-gradient-driven anomalies, and residual effects from g-jitter. In its proposed configuration, the NASA Lewis Research Center's Stereo Imaging Velocimeter will consist of at least two charged coupled device (CCD) cameras, oriented at some relative angle with respect to each other. The cameras will observe a fluid experiment that has been seeded with tracer particles that are neutrally buoyant to permit accurate flow tracking. Except for the tracer particles, this measurement technique will be nonintrusive. Velocity accuracies will be on the order of 1 to 5 percent of full field. Each camera will make a two-dimensional record of the motion of the seed particles in the observation volume. Three-dimensional data will be obtained by computationally combining the two-dimensional information.

Source record↗

Completing the Feedback Loop: The Impact of Chlorophyll Data Assimilation on the Ocean State

In anticipation of the integration of a full biochemical model into the next generation GMAO coupled system, an intermediate solution has been implemented to estimate the penetration depth (1Kd_PAR) of ocean radiation based on the chlorophyll concentration. The chlorophyll is modeled as a tracer with sources-sinks coming from the assimilation of MODIS chlorophyll data. Two experiments were conducted with the coupled ocean-atmosphere model. In the first, climatological values of Kpar were used. In the second, retrieved daily chlorophyll concentrations were assimilated and Kd_PAR was derived according to Morel et al (2007). No other data was assimilated to isolate the effects of the time-evolving chlorophyll field. The daily MODIS Kd_PAR product was used to validate the skill of the penetration depth estimation and the MERRA-OCEAN re-analysis was used as a benchmark to study the sensitivity of the upper ocean heat content and vertical temperature distribution to the chlorophyll input. In the experiment with daily chlorophyll data assimilation, the penetration depth was estimated more accurately, especially in the tropics. As a result, the temperature bias of the model was reduced. A notably robust albeit small (2-5 percent) improvement was found across the equatorial Pacific ocean, which is a critical region for seasonal to inter-annual prediction.

MERRA-OCEAN↗