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At least 91 records · Page 5

Dynamic sparse x-ray nanotomography reveals ionomer hydration mechanism in polymer electrolyte fuel-cell catalyst

Tomographic imaging of time-evolving samples is a challenging yet important task for various research fields. At the nanoscale, current approaches face limitations of measurement speed or resolution due to lengthy acquisitions. We developed a dynamic nanotomography technique based on sparse dynamic imaging and 4D tomography modeling. We demonstrated the technique, using ptychographic x-ray computed tomography as its imaging modality, on resolving the in situ hydration process of polymer electrolyte fuel cell (PEFC) catalyst. The technique provides a 40-time increase in temporal resolution compared to conventional approaches, yielding 28 nm half-period spatial and 12 min temporal resolution. The results allow a quantitative characterization of the water intake process inside PEFC catalysts with nanoscale resolution, which is crucial for understanding their electrochemical mechanisms and optimizing their performance. Our technique enables high-speed operando nanotomography studies and paves the way for wider application of dynamic tomography at the nanoscale.

Science & Technology - Other Topics↗

Exploring baryon resonances with transition generalized parton distributions: status and perspectives

QCD gives rise to a rich spectrum of excited baryon states. Understanding their internal structure is important for many areas of nuclear physics, such as nuclear forces, dense matter, and neutrino-nucleus interactions. Generalized parton distributions (GPDs) are an established tool for characterizing the QCD structure of the ground-state nucleon. They are used to create 3D tomographic images of the quark/gluon structure and quantify the mechanical properties such as the distribution of mass, angular momentum, and forces in the system. Transition GPDs extend these concepts to N → N* transitions and can be used to characterize the 3D structure and mechanical properties of baryon resonances. They can be probed in high-momentum-transfer exclusive electroproduction processes with resonance transitions e + N → e' + M + N*, such as deeply-virtual Compton scattering (M = γ) or meson production (M = π, K, etc.), and in related photon/hadron-induced processes. This White Paper describes a research program aiming to explore baryon resonance structure with transition GPDs. This includes the properties and interpretation of the transition GPDs, theoretical methods for structures and processes, first experimental results from JLab 12 GeV, future measurements with existing and planned facilities (JLab detector and energy upgrades, COMPASS/AMBER, EIC, EicC, J-PARC, LHC ultraperipheral collisions), and the theoretical and experimental developments needed to realize this program.

Experimental Nuclear Physics↗

Scalable FBP decomposition for cone-beam CT reconstruction

Filtered Back-Projection (FBP) is a fundamental compute intense algorithm used in tomographic image reconstruction. Cone-Beam Computed Tomography (CBCT) devices use a cone-shaped X-ray beam, in comparison to the parallel beam used in older CT generations. Distributed image reconstruction of cone-beam datasets typically relies on dividing batches of images into different nodes. This simple input decomposition, however, introduces limits on input/output sizes and scalability.We propose a novel decomposition scheme and reconstruction algorithm for distributed FPB. This scheme enables arbitrarily large input/output sizes, eliminates the redundancy arising in the end-to-end pipeline and improves the scalability by replacing two communication collectives with only one segmented reduction. Finally, we implement the proposed decomposition scheme in a framework that is useful for all current-generation CT devices (7th gen). In our experiments using up to 1024 GPUs, our framework can construct 40963 volumes, for real-world datasets, in under 16 seconds (including I/O).

Chen, Peng↗

TomoTwin: A simple digital twin for synchrotron tomography

A digital twin for synchrotron-based tomography for generating synthetic datasets from ground-truth phantoms. The code outputs greyscale projection images / tomographic volumes with realistic artifacts such as noise and phase-contrast and emulates their dependence on the acquisition parameters defining the beam and detector configuration. Some ground-truth phantoms are included with the code.

TEKAWADE, ANIKET↗

Strong intracellular signal inactivation produces sharper and more robust signaling from cell membrane to nucleus

For a chemical signal to propagate across a cell, it must navigate a tortuous environment involving a variety of organelle barriers. In this work we study mathematical models for a basic chemical signal, the arrival times at the nuclear membrane of proteins that are activated at the cell membrane and diffuse throughout the cytosol. Organelle surfaces within human B cells are reconstructed from soft X-ray tomographic images, and modeled as reflecting barriers to the molecules’ diffusion. We show that signal inactivation sharpens signals, reducing variability in the arrival time at the nuclear membrane. Inactivation can also compensate for an observed slowdown in signal propagation induced by the presence of organelle barriers, leading to arrival times at the nuclear membrane that are comparable to models in which the cytosol is treated as an open, empty region. In the limit of strong signal inactivation this is achieved by filtering out molecules that traverse non-geodesic paths.

59 BASIC BIOLOGICAL SCIENCES↗

Nanoscale x-ray and electron tomography

We present that three-dimensional (3D) tomographic imaging of the structural, chemical, and physical properties of a material provides key knowledge that links the structure of a material to both its processing and structure that is central to studies across a broad spectrum of materials. For many decades, tomography using x-rays or electrons has proven to be an essential 3D characterization tool. In recent years, advances in technology have significantly pushed the envelope of these techniques in many respects, enabling new imaging capabilities at the nanometer and atomic scale. This article highlights several such developments in nanoscale x-ray and electron tomography. The five articles that appear in this issue of MRS Bulletin discuss research frontiers that include multimodal x-ray tomography at the nanoscale, x-ray spectroscopic tomography, dark-field x-ray microscopy, electron nanotomography for functional nanomaterials, and atomistic imaging by electron tomography. Lastly, these articles give a holistic view of the status of these techniques and promising future directions, as well highlighting their applications for scientific problems.

36 MATERIALS SCIENCE↗

Relocation of the 8 September 2023 High Atlas, Morocco, Earthquake Aftershock Sequence

The earthquake that occurred on 8 September 2023, with a magnitude of 6.8, was the most destructive earthquake event in Morocco in the past decade. This earthquake took place in the Al Haouz region, located in the western part of the High Atlas Mountain range. To better understand what caused and triggered this earthquake, the earthquake catalogs including P and S arrival times were collected from the Moroccan seismic network and combined with regional data from the International Seismological Centre. The mainshock and aftershocks were relocated by using iLoc, a state-of-the-art single-event location algorithm, and then by the multiple event location double-difference algorithm, hypoDD. The improved earthquake relocations using iLoc and the double-difference methods provide sharper lineation of seismicity and agree well with tomographic images of the earthquake zone. Finally, the seismicity distribution and the focal mechanism of the mainshock indicate that the earthquake sequence has occurred along the South Atlas fault system.

58 GEOSCIENCES↗

SU(n) and Quantum SU(n) Symmetries in Physical Systems [Slides]

Presence of SU(n) or other Lie group symmetry in a physical system is its powerful, usually underutilized property. In many cases it allows for finding analytical solutions to nonlinear differential equations describing this system. Power of the method is presented on diversified examples from mathematical physics: Lie-group symmetries in finding solutions of generalized, multidimensional theory of gravity; analytical Dirac–equation solutions for description of conducting polymers; stability of qubit states in quantum computers; spatial defects in condensed matter; reconstruction of 3D object from its 2D tomographic image; significant improvement of numerical solutions stability for Euler equations. The next question after obtaining such Lie group symmetric solution is: does a generalized solution with appropriate quantum group symmetry exists for the given physical system, and if yes what is the physical meaning of the deformation parameter q introduced by such solution. In many cases it can be identified. Any SU(n) solution is by its nature singular, assuming a perfect symmetry of the physical system discussed. Such solution gives a powerful insight to theoretical physics, yet the assumption may be too demanding for experimental applications. Deformation parameter q from a quantum group symmetry allows for a continuum of solutions, more applicable to experiments.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Earthquake Relocation in Rock Valley, NV Using Absolute and Differential Times

In this brief report we document algorithmic choices and updates to our code related to the earthquake relocation portion of our tomographic imaging algorithm. We show results of these improvements by relocating over 40,000 events located within 20-30 km of the Rock Valley Direct Comparison (RV/DC) site using both absolute and differential arrival times within the context of two different 3-D Earth models. Accurate hypocentral locations and Earth models are important to the ultimate goals of the RV/DC program, which will co-locate a chemical explosion with a shallow earthquake within Rock Valley, southern Nevada, to investigate differences between the source types and improve our analysis algorithms for both types (Snelson et al., 2022). Our improvements to our relocation algorithms comprise just one step toward achieving these goals

58 GEOSCIENCES↗

Overview on the theory and phenomenology of generalized parton distributions

We give a brief overview on the theory and phenomenology of generalized parton distributions (GPDs), including the recently developed framework of single-diffractive hard exclusive process for matching GPDs to experimental observables. We concentrate on the extraction of GPDs from experimental processes, especially on the challenges and potential solutions regarding the separation of different GPDs and the extraction of $x$-dependence of GPDs, which is critically important for constructing the tomographic images and matching the $x$-moments of GPDs to various emergent hadron properties.

Qiu, Jianwei↗

Riverbed Temperature and 4D ERT Monitoring Reveals Heterogenous Horizontal and Vertical Groundwater-Surface Water Exchange Flows Under Dynamic Stage Conditions

Groundwater surface water exchange plays a critical role in physical, biological, and geochemical function of coastal and riverine systems. Observing exchange flow behavior in heterogeneous systems is a primary challenge, particularly when flows are governed by dynamic river stage or tidal variations. In this paper we demonstrate a novel application of time-lapse 3D electrical resistivity tomography and temperature monitoring where an array of thermistors installed beneath a riverbed double as resistivity electrodes. We use the array to monitor stage driven exchange flows over a 6-day period in a dynamic, stage-driven high order stream. We present a method for addressing the otherwise confounding effects of the moving river-surface boundary on the raw resistivity data, thereby enabling successful tomographic imaging. Temperature time-series at each thermistor location and time-lapse 3D images of changes in bulk electrical conductivity together provide a detailed description of exchange dynamics over a 10-meter by 45-meter section of the riverbed, to a depth of approximately 5 m. Results reveal highly variable flux behavior throughout the monitoring domain including both horizontal and vertical exchange flows.

54 ENVIRONMENTAL SCIENCES↗

CP Puppis - No ordinary old nova

We present spectrophotometric data for the old nova CP Puppis (Nova Puppis 1942) that demonstrates the simultaneous existence of two distinct periods for the system. We find that the photometric period of 0.06834(7) day is 11 percent longer than the spectroscopic period. We also present Doppler tomographic images of CP Pup that indicate the existence of an accretion disk in the system. Finally, we interpret the observational evidence in terms of a DQ Herculis model and an SU Ursae Majoris model for CP Pup. While the evidence mildly supports both interpretations, it is insufficient for us to conclusively classify CP Pup as either a DQ Her system or an SU UMa system.

White, James C., II↗

Three-dimensional spherical models of layered and whole mantle convection

We present numerical calculations of three-dimensional spherical shell thermal convection for constant viscosity and stratified viscosity models of whole-layer and two-layer mantle convection. These four examples are intended to provide theoretical guidance for determining the style of convection that is occurring in Earth's mantle. An impermeable interface between the upper and lower convecting shells in the two-layer solutions is placed at a depth of 670 km to coincide with the mantle seismic discontinuity that divides the upper and lower mantle. The interface results in an internal thermal boundary layer that raises the mean temperature in the lower shell by about 1400 K compared to the whole-layer solutions. The patterns of convection in the upper part of the whole-layer solutions are dominated by narrow arcuate sheetlike downflows in a background of weak upflow. In contrast, the upper shells of the two-layer solutions have complicated networks of convective rolls with the upflows and downflows having very similar structure. The structure of convection in the lower shells is similar to that in the lower part of the whole-layer solutions. Based on the horizontal structure of subduction zones on Earth's surface and on tomographic images of temperature variations in Earth's mantle, we conclude that the style of convection in Earth's mantle is more like that of the whole-mantle models.

Glatzmaier, Gary A.↗

Magnetospheric Radio Tomography: Observables, Algorithms, and Experimental Analysis

This grant supported research towards developing magnetospheric electron density and magnetic field remote sensing techniques via multistatic radio propagation and tomographic image reconstruction. This work was motivated by the need to better develop the basic technique of magnetospheric radio tomography, which holds substantial promise as a technology uniquely capable of imaging magnetic field and electron density in the magnetosphere on large scales with rapid cadence. Such images would provide an unprecedented and needed view into magnetospheric processes. By highlighting the systems-level interconnectedness of different regions, our understanding of space weather processes and ability to predict them would be dramatically enhanced. Three peer-reviewed publications and 5 conference presentations have resulted from this work, which supported 1 PhD student and 1 postdoctoral researcher. One more paper is in progress and will be submitted shortly. Because the main results of this research have been published or are soon to be published in refereed journal articles listed in the reference section of this document, we provide here an overview of the research and accomplishments without describing all of the details that are contained in the articles.

Cummer, Steven↗

Direct Observations of Nucleation in a Nondilute Multicomponent Alloy

The chemical pathways leading to gamma'(L1(sub 2)) nucleation from nondilute Ni-5.2 Al-14.2 Cr at. %, gama(fcc), at 873 K are followed with radial distribution functions and isoconcentration surface analyses of direct-space atom-probe tomographic images. Although Cr atoms initially are randomly distributed, a distribution of congruent Ni3Al short-range-order domains (SRO), [R] approx. equals 0.6 nm, results from Al diffusion during quenching. Domain site occupancy develops as their number density increases leading to Al-rich phase separation by gamma'-nucleation, [R]=0.75 nm, after SRO occurs.

Sudbrack, Chantal K.↗

Medical tomograph system using ultrasonic transmission

Ultrasonic energy transmission in rectilinear array scanning patterns of soft tissue provides projection density values of the tissue which are recorded as a function of scanning position and angular relationship, .theta., of the subject with a fixed coordinate system. A plurality of rectilinear scan arrays in the same plane for different angular relationships .theta..sub.1 . . . .theta..sub.n thus recorded are superimposed. The superimposition of intensity values thus yields a tomographic image of an internal section of the tissue in the scanning plane.

Heyser, Richard C.↗

Measurements on NASA Langley Durable Combustor Rig by TDLAT: Preliminary Results

Detailed knowledge of the internal structure of high-enthalpy flows can provide valuable insight to the performance of scramjet combustors. Tunable Diode Laser Absorption Spectroscopy (TDLAS) is often employed to measure temperature and species concentration. However, TDLAS is a path-integrated line-of-sight (LOS) measurement, and thus does not produce spatially resolved distributions. Tunable Diode Laser Absorption Tomography (TDLAT) is a non-intrusive measurement technique for determining two-dimensional spatially resolved distributions of temperature and species concentration in high enthalpy flows. TDLAT combines TDLAS with tomographic image reconstruction. Several separate line-of-sight TDLAS measurements are analyzed in order to produce highly resolved temperature and species concentration distributions. Measurements have been collected at the University of Virginia's Supersonic Combustion Facility (UVaSCF) as well as at the NASA Langley Direct-Connect Supersonic Combustion Test Facility (DCSCTF). Measurements collected at the DCSCTF required significant modifications to system hardware and software designs due to its larger measurement area and shorter test duration. Initial LOS measurements from the NASA Langley DCSCTF operating at an equivalence ratio of 0.5 are presented. Results show the capability of TDLAT to adapt to several experimental setups and test parameters.

Busa, Kristin↗

Electrical Impedance Tomography Technology (EITT) Project

Development of a portable, lightweight device providing two-dimensional tomographic imaging of the human body using impedance mapping. This technology can be developed to evaluate health risks and provide appropriate medical care on the ISS, during space travel and on the ground.

Technology Portfolio System↗