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Pair breaking in superconductors with strong spin-orbit coupling
Here we study the influence of symmetry-breaking perturbations on superconductivity in multiorbital materials, with a particular focus on an external magnetic field. We introduce the field-fitness function which characterizes the pair-breaking effects of the perturbation on a given superconducting state. For even-parity superconductors we find that this field-fitness function for an external magnetic field is one, implying that the paramagnetic response is controlled only by a generalized effective g factor. For odd-parity superconductors, the interplay of the effective g factor and the field-fitness function can lead to counterintuitive results. We demonstrate this for p-wave pairing in the effective j = $\frac{3}{2}$ electronic states of the Luttinger-Kohn model.
Correlated phases in spin-orbit-coupled rhombohedral trilayer graphene
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Emergent bright excitons with Rashba spin-orbit coupling in atomic monolayers
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Topological superconductivity induced by spin-orbit coupling, perpendicular magnetic field, and superlattice potential
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Finite-element methods for noncollinear magnetism and spin-orbit coupling in real-space pseudopotential density functional theory
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Magnetism and Spin-Orbit Coupling in Iron Chalcogenide Superconductors
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Theoretical study of the spin-orbit coupling constants of C/2p/3Pi u, d/3p/3Pi u, k/4p/3Pi u, i/3d/3Pi g, r/4d/3Pi g, j/3d/3Delta g, and /4f/3 Delta u states of H2
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XTE Observations of PSR 1259-63 and a Test of Spin Orbit Coupling in the 4U0115+63 System
During this report period, Mallory Roberts went to GSFC to analyze the data from two minor outbursts, which occurred from 4UO115+63. Unfortunately, the outbursts were not of sufficient duration to do a unique orbital determination (which was the scientific goal of the experiment). As this report is being written, 4UO115+63 is undergoing its first major outburst in four years. We are planning on adding our RXTE PCA data to any public ASM or PCA data that is obtained through the duration of this outburst, and combining it with our BATSE data from 1994 and 1995 outbursts in order to learn something about the orbital evolution in this system. We have formed a collaboration with colleagues at MIT who are working on the ASM data for this outburst. Thus, work on the original data will continue, with no further funding, and we are hopeful that some important questions with regard to the orbital timing will finally be resolved. The PSR 1259-63 data were originally analyzed by Barry Giles, who reported that no pulsations or flux were seen from this source near apastron. Recently, a new background model for low-count rate sources has been developed for the PCA. We intend to use this new background model to reanalyze these data to see if we can improve the upper limit to the flux. This work will also continue with no further funding.
Low-Scaling Perturbative Spin-Orbit Coupling for Closed-Shell Time-Dependent DFT
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Uncovering spin-orbit coupling-independent hidden spin polarization of energy bands in antiferromagnets
Abstract Many textbook physical effects in crystals are enabled by some specific symmetries. In contrast to such ‘apparent effects’, ‘hidden effect X’ refers to the general condition where the nominal global system symmetry would disallow the effect X, whereas the symmetry of local sectors within the crystal would enable effect X. Known examples include the hidden Rashba and/or hidden Dresselhaus spin polarization that require spin-orbit coupling, but unlike their apparent counterparts are demonstrated to exist in non-magnetic systems even in inversion-symmetric crystals. Here, we discuss hidden spin polarization effect in collinear antiferromagnets without the requirement for spin-orbit coupling (SOC). Symmetry analysis suggests that antiferromagnets hosting such effect can be classified into six types depending on the global vs local symmetry. We identify which of the possible collinear antiferromagnetic compounds will harbor such hidden polarization and validate these symmetry enabling predictions with first-principles density functional calculations for several representative compounds. This will boost the theoretical and experimental efforts in finding new spin-polarized materials.
Signatures of enhanced spin-triplet superconductivity induced by interfacial properties
While spin-triplet pairing remains elusive in nature, there is a growing effort to realize proximity-induced equal-spin triplet superconductivity in junctions with magnetic regions or an applied magnetic field and common s-wave superconductors. To enhance such spin-triplet contribution, it is expected that junctions with a weak interfacial barrier and strong spin-orbit coupling are desirable. Intuitively, a weak interfacial barrier enables a robust proximity-induced superconductivity and strong spin-orbit coupling promotes spin mixing, converting spin-singlet into spin-triplet superconductivity. In contrast, we reveal a nonmonotonic spin-triplet contribution with the strength of the interfacial barrier and spin-orbit coupling. This picture is established by considering different signatures in conductance and superconducting correlations, as well as by performing self-consistent calculations. As a result, we identify a strongly enhanced spin-triplet superconductivity, realized for an intermediate strength of interfacial barrier and spin-orbit coupling. In junctions with magnetic regions, an enhanced spin-triplet superconductivity leads to a large magnetoanisotropy of conductance and superconducting correlations. Furthermore, this picture of an enhanced spin-triplet superconductivity is consistent with experiments demonstrating a huge increase in the conductance magnetoanisotropy, which we predict can be further enhanced at a finite bias.
Unconventional supercurrent phase in Ising superconductor Josephson junction with atomically thin magnetic insulator
Abstract In two-dimensional (2D) NbSe 2 crystal, which lacks inversion symmetry, strong spin-orbit coupling aligns the spins of Cooper pairs to the orbital valleys, forming Ising Cooper pairs (ICPs). The unusual spin texture of ICPs can be further modulated by introducing magnetic exchange. Here, we report unconventional supercurrent phase in van der Waals heterostructure Josephson junctions (JJs) that couples NbSe 2 ICPs across an atomically thin magnetic insulator (MI) Cr 2 Ge 2 Te 6 . By constructing a superconducting quantum interference device (SQUID), we measure the phase of the transferred Cooper pairs in the MI JJ. We demonstrate a doubly degenerate nontrivial JJ phase ( ϕ ), formed by momentum-conserving tunneling of ICPs across magnetic domains in the barrier. The doubly degenerate ground states in MI JJs provide a two-level quantum system that can be utilized as a new dissipationless component for superconducting quantum devices. Our work boosts the study of various superconducting states with spin-orbit coupling, opening up an avenue to designing new superconducting phase-controlled quantum electronic devices.
Spin–phonon interactions and magnetoelectric coupling in Co 4 B 2 O 9 ( B = Nb, Ta)
In order to explore the consequences of spin–orbit coupling on spin–phonon interactions in a set of chemically similar mixed metal oxides, we measured the infrared vibrational properties of Co 4 B 2 O 9 (B = Nb, Ta) as a function of temperature and compared our findings with lattice dynamics calculations and several different models of spin–phonon coupling. Frequency vs temperature trends for the Co 2+ shearing mode near 150 cm –1 reveal significant shifts across the magnetic ordering temperature that are especially large in relative terms. Bringing these results together and accounting for noncollinearity, we obtain spin–phonon coupling constants of –3.4 and –4.3 cm –1 for Co 4 Nb 2 O 9 and the Ta analog, respectively. Analysis reveals that these coupling constants are derived from interlayer (rather than intralayer) exchange interactions and that the interlayer interactions contain competing antiferromagnetic and ferromagnetic contributions. At the same time, beyond-Heisenberg terms are minimized due to fortuitous symmetry considerations, different from most other 4d- and 5d-containing oxides. Comparison with other contemporary oxides shows that spin–phonon coupling in this family of materials is among the strongest ever reported, suggesting an origin for magnetoelectric coupling.