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The role of electronic mechanisms in surface erosion and glow phenomena

Experimental studies of desorption induced by electronic transitions (DIET) are described. Such studies are producing an increasingly complete picture of the dynamical pathways through which incident electronic energy is absorbed and rechanneled to produce macroscopic erosion and glow. These mechanistic studies can determine rate constants for erosion and glow processes in model materials and provide valuable guidance in materials selection and development. Extensive experiments with electron, photon, and heavy particle irradiation of alkali halides and other simple model materials have produced evidence showing that: (1) surface erosion, consisting primarily in the ejection or desorption of ground-state neutral atoms, occurs with large efficiencies for all irradiated species; (2) surface glow, resulting from the radiative decay of desorbed atoms, likewise occurs for all irradiating species; (3) the typical mechanism for ground-state neutral desorption is exciton formation, followed by relaxation to a permanent, mobile electronic defect which is the precursor to bond-breaking in the surface or near-surface bulk of the material; and (4) the mechanisms for excited atom formation may include curve crossing in atomic collisions, interactions with surface defect or impurity states, or defect diffusion.

Haglund, Richard F., Jr.↗

Mechanism for the thermal dependence of the Cr to Nd energy transfer in garnets

The temperature dependence of the Cr-Nd energy transfer is found to be due to the thermal variation of the radiative decay probability of Cr. The validity of this conjecture is checked in the Gd3Sc2Ga3O12 and CaMg2Y2Ge3O12 crystals. It is also found that above 200 K, the nonradiative energy transfer rate from Cr to Nd is greater in Gd3Sc2Ga3O12 than in CaMg2Y2Ge3O12.

Armagan, Guzin↗

Redistribution in astrophysically important hydrogen lines

Under typical solar chromospheric conditions for hydrogen radiators, strong collisions due to both electrons and ions are well separated in time, so that a binary collision theory for collisional redistribution is applicable. However, a simple impact approximation may not be used, but rather a unified type theory is required in which frequency dependent line shape parameters are used to describe both impact and quasi-static regions of the spectrum. In addition, correlated terms which describe absorption and emission during a collision are important, and, in fact, without correlated terms describing both transfer of excitation and emission during the same collision unphysical predictions (such as negative intensities) would be obtained. In this paper theory is specifically developed for the coupled Lyman-alpha, Lyman-beta, Hydrogen-alpha system, and equations of statistical equilibrium and absorption and emission coefficients are given. All correlated events are examined and emission during a collision is found to be important in the line wings. Stimulated emission and absorption is also included within a broadband approximation. The major approximation is to ignore lower state interaction. It is found that for Lyman-beta Raman-coupling with Hydrogen-alpha occurs and the overall scattering of radiation in the line wings is mostly coherent. In contrast, for Hydrogen-alpha, incoherent redistribution due to lower state radiative decay (which occurs even in the absence of collisions) is found to dominate the coherent scattering. Finally, in the Lyman series the dominant incoherent contribution is associated with cascade transitions and inelastic collisions between different principal quantum states.

Cooper, J.↗

High-energy continuum emission from solar flares

The properties of solar flare continuum emission at energies of greater than 300 keV have been determined from observations obtained during the 21st solar maximum by gamma-ray detectors aboard the SMM and Hinotori satellites. The temporal structure of the high-energy continuum is modeled by two-step acceleration and particle trapping. The results suggest that the very high-energy emission noted must be a mixture of pion-decay radiation and primary electron bremsstrahlung.

Vestrand, W. Thomas↗

Approximate formulation of redistribution in the Ly-alpha, Ly-beta, H-alpha system

Simple approximate formulas are given for the coupled redistribution of Ly-alpha, Ly-beta, and H-alpha, by using well-defined approximations to an essentially exact formulation. These formulas incorporate all the essential physics including Raman scattering, lower state radiative decay, and correlated terms representing emission during a collision which must be retained in order that the emission coefficients are properly behaved in the line wings. Approximate expressions for the appropriate line broadening parameters are collected. Finally, practical expressions for the source functions are given. These are formulated through newly introduced nonimpact redistribution functions, which are shown to be reasonably approximated by existing (ordinary and generalized) redistribution functions.

Cooper, J.↗

The grand unified photon spectrum: A coherent view of the diffuse extragalactic background radiation

The spectrum of diffuse extragalactic background radiation (DEBRA) at wavelengths from 10(exp 5) to 10(exp -24) cm is presented in a coherent fashion. Each wavelength region, from the radio to ultra-high energy photons and cosmic rays, is treated both separately and as part of the grand unified photon spectrum (GUPS). A discussion of, and references to, the relevant literature for each wavelength region is included. This review should provide a useful tool for those interested in diffuse backgrounds, the epoch of galaxy formation, astrophysical/cosmological constraints to particle properties, exotic early Universe processes, and many other astrophysical and cosmological enterprises. As a worked example, researchers derive the cosmological constraints to an unstable-neutrino spies (with arbitrary branching ratio to a radiative decay mode) that follow from the GUPS.

Ressell, M. Ted↗

Spectroscopic investigation of Cr to Tm energy transfer in yttrium aluminum garnet crystals

A series of experiments has been conducted in order to examine the nature of the energy transfer process between the Cr(3+) and Tm(3+) ions in YAG. Data are obtained on various samples doped with Cr(3+) and/or Tm(3+). These data include absorption, luminescence, excitation spectra and time-resolved response to pulsed excitation. The measurements were carried out over a range of temperatures from 78 to 350 K. The rate of nonradiative energy transfer from Cr(3+) to Tm(3+) depends on temperature, and in the region from 200 to 350 K, this dependence is due primarily to the thermal variation in the radiative decay probability of the Cr ion.

Armagan, G.↗

Infrared and optical imagery of the Crab Nebula

The paper presents 1.644 micron forbidden-line Fe II and 1.570 micron continuum images of the Crab Nebula which are compared with optical H-alpha, forbidden-line O III, and 5100 A continuum data. While the same prominent filaments are generally apparent in all lines, no substantial variations within the nebula in the strength and morphology of forbidden-line Fe II relative to the other lines are found. The infrared to optical continuum ratio of the synchrotron nebula shows 15 - 20 percent variations which are dominated by features which appear related to the position of the pulsar. These are interpreted as variations of 0.15 in the spectral index and it is suggested that they are related to the radiative decay of energetic particles and the paths over which these particles travel from the pulsar throughout the nebula.

Hester, J. Jeff↗

N(2P) in the dayglow - Measurement and theory

During the ATLAS-1 mission, the first dayglow altitude profiles were obtained of the N(2P) emission at 3466 A. These observations were made in the sunlit thermosphere using the Imaging Spectrometric Observatory. As all previous work on this emission has been done under auroral conditions, this study represents the first examination of the photochemical sources and sinks of N(2P) in the normal daytime thermospheric, with comparison with measurements. We find that the observations are explained by a model in which the major source is photodissociation of N2, and quenching by O is the principal low-altitude loss process, with radiative decay to N(2D) dominating above 200 km. As the dominant loss processes are likely to result in the production of N(2D), N(2P) could be a moderate source of N(2D) and may be a factor to be taken into consideration in modeling NO.

Torr, Marsha R.↗

Induced ClO vacuum ultraviolet fluorescence

Some vibronic transitions of ClO such as G(v-prime = 11 )-X(v-double prime = 10), G(v-prime = 5)-X(v-double prime = 3) and H(v-prime = 4)-X(v-double prime = 2), which promote overtones of X(2pi3/2) to bound Rydberg states, are nearly resonant with the 130.6 nm O-atom emission line and possess sizable Franck-Condon factors. On this basis broadband detection of 'O atom' fluorescence in experiments involving vibrationally excited ClO(X) is ascribed to the radiative decay of ClO(G, H) rather than to the formation of O atoms; these observations raise the probability of monitoring ClO(X; v = 0) by VUV-induced fluorescence.

Colussi, A. J.↗

Measurement of the transition probability of the C III 190.9 nanometer intersystem line

A radio-frequency ion trap has been used to store C(2+) ions created by electron bombardment of CO. The transition probability for the 2s2p 3Po1-2s2 1S0 intersystem line of C m has been measured by recording the radiative decay at 190.9 nm. The measured A-value is 121 +/- 7/s and agrees, within mutual uncertainty limits, with that of Laughlin et al. (1978), but is 20 percent larger than that of Nussbaumer and Storey (1978). The effective collision mixing rate coefficient among the fine structure levels of 3Po and the combined quenching and charge transfer rate coefficients out of the 3Po1 level with the CO source gas have also been measured.

Kwong, Victor H. S.↗

A physical model of the infrared-to-radio correlation in galaxies

We explore the implications of the IR-radio correlation in star-forming galaxies, using a simple physical model constrained by the constant global ratio q of IR to radio emission and by the radial falloff of this ratio in disks of galaxies. The modeling takes into account the diffusion, radiative decay, and escape of cosmic-ray electrons responsible for the synchrotron emission, and the full range of optical depths to dust-heating photons. We introduce two assumptions: that dust-heating photons and radio-emitting cosmic-ray electrons are created in constant proportion to each other as part of the star formation activity, and that gas and magnetic field are well coupled locally, expressed as B proportional to n exp beta, with beta between 1/3 and 2/3. We conclude that disk galaxies would maintain the observed constant ratio q under these assumptions if the disk scale height h(0) and the escape scale length l(esc) for cosmic-ray electrons followed a relation of the form l(esc) proportional to h(0) exp 1/2; the IR-to-radio ratio will then depend very weakly on interstellar density, and, therefore, on magnetic field strength or mean optical depth.

Helou, G.↗

Voyager investigation of the cosmic diffuse background: Observations of rocket-studied locations with Voyager

Attachments to this final report include 2 papers connected with the Voyager work: 'Voyager Observations of Dust Scattering Near the Coalsack Nebula' and 'Search for the Intergalactic Medium'. An appendix of 12 one-page write-ups prepared in connection with another program, UVISI, is also included. The one-page write-ups are: (1) Sky survey of UV point sources to 600 times fainter than previous (TD-1) survey; (2) Diffuse galactic light: starlight scattered from dust at high galactic latitude; (3) Optical properties of interstellar grains; (4) Fluorescence of molecular hydrogen in the interstellar medium; (5) Line emission from hot interstellar medium and/or hot halo of galaxy; (6) Integrated light of distant galaxies in the ultraviolet; (7) Intergalactic far-ultraviolet radiation field; (8) Radiation from recombining intergalactic medium; (9) Radiation from re-heating of intergalactic medium following recombination; (10) Radiation from radiative decay of dark matter candidates (neutrino, etc.); (11) Reflectivity of the asteroids in the Ultraviolet; and (12) Zodiacal light.

Henry, Richard C.↗

Possible Detection of Pi(exp 0)-Decay Gamma-Ray Emission from Cyg OB2 by EGRET

We report possible detection of pi (exp 0) decay radiation from Cyg OB2, a nearby (1.7 kpc) massive OB star association. The EGRET flux (greater than 100 MeV) maps clearly indicate a point source whose error circle includes both Cyg OB2 and Cyg X-3. We show that Cyg X-3 is unlikely to be the counterpart for the EGRET source, because of the marginal spatial consistency and the lack of the 4.8 hour modulation seen in other high energy emissions from Cyg X-3. If confirmed, this will be the first detection by EGRET of massive stars.

Chen, W.↗

The Middle Ultraviolet-Visible Spectrum of H2 Excited by Electron Impact

The electron-impact-induced emission spectrum of H2 has been measured in the extended wavelength region 175-530 mm at a spectral resolution of 1.7 mm (FWHM). The laboratory spectra are characterized by underlying H2 (a (sup 3) Sigma(sup +, sub g) to b (sup 3) Sigma(sup +, sub u) continuum emission. together with many strong lines assigned to the radiative decay of the gerade singlet states of H2, and to members of the H Balmer series resulting from dissociative excitation of H2.

James, Geoffrey K.↗

CdZnTe Background Measurements at Balloon Altitudes with PoRTIA

Measurements of the CdZnTe internal background at balloon altitudes are essential to determine which physical processes make the most important background contributions. We present results from CdZnTe background measurements made by PoRTIA, a small CdZnTe balloon instrument that was flown three times in three different shielding configurations. PoRTIA was passively shielded during its first flight from Palestine, Texas and actively shielded as a piggyback instrument on the GRIS balloon experiment during its second and third flights from Alice Springs, Australia, using the thick GRIS Nal anticoincidence shield. A significant CdZnTe background reduction was achieved during the third flight with PoRTIA placed completely inside the GRIS shield and blocking crystal, and thus completely surrounded by 15 cm of Nal. A unique balloon altitude background data set is provided by CdZnTe and Ge detectors simultaneously surrounded by the same thick anticoincidence shield; the presence of a single coxial Ge detector inside the shield next to PoRTIA allowed a measurement of the ambient neutron flux inside the shield throughout the flight. These neutrons interact with the detector material to produce isomeric states of the Cd, Zn and Te nuclei that radiatively decay; calculations are presented that indicate that these decays may explain most of the fully shielded CdZnTe background.

Parsons, A.↗

The FERRUM Project: Experimental Transition Probabilities of [Fe II] and Astrophysical Applications

We report on experimental transition probabilities for thirteen forbidden [Fe II] lines originating from three different metastable Fe II levels. Radiative lifetimes have been measured of two metastable states by applying a laser probing technique on a stored ion beam. Branching ratios for the radiative decay channels, i.e. M1 and E2 transitions, are derived from observed intensity ratios of forbidden lines in astrophysical spectra and compared with theoretical data. The lifetimes and branching ratios are combined to derive absolute transition probabilities, A-values. We present the first experimental lifetime values for the two Fe II levels a(sup 4)G(sub 9/2) and b(sup 2)H(sub 11/2) and A-values for 13 forbidden transitions from a(sup 6)S(sub 5/2), a(sup 4)G(sub 9/2) and b(sup 4)D(sub 7/2) in the optical region. A discrepancy between the measured and calculated values of the lifetime for the b(sup 2)H(sub 11/2) level is discussed in terms of level mixing. We have used the code CIV3 to calculate transition probabilities of the a(sup 6)D-a(sup 6)S transitions. We have also studied observational branching ratios for lines from 5 other metastable Fe II levels and compared them to calculated values. A consistency in the deviation between calibrated observational intensity ratios and theoretical branching ratios for lines in a wider wavelength region supports the use of [Fe II] lines for determination of reddening.

Hartman, H.↗

CHANDRA Observations of V407 Vul: Confirmation of the Spin-up

V407 Vu1 (RX J1914.4+2456) is a candidate double-degenerate binary with a putative 1.756 mHz (9.5 min) orbital frequency. In a previous timing study using archival ROSAT and ASCA data we reported evidence for an increase of this frequency at a rate consistent with expectations for gravitational radiation from a detached ultracompact binary system. Here we report the results of new Chandra timing observations which confirm the previous indications of spin-up of the X-ray frequency, and provide much tighter constraints on the frequency derivative, nu (raised dot). We obtained with Chandra a total of 90 ksec of exposure in two epochs separated in time by 11.5 months. The total time span of the archival ROSAT, ASCA and new Chandra data is now approximately equal to 10.5 years. This more than doubles the interval spanned by the ROSAT and ASCA data alone, providing much greater sensitivity to a frequency derivative. With the addition of the Chandra data an increasing frequency is unavoidable, and the mean nu (raised dot) is 7.0 plus or minus 0.8 x l0(exp -18) Hz per second. Although a long-term spin-up trend is confirmed, there is excess variance in the phase timing residuals, perhaps indicative of shorter timescale torque fluctuations or phase instability associated with the source of the X-ray flux. Power spectral searches for periods longward of the 9.5 minute period do not find any significant modulations, however, the sensitivity of searches in this frequency range are somewhat compromised by the dithering of the Chandra attitude. The observed spin-up is of a magnitude consistent with that expected from gravitational radiation decay, however, the factor of approximately equal to 3 variations in flux combined with the timing noise could conceivably result from accretion-induced spin-up of a white dwarf. Continued monitoring to explore correlations of torque with X-ray flux could provide a further test of this hypothesis.

Strohmayer, T.↗