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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS1985

Astronomical identification of the C3H radical

The C3H radical has been identified in the millimeter-wave spectra of IRC +10216 and TMC-1. In IRC +10216, four rotational transitions have been observed, three in the lower fine-structure ladder (2Pi1/2) and one in the upper (2Pi3/2), each a resolved or partially resolved lambda-doublet. In TMC-1, both lambda components of the lowest lying 3/2-1/2 transition of the 2Pi1/2 ladder have been observed, each with well-resolved hfs. In IRC +10216, the excitation of C3H is similar to that of SiCC: the rotational temperature Trot within the 2Pi1/2 ladder is low (8.5 K), because of rapid radiative decay, while Trot across the ladders is high (about 52 K), because interconnecting far-IR radiative transitions are only weakly permitted. The column density of C3H in IRC +10216 averaged over the estimated source diameter of 84 arcsec is 2.8 x 10 to the 13th/sq cm, an order of magnitude less than that of C2H and C4H.

Thaddeus, P.↗
DOE OSTI2025

$η(') → π0γγ$ decays: Test of meson exchange models and searches of leptophobic $B$ bosons

We analyze the vector and scalar meson exchange contributions to the doubly radiative decays $η(') → π0γγ$ and $η → ηγγ$, and study the sensitivity of these decays to a leptophobic B boson in the sub-GeV mass range. Our results are relevant for studies of these decays at existing (A2, BESIII, KLOE-2) and forthcoming $η/η'$-factories, such as the JEF and REDTOP experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Improved measurements of the Dalitz decays η / η ′ → γ e + e −

Based on a data sample of 10 billion J / ψ events collected with the BESIII detector, improved measurements of the Dalitz decays η / η ′ → γ e + e − are performed, where the η and η ′ are produced through the radiative decays J / ψ → γ η / η ′ . The branching fractions of η → γ e + e − and η ′ → γ e + e − are measured to be ( 7.07 ± 0.05 ± 0.23 ) × 10 − 3 and ( 4.83 ± 0.07 ± 0.14 ) × 10 − 4 , respectively. Within the single-pole model, the parameter of electromagnetic transition form factor for η → γ e + e − is determined to be Λ η = ( 0.749 ± 0.027 ± 0.007 ) GeV / c 2 . Within the multipole model, we extract the electromagnetic transition form factors for η ′ → γ e + e − to be Λ η ′ = ( 0.802 ± 0.007 ± 0.008 ) GeV / c 2 and γ η ′ = ( 0.113 ± 0.010 ± 0.002 ) GeV / c 2 . The results are consistent with both theoretical predictions and previous measurements. The characteristic sizes of the interaction regions for the η and η ′ are calculated to be ( 0.645 ± 0.023 ± 0.007 ) fm and ( 0.596 ± 0.005 ± 0.006 ) fm , respectively. In addition, we search for the dark photon in η / η ′ → γ e + e − , and the upper limits of the branching fractions as a function of the dark photon are given at 90% confidence level. Published by the American Physical Society 2024

Astronomy & Astrophysics↗
DOE OSTI2024

Search for η c ( 2 S ) → 2 ( π + π − ) and improved measurement of χ c J → 2 ( π + π − )

We search for the hadronic decay η c ( 2 S ) → 2 ( π + π − ) in the ψ ( 3686 ) → γ η c ( 2 S ) radiative decay using ( 27.12 ± 0.14 ) × 10 8 ψ ( 3686 ) events collected by the BESIII detector at the BEPCII collider. No significant signal is found, and the upper limit of B [ ψ ( 3686 ) → γ η c ( 2 S ) ] B [ η c ( 2 S ) → 2 ( π + π − ) ] is determined to be 1.43 × 10 − 6 at the 90% confidence level. Using ψ ( 3686 ) → γ χ c J transitions, we also measure the branching fractions of B [ χ c J ( J = 0 , 1 , 2 ) → 2 ( π + π − ) ] , which are B [ χ c 0 → 2 ( π + π − ) ] = ( 2.127 ± 0.002 ( stat ) ± 0.101 ( syst ) ) % , B [ χ c 1 → 2 ( π + π − ) ] = ( 0.685 ± 0.001 ( stat ) ± 0.031 ( syst ) ) % , and B [ χ c 2 → 2 ( π + π − ) ] = ( 1.153 ± 0.001 ( stat ) ± 0.063 ( syst ) ) % . Published by the American Physical Society 2024

Ablikim, M.↗
DOE OSTI2022

Simulation of the photodetachment spectra of the nitrate anion (NO 3 ₋ ) in the B ~ 2 E' energy range and non-adiabatic electronic population dynamics of NO 3

The photodetachment spectrum of the nitrate anion (NO 3 ₋ ) in the energy range of the NO 3 second excited state is simulated from first principles using quantum wave packet dynamics. The prediction at 10 K and 435 K relies on the use of an accurate full-dimensional fully coupled five state diabatic potential model utilizing an artificial neural network. The ability of this model to reproduce experimental spectra was demonstrated recently for the lower energy range. Analysis of the spectra indicates a weaker Jahn–Teller coupling compared to the first excited state. The detailed non-adiabatic dynamics is studied by computing the population dynamics. An ultra-fast non-statistical radiationless decay is found only among the Jahn–Teller components, which is followed by a slow statistical non-radiative decay among the different state manifolds. The latter is reproduced perfectly by a simple first order kinetics model. The dynamics in the second excited state is not affected by the presence of a conical intersection with the first excited state manifold.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Search for lepton-flavor-violating tau-lepton decays to ℓγ at Belle

Charged lepton flavor violation is forbidden in the Standard Model but possible in several new physics scenarios. In many of these models, the radiative decays τ ± → ℓ ± γ (ℓ = e, μ) are predicted to have a sizeable probability, making them particularly interesting channels to search at various experiments. An updated search via τ ± → ℓ ± γ using full data of the Belle experiment, corresponding to an integrated luminosity of 988 fb –1 , is reported for charged lepton flavor violation. No significant excess over background predictions from the Standard Model is observed, and the upper limits on the branching fractions, B(τ ± → μ ± γ) ≤ 4.2 × 10 –8 and B(τ ± → e ± γ) ≤ 5.6 × 10 –8 , are set at 90% confidence level.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Toward radiative-limited coherence of erbium dopants in a nanophotonic resonator

Atomic-like emitters in the solid state serve as important resources in the advancement of future quantum networks. In particular, intra-4f optical transitions of rare earth ions exhibit excellent coherence properties thanks to the shielding effect of outer electrons. Still, the presence of various dephasing channels in solid state hosts introduces additional decoherence beyond the radiative decay, causing the coherence time of most rare earth doped materials to be over an order of magnitude lower than the radiative limit. Such obstacle prevents the emission of indistinguishable photons from rare earth ions, which is an essential requirement for various quantum applications. In this work, we perform optical coherence study on erbium ions doped in thin-film lithium niobate by patterning photonic crystal resonators with quality factor around 100 k and sub-λ3 mode volume. Leveraging the combination of long coherence and strong Purcell enhancement in the cavity, we show that the coherence time measured with photon echo approaches the radiative limit (80%), representing a 50-fold improvement compared to the waveguide case. Our results present promising prospects toward utilizing rare earth doped materials as quantum repeaters and sources of indistinguishable photons.

Physics↗
NASA NTRS1986

Dissociative excitation of the N(+)(5S) state by electron impact on N2 - Excitation function and quenching

Metastable N(+)(5S) ions were produced in the laboratory by dissociative excitation of N2 with energetic electrons. The resulting radiative decay of the N(+)(5S) state was observed with sufficient resolution to completely resolve the doublet from the nearby N2 molecular radiation. The excitation function was measured from threshold to 500 eV. The cross section peaks at a high electron energy and also exhibits a high threshold energy both of which are typical of dissociative excitation-ionization processes. This finding complicates the explanation of electron impact on N2 as the mechanism for the source of the 2145 A 'auroral mystery feature' by further increasing the required peak cross section. It is suggested that the apparent N(+)(5S) quenching in auroras may be an artifact due to the softening of the electron energy spectrum in the auroral E region.

Erdman, P. W.↗
DOE OSTI2025

A machine learning framework for accurate and robust analysis of radiation detector pulses

The microscopic properties of atomic nuclei are used to study various scientific questions. They are essential for understanding the fundamental forces of nature and the chemical evolution of the universe. Detecting decay radiation from radioactive nuclei makes it possible to probe these fundamental nuclear properties. Detector waveform traces may contain additional information about the radiation. Generally, advanced signal processing techniques are needed to extract this additional information, often involving fitting the waveform with model response functions using non-linear least-squares optimization with second-order gradient methods. While this is a powerful technique, it is also computationally expensive, leading to slow processing time, which scales with the volume of data. To address this problem, we have developed a machine learning (ML) approach that infers the characteristics of traces from a model detector response function. In particular, we are interested in classifying whether a single recorded trace consists of one or two pulse constituents and estimating the pulse parameters. Furthermore, our proposed ML method can precisely extract the pulses’ parameters, such as energy and timing information, and accurately classify the pulse multiplicity of a trace. Unlike non-learning-based approaches, our ML approach uses neural networks that are significantly faster at inference, as they do not require any optimization during this stage.

Curve fitting↗
NASA NTRS1980

Observations of extreme ultraviolet emissions from the Saturnian plasmasphere

Emission signals from the Saturnian plasmasphere at wavelengths shortward of 800 A have been detected by the Pioneer ultraviolet photometer. The surface brightness of the emissions is about 0.3 + or - 0.2 R. These short-wavelength emissions are interpreted as arising primarily from the radiative decay of electron-excited atomic oxygen ions (O(2+)), in the region between 5 and 7 Saturn radii from Saturn. The total power radiated by the Saturnian plasma inferred from these ultraviolet measurements is about 2 x 10 to the 16th erg/sec, consistent with in situ plasma measurements. From the observed energy loss rate it is estimated that the ions are introduced into the plasma torus at a rate of 8 x 10 to the 25th ions/sec, possibly through the sputtering of water ice on the surface of Tethys and Dione by particle impact.

Wu, F. M.↗
NASA NTRS1992

Gamma rays from pion decay - Evidence for long-term trapping of particles in solar flares

The energy spectrum and time dependence of the 50 MeV to 2 GeV gamma rays observed from the 1991 June 11 solar flare are analyzed. It is shown that the emission detected at the late phase of this flare with EGRET on the Compton Gamma-Ray Observatory can be explained by a model in which the bulk of the particles were accelerated during the impulsive phase and subsequently trapped in coronal magnetic loops. The observed spectrum was fit with a combination of pion decay radiation and primary electron bremsstrahlung. The 1991 June 11 data are compared with data for the 1982 June 3 and 1991 June 15 flares from which pion decay emission was also observed. The fact that the fluxes from these three flares are ordered in time in accordance with the predicted time dependence of emission produced by trapped particles provides support for the model.

Mandzhavidze, Natalie↗
DOE OSTI2021

Lower limits for non-radiative recombination loss in organic donor/acceptor complexes

Understanding the factors controlling radiative and non-radiative transition rates for charge transfer states in organic systems is important for applications ranging from organic photovoltaics (OPV) to lasers and LEDs. Here we explore the role of charge-transfer (CT) energetics, lifetimes, and photovoltaic properties in the limit of very slow non-radiative rates by using a model donor/acceptor system with photoluminescence dominated by thermally activated delayed fluorescence (TADF). This blend exhibits an extremely high photoluminescence quantum efficiency (PLQY = ~22%) and comparatively long PL lifetime, while simultaneously yielding appreciable amounts of free charge generation (photocurrent external quantum efficiency EQE of 24%). In solar cells, this blend exhibits non-radiative voltage losses of only ~0.1 V, among the lowest reported for an organic system. Notably, we find that the non-radiative decay rate, k nr , is on the order of 10 5 s -1 , approximately 4–5 orders of magnitude slower than typical OPV blends, thereby confirming that high radiative efficiency and low non-radiative voltage losses are achievable by reducing k nr . Furthermore, despite the high radiative efficiency and already comparatively slow k nr , we find that k nr is nevertheless much faster than predicted by Marcus–Levich–Jortner two-state theory and we conclude that CT-local exciton (LE) hybridization is present. Our findings highlight that it is crucial to evaluate how radiative and non-radiative rates of the LE states individually influence the PLQY of charge-transfer states, rather than solely focusing on the PLQY of the LE. This conclusion will guide material selection in achieving low non-radiative voltage loss in organic solar cells and high luminescence efficiency in organic LEDs.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Nuclear Data Sheets for A=48

Experimental nuclear structure data from various reactions and decays are compiled and evaluated for all known nuclides with mass number A=48 (S, Cl, Ar, K, Ca, Sc, Ti, V, Cr, Mn, Fe, Co, Ni). For each nuclide, detailed evaluated nuclear structure information is presented for each individual reaction and decay, and the best values combining all available data are recommended for spectroscopic properties, such as level energies, half-lives, γ-ray energies and intensities, decay radiations. No excited states have been identified in 48 S, 48 Cl, 48 Co and 48 Ni, among which the first three even have no measured ground-state half-lives and decay modes. For 48 Fe, a level scheme with a sequence of excited states was established for the first time from a recent one-neutron removal measurement by 2021Ya33. Data for excited states in 48 Ar, 48 K and 48 Mn remain limited; no decay scheme has been measured for 48 Ar and 48 K yet, while the decay scheme for 48 Ni is incomplete due to unobserved levels. 48 Ti is the most studied nuclide through various reactions and decays, followed by 48 V, 40 Ca, 48 Sc, and 48 Cr, among which no decay event to 48 Sc has been observed and the decay schemes for 48 V and 48 Cr are considered as incomplete. Furthermore, this work supersedes the previous full evaluations of A=48: 2006Bu08, 1993Bu04, 1985Al14, 1978Be01.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Relic neutrino decay solution to the excess radio background

Abstract The excess radio background detected by ARCADE 2 represents a puzzle within the standard cosmological model. There is no clear viable astrophysical solution, and therefore, it might indicate the presence of new physics. Radiative decays of a relic neutrino ν_i (either i=1, or i=2, or i=3) into a sterile neutrino ν_ s, assumed to be quasi-degenerate, provide a solution that currently evades all constraints posed by different cosmological observations and reproduces very well the ARCADE 2 data. We find a very good fit to the ARCADE 2 data with best fit values τ_i = 1.46 × 10^21 s and Δ m_i = 4.0 × 10^-5 eV, where τ_i is the lifetime and Δ m_i is the mass difference between the decaying active neutrino and the sterile neutrino. On the other hand, if relic neutrino decays do not explain ARCADE 2 data, then these place a stringent constraint Δ m_i^3/2τ_i ≳ 2 × 10^14 eV^3/2 s in the range 1.4 × 10^-5 eV<Δ m_i < 2.5 × 10^-4 eV. The solution also predicts a stronger 21 cm absorption global signal than the predicted one from the ΛCDM model, with a contrast brightness temperature T_21 = -238^+21_-20 mK (99% C.L.) at redshift z≃ 17. This is in mild tension with the even stronger signal found by the EDGES collaboration, T_21 = - 500^+200_-500 mK, suggesting that this might have been overestimated, possibly receiving a contribution from some unidentified foreground source.

Astronomy & Astrophysics↗
DOE OSTI2022

On the Interplay between CT and Singlet Exciton Emission in Organic Solar Cells with Small Driving Force and Its Impact on Voltage Loss

The interplay between free charge carriers, charge transfer (CT) states and singlet excitons (S 1 ) determines the recombination pathway and the resulting open circuit voltage (V OC ) of organic solar cells. By combining a well-aggregated low bandgap polymer with different blend ratios of the fullerenes PCBM and ICBA, the energy of the CT state (E CT ) is varied by 130 meV while leaving the S 1 energy of the polymer (E S 1 ) unaffected. It is found that the polymer exciton dominates the radiative properties of the blend when approaches E CT , while the V OC remains limited by the non-radiative decay of the CT state. It is concluded that an increasing strength of the exciton in the optical spectra of organic solar cells will generally decrease the non-radiative voltage loss because it lowers the radiative V OC limit (V OC,rad ), but not because it is more emissive. The analysis further suggests that electronic coupling between the CT state and the S 1 will not improve the V OC , but rather reduce the V OC,rad . It is anticipated that only at very low CT state absorption combined with a fairly high CT radiative efficiency the solar cell benefit from the radiative properties of the singlet excitons.

14 SOLAR ENERGY↗
NASA NTRS1972

Optical radiation from regions downstream of mercury bombardment thrusters.

Use of a 0.5-m focal length, plane grating monochromator to measure the radiance of spectral radiation emanating from regions downstream of a mercury bombardment thrustor in the wavelength range investigated was 2800 to 6000 A. This radiation was due primarily to the radiative decay of excited mercury atoms exhausted from the thrustor. Radiance values ranged from 10 to the minus 11th to 10 to the min scm/ster varying with wavelength. For resonant radiation, the spectral radiance may exceed 10 to the minus 8th W/sq cm/ster. From such radiance measurements, it was concluded that the thrustor background radiation should not interfere with the control functions of a star tracker viewing through the thrustor exhaust, provided that the tracker is designed to operate with a sufficiently small field of view. Problems may be encountered, however, during the spacecraft acquisition phase where a larger field of view may be required. Here the thrustor exhaust radiation may be comparable to the star light flux. This problem may be circumvented by locating the tracker view axis so as not to view downstream of the thrustor.

Milder, N. L.↗
NASA NTRS1977

Inclusive gamma-ray spectra from psi/3095/ and psi-prime/3684/ decays

Inclusive gamma-ray experiments were carried out in a e(+)e(-) colliding-beam apparatus with NaI(Tl) arrays as detectors. The inclusive gamma-ray spectra, after cosmic-ray background subtraction, are shown as histograms for the decays of the psi(3095) and psi-prime(3684). The psi spectrum has no significant narrow structure, while the psi-prime spectrum shows at least four peaks. Three major radiative decays of the psi-prime(3684) are found, and their respective branching fractions are computed.

Biddick, C. J.↗