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Direct Numerical Simulations of Blended Ammonia/Hydrogen/Nitrogen Premixed Flames in Intense Sheared Turbulence.
Abstract not provided.
Filtered Density Function Simulations of a Near-Limit Turbulent Lean Premixed Flame
Not provided.
THE YIELD OF NITRIC OXIDE FROM PREMIXED FLAMES OF HYDROGEN AND HYDROCARBONS WITH NITROUS OXIDE
Yield of nitric oxide from hydrogen & hydrocarbons with nitrous oxide
On stability of premixed flames in stagnation - Point flow
A quantitative description of flame stabilization in stagnation-point flow is proposed. Asymptotic and stability analyses are made for a flame model where the density of the gas is assumed to be constant and the reaction zone is assumed to be narrow and concentrated over the flame front. It is shown that, if blowing is sufficiently strong, the corrugations disappear and a plane flame results. The phenomena cannot be fully described by means of classical linear stability analysis.
An experimental study on extinction and stability of stretched premixed flames
Law et al. (1981) and Ishizuka et al. (1982) have experimentally investigated the effects of flame stretch, preferential diffusion, and downstream heat loss on the extinction and stability of propane/air flames. The obtained results suggest that in the case of rich propane/air mixtures downstream heat loss, in addition to flame stretch, is needed for flame extinction. In the case of lean mixtures, flames can be extinguished by flame stretch alone. The data obtained in connection with the present study provide convincing evidence regarding the correctness of the previous results on the nature of flame extinction due to stretch. It is found that, in accordance with theoretical predictions, extinction by stretch alone is possible only when there is a deficiency regarding the less mobile reactant.
Effect of reactive intermediates on the propagation of turbulent premixed flames
The most simple version of the Bray and Libby model of turbulent flame propagation has been extended to include a two-step reaction mechanism in which reactants decompose into reactive intermediates which then form products. A transport equation for the joint pdf of intermediate and product concentrations was derived, the pdf parameterized, and transport equations for the parameters obtained. The one-dimensional concentration equations were then solved for the parameters of the pdf and the turbulent kinetic energy. Flame speed and angle are recovered as eigenvalues of the problem. The results show the essential features observed in experiments. The product pdf is composed of peaks at zero and unity product concentration, with a continuous structure representing partially reacted gas. The intermediates pdf has a peak at zero concentration and a broad bell-shaped distribution at nonzero concentration, representing partially reacted gas. The results also show the effect of partitioning of energy release on the flame thickness and speed.
The behavior of fuel-lean premixed flames in a standard flammability limit tube under controlled gravity conditions
Fuel-lean flames in methane-air mixtures from 4.90 to 6.20 volume percent fuel and propane-air mixtures from 1.90 to 3.00 volume percent fuel were studied in the vicinity of the limit for a variety of gravity conditions. The limits were determined and the behavior of the flames studied for one g upward, one g downward, and zero g propagation. Photographic records of all flammability tube firings were obtained. The structure and behavior of these flames were detailed including the variations of the curvature of the flame front, the skirt length, and the occurrence of cellular instabilities with varying gravity conditions. The effect of ignition was also discussed. A survey of flame speeds as a function of mixture strength was made over a range of lean mixture compositions for each of the fuels studied. The results were presented graphically with those obtained by other researchers. The flame speed for constant fractional gravity loadings were plotted as a function of gravity loadings from 0.0 up to 2.0 g's against flame speeds extracted from the transient gravity flame histories for corresponding gravity loadings. The effects of varying gravity conditions on the extinguishment process for upward and downward propagating flames were investigated.
The Effect of Gravity on Premixed Flame Propagation and Extinction in a Vertical Standard Flammability Tube
The effect of gravity on the upward and downward flame propagation in lean methane/air and lean propane/air mixtures was studied using plexiglass flammability tubes with ignition at the open-end gravity levels which ranged from microgravity (0 + or - 0.1 g) to 1.77 g. The lean limits were found to be about 5.25, 5.25, and 5.85 percent methane in air; and about 2.15, 2.06, and 2.20 percent propane in air for 1 g upward propagation, 0 g, and 1 g downward propagation, respectively. The propane/air flames observed were stable, irrespective of the g level. On the other hand, lean methane/air flames were found to be sporadically unstable for upward propagation at g levels less than 0.5 g, and for donward propagation at g = 1.0. The extinction process observed was the same for both systems studied: at g = 0, the flame extinguished from the edge toward the center, while at g of 1 and above, the flame extinguished from the center toward the edge.
Structure and dynamics of premixed flames in microgravity
In this report we describe the research performed at the Naval Research Laboratory in support of the NASA Microgravity Science and Applications Program over the past three years with emphasis on the work performed since February 1992, the beginning of the current project. The focus of our research has been on investigating fundamental combustion questions concerning the propagation and extinction of gas-phase flames in microgravity and earth-gravity environments. Our approach to resolving these fundamental questions has been to use detailed time-dependent, multidimensional numerical models to perform carefully designed computational experiments. The basic questions we have addressed, a general description of the numerical approach, and a summary of the results are described in this report. More detailed discussions are available in the papers published which are referenced herein.
Premixed Flame Propagation in an Optically Thick Gas
Flame propagation in both the optically thin and the optically thick regime of radiative transport was studied experimentally using particle-laden gas mixtures. Data on flame shapes, propagation rates, peak pressure, maximum rate of pressure rise, and thermal decay in the burned gases are consistent with the hypothesis that, at low particle loadings, the particles act to increase the radiative loss from the gases, whereas at higher loadings, reabsorption of emitted radiation becomes significant. The reabsorption acts to decrease the net radiative loss and augment conductive heat transport. It is speculated that, in sufficiently large systems, in which the absorption length is much smaller than the system size, flammability limits might not exist at microgravity conditions because emitted radiation would not constitute a loss mechanism.
Effect of finite-rate chemistry and unequal Schmidt numbers on turbulent non-premixed flames modeled with single-step chemistry
The interaction between a quasi-laminar flame and a turbulent flowfield is investigated through direct numerical simulations (DNS) of reacting flow in two- and three-dimensional domains. Effects due to finite-rate chemistry are studied using a single step global reaction A (fuel) + B (oxidizer) yields P (product), and by varying a global Damkoehler number, as a result of which the turbulence-chemistry interaction in the flame is found to generate a wide variety of conditions, ranging from near-equilibrium to near-extinction. Differential diffusion effects are studied by changing the Schmidt number of one reactive species to one-half. It is observed that laminar flamelet response is followed within the turbulent flowfield, except in regions where transient effects seem to dominate.
Structure of turbulent non-premixed flames modeled with two-step chemistry
Direct numerical simulations of turbulent diffusion flames modeled with finite-rate, two-step chemistry, A + B yields I, A + I yields P, were carried out. A detailed analysis of the turbulent flame structure reveals the complex nature of the penetration of various reactive species across two reaction zones in mixture fraction space. Due to this two zone structure, these flames were found to be robust, resisting extinction over the parameter ranges investigated. As in single-step computations, mixture fraction dissipation rate and the mixture fraction were found to be statistically correlated. Simulations involving unequal molecular diffusivities suggest that the small scale mixing process and, hence, the turbulent flame structure is sensitive to the Schmidt number.
Verification and Improvement of Flamelet Approach for Non-Premixed Flames
Studies in the mathematical modeling of the high-speed turbulent combustion has received renewal attention in the recent years. The review of fundamentals, approaches and extensive bibliography was presented by Bray, Libbi and Williams. In order to obtain accurate predictions for turbulent combustible flows, the effects of turbulent fluctuations on the chemical source terms should be taken into account. The averaging of chemical source terms requires to utilize probability density function (PDF) model. There are two main approaches which are dominant in high-speed combustion modeling now. In the first approach, PDF form is assumed based on intuitia of modelliers (see, for example, Spiegler et.al.; Girimaji; Baurle et.al.). The second way is much more elaborate and it is based on the solution of evolution equation for PDF. This approach was proposed by S.Pope for incompressible flames. Recently, it was modified for modeling of compressible flames in studies of Farschi; Hsu; Hsu, Raji, Norris; Eifer, Kollman. But its realization in CFD is extremely expensive in computations due to large multidimensionality of PDF evolution equation (Baurle, Hsu, Hassan).
Quantitative Studies on the Propagation and Extinction of Near-Limit Premixed Flames under Normal- and Micro-gravity
Strained laminar flames have been systematically studied, as the understanding of their structure and dynamic behavior is of relevance to turbulent combustion.. Most of these studies have been conducted in opposed-jet, stagnation-type flow configurations. Studies at high strain rates are important in quantifying and understanding the response of vigorously burning flames and determine extinction states. Studies of weakly strained flames can be of particular interest for all stoichiometries. For example, the laminar flame speeds, S(sup o)(sub u), can be accurately determined by using the counterflow technique only if measurements are obtained at very low strain rates. Furthermore, near-limit flames are stabilized by weak strain rates. Previous studies have shown that near-limit flames are particularly sensitive to chain mechanisms, thermal radiation, and unsteadiness. The stabilization and study of weakly strained flames is complicated by the presence of buoyancy that can render the flames unstable to the point of extinction. Thus, the use of microgravity (mu-g) becomes essential in order to provide meaningful insight into this important combustion regime. In our past studies the laminar flame speeds and extinction strain rates were directly measured at ultra-low strain rates. The laminar flame speeds were measured by having a positively strained planar flame undergoing a transition to a negatively strained Bunsen flame and by measuring the propagation speed during that transition. The extinction strain rates of near-limit flames were measured in mu-g. Results obtained for CH4/air and C3H8/air mixtures are in agreement with those obtained by Maruta et al.
Quantitative Studies on the Propagation and Extinction of Near-Limit Premixed Flames Under Normal and Microgravity
The main objective of this research is to introduce accurate fluid mechanics measurements diagnostics in the 2.2-s drop tower for the determination of the detailed flow-field at the states of extinction. These results are important as they can then be compared with confidence with detailed numerical simulations so that important insight is provided into near-limit phenomena that are controlled by not well-understood kinetics and thermal radiation processes. Past qualitative studies did enhance our general understanding on the subject. However, quantitative studies are essential for the validation of existing models that subsequently be used to describe near-limit phenomena that can initiate catastrophic events in micro- and/or reduced gravity environments.
Gaseous Non-Premixed Flame Research Planned for the International Space Station
Thus far, studies of gaseous diffusion flames on the International Space Station (ISS) have been limited to research conducted in the Microgravity Science Glovebox (MSG) in mid-2009 and early 2012. The research was performed with limited instrumentation, but novel techniques allowed for the determination of the soot temperature and volume fraction. Development is now underway for the next experiments of this type. The Advanced Combustion via Microgravity Experiments (ACME) project consists of five independent experiments that will be conducted with expanded instrumentation within the stations Combustion Integrated Rack (CIR). ACMEs goals are to improve our understanding of flame stability and extinction limits, soot control and reduction, oxygen-enriched combustion which could enable practical carbon sequestration, combustion at fuel lean conditions where both optimum performance and low emissions can be achieved, the use of electric fields for combustion control, and materials flammability. The microgravity environment provides longer residence times and larger length scales, yielding a broad range of flame conditions which are beneficial for simplified analysis, e.g., of limit behaviour where chemical kinetics are important. The detailed design of the modular ACME hardware, e.g., with exchangeable burners, is nearing completion, and it is expected that on-orbit testing will begin in 2016.
Sensitivity of predictions to chemical kinetics models in a temporally evolving turbulent non-premixed flame
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