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At least 91 records · Page 5

Search for extraterrestrial intelligence/high resolution microwave survey team member

This semiannual status report describes activities conducted by the Principal Investigator during the first half of this third year of the NASA High Resolution Microwave Survey (HRMS) Investigator Working Group (IWG). As a (HRMS) Team Member with primary interest in the Sky Survey activity, this investigator attended IWG meetings at NASA/Ames and U.C.-Santa Cruz in Apr. and Aug. 1992, and has traveled independently to NRAO/Kitt Peak, Arizona (April 1993) and Woodbury, Georgia (July 1993). During the July 1993 visit to the Georgia Tech Research Corporation/Woodbury Research Facility, an experiment was conducted to study the effects of interference from C-band (3.7 - 4.2 GHz) geostationary spacecraft on the Sky Survey operation in that band. At the first IWG meeting in April of this year, results of a SETI observation conducted at the 203 GHz positronium hyperfine resonance using the NRAO facility at Kitt Peak, AZ, were presented, as well as updates on the development of the spaceborne RFI data bases developed for the project. At the second meeting, results of the study of interference from C-band geostationary spacecraft were presented. Likewise, a presentation was made at the accompanying 1993 Bioastronomy Symposium describing the SETI observation at the positronium hyperfine resonance.

Steffes, Paul G.↗

The annihilation of positrons in the cold phase of the interstellar medium revisited

The positron cross sections in H and H2 media are reevaluated, taking into account new experimental results. Using a Monte Carlo simulation, we find a positronium fraction before thermalization of 0.90 for H2, in good agreement with the previous experimental result given by Brown et al. (1986). For H we obtain an upper limit of 0.98. We study the behavior of the charge exchange annihilation in a cold phase (molecular cloud). We calculate a formula for the slowing-down time t, before annihilation lasting Delta t, via charge exchange, of a positron beam with a given energy for different medium densities and initial energies. An upper limit of 0.7 MeV for the initial energy of the positrons, annihilating in the molecular cloud G0.86 - 0.08 near the gamma ray source positronium and gives new time constraints on their possible observation.

Wallyn, P.↗

Demonstration of o-Ps detection with a cylindrical array of NaI detectors

Ortho-positronium (o-Ps) is a bound state of an electron and positron that can provide a means of searching for new physics. We searched and identified o-Ps in our cylindrical array of NaI(Tl) scintillators, developing a technique for tagging on o-Ps with any one of the 24 bars in the array. With high angular efficiency and this new technique, such an experimental setup could be used in a fundamental symmetries search. In particular, we explore the possibility of using such a setup with a search for CP- or CPT-violation in o-Ps.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Influence of Water, Vacuum, and Temperature on Surface Conditions of a Zeolite‐based Molecular Sieve

Molecular sieves such as zeolite-based materials are ubiquitous in industrial separation processes. However, there is a significant gap in understanding the surface properties and adsorption mechanisms for commercial zeolites, as most research focuses on pure zeolite powders rather than industrially relevant forms. Here, this work addresses this gap in understanding by employing advanced characterization techniques, including positron annihilation spectroscopy, X-ray diffraction, scanning electron microscopy, X-ray fluorescence spectroscopy, X-ray photoelectron spectroscopy, liquid nitrogen sorption, and Fourier-transform infrared spectroscopy, to investigate the adsorption and desorption behavior of water in commercial zeolite 13X. Our research reveals insights into the pore-filling mechanisms, the impact of material binders on adsorption properties, and the dynamics of hydration and drying processes for zeolites. Monitoring changes on a minute scale allowed the distinction between fast and slow processes leading to sample drying. The identification of positronium bound to Na + ions indicated that water molecules remain in the vicinity of Na + ions after air-drying zeolite 13X. These findings highlight the importance of various environmental conditions in restoring zeolite properties to baseline after hydration, with significant implications for optimizing industrial processes. This work sets the direction for further research aimed at developing more efficient and robust separation techniques.

Beads Binder↗

Measurement and analysis of the Doppler broadened energy spectra of gamma radiation originating from the annihilation of positrons incident on clean and adsorbate-covered surfaces

We present measurements and theoretical modeling demonstrating the capability of coincidence Doppler broadened (CDB) annihilation gamma spectroscopy to provide element-specific information from the topmost atomic layer of surfaces. Our measurements show that the energy spectra of Doppler-shifted annihilation gamma photons emitted following the annihilation of positrons from the topmost atomic layers of clean and adsorbate covered surfaces of gold (Au), silver (Ag) and copper (Cu) differ significantly. The shape of the Doppler-broadened gamma spectrum, as analyzed using ratio curves, indicates that the elemental composition of the surface can still be identified despite contributions from positronium annihilation and a significant reduction in core electron annihilation. We estimate the chemical composition of the various probed surfaces by modeling the ratios of the measured Doppler spectra with respect to the Doppler spectra from a clean Cu surface using a linear combination of calculated ratio curves. The fitting of the experimental ratio curves was used to obtain an estimate of the elemental composition of Cu surfaces with sulfur segregation, oxygen adsorption, a thin film of Selenium (Se), and a single layer of graphene (SLG). A similar analysis was performed on the Ag surface with environmental adsorbates, the same surface after argon ion sputtering, as well as a sputter cleaned Au surface. The surface compositions obtained from the analysis of the CDB data were compared to the compositions obtained using positron annihilation induced Auger electron spectroscopy (PAES). Our results show that CDB can detect, identify, and quantify, sub-monolayer adsorbates and a single atomic layer deposited on metal substrates.

Lotfimarangloo, Sima [Univ. of Texas, Arlington, T↗

Hydrated doped-BaZrO 3 proton conductors studied by positron annihilation lifetime spectroscopy

The study of defect chemistry for doped BaZrO 3 proton conductors is of particular interest because of defect interactions that can affect the proton conductivity of the material. Protons incorporated due to the material's hydration can be trapped by negatively charged immobile dopants, reducing proton mobility. The reduction of the proton conduction impedes using BaZrO 3 materials in energy conversion applications at intermediate temperatures (300°C – 600°C). The probing of proton trapping in doped BaZrO 3 is hindered by the limited availability of techniques sensitive to defect chemistries. In this work, we used positron annihilation lifetime spectroscopy (PALS) to study the defect chemistry of Y-doped and Sc-doped BaZrO 3 . Using a two-state positron trapping model we showed that PALS can be used to study the defect chemistry of hydrated dense proton conductors. Positron trapping rates and lifetimes were correlated with doping levels of the materials. Probability significance t-tests were carried out for PALS parameters to verify whether there are differences/similarities for various populations: non-doped/doped, level and type of doping, high temperature, and surface effects. Further, the results revealed that the initial doping generates a significant number of traps available for positrons. Doping in yttrium increased the positron trapping rate, while this effect was not observed with scandium. Low-temperature hydration affects specimens significantly inhibiting positron trapping at undoped BaZrO 3 material and highly doped specimens. Positronium formation in rough surface layers, and highly doped specimens was detected but does not exceed 1%.

36 MATERIALS SCIENCE↗

A buffer-gas trap for the NEPOMUC positron beam: optimization studies with electrons

Buffer-gas traps (BGTs) use inelastic interactions with nitrogen molecules to capture positrons from a continuous beam. These devices are invaluable for high-resolution studies of matter–antimatter interactions, antihydrogen research and positronium laser spectroscopy. We present a new project with the goal of producing a non-neutral plasma containing ${\sim }10^8$ low-energy positrons by installing a BGT on the NEPOMUC (NEutron induced POsitron source MUniCh) high-intensity positron beam. Details of the BGT are outlined and results are presented from experiments in which an electron beam, with a similar intensity and energy spread to the remoderated NEPOMUC beam, was used to create pulses of non-neutral electron plasma. The device is a vital component of the APEX (A Positron Electron eXperiment) project, which aims to create a low-temperature electron–positron pair plasma.

Physics↗

Antihydrogen chemistry

A survey of antimatter reactions is presented, including the formation of the antihydrogen atom and anionic, cationic, and molecular species by collisional and radiative processes. Our approach is rooted in the detailed knowledge available for many matter counterpart (hydrogenic) reactions, due to their importance in controlling early Universe chemistry. We point out that the availability of trapped antihydrogen at densities similar to those pertaining to the epoch of hydrogen chemistry will soon be available. In addition, using modern atomic physics techniques, it should be feasible to control antimatter in the laboratory to facilitate antihydrogen chemistry. Our purpose is to summarize what is known from hydrogen chemistry that is of relevance for antimatter and to indicate, based on possible reaction rates, which processes may be fruitful to pursue to create new antimatter entities as probes of fundamental symmetries. We include antihydrogen, positrons, and antiprotons in our discussion and additionally the electron due to its propensity to form positronium and perhaps to participate in certain reactions. We attempt to indicate whether further theoretical/computational work is necessary to add to the assessment of reaction rates, and we discount processes where the projected rates are too low to be of interest, given foreseeable experimental capabilities.

74 ATOMIC AND MOLECULAR PHYSICS↗

Theory of low-energy positron-helium scattering.

Positron-helium scattering below positronium threshold, using adiabatic method previously tested in positron hydrogen scattering, presenting phase shifts and momentum transfer cross section computations

POSITRON↗

Planetary geology, stellar evolution and galactic cosmology

Field studies of selected basalt flows in the Snake River Plain, Idaho, were made for comparative lunar and Mars geological investigations. Studies of basalt lava tubes were also initiated in Washington, Oregon, Hawaii, and northern California. The main effort in the stellar evolution research is toward the development of a computer code to calculate hydrodynamic flow coupled with radiative energy transport. Estimates of the rotation effects on a collapsing cloud indicate that the total angular momentum is the critical parameter. The study of Paschen and Balmer alpha lines of positronium atoms in the center of a galaxy is mentioned.

Source record↗

Analysis of the 0.511 MeV radiation at the OSO-7 satellite

Observations of the 0.511 MeV positron annihilation, gamma ray on the OSO-7 satellite are presented. Variables which affect the counting rate are discussed. An upper limit flux of .0076 photons/sq cm/sec is obtained for the quiet sun and a positive solar flux of .063(+ or - .0002) photons/sq cm/sec is obtained for the 3B flare of 4 August 1972. The width of this annihilation line gives an upper limit temperature for the annihilation region of approximately 6 million K. An analysis of the line width and position also shows that the contribution to the line from positronium annihilation is less than 100% at the 99% confidence level. An upper limit is also found for an isotropic cosmic flux.

Dunphy, P. P.↗

Rigorous precision p-wave positron-hydrogen scattering calculation

Rigorous lower-bound p-wave positron-hydrogen phase shifts are calculated below the positronium pickup threshold. The wave function is expanded in terms of the two linearly independent D functions each multiplied by an associated Hilleraas-type radial function with two parameters. Adiabatic and nonadiabatic corrections have been included. The results are found to be larger than Armstead's (1968) in all cases near the upper edge of his estimated uncertainty.

Bhatia, A. K.↗

Annihilation during positron-hydrogen collisions

Using the precision s- and p-wave elastic-scattering wave functions obtained previously, we have calculated the annihilation rate for positrons colliding with hydrogen atoms below the positronium-formation threshold. The s-wave results agree well with those of Humberston, while the p-wave results, which are new, contribute about 20% of the total at the higher energies.

Bhatia, A. K.↗