Intensity measurements, self-broadening coefficients, and rotational intensity distribution for lines of the oxygen B band at 6880 A
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Giver, L. P.↗
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Line Profile Measurements of Atomic Oxygen at 1300 A with a VUV Raman Shifter
We are currently developing an atomic oxygen diagnostic to study the degree of oxygen dissociation in ground-based facilities. The absorption of the (sub 3)P - (sup 3)S(sup 0) resonance triplet in the vacuum ultraviolet is a direct measure of the ground state number density of atomic oxygen. Although the integrated line strength is well known for these transitions, the line profile is not. We report the results of a series of experiments in which the line profile is measured in shock-heated oxygen. An ArF excimer laser and a hydrogen Raman shifter generate tunable VUV radiation at the resonance wavelength. The test gas is dissociated oxygen, generated in the Electric Arc Shock Tube (EAST) Facility at NASA-Ames Research Center. By measuring the absorption of known concentrations of atomic oxygen, we are able to study the absorption line profile. The results will serve as a calibration to apply this diagnostic in other flowfields.
Sharma, Surendra P.↗
Atmospheric odd oxygen production due to the photodissociation of ordinary and isotopic molecular oxygen
Line-by-line calculations are performed to determine the contributions of the Schumann-Runge bands of ordinary and isotopic oxygen to the photodissociation of these molecules at different altitudes. The contributions to the dissociation rates of the satellite lines and of the first and higher vibrational states of the initial molecular states are found to be insignificant. At 70 km, (O-16)(O-18) is found to produce 10 times as much odd oxygen as would be produced if the isotope did not have selective absorption, and 6 percent of the odd oxygen produced is due to this isotope. It is noted that the excess odd oxygen produced is not enough to explain the excess quantity of ozone observed in the atmosphere, which cannot be accounted for in photochemical models. Comparison with previous results is made.
Omidvar, K.↗
Abundance studies of oxygen and nitrogen in nebulae - Uses of the far-infrared emission lines
The potential of infrared forbidden emission lines for studying nebular abundances is discussed, with emphasis on the far-infrared fine-structure lines of oxygen and nitrogen. Observations of these transitions provide fundamentally new diagnostics of the physical conditions in ionized nebulae, and make it possible for the first time to study the abundances of these species in the inner parts of the Galaxy. These new tools for nebular abundance studies are only beginning to be exploited. The results derived so far from such studies are reviewed, and future prospects and applications of these techniques are discussed.
Dinerstein, Harriet L.↗
Solar wind physics
A double-chambered gas proportional counter was constructed to detect and identify solar wind ions after acceleration by a high voltage power supply. It was determined that the best method of detecting deuterium in the solar wind is to use a tritium target as proposed for IMP H and J. The feasibility of detecting H(+) and He(+) ions of interstellar origin is considered. A program is described to carry out ground-based astronomical observations of faint, diffuse optical emission lines from interstellar gas. Hydrogen and oxygen emission lines from galactic sources were detected and the galactic and geocoronal H alpha and beta lines were clearly resolved.
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Dynamical Studies of the Middle Atmosphere Using High Resolution Doppler Imager Observations
This report summarizes the activities of NASA grant NAG5-11068, "Dynamicai Studies of the Middle Atmosphere Using High Resolution Doppler Imager Observations." The High Resolution Doppler Imager (HRDI) on the Upper Atmosphere Research Satellite (UARS) has been providing direct measurements of the Earth's horizontal wind field in the stratosphere, mesosphere and lower thermosphere. Mesospheric temperatures, ozone, and O((sup 1) D) densities, and stratospheric aerosol extinctions coefficients, are also retrieved. The goal of HRDI is to measure the vector winds in the stratosphere (10-40 km), mesosphere, and lower thermosphere (approximately 50-120 km) during the day, and the lower thermosphere at night (approximately 95 km) to an accuracy of 5 m/s. The horizontal wind vector is measured by observing the Doppler shift of rotational lines of molecular oxygen along two lines of sight. In addition to winds, temperatures and volume emission rates are determined in the mesosphere and lower thermosphere, from which ozone and O((sup 1) D) concentrations can be derived, and aerosol scattering coefficients are determined in the stratosphere. UARS was launched on September 12, 1991, into a 585-km circular orbit inclined 57 degrees to the equator HRDI was activated September 28, 1991 and following a period of checkout and adjustment of the instrument parameters, scientific observations began November 2, 199 1. HRDI operated nearly continuously from launch until April 1995. At that time the UARS solar array drive failed, forcing the instruments to time-share the available power. From July 1995 to July 1996 HRDI operated approximately 50% of the time. At that point, one of the three spacecraft batteries failed and from then until September 1998 the duty cycle was less than 20% per month, At that time it was determined that HRDI could operate during each daytime pass, which increased the daytime duty cycle to close to l00%, while nighttime operations were limited to about a week per month. In the fall of 1999, the second tape recorder failed requiring a real time contact with a TRDSS satellite to retrieve that data. This resulted in about 60% data collection efficiency. Finally, in the summer of 2000, the second star sensor failed requiring the spacecraft attitude to be controlled by a three axis magnetometer and sun sensor. This resulted in a loss of attitude knowledge but operations continue with the anticipation of correcting the attitude. A new method for determining the tide and mean structure from satellite data in conjunction with a new tidal model has been devised. For brevity, it shall be referred to as the TMAT or Tide-Mean Assimilation Technique. Most previous methods of tidal analysis are based on various ways of slicing the data set.
Skinner, Wilbert↗
Chandra Observations of Comet 2P/Encke 2003: First Detection of a Collisionally Thin, Fast Solar Wind Charge Exchange System
We report the results of 15 hr of Chandra observations of comet 2P/Encke 2003 on November 24. X-ray emission from comet Encke was resolved on scales of 500-40,000 km, with unusual morphology due to the presence of a low-density, collisionally thin (to charge exchange) coma. A light curve with peak-to-peak amplitude of 20% consistent with a nucleus rotational period of 11.1 hr was found, further evidence for a collisionally thin coma. We confirm emission lines due to oxygen and neon in the 800-1000 eV range but find very unusual oxygen and carbon line ratios in the 200-700 eV range, evidence for low-density, high effective temperature solar wind composition. We compare the X-ray spectral observation results to contemporaneous measurements of the coma and solar wind made by other means and find good evidence for the dominance of a postshock bubble of expanding solar wind plasma, moving at 600 km/s with charge state composition between that of the "fast" and "slow" solar winds.
Lisse, C. M.↗
The ultraviolet dayglow. IV - The spectrum and excitation of singly ionized oxygen
The emission line spectrum of singly ionized atomic oxygen (O II) dominates the day airglow spectrum in the extreme ultraviolet below 834 A. The strongest resonance line, at 834 A, is optically thick and an analysis of height profiles obtained from rocket observations between 140 and 265 km in specific viewing directions indicates that the principal excitation source is direct photoionization of neutral atomic oxygen. Strong emission at 538-539 A is most likely due to the quartet rather than the doublet transitions, which both occur at these wavelengths and which are not spectrally resolved in the data. The intensities of the weaker lines are consistent with recent laboratory measurements of transition branching ratios. Several strong O II lines near He I 584 produce severe contamination of low-altitude (less than 400 km) measurements of geocoronal helium emission made with thin-film broadband photometers.
Feldman, P. D.↗
Reversible oxidation and reduction of gold-supported iron oxide islands at room temperature
Monolayer iron oxides grown on metal substrates have widely been used as model systems in heterogeneous catalysis. By means of ambient-pressure scanning tunneling microscopy (AP-STM), we studied the in situ oxidation and reduction of FeO(111) grown on Au(111) by oxygen (O 2 ) and carbon monoxide (CO), respectively. Oxygen dislocation lines present on FeO islands are highly active for O 2 dissociation. X-ray photoelectron spectroscopy measurements distinctly reveal the reversible oxidation and reduction of FeO islands after sequential exposure to O 2 and CO. Here, our AP-STM results show that excess O atoms can be further incorporated on dislocation lines and react with CO, whereas the CO is not strong enough to reduce the FeO supported on Au(111) that is essential to retain the activity of oxygen dislocation lines.
36 MATERIALS SCIENCE↗
Molecular rotational line profiles from oxygen-rich red giant winds
We have developed a radiative transfer model of the dust and gas envelopes around late-type stars. The gas kinetic temperature for each star is calculated by solving equations of motion and the energy balance simultaneously. The main processes include viscous heating and adiabatic and radiative cooling. Heating is dominated by viscosity as the grains stream outward through the gas, with some contribution in oxygen-rich stars by near-IR pumping of H2O followed by collisional de-excitation in the inner envelope. For O-rich stars, rotational H2O cooling is a dominant mechanism in the middle part of the envelope, with CO cooling being less significant. We have applied our model to three well-studied oxygen-rich red giant stars. The three stars cover a wide range of mass-loss rates, and hence they have different temperature structures. The derived temperature structures are used in calculating CO line profiles for these objects. Comparison of the dust and gas mass-loss rates suggests that mass-loss rates are not constant during the asymptotic giant branch phase. In particular, the results show that the low CO 1-0 antenna temperatures of OH/IR stars reflect an earlier phase of much lower mass-loss rate.
Justtanont, K.↗
Thermophysical properties of oxygen from the freezing liquid line to 600 R for pressures to 5000 psia
Data on oxygen properties commonly used for engineering calculations over wide temperature and pressure range
Mccarty, R. D.↗
The influence of thermospheric winds on the auroral red-line profile of atomic oxygen.
Discussion of the effect of thermospheric winds on the emission profile of lambda 6300. It is shown that meridional winds play a significant role in determining the shape of this emission and that the conventional diffusion of O(super 1 D) hypothesis, although important, is not adequate to explain the observed features completely.
Hays, P. B.↗
Carbon and oxygen X-ray line emission from the interstellar medium
A soft X-ray, 0.3-1.0 keV spectrum from a 1 sr region which includes a portion of the North Polar Spur, obtained by three rocketborne lithium-drifted silicon detectors, shows the C V, C VI, O VII and O VIII emission lines. The spectrum is well fitted by a two-component, modified Kato (1976) model, where the coronal emission is in collisional equilibrium, with interstellar medium and North Polar Spur temperatures of 1.1 and 3.8 million K, respectively.
Schnopper, H. W.↗
The neutral oxygen spectrum. 1: Collisionally excited level populations and line intensities under optically thin conditions
This is the first paper in a projected program to produce quantitative information on the spectrum of the neutral oxygen atom under a variety of excitation conditions. Radiative rates and effective collision strengths are assembled from the recent literature where available, or are calculated for as yet untreated transitions using the University College superstructure/distorted-wave computer package, to produce a complete set of atomic data for a 13 hybrid level model of neutral oxygen. Level populations and relative intensities for 28 allowed, inter-combination, and forbidden oxygen lines are computed, under optically thin conditions, for the electron density range 4.0 less than log N(sub e) less than 12.0 and the electron temperature values T(sub e) = 5000, 10,000, 20,000, 50,000, and 100,000 K. Preliminary applications to observed intercombination/allowed and forbidden/allowed line ratios are discussed.
Bhatia, A. K.↗
Twilight and nighttime ionospheric temperatures from oxygen wavelengths 6300 and 5577 spectral line profiles
Fabry-Perot interferometer measurements of atomic oxygen 6300 A and 5577 A line profiles from twilight and nightglow are used to determine the neutral temperatures in F2 and E regions of the earth's ionosphere. The exospheric temperatures T sub n (infinity) determined from the 6300 A profiles are usually somewhat higher than those calculated from Jacchia's model, with differences as large as approximately 300 K noted when T sub n (infinity) = 1500 to 1600 K. The post-sunset and pre-dawn rate of change of T sub n (infinity) is often substantially larger than the Jacchia prediction. The 5577 A (E-region) measured temperatures range from 200 to 220 K on quiet nights to 500 to 600 K during geomagnetic storms.
Feibelman, W. A.↗
Line Narrowing Parameter Measurement by Modulation Spectroscopy
Accurate Characterization of Oxygen A-Band Line Parameters by Wavelength Modulation Spectroscopy with tunable diode lasers is an ongoing research at Old Dominion University, under sponsorship from NASA Langley research Center. The work proposed here will be undertaken under the guidance of Dr. William Chu and Dr. Lamont Poole of the Aerosol Research Branch at NASA Langley-Research Center in Hampton, Virginia. The research was started about two years ago and utilizes wavelength modulation absorption spectroscopy with higher harmonic detection, a technique that we developed at Old Dominion University, to obtain the absorption line characteristics of the Oxygen A-band rovibronic lines. Accurate characterization of this absorption band is needed for processing of data that will be obtained in experiments such as the NASA Stratospheric Aerosol and Gas Experiment III (SAGE III) as part of the US Mission to Planet Earth. The research work for Summer Fellowship undertook a measurement of the Dicke line-narrowing parameters of the Oxygen A-Band lines by using wavelength modulation spectroscopy. Our previous theoretical results had indicated that such a measurement could be done sensitively and in a convenient fashion by using this type of spectroscopy. In particular, theoretical results had indicated that the signal magnitude would depend on pressure in a manner that was very sensitive to the narrowing parameter. One of the major tasks undertaken during the summer of 1998 was to establish experimentally that these theoretical predictions were correct. This was done successfully and the results of the work are being prepared for publication. Experimental Results were obtained in which the magnitude of the signal was measured as a function of pressure, for various harmonic detection orders (N = 1, 2, 3, 4, 5). A comparison with theoretical results was made, and it was shown that the agreement between theory and experiment was very good. More importantly, however, it was shown that the measurement was yielded a very sensitive technique for obtaining the narrowing parameter that describes the deviation of Oxygen A-band lines from the Voigt profile. In particular, it was seen that the best fits were obtained consistently when the narrowing parameter value used was 0.022 1/cm, 1/Atm, Previous work, upon which the current work was based has resulted in several accurate measurements of properties of particular lines of the Oxygen A band. For example, this work has resulted in the measurement of the collision cross sections of several lines including the RQ(13,14) and the RR(15,15) lines. A major achievement of achievement of the work was also the demonstration that the technique we have developed can accurately probe the structure of the absorption lineshape function. In particular, the method we have developed is very well suited for experimentally probing the characteristics of lines in their wings. This work was accepted for publication in the Journal of Applied Physics, and is scheduled to appear in the December 15, 1998 issue.
Dharamsi, Amin N.↗
Excitation of the auroral green line by dissociative recombination of the oxygen molecular ion - Analysis of two rocket experiments.
Excitation of auroral green line by dissociative recombination of oxygen molecular ions, using photometric and electron flux rocket sounding data
Doering, J. P.↗
Two-dimensional photometry of planetary nebulae
Monochromatic images of three planetary nebulae, NGC 6720, NGC 7662 and NGC 2392, were taken using narrow band interference filters centered on the forbidden emission lines of Oxygen I, II, III, Nitrogen II, Sulfur II and the permitted emission lines of Hydrogen I, Helium I and Helium II. The data was taken with a silicon intensified vidicon using the Palomar 1.5 meter telescope and was recorded digitally to an encoding level of 12 bits. The data was processed at the Image Processing Laboratory of the Jet Propulsion Laboratory. The calibrated images were used to investigate the three dimensional structure of the nebulae and to generate two-dimensional electron and temperature maps.
Kupferman, P. N.↗