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DOE OSTI2025

Nanomechanical squeezing: Toward quantum imaging with atomic force microscopy

Leveraging quantum effects in mechanical oscillators promises major advancements in nanometrology, including sensing and imaging. Microscopic cantilevers serve as versatile force sensors with broad applications in nanoscience, nanotechnology, and, increasingly, quantum sensing. Here, we theoretically model and investigate the quantum mechanics of cantilever probes in atomic force microscopy under conditions of reduced thermal noise. Specifically, our model captures the cantilever interaction with a surface via long-range attractive van der Waals forces and short-range repulsive-adhesive interactions described by the Derjaguin-Muller-Toporov model. We find that when the probe resides within the attractive interaction regime, a coherent state emerges, whereas, in the repulsive regime, a squeezed state forms for the cantilever's deformation state. Our calculations explain the functional role of interaction potentials in the quantum dynamics of macroscopic mechanical systems, which are proving useful in quantum sensing and information processing. The presented calculations can be extended to investigate other interaction forces relevant to atomic force microscopy.

Al-Sawai, Wael M. [Lamar Univ., Beaumont, TX (Unit↗

DOE OSTI2024

Seasonal variability and predictability of monsoon precipitation in Southern Africa

Rainfed agriculture is the mainstay of economies across Southern Africa (SA), where most precipitation is received during the austral summer monsoon. This study aims to further our understanding of monsoon precipitation predictability over SA. We use three natural climate forcings, El Niño–Southern Oscillation, Indian Ocean Dipole (IOD), and the Indian Ocean Precipitation Dipole (IOPD)—the dominant precipitation variability mode—to construct an empirical model that exhibits significant skill over SA during monsoon in explaining precipitation variability and in forecasting it with a five-month lead. While most explained precipitation variance (50%–75%) comes from contemporaneous IOD and IOPD, preconditioning all three forcings is key in predicting monsoon precipitation with a zero to five-month lead. Seasonal forecasting systems accurately represent the interplay of the three forcings but show varying skills in representing their teleconnection over SA. This makes them less effective at predicting monsoon precipitation than the empirical model.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Effects of Heave Plate Topology on Reaction Forces

Multi-body wave energy converters often rely on "heave plates" to generate the reaction forces required for energy harvesting. However, the influence of threedimensional heave plate topology on these reaction forces is relatively unexplored in the literature. Using laboratory experiments, we investigate the reaction forces generated by three distinct heave plate topologies: A flat hexagonal plate, an open hexagonal-conic, and an enclosed hexagonalconic (i.e., interior cavity flooded with water). Though the flat plate is the least massive of the topologies, it generates the greatest total reaction force for nearly all experimental cases due to higher fluid force. Our results also demonstrate that the flat plate generally experiences the greatest force variability between the three topologies, especially during relatively large oscillations (KC greater than 2). Globally, force variability increases with the Keulegan Carpenter (KC) number. These results highlight the importance of heave plate topology on multi-body point wave energy converter performance.

heave plate↗

DOE OSTI2023

Writing the Programs of Programmable Catalysis

It has long been known that non-steady state and periodic catalytic reactor operation in terms of temperature, pressure, and composition can lead to higher overall productivity and/or product selectivity than the best steady operation. Recently, the emergence of catalysts whose intrinsic properties can be made to oscillate with time, introduces advanced forcing capabilities that can be “programmed” into the catalysts to broaden the scope and applicability of periodic operation to surface chemistry. In this work, an algorithmic approach is implemented to significantly accelerate the discovery and optimization of periodic steady states of catalytic reactors. Decomposition of complex dynamics into fundamental mechanistic fast–slow steps is seen to improve conceptual understanding of the relationship between binding energy oscillation protocols and overall catalytic rates. Finding structured forcing protocols, optimally tailored to the multiple time scales of a given individual mechanism, requires an efficient search of high-dimensional parameter spaces. Here, this is enabled here through active learning (Bayesian optimization, enhanced by our proposed Bayesian continuation). Implementation of these methods is shown to accelerate the evaluation of catalyst programs by up to several orders of magnitude. Faster screening of programmable catalysts to discover periodic steady states enables the optimization of catalytic operating protocols and thus opens the possibility for catalyst engineering based on optimal forcing programs to control rate and product selectivity, even for complex multistep catalytic mechanisms.

catalysis↗

DOE OSTI2021

Influence of Heave Plate Topology on Reaction Force

In this study, we explore the role of heave plate topology on fluid reaction forces using three, representative shapes: a hexagonal flat plate, a hexagonal conic with an open top, and the same with a closed top that encloses a fluid mass. We force each test article sinusoidally in a quiescent tank and decompose the reaction force using forms of the Morison equation for phase-invariant and phase-dependent parameterizations. We find that a flat plate generates 5.3 % more fluid reaction force than the open conic topology, and 21.4% more than the enclosed conic. Asymmetric topologies generate asymmetric reaction forces, but the magnitude of asymmetry is limited by nearly symmetric fluid inertia forces, which dominate over drag for these test articles. Additionally, we observe asymmetric vortex dynamics for the flat plate when the Keulegan-Carpenter number is between 1 and 2, accompanied by a shift in the phase of the peak force by of the oscillation period. As a consequence of this shift, the hydrodynamic coefficients estimated from the phase-dependent Morison equation decomposition are asymmetric, suggesting that phase-dependent representations may not provide physical insight in some hydrodynamic regimes.

added mass↗

DOE OSTI2023

Electro-optic transduction in silicon via gigahertz-frequency nanomechanics

Interfacing electronics with optical fiber networks is key to the long-distance transfer of classical and quantum information. Piezo-optomechanical transducers enable such interfaces by using gigahertz-frequency acoustic vibrations as mediators for converting microwave photons to optical photons via the combination of optomechanical and piezoelectric interactions. However, despite successful demonstrations, efficient quantum transduction remains out of reach due to the challenges associated with hybrid material integration and increased loss from piezoelectric materials when operating in the quantum regime. Here, we demonstrate an alternative approach in which we actuate 5-GHz phonons in a conventional silicon-on-insulator platform. In our experiment, microwave photons resonantly drive a phononic crystal oscillator via the electrostatic force realized in a charge-biased narrow-gap capacitor. The mechanical vibrations are subsequently transferred via a phonon waveguide to an optomechanical cavity, where they transform into optical photons in the sideband of a pump laser field. Operating at room temperature and atmospheric pressure, we measure a microwave-to-optical photon conversion efficiency of 1.72±0.14×10 −7 in a 3.3 MHz bandwidth. Our results mark a stepping stone towards quantum transduction with integrated devices made from crystalline silicon, which promise efficient high-bandwidth operation and integration with superconducting qubits. Additionally, the lack of need for piezoelectricity or other intrinsic nonlinearities makes our approach applicable to a wide range of materials for potential applications beyond quantum technologies.

42 ENGINEERING↗

DOE OSTI2024

Subpolar North Atlantic Mean State Affects the Response of the Atlantic Meridional Overturning Circulation to the North Atlantic Oscillation in CMIP6 Models

Abstract The Atlantic meridional overturning circulation (AMOC) plays an important role in climate, transporting heat and salt to the subpolar North Atlantic. The AMOC’s variability is sensitive to atmospheric forcing, especially the North Atlantic Oscillation (NAO). Because AMOC observations are short, climate models are a valuable tool to study the AMOC’s variability. Yet, there are known issues with climate models, like uncertainties and systematic biases. To investigate this, preindustrial control experiments from models participating in the phase 6 of Coupled Model Intercomparison Project (CMIP6) are evaluated. There is a large, but correlated, spread in the models’ subpolar gyre mean surface temperature and salinity. By splitting models into groups of either a warm–salty or cold–fresh subpolar gyre, it is shown that warm–salty models have a lower sea ice cover in the Labrador Sea and, hence, enable a larger heat loss during a positive NAO. Stratification in the Labrador Sea is also weaker in warm–salty models, such that the larger NAO-related heat loss can also affect greater depths. As a result, subsurface density anomalies are much stronger in the warm–salty models than in those that tend to be cold and fresh. As these anomalies propagate southward along the western boundary, they establish a zonal density gradient anomaly that promotes a stronger delayed AMOC response to the NAO in the warm–salty models. These findings demonstrate how model mean state errors are linked across variables and affect variability, emphasizing the need for improvement of the subpolar North Atlantic mean states in models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

CP-violating axion interactions II: axions as dark matter

Axions provide a solution to the strong CP problem and are excellent dark matter candidates. The presence of additional sources of CP violation, for example to account for the matter/antimatter asymmetry of the universe, can lead to CP-violating interactions between axions and Standard Model fields. In case axions form a coherent dark matter background, this leads to time-oscillating fundamental constants such as the fine-structure constant and particle masses. In this work we compare the sensitivity of various searches for CP-odd axion interactions. These include fifth-force experiments, searches for time-oscillating constants induced by axion dark matter, and direct limits from electric dipole moment experiments. We show that searches for oscillating constants can outperform fifth-force experiments in the regime of small axion masses, but, in general, do not reach the sensitivity of electric dipole moment experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Electron-phonon coupling induced intrinsic Floquet electronic structure

Floquet states are a topic of intense contemporary interest, which is often induced by coherent external oscillating perturbation (e.g., laser, or microwave) which breaks the continuous time translational symmetry of the systems. Usually, electron–phonon coupling modifies the electronic structure of a crystal as a non-coherent perturbation and seems difficult to form Floquet states. Surprisingly, we found that the thermal equilibrium electron–phonon coupling in M(MoS) 3 and M(MoSe) 3 (where M is a metallic element) exhibits a coherent behavior, and the electronic structure can be described by the Floquet theorem. Such a coherent Floquet state is caused by a selective giant electron–phonon coupling, with thermodynamic phonon oscillation serving as a driving force on the electronic part of the system. The quasi-1D Dirac cone at the Fermi energy has its band gap open and close regularly. Similarly, the electric current will oscillate even under a constant voltage.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Muon-neutrino disappearance with multiple liquid argon time projection chambers in the Fermilab Booster neutrino beam

The Short Baseline Neutrino (SBN) program consists of three liquid argon time projection chamber (LArTPC) experiments: SBND, MicroBooNE and ICARUS, with 110 m, 470 m and 600 m baselines respectively. The detectors are located in the Booster Neutrino Beam (BNB) at Fermilab which has a peak energy around 0.7 GeV and contains predominantly muon neutrinos. The baseline and energy range of the SBN program is conducive to measuring neutrino oscillation parameters under various sterile neutrino hypotheses. Sterile neutrinos have been proposed as a possible solution to the numerous short baseline anomalies. The proposed particles must be sterile in nature such that they do not interact via the weak force, however they may undergo oscillations with the active neutrino flavours. Their existence may consequently be confirmed through measurements of the appearance and disappearance of the active flavours. The analyses presented in this thesis aimed to calculate and understand the sensitivity of the SBN program to measuring the ?µ disappearance parameters under the (3+1) sterile neutrino oscillation hypothesis. The sensitivity of SBN to measuring the ?µ disappearance sterile oscillation parameters, sin2 2?µµ, ?m2 41, was calculated through semi-exclusive joint fits of the ?µ CC 0p and ?µ CC Other reconstructed neutrino energy spectra. The first iteration used truth-level Monte Carlo (MC) events, and determined that the 5s SBN sensitivity is comparable to the 90% MINOS/MINOS+ confidence level and supersedes the 90% MiniBooNE confidence level across entire phase space. Semi-exclusive joint fits of the aforementioned sample spectra were performed between the MC and multiple mock data sets in SBND. This analysis assessed the accuracy with which the near detector can disentangle systematic from physics effects in the oscillation analysis. The result was a 5.49% discrepancy between the ICARUS Monte Carlo and mock data event rates, when the systematic constraints from the near detector fit were extrapolated to the far detector. The second iteration of the SBN sensitivity analysis involved the application of an event selection procedure developed in SBND, following the full reconstruction chain. ?µ CC 0p events were selected from sample of neutrinos with 84.5% efficiency and 84.3% purity. The sterile neutrino sensitivity was determined once more at the near detector with these samples, and was shown to be consistent with the truth-level studies.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2022

Optimizing Magnetic Force Microscopy Resolution and Sensitivity to Visualize Nanoscale Magnetic Domains

Magnetic force microscopy (MFM) enables mapping local magnetic fields across a sample surface with nanoscale resolution. To perform MFM, an atomic force microscopy (AFM) probe whose tip has been magnetized vertically (i.e., perpendicular to the probe cantilever) is oscillated at a fixed height above the sample surface. The resultant shifts in the oscillation phase or frequency, which are proportional to the magnitude and sign of the vertical magnetic force gradient at each pixel location, are then tracked and mapped. Although the spatial resolution and sensitivity of the technique increases with decreasing lift height above the surface, this seemingly straightforward path to improved MFM images is complicated by considerations such as minimizing topographical artifacts due to shorter range van der Waals forces, increasing the oscillation amplitude to further improve sensitivity, and the presence of surface contaminants (in particular water due to humidity under ambient conditions). In addition, due to the orientation of the probe's magnetic dipole moment, MFM is intrinsically more sensitive to samples with an out-of-plane magnetization vector. Here, high-resolution topographical and magnetic phase images of single and bicomponent nanomagnet artificial spin-ice (ASI) arrays obtained in an inert (argon) atmosphere glovebox with <0.1 ppm O 2 and H 2 O are reported. Further, optimization of lift height and drive amplitude for high resolution and sensitivity while simultaneously avoiding the introduction of topographical artifacts is discussed, and detection of the stray magnetic fields emanating from either end of the nanoscale bar magnets (~250 nm long and <100 nm wide) aligned in the plane of the ASI sample surface is shown. Likewise, using the example of a Ni-Mn-Ga magnetic shape memory alloy (MSMA), MFM is demonstrated in an inert atmosphere with magnetic phase sensitivity capable of resolving a series of adjacent magnetic domains each ~200 nm wide.

47 OTHER INSTRUMENTATION↗

DOE OSTI2026

Hierarchical Testing of a Hybrid Machine Learning‐Physics Global Atmosphere Model

Machine learning (ML)-based models have demonstrated high skill and computational efficiency, often outperforming conventional physics-based models in weather and subseasonal predictions. While prior studies have assessed their fidelity in capturing synoptic-scale atmospheric dynamics, their performance across timescales and under out-of-distribution forcing, such as +3K or +4K uniform-warming forcings, and the sources of biases remain elusive, to establish the model's reliability for Earth science. Here, we design three sets of experiments targeting synoptic-scale phenomena, interannual variability, and out-of-distribution uniform-warming forcings. We evaluate the Neural General Circulation Model (NeuralGCM), a hybrid model integrating a dynamical core with ML-based component, against observations and physics-based Earth system models (ESMs). At the synoptic scale, NeuralGCM captures the evolution and propagation of extratropical cyclones with performance comparable to ESMs. At the interannual scale, when forced by El Niño-Southern Oscillation sea surface temperature (SST) anomalies, NeuralGCM successfully reproduces associated teleconnection patterns but exhibits deficiencies in capturing nonlinear response. Under out-of-distribution uniform-warming forcings, NeuralGCM simulates similar responses in global-average temperature and precipitation and reproduces large-scale tropospheric circulation features similar to those in ESMs. Notable weaknesses include overestimating the tracks and spatial extent of extratropical cyclones, biases in the teleconnected wave train triggered by tropical SST anomalies, and differences in upper-level warming and stratospheric circulation responses to SST warming compared to physics-based ESMs. The causes of these weaknesses were explored. Despite the noted weaknesses, NeuralGCM reproduces responses across experiments reasonably and performs comparably to ESMs. By integrating a dynamical core with ML, NeuralGCM shows potential for developing ML-based ESMs.

global warming↗

DOE OSTI2025

A Fundamentally New Coupled Approach to Contact Mechanics via the Dirichlet‐Neumann Schwarz Alternating Method

Contact phenomena are crucial for understanding the behavior of mechanical systems. However, existing computational approaches for simulating mechanical contact often face numerical challenges, such as inaccurate physical predictions, energy conservation errors, and unwanted oscillations. Here, we introduce an alternative technique for simulating dynamic contact based on the non‐overlapping Schwarz alternating method, originally developed for domain decomposition. In multibody contact scenarios, this method treats each body as a separate, non‐overlapping domain and prevents interpenetration using an alternating Dirichlet–Neumann iterative process. This approach has a strong theoretical foundation, eliminates the need for contact constraints, and offers flexibility, making it ideal for multiscale and multiphysics applications. We conducted a numerical comparison between the Schwarz method and traditional methods, such as the Lagrange multiplier and penalty methods, focusing on a benchmark impact problem. Our results indicate that the Schwarz alternating method outperforms traditional methods in several key areas: it provides more accurate predictions for various measurable quantities and demonstrates exceptional energy conservation capabilities. To address unwanted oscillations in contact velocities and forces, we explored various algorithms and stabilization techniques, ultimately opting for the naïve‐stabilized Newmark scheme for its simplicity and effectiveness. Additionally, we validated the efficiency of the Schwarz method in a three‐dimensional impact problem, highlighting its inherent capacity to accommodate different mesh topologies, time‐integration schemes, and time steps for each interacting body.

Schwarz alternating method↗

DOE OSTI2022

Momentum conservation in current drive and alpha-channeling-mediated rotation drive

Alpha channeling uses waves to extract hot ash from a fusion plasma, transferring energy from the ash to the wave. It has been proposed that this process could create a radial electric field, efficiently driving E × B rotation. However, existing theories ignore the nonresonant particles, which play a critical role in enforcing momentum conservation in quasilinear theory. Because cross field charge transport and momentum conservation are fundamentally linked, this non-consistency throws the rotation drive into question. This paper has two main goals. First, we provide a pedantic and cohesive introduction to the recently developed simple, general, self-consistent quasilinear theory for electrostatic waves that explains the torques which allow for current drive parallel to the magnetic field, and charge extraction across it; a theory that has largely resolved the question of rotation drive by alpha channeling. We show how the theory reveals a fundamental difference between the reaction of nonresonant particles to plane waves that grow in time vs steady-state waves that have a nonuniform spatial structure, allowing rotation drive in the latter case while precluding it in the former, and we review the local and global conservation laws that lead to this result. Second, we provide two new results in support of the theory. First, we provide a novel two-particle Hamiltonian model that rigorously establishes the relationship between charge transport and momentum conservation. Second, we compare the new quasilinear theory to the oscillation-center theories of ponderomotive forces, showing how the latter often obscure the time-dependent nonresonant recoil, but ultimately lead to similar results.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Integrable symplectic maps with a polygon tessellation

Identifying integrable dynamics remains a formidable challenge, and despite centuries of research, only a handful of examples are known to date. In this article, we explore a distinct form of area-preserving (symplectic) mappings derived from the stroboscopic Poincaré cross section of a kicked rotator—an oscillator subjected to an external force periodically switched on in short pulses. The significance of this class of problems extends to various applications in physics and mathematics, including particle accelerators, crystallography, and studies of chaos. Notably, Suris's theorem constrains the integrability within this category of mappings, outlining potential scenarios with analytic invariants of motion. In this paper, we challenge the assumption of the analyticity of the invariant by exploring piecewise linear transformations on a torus ( T 2 ) and associated systems on the plane ( R 2 ), incorporating arithmetic quasiperiodicity and discontinuities. Introducing a new automated technique, we discovered previously unknown scenarios featuring polygonal invariants that form perfect tessellations and, moreover, fibrations of the plane or torus. This work reveals a novel category of planar tilings characterized by discrete symmetries that emerge from the invertibility of transformations and are intrinsically linked to the presence of integrability. Our algorithm relies on the analysis of the Poincaré rotation number and its piecewise monotonic nature for integrable cases, contrasting with the noisy behavior in the case of chaos, thereby allowing for clear separation. Some of the newly discovered systems exhibit the peculiar behavior of “integrable diffusion,” characterized by infinite and quasirandom hopping between tiles while being confined to a set of invariant segments. Finally, through the implementation of a smoothening procedure, all mappings can be generalized to quasi-integrable scenarios with suppressed volume occupied by chaotic trajectories, thereby opening doors to potential practical applications. Published by the American Physical Society 2024

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

East Pacific ENSO Offers Early Predictive Signals for Harvest Yields

Abstract Annual wheat yields have steadily risen over the past century, but harvests remain highly variable and dependent on myriad weather conditions during a long growing season. In Kansas, for example, the 2014 crop year brought the lowest average yield in decades at 28 bushels per acre, while in 2016 farmers in the Wheat State, as Kansas is often called, enjoyed a historic high of 57 bushels per acre. It is broadly known that remote forces like El Niño–Southern Oscillation contribute to meteorological outcomes across North America, including in the wheat-growing regions of the U.S. Midwest, but the differential imprints of ENSO phases and flavors have not been well explored as leading indicators for harvest outcomes in highly specific agricultural regions, such as the more than 7 million acres upon which wheat is grown in Kansas. Here, we demonstrate a strong, steady, and long-term association between a simple “wheat yield index” and sea surface temperature anomalies, more than a year earlier, in the East Pacific, potentially offering insights into forthcoming harvest yields several seasons before planting commences.

Meteorology & Atmospheric Sciences↗

DOE OSTI2024

Investigating the Relative Contribution from Tropical Indo-Pacific SST to Asian Monsoon Precipitation Variability Using LIM

Abstract A critical issue is determining the factors that control the year-to-year variability in precipitation over southern Asia. In this study, we employ a cyclostationary linear inverse model (CS-LIM) to quantify the relative contribution of tropical Pacific and Indian Ocean sea surface temperature anomalies (SSTAs) to the interannual variability of the Asian monsoon, especially Indian summer monsoon rainfall (ISMR). Through a series of CS-LIM experiments, we isolate the impacts of the direct forcing from Pacific SSTAs, Indian Ocean SSTAs, and their interaction on Asian monsoon rainfall variability. Our results reveal distinct patterns of influence with the direct forcing from the Pacific (Indian) Ocean tending to enhance (reduce) the magnitude of precipitation variability, while the Indo-Pacific interaction acts to strongly damp the variability of Asian monsoon precipitation, especially over India. We further investigate these specific impacts on ISMR by analyzing the relationship between tropical Indo-Pacific SSTAs and the leading three empirical orthogonal functions (EOFs) of ISMR. The results from our CS-LIM experiments indicate that the direct forcing from El Niño–Southern Oscillation (ENSO) enhances the variability of the first and third EOFs, while the Indian Ocean SSTA opposes ENSO’s effects, which is consistent with previous studies. Our new results show that the tropical Indo-Pacific interaction strongly damps ISMR variability, which is due to the ENSO-induced Indian Ocean dipole (IOD) opposing the direct impacts from ENSO on ISMR. Additionally, reduced ENSO amplitude and duration associated with the Indo-Pacific interaction may also contribute to the damping effect on ISMR, but this requires further study to understand the relevant mechanisms.

Meteorology & Atmospheric Sciences↗

DOE OSTI2022

Quantum enhanced metrology in the search for fundamental physical phenomena

These notes summarize lectures given at the 2019 Les Houches summer school on Quantum Information Machines. They describe and review an application of quantum metrology concepts to searches for ultralight dark matter. In particular, for ultralight dark matter that couples as a weak classical force to a laboratory harmonic oscillator, quantum squeezing benefits experiments in which the mass of the dark matter particle is unknown. This benefit is present even if the oscillatory dark matter signal is much more coherent than the harmonic oscillator that it couples to, as is the case for microwave frequency searches for dark matter axion particles.

Lehnert, Konrad↗