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All sources NASA NTRS DOE OSTI

DOE OSTI2026

Measuring Loss Tangents of Substrates for Superconducting Qubits with Part-per-Billion Precision

We report precision measurements of dielectric loss tangents in substrates for superconducting qubits using an ultra-high quality factor niobium SRF cavity operating at millikelvin temperatures and low electric fields. Multiple substrate types and surface treatments are compared to assess how processing impacts microwave dissipation. The RF results are correlated with materials analysis, including ToF-SIMS and XPS, to identify dominant loss mechanisms. This combined study links microscopic surface chemistry to macroscopic performance and provides a framework for materials-driven improvements in qubit coherence and device design.

Bafia, Daniel [Fermilab]↗

DOE OSTI2026

Measuring Loss Tangents of Substrates for Superconducting Qubits with Part-per-Billion Precision

Bafia, Daniel [Fermilab]↗

DOE OSTI2021

Spin-texture-driven electrical transport in multi-Q antiferromagnets

Abstract Unusual magnetic textures can be stabilized in f -electron materials due to the interplay between competing magnetic interactions, complex Fermi surfaces, and crystalline anisotropy. Here we investigate CeAuSb 2 , an f -electron incommensurate antiferromagnet hosting both single- Q and double- Q spin textures as a function of magnetic fields ( H ) applied along the c axis. Experimentally, we map out the field-temperature phase diagram via electrical resistivity and thermal expansion measurements. Supported by calculations of a Kondo lattice model, we attribute the puzzling magnetoresistance enhancement in the double- Q phase to the localization of the electronic wave functions caused by the incommensurate magnetic texture.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Spatiotemporal imaging and manipulation of surface plasmons

Abstract Surface plasmon polaritons (SPPs) are travelling surface waves that have shown promise for applications in nanophotonics as they provide a direct route toward photon-mediated electrical signal generation – a central paradigm for speeding up and scaling down photonic elements. SPP waves have also generated fundamental interest due to their high-field strength and sub-wavelength confinement, properties that have enabled the surface-enhanced Raman effect. Over the last decade, photoemission electron microscopy (PEEM) has emerged as a pioneering technique for imaging surface electric fields through ultrashort laser pulse mediated electron emission and has therefore become an indispensable tool for characterizing plasmonic phenomena at interfaces in a variety of materials. PEEM offers nanometer spatial resolution and femtosecond temporal resolution, allowing SPPs to be prepared, monitored, and manipulated on the nanometer-femtosecond scale. Through a brief review of recent reports, we aim to introduce PEEM-based SPP imaging and manipulation modalities and highlight their utility in the context of emerging nanoscale and quantum materials science advancements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2008

Chemical Detection using Electrically Open Circuits having no Electrical Connections

This paper presents investigations to date on chemical detection using a recently developed method for designing, powering and interrogating sensors as electrically open circuits having no electrical connections. In lieu of having each sensor from a closed circuit with multiple electrically connected components, an electrically conductive geometric pattern that is powered using oscillating magnetic fields and capable of storing an electric field and a magnetic field without the need of a closed circuit or electrical connections is used. When electrically active, the patterns respond with their own magnetic field whose frequency, amplitude and bandwidth can be correlated with the magnitude of the physical quantities being measured. Preliminary experimental results of using two different detection approaches will be presented. In one method, a thin film of a reactant is deposited on the surface of the open-circuit sensor. Exposure to a specific targeted reactant shifts the resonant frequency of the sensor. In the second method, a coating of conductive material is placed on a thin non-conductive plastic sheet that is placed over the surface of the sensor. There is no physical contact between the sensor and the electrically conductive material. When the conductive material is exposed to a targeted reactant, a chemical reaction occurs that renders the material non-conductive. The change in the material s electrical resistance within the magnetic field of the sensor alters the sensor s response bandwidth and amplitude, allowing detection of the reaction without having the reactants in physical contact with the sensor.

Woodward, Stanley E.↗

NASA NTRS1981

Two-dimensional electron beam charging model for polymer films

A two-dimensional model is developed to describe the charging of strips of thin polymer films above a grounded substrate exposed to a uniform mono-energetic electron beam. The study is motivated by the observed anomalous behavior of geosynchronous satellites, which has been attributed to differential charging of the satellite surfaces exposed to magnetospheric electrons. Surface and bulk electric fields are calcuated at steady state in order to identify regions of high electrical stress, with emphasis on behavior near the material's edge. The model is used to study the effects of some of the experimental parameters, notably beam energy, beam angle of incidence, beam current density, material thickness and material width. Also examined are the consequences of a central gap in the material and a discontinuity in the material thickness.

Reeves, R. D.↗

DOE OSTI2025

Pathway to tune sputter coated Nb$_3$Sn with Zr

Superconducting radio frequency (SRF) cavities are essential elements of many modern-day particle accelerators such as, European XFEL (DESY), LCLS II-HE (SLAC) and PIP II (Fermilab). Nb$_3$Sn superconducting material promises significant potential to exceed the performance of conventional niobium based SRF cavities. We aim to advance the ongoing R$&$D efforts to achieve Nb$_3$Sn coated cavities with high material quality. In this work, we have developed to achieve a route for effectively reducing the intrinsic defects in magnetron sputter coated Nb$_3$Sn SRF cavities and eventually improve the overall RF performance. We have observed that Zr is mainly being incorporated as ZrO$_2$ precipitates of average dimensions ranging from 20-100nm. By increasing the concentration of Zr, we have three major effects in the physical properties. Firstly, we noted that the density of the surface and bulk voids as well as their average dimensions are dramatically reduced on increasing the Zr content in Nb$_3$Sn. These surface voids are believed to be detrimental to cavity applications due to increase the local dissipation of electric and magnetic fields. These results indicate that inclusion of Zr in Nb$_3$Sn sputtered coating will improve the material quality and might help to reduce the overall RF power dissipation. Secondly, we observed that increasing Zr concentration from 0 to 2.4% substantially improves both superconducting transition temperature (Tc) and upper critical magnetic field (Hc2). However, on further increasing the Zr concentration to 24%, we noticed a small decrement in the Hc2 value. These results infer that the increase in Zr concentration up to an optimal concentration will be beneficial to enhance the superconducting properties. Increase in Tc promises lesser RF losses and improvement in accelerating gradient, whereas the increase in Hc2 suggests more efficient flux pinning which could give rise to high quality factors in presence of multi-Tesla magnetic field. Additionally, we also observed that increasing Zr concentration possibly prevents the oxygen diffusion and leads to thinner formation of primary surface oxide (Nb$_2$O$_5$ and SnO). This study gives a route to tune Zr fraction in Nb3Sn to modify the physical properties that control the high field performance of Nb3Sn RF cavities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2019

Controlling spins with surface magnon polaritons

Polaritons in metals, semimetals, semiconductors, and polar insulators can allow for extreme confinement of electromagnetic energy, providing many promising opportunities for enhancing typically weak light-matter interactions such as multipolar radiation, multiphoton spontaneous emission, Raman scattering, and material nonlinearities. These extremely confined polaritons are quasielectrostatic in nature, with most of their energy residing in the electric field. As a result, these “electric” polaritons are far from optimized for enhancing emission of a magnetic nature, such as spin relaxation, which is typically many orders of magnitude slower than corresponding electric decays. Here, we take concepts of “electric” polaritons into magnetic materials, and propose using surface magnon polaritons in negative magnetic permeability materials to strongly enhance spin relaxation in nearby emitters. Specifically, we provide quantitative examples with MnF 2 and FeF 2 , enhancing spin transitions in the THz spectral range. In this work we find that these magnetic polaritons in 100-nm thin films can be confined to lengths over 10 000 times smaller than the wavelength of a photon at the same frequency, allowing for a surprising 12 orders of magnitude enhancement in magnetic dipole transitions. This takes THz spin-flip transitions, which normally occur at timescales on the order of a year, and forces them to occur at sub-ms timescales. Our results suggest an interesting platform for polaritonics at THz frequencies, and more broadly, a way to use polaritons to control light-matter interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Estimation of mean electron energy in helium surface ionization waves on dielectric substrates

Abstract The determination of basic plasma parameters in atmospheric pressure discharges is critical to advancing their use in applications. Atmospheric pressure plasma jets have found use in the fields of medicine, agriculture, material modification and others. Atmospheric pressure plasma jets often generate plasma surface ionization waves (SIW) which interact with and propagate over surfaces. Electrical diagnostics are challenging in SIW due to high collision frequencies and small scale of the plasma discharge. This work employs a passive optical emission line ratio technique to estimate the mean electron energy in SIW over planar dielectric substrates. The method uses an intensity ratio of two helium triplet lines: He( 3 3 S ) at 706.5 nm and He( 3 3 D ) at 587.56 nm. A collisional-radiative model is used to correlate line ratio to mean electron energy and determine dependencies on electron density and He/air gas mixture. Mean electron energies ranging from 3–8 eV are determined in He/air mixtures and are found to remain constant as the surface wave propagates radially. This work provides a 2D, time-resolved, mean electron energy diagnostic for surface ionization wave propagation and validation of numerical modeling in atmospheric pressure systems with spatially varying He/air gas mixtures. The model in question is designed for use with any He line ratio in the n = 3 excitation level.

Morsell, Joshua (ORCID:0000000331073002)↗

NASA NTRS2010

Methods of Using a Magnetic Field Response Sensor Within Closed, Electrically Conductive Containers

Magnetic field response sensors are a class of sensors that are powered via oscillating magnetic fields, and when electrically active, respond with their own magnetic fields with attributes dependent upon the magnitude of the physical quantity being measured. A magnetic field response recorder powers and interrogates the magnetic sensors [see Magnetic-Field-Response Measurement- Acquisition System, NASA Tech Briefs Vol. 30, No, 6 (June 2006, page 28)]. Electrically conductive containers have low transmissivity for radio frequency (RF) energy and thus present problems for magnetic field response sensors. It is necessary in some applications to have a magnetic field response sensor s capacitor placed in these containers. Proximity to conductive surfaces alters the inductance and capacitance of the sensors. As the sensor gets closer to a conductive surface, the electric field and magnetic field energy of the sensor is reduced due to eddy currents being induced in the conductive surface. Therefore, the capacitors and inductors cannot be affixed to a conductive surface or embedded in a conductive material. It is necessary to have a fixed separation away from the conductive material. The minimum distance for separation is determined by the desired sensor response signal to noise ratio. Although the inductance is less than what it would be if it were not in proximity to the conductive surface, the inductance is fixed. As long as the inductance is fixed, all variations of the magnetic field response are due to capacitance changes. Numerous variations of inductor mounting can be utilized, such as providing a housing that provides separation from the conductive material as well as protection from impact damage. The sensor can be on the same flexible substrate with a narrow throat portion of the sensor between the inductor and the capacitor, Figure 1. The throat is of sufficient length to allow the capacitor to be appropriately placed within the container and the inductor placed outside the container. The throat is fed through the orifice in the container wall (e.g., fuel tank opening) and connects to the inductor and capacitor via electrical leads to form a closed circuit, Figure 2. Another embodiment is to have the inductor and capacitor fabricated as separate units. In this embodiment, the inductor is mounted external to the container, and the capacitor is mounted internal to the container, Figure 1. Electrical leads are fed through the orifice to connect the inductor and capacitor, Figure 2. When a container holding multiple sensors is made of a conductive material, an antenna can be placed internal to the container. An internal antenna allows all components of the sensors to reside inside the container. The antenna must be separated from the container wall s conductive surface. Additionally, the inductors must be maintained in a fixed position relative to and separated from the container

Woodward, Stanley E.↗

DOE OSTI2025

Impact of CuInP 2 S 6 –metal interfaces on the stabilization of polar phases and polarization switching

The multifunctionality of two-dimensional ferroelectric CuInP 2 S 6 (CIPS) arises from the existence of multiple polar phases combined with a high ionic conductivity that facilitates polarization switching in unusual ways. The van der Waals (vdW) layered structure provides ultrathin flakes and ideal interfaces to integrate with other materials for microelectronics and neuromorphic elements. However, device integration necessitates metal contacts to read, write, or transmit signals. In this work, we find that different types of metal–CIPS interfaces strongly impact the stabilization of specific polar phases and the field-induced transitions between the polarization states. Cu electrodes initially suppress the piezoresponse, whereas, at CIPS–Ag interfaces, the electromechanical signal is increased. Under electric fields, the Cu electrodes, Ag electrodes and surrounding CIPS surfaces can show distinct switching behavior as different phases and polarization orientations are stabilized. These findings highlight that metal–CIPS interfaces provide the opportunity to optimize functional material properties.

Ferroelectrics and multiferroics↗

NASA NTRS1973

Summary of scientific results

The accomplishments of the Apollo 17 flight are summarized. The basic objective of the mission was to sample basin-rim highland material and adjacent mare material and to investigate the geological evolutionary relationship between these two major units. The lunar experiments which were conducted include: (1) lunar field geology, (2) surface electrical experiments, (3) lunar traverse gravimeter experiments, (4) lunar seismic profiling experiment, (5) lunar ejecta and meteorites experiment, (6) analysis of lunar atmosphere composition, and (7) heat flow experiments.

Parker, R. A.↗

NASA NTRS1981

Design of an arc-free thermal blanket

The success of a multilayer thermal blanket in eliminating arcing is discussed. Arcing is eliminated by limiting the surface potential to well below the threshold level for discharge. This is achieved by enhancing the leakage current which results in conduction of the excess charge to the spacecraft structure. The thermal blanket consists of several layers of thermal control (space approved) materials, bonded together, with Kapton on the outside, arranged in such a way that when the outer surface is charged by electron irradiation, a strong electric field is set up on the Kapton layer resulting in a greatly improved conductivity. The basic properties of matter utilized in designing this blanket method of charge removal, and optimum thermo-optical properties are summarized.

Fellas, C. N.↗

NASA NTRS1981

Two-dimensiosnal electron beam charging model for polymer films

A two dimensional model was developed to describe the charging of thin polymer films exposed to a uniform mon-energetic electron beam. The study was motivated by observed anomalous behavior of geosynchronous satellites which was attributed to electrical discharges associated with the differential charging of satellite surfaces of magnetospheric electrons. Electric fields both internal and external to the irradiated specimen were calculated at steady state in order to identify regions of high electrical stress. Particular emphasis was placed on evaluating the charging characteristics near the material's edge. The model was used to identify and quantify the effects of some of the experimental parameters notably: beam energy; beam angle of incidence; beam current density; material thickness; and material width. Simulations of the following situations were also conducted: positive or negative precharging over part of the surface; a central gap in the material; and a discontinuity in the material's thickness.

Reeves, R. D.↗

NASA NTRS1972

Previous design restraints and radiation damage effects of low energy particles

Spacecraft design fluences and damage by low energy electrons and protons are summarized. For electron energies 5 MeV, the design fluence is 10 to the 11th power electrons/sq cm; for energies 5 MeV, the integral spectrum is assumed to go as 1/E sq. The design fluences for proton energies 30 MeV is 1.5 x 10 to the 9th power protons/sq cm; for energies 100 MeV, it is 5 x 10 to the 14th power protons/sq cm. The radioisotope thermoelectric generator gamma and neutron radiation constraints are listed. Damage due to electron energies 0.5 MeV and proton energies 10 MeV are summarized for effects on spacecraft thermal surfaces, reflective surfaces, and refractive materials. The high frequency noise figure for field effect transistors may increase markedly, and another effect is the buildup of charge on insulating surfaces, resulting in large electric fields.

Trainor, J. H.↗

NASA NTRS1985

Electric propulsion produced environments and possible interactions with the SP-100 power system

An examination of a conceptual SP-100 type power system has been conducted to assess the effect of possible electric thruster induced contamination. The operating characteristics and known exhaust plume properties of various electric thrusters are summarized along with the natural environment and its effects to provide background for the contamination discussion. Charge buildup on nonconducting surfaces, differential charging of surfaces and arcing should be moderated by the operation of an electric thruster system. Thin film deposition of eroded thruster materials is a possible contamination mechanism. Electric thruster field efflux and propellant condensation should have only a minor contaminating effect upon a nuclear power system.

Deininger, W. D.↗

NASA NTRS1999

Electric Field Double Probe Measurements on Satellites with Very Low Perigees

Measurements of DC and AC electric Fields at low altitudes (less than 150 km) in the Earth's ionosphere address a wide array of important scientific questions including Joule Heating, the closure of field aligned currents, and the deviation of E x B electron velocities from ion velocity vectors influenced by collisions. Double probes represent a well-proven technique for gathering high quality DC and AC electric field measurements for which the design of the boom system is of critical importance for the success of the experiment. In general, ionospheric DC electric field instruments that achieve accuracies of 0.1 mV/m or better, place sensors at large distances from the spacecraft body in order to extend well beyond the spacecraft wake and sheath and to achieve the large signal-to-noise ratios for DC and long wavelength measurements. Additional sets of sensors inboard of the primary, outermost sensors provide useful additional information, both for diagnostics of the plasma contact potentials, which particularly enhance the DC electric field measurements on non-spinning spacecraft, and for wavelength and phase velocity measurements that use the spaced receiver or "Interferometer" technique. Accurate attitude knowledge enables V x B contributions to be subtracted from the measured potentials, and permits the measured components to be rotated into meaningful geophysical reference frames. This presentation discusses the expected performance of electric field double probe experiments and their boom mechanisms on both spinning and non-spinning satellite platforms with very low perigees. Careful selection of probe surface materials, such as titanium nitride, for the low perigee environment, as well as thermal considerations are also discussed.

Pfaff, R. F., Jr.↗

NASA NTRSDate not supplied

Development of a Comprehensive Physics-Based Model for Study of NASA Gateway Lunar Dust Contamination

NASA is committed to landing the first woman and first person of color on the Moon by 2025 to begin a sustaining presence. A major component of this mission is NASA’s orbiting lunar outpost, Gateway, that will be subjected to the harsh environment of space during its 7-day orbit around the Moon. One aspect of this environment that is not well quantified is microscopic lunar regolith particles, or simply, lunar dust. As Apollo 17 Mission Commander Eugene Cernan said, “I think dust is probably one of our greatest inhibitors to a nominal operation on the moon. I think we can overcome other physiological or physical or mechanical problems except dust” [1]. These dust particles, most of which are smaller than the width of two human hairs and of highly irregular shape, are composed mainly of dielectric materials. Such characteristics can allow the dust particles to collect electric charge from the surrounding environment, resulting in electrostatic interactions between the dust, electromagnetic fields, and electrically charged surfaces [2-3]. Due to the nature of these fields, dust can collect on and contaminate charged surfaces. Lunar dust introduced into the Gateway environment by a lunar ascent vehicle element returning from the surface of the Moon presents risks to Gateway hardware such as radiators, solar arrays, antennae, and docking mechanisms. To quantify this risk and inform NASA, International Partner, and Commercial Provider stakeholders, Booz Allen, in partnership with NASA, is developing a toolset to model the interaction of charged lunar dust particles with the cis-lunar and deep-space environments. This includes a comprehensive physics model of the space plasma and solar radiation environment and electromagnetic interaction of spacecraft and lunar dust. Spacecraft charging and plasma environment are solved using the open-source code from The French Aerospace Lab (ONERA) and the European Space Agency (ESA), known as Spacecraft Plasma Interaction Software (SPIS) [4]. The physics of particle charging and motion is handled by a time-dependent implementation of Orbital-Motion-Limited (OML) theory which accounts for plasma flows and positive potential grains [5-7], using Siemens STAR-CCM+ as the framework. Model validation includes lab experiments by NASA experts and academia, as well as future on-orbit dust detecting payloads on the exterior of Gateway and Commercial Lunar Payload Services (CLPS) missions to the lunar surface [7-9]. The results and analyses will inform Gateway Program system owners at risk for lunar dust contamination.

Complex Plasma↗