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Comparisons of Bispectral and Polarimetric Retrievals of Marine Boundary Layer Cloud Microphysics: Case Studies Using a LES- Satellite Retrieval Simulator

Many passive remote-sensing techniques have been developed to retrieve cloud microphysical properties from satellite-based sensors, with the most common approaches being the bispectral and polarimetric techniques. These two vastly different retrieval techniques have been implemented for a variety of polar-orbiting and geostationary satellite platforms, providing global climatological data sets. Prior instrument comparison studies have shown that there are systematic differences between the droplet size retrieval products (effective radius) of bispectral (e.g., MODIS, Moderate Resolution Imaging Spectroradiometer) and polarimetric (e.g., POLDER, Polarization and Directionality of Earth's Reflectances) instruments. However, intercomparisons of airborne bispectral and polarimetric instruments have yielded results that do not appear to be systematically biased relative to one another. Diagnosing this discrepancy is complicated, because it is often difficult for instrument intercomparison studies to isolate differences between retrieval technique sensitivities and specific instrumental differences such as calibration and atmospheric correction. In addition to these technical differences the polarimetric retrieval is also sensitive to the dispersion of the droplet size distribution (effective variance), which could influence the interpretation of the droplet size retrieval. To avoid these instrument-dependent complications, this study makes use of a cloud remote-sensing retrieval simulator. Created by coupling a large-eddy simulation (LES) cloud model with a 1-D radiative transfer model, the simulator serves as a test bed for understanding differences between bispectral and polarimetric retrievals. With the help of this simulator we can not only compare the two techniques to one another (retrieval intercomparison) but also validate retrievals directly against the LES cloud properties. Using the satellite retrieval simulator, we are able to verify that at high spatial resolution (50m) the bispectral and polarimetric retrievals are highly correlated with one another within expected observational uncertainties. The relatively small systematic biases at high spatial resolution can be attributed to different sensitivity limitations of the two retrievals. In contrast, a systematic difference between the two retrievals emerges at coarser resolution. This bias largely stems from differences related to sensitivity of the two retrievals to unresolved inhomogeneities in effective variance and optical thickness. The influence of coarse angular resolution is found to increase uncertainty in the polarimetric retrieval but generally maintains a constant mean value.

Miller, Daniel J.↗

Evaluation of the Impacts of Biomass Burning Aerosols on the NASA GEOS Sub-Seasonal Climate Forecasts

Emission sources of trace gases and aerosol particles in the South American (SA)and African (Af) continents have a strong seasonal and space variability associated with the extensive vegetation fires activities. In both continents, during the austral winter, the fires affect mainly tropical forest and savannah-type biomes and are mostly associated with deforestation and agricultural/pasture land management. Smoke aerosol particles, on average, contribute to at least 90% of the total aerosol optical depth (AOD) in the visible spectrum in the case of the South America regional smoke. Smoke aerosols also act as cloud condensation nuclei affecting cloud microphysics properties and therefore, changing the radiation budget, hydrological cycle and global circulation patterns over disturbed areas (Kaufman, 1995; Rosenfeld, 1999; Andreae,et al., 2004; Koren et al., 2004, Zhang, 2008; Ott et al., 2010; Randles et al., 2013). This study aims to evaluate and quantify the impact of including a comprehensive emission field of biomass burning aerosol on the performance of a seasonal climate forecast system, not only regarding the AOD itself but mainly on the meteorological state variable (e.g., precipitation and temperature). To address the questions put above, we designed two numerical experiments: 1- named"AERO_CTL" which applies the Quick Fire Emissions Dataset (QFED) emissions estimated with intra-diurnal variation (hereafter, BBE), and 2- named "AERO_CLM" where the sourcee mission is based on a climatology of the QFED emissions, with only monthly variation(hereafter, BBCLIM). Hindcast simulations were produced using the Goddard Earth ObservingSystem global circulation model, version 5, sub-seasonal to seasonal (GEOS5-S2S) system with a nominal spatial resolution of 56km (Rienecker et al., 2008). In both experiments, the aerosol feedbacks from cloud developments and radiation interactions were accounted. The two experiments consisted of 4 members each and ran from June to November spanning over the years 2000 to 2015. Model performance was evaluated by calculating statistical metrics on the mean area of SA and Af. Our results demonstrated that the skill model in predicting AOD is significantly improve when BBE source emission is applied over SA, but not over the Afcontinent. Over SA, the correlation between the AERO_CTL model configuration and MERRA-2 is 0.93 (R2= 0.86, RMS=0.02, BIAS=0.01), while the AERO_CLM model presents a value of0.81 (R2= 0.65, RMS=0.04, BIAS=0.06). However, the AERO_CTL experiment better represents the inter-annual variability of the AOS in both regions. The gain of the skill in predicting the AOD by the AERO_CTL experiment is also seen in some meteorological variables. We observed an increase in the model skill in predicting the 2-meter temperature and precipitation of up to 0.3 for the AERO_CTL experiment in comparison to the AERO_CLM. AERO_CLM. According to the analyzed hindcast, we inferred that representing the BBE more realistically implies in a significant gain of skills in the seasonal climate forecasting over SA and Af continents.

Aerosol↗

The Cirrus Parcel Model Comparison Project

The cirrus Parcel Model Comparison Project involves the systematic comparison of current models of ice crystal nucleation and growth for specified, typical, cirrus cloud environments. In Phase 1 of the project reported here, simulated cirrus cloud microphysical properties are compared for situations of "warm" (-40 C) and "cold" (-60 C) cirrus subject to updrafts of 4, 20 and 100 centimeters per second, respectively. Five models are participating in the project. These models employ explicit microphysical schemes wherein the size distribution of each class of particles (aerosols and ice crystals) is resolved into bins. Simulations are made including both homogeneous and heterogeneous ice nucleation mechanisms. A single initial aerosol population of sulfuric acid particles is prescribed for all simulations. To isolate the treatment of the homogeneous freezing (of haze drops) nucleation process, the heterogeneous nucleation mechanism is disabled for a second parallel set of simulations. Qualitative agreement is found amongst the models for the homogeneous-nucleation-only simulations, e.g., the number density of nucleated ice crystals increases with the strength of the prescribed updraft. However, non-negligible quantitative differences are found. Systematic bias exists between results of a model based on a modified classical theory approach and models using an effective freezing temperature approach to the treatment of nucleation. Each approach is constrained by critical freezing data from laboratory studies. This information is necessary, but not sufficient, to construct consistent formulae for the two approaches. Large haze particles may deviate considerably from equilibrium size in moderate to strong updrafts (20-100 centimeters per second) at -60 C when the commonly invoked equilibrium assumption is lifted. The resulting difference in particle-size-dependent solution concentration of haze particles may significantly affect the ice nucleation rate during the initial nucleation interval. The uptake rate for water vapor excess by ice crystals is another key component regulating the total number of nucleated ice crystals. This rate, the product of ice number concentration and ice crystal diffusional growth rate, partially controls the peak nucleation rate achieved in an air parcel and the duration of the active nucleation time period.

Lin, Ruei-Fong↗

GCSS Cirrus Parcel Model Comparison Project

The Cirrus Parcel Model Comparison Project, a project of GCSS Working Group on Cirrus Cloud Systems (WG2), involves the systematic comparison of current models of ice crystal nucleation and growth for specified, typical, cirrus cloud environments. The goal of this project is to document and understand the factors resulting in significant inter-model differences. The intent is to foment research leading to model improvement and validation. In Phase 1 of the project reported here, simulated cirrus cloud microphysical properties are compared for situations of "warm" (-40 C) and "cold" (-60 C) cirrus subject to updrafts of 4, 20 and 100 cm/s, respectively. Five models participated. These models employ explicit microphysical schemes wherein the size distribution of each class of particles (aerosols and ice crystals) is resolved into bins. Simulations are made including both homogeneous and heterogeneous ice nucleation mechanisms. A single initial aerosol population of sulfuric acid particles is prescribed for all simulations. To isolate the treatment of the homogeneous freezing (of haze drops) nucleation process, the heterogeneous nucleation mechanism is disabled for a second parallel set of simulations. Qualitative agreement is found for the homogeneous-nucleation-only simulations, e.g., the number density of nucleated ice crystals increases with the strength of the prescribed updraft. However, non-negligible quantitative differences are found. Detailed analysis reveals that the homogeneous nucleation formulation, aerosol size, ice crystal growth rate (particularly the deposition coefficient), and water vapor uptake rate are critical components that lead to differences in predicted microphysics. Systematic bias exists between results based on a modified classical theory approach and models using an effective freezing temperature approach to the treatment of nucleation. Each approach is constrained by critical freezing data from laboratory studies, but each includes assumptions that can only be justified by further laboratory data. Consequently, it is not yet clear if the two approaches can be made consistent. Large haze particles may deviate considerably from equilibrium size in moderate to strong updrafts (20-100 cm/s) at -60 C when the commonly invoked equilibrium assumption is lifted. The resulting difference in particle-size-dependent solution concentration of haze particles may significantly affect the ice nucleation rate during the initial nucleation interval. The uptake rate for water vapor excess by ice crystals is another key component regulating the total number of nucleated ice crystals. This rate, the product of ice number concentration and ice crystal diffusional growth rate, which is sensitive to the deposition coefficient when ice particles are small, partially controls the peak nucleation rate achieved in an air parcel and the duration of the active nucleation time period. The effects of heterogeneous nucleation are most pronounced in weak updraft situations. Vapor competition by the nucleated (heterogeneous) ice crystals limits the achieved ice supersaturation and thus suppresses the contribution of homogeneous nucleation. Correspondingly, ice crystal number density is markedly reduced. Definitive laboratory and atmospheric benchmark data are needed for the heterogeneous nucleation process. Inter-model differences are correspondingly greater than in the case of the homogeneous nucleation process acting alone.

Lin, Ruei-Fong↗

The DC-8 Submillimeter-Wave Cloud Ice Radiometer

An airborne radiometer is being developed to demonstrate the capability of radiometry at submillimeter-wavelengths to characterize cirrus clouds. At these wavelengths, cirrus clouds scatter upwelling radiation from water vapor in the lower troposphere. Radiometric measurements made at multiple widely spaced frequencies permit flux variations caused by changes in scattering due to crystal size to be distinguished from changes in cloud ice content. Measurements at dual polarizations can also be used to constrain the mean crystal shape. An airborne radiometer measuring the upwelling submillimeter-wave flux should then able to retrieve both bulk and microphysical cloud properties. The radiometer is being designed to make measurements at four frequencies (183 GHz, 325 GHz, 448 GHz, and 643 GHz) with dual-polarization capability at 643 GHz. The instrument is being developed for flight on NASA's DC-8 and will scan cross-track through an aircraft window. Measurements with this radiometer in combination with independent ground-based and airborne measurements will validate the submillimeter-wave radiometer retrieval techniques. The goal of this effort is to develop a technique to enable spaceborne characterization of cirrus, which will meet a key climate measurement need. The development of an airborne radiometer to validate cirrus retrieval techniques is a critical step toward development of spaced-based radiometers to investigate and monitor cirrus on a global scale. The radiometer development is a cooperative effort of the University of Colorado, Colorado State University, Swales Aerospace, and Jet Propulsion Laboratory and is funded by the NASA Instrument Incubator Program.

Walter, Steven J.↗

Cirrus Parcel Model Comparison Project: The Critical Components to Simulate Cirrus Initiation Explicitly - Phase 1

The Cirrus Parcel Model Comparison Project, a project of the GCSS (GEWEX Cloud System Studies) Working Group on Cirrus Cloud Systems, involves the systematic comparison of current models of ice crystal nucleation and growth for specified, typical, cirrus cloud environments. In Phase I of the project reported here, simulated cirrus cloud microphysical properties are compared for situations of "warm" (40 C) and "cold" (-60 C) cirrus, both subject to updrafts of 4, 20 and 100 centimeters per second. Five models participated. The various models employ explicit microphysical schemes wherein the size distribution of each class of particles (aerosols and ice crystals) is resolved into bins or treated separately. Simulations are made including both the homogeneous and heterogeneous ice nucleation mechanisms. A single initial aerosol population of sulfuric acid particles is prescribed for all simulations. To isolate the treatment of the homogeneous freezing (of haze droplets) nucleation process, the heterogeneous nucleation mechanism is disabled for a second parallel set of simulations. Qualitative agreement is found for the homogeneous-nucleation- only simulations, e.g., the number density of nucleated ice crystals increases with the strength of the prescribed updraft. However, significant quantitative differences are found. Detailed analysis reveals that the homogeneous nucleation rate, haze particle solution concentration, and water vapor uptake rate by ice crystal growth (particularly as controlled by the deposition coefficient) are critical components that lead to differences in predicted microphysics. Systematic bias exists between results based on a modified classical theory approach and models using an effective freezing temperature approach to the treatment of nucleation. Each approach is constrained by critical freezing data from laboratory studies, but each includes assumptions that can only be justified by further laboratory research. Consequently, it is not yet clear if the two approaches can be made consistent. Large haze particles may deviate considerably from equilibrium size in moderate to strong updrafts (20-100 centimeters per second) at -60 C when the commonly invoked equilibrium assumption is lifted. The resulting difference in particle-size- dependent solution concentration of haze particles may significantly affect the ice particle formation rate during the initial nucleation interval. The uptake rate for water vapor excess by ice crystals is another key component regulating the total number of nucleated ice crystals. This rate, the product of particle number concentration and ice crystal diffusional growth rate, which is particularly sensitive to the deposition coefficient when ice particles are small, modulates the peak particle formation rate achieved in an air parcel and the duration of the active nucleation time period. The effects of heterogeneous nucleation are most pronounced in weak updraft situations. Vapor competition by the heterogeneously nucleated ice crystals may limit the achieved ice supersaturation and thus suppresses the contribution of homogeneous nucleation. Correspondingly, ice crystal number density is markedly reduced. Definitive laboratory and atmospheric benchmark data are needed for the heterogeneous nucleation process. Inter-model differences are correspondingly greater than in the case of the homogeneous nucleation process acting alone.

Lin, Ruei-Fong↗

Evaluation of NCAR Icing/SLD Forecasts, Tools and Techniques Used During The 1998 NASA SLD Flight Season

Supercooled Large Droplet (SLD) icing conditions were implicated in at least one recent aircraft crash, and have been associated with other aircraft incidents. Inflight encounters with SLD can result in ice accreting on unprotected areas of the wing where it can not be removed. Because this ice can adversely affect flight characteristics of some aircraft, there has been concern about flight safety in these conditions. The FAA held a conference on in-flight icing in 1996 where the state of knowledge concerning SLD was explored. One outcome of these meetings was an identified need to acquire SLD flight research data, particularly in the Great Lakes Region. The flight research data was needed by the FAA to develop a better understanding of the meteorological characteristics associated with SLD and facilitate an assessment of existing aircraft icing certification regulations with respect to SLD. In response to this need, NASA, the Federal Aviation Administration (FAA), and the National Center for Atmospheric Research (NCAR) conducted a cooperative icing flight research program to acquire SLD flight research data. The NASA Glenn Research Center's Twin Otter icing research aircraft was flown throughout the Great Lakes region during the winters of 1996-97 and 1997-98 to acquire SLD icing and meteorological data. The NASA Twin Otter was instrumented to measure cloud microphysical properties (particle size, LWC (Liquid Water Content), temperature, etc.), capture images of wing and tail ice accretion, and then record the resultant effect on aircraft performance due to the ice accretion. A satellite telephone link enabled the researchers onboard the Twin Otter to communicate with NCAR meteorologists. who provided real-time guidance into SLD icing conditions. NCAR meteorologists also provided preflight SLD weather forecasts that were used to plan the research flights, and served as on-board researchers. This document contains an evaluation of the tools and techniques NCAR forecasters used to predict the location of SLD icing conditions during the winter of 1997-1998. The objectives of this report are to: (1) assess the tools used to forecast in-flight icing. (2) assess the success/failure rate of the forecasts, and (3) discuss suggested changes to forecast techniques.

Bernstein, Ben C.↗

Sensitivity of Stratocumulus Optical Depths to Droplet Concentrations: Satellite Observations and Large-Eddy Simulations

A number of observations and simulations have shown that increased droplet concentrations in ship tracks increase their total cross-sectional area, thereby enhancing cloud albedo and providing a negative (cooling) radiative forcing at the surface and the top of the atmosphere. In some cases cloud water has been found to be enhanced in ship tracks, which has been attributed to suppression of drizzle and implies an enhanced susceptibility of cloud albedo to droplet concentrations. However, observations from aircraft and satellite indicate that on average cloud water is instead reduced in daytime ship tracks. Such a reduction in liquid water may be attributable to cloud-burning caused by solar heating by soot within the ship exhaust, or by increased precipitation resulting from giant nuclei in the ship exhaust. We will summarize the observational evidence and present results from large-eddy simulations that evaluate these mechanisms. Along the way we will present our insights into the interpretation of satellite retrievals of cloud microphysical properties.

Ackerman, A. S.↗

Cirrus Parcel Model Comparison Phase 2

The Cirrus Parcel Model Comparison (CPMC) project, a project of the GEWEX Cloud System Study Working Group on cirrus clouds (GCSS WG2), is an international effort to advance our knowledge of numerical simulations of cirrus cloud initiation. This project was done in two phases. In Phase 1 of CPMC, the critical components determining the predicted cloud microphysical properties were identified using parcel models in which the aerosol and ice crystal size distributions are explicitly resolved, the formulation of the homogeneous freezing of aqueous solution droplets, especially the gradient of nucleation rate with respect to solution concentration; aerosol growth modeling; and the mass accommodation coefficient of water vapor on ice surface (the deposition coefficient). In Phase 1, all simulations were conducted using a given background aerosol distribution. To complete the comparison study, participant model responses to a range of background aerosol distributions are investigated in Phase 2.

Lin, Ruei-Fong↗

Vertical Profiles of Mars 1.27 Micrometer O2 Dayglow from MRO CRISM Limb Spectra: Seasonal/global Behaviors, Comparisons to LMDGCM Simulations, and a Global Definition for Mars Water Vapor Profiles

Since July of 2009, The Compact Reconnaissance Imaging Spectral Mapper (CRISM) onboard the Mars Re- connaissance Orbiter (MRO) has periodically obtained pole-to-pole observations (i.e., full MRO orbits) of limb scanned visible/near IR spectra (lambda= 0.4 - 4.0 micrometers, delta lambda approx. 10 nm- Murchie et al., 2007). These CRISM limb observations support the first seasonally and spatially extensive set of Mars 1.27 micometers O2 (1 delta(sub g)) day-glow profile retrievals (approx. 1100) over greater than or equal to 8-80 km altitudes. Their comparison to Laboratoire de Meteorologie Dynamique (LMD) global climate model (GCM) simulated O2 (1 delta(sub g)) volume emission rate (VER) profiles, as a function of altitude, latitude, and season (solar longitude, L(sub s), supports several key conclusions regarding Mars atmospheric water vapor (which is derived from O2 (1 delta(sub g)) emission rates), Mars O3, and the collisional de-excitation of O2 (1 delta(sub g)) in the Mars CO2 atmosphere. Current (Navarro et al., 2014) LMDGCM simulations of Mars atmospheric water vapor fall 2-3 times below CRISM derived water vapor abundances at 20-40 km altitudes over low-to-mid latitudes in northern spring (L(sub s) = 30-60 deg), and northern mid-to-high latitudes over northern summer (L(sub s) = 60-140 deg). In contrast, LMDGCM simulated water vapor is 2-5 times greater than CRISM derived values at all latitudes and seasons above 40 km, within the aphelion cloud belt (ACB), and over high-southern to mid-southern latitudes in southern summer (L(sub s) = 190-340 deg) at 15-35 km altitudes. Overall, the solstitial summer-to-winter hemisphere gradients in water vapor are reversed between the LMDGCM modeled versus the CRISM derived water vapor abundances above 10-30 km altitudes. LMDGCM-CRISM differences in water vapor profiles correlate with LMDGCM-CRISM differences in cloud mixing profiles; and likely reflect limitations in simulating cloud microphysics and radiative forcing, both of which restrict meridional transport of water from summer- to-winter hemispheres on Mars (Clancy et al., 1996; Montmessin et al., 2004; Steele et al., 2014; Navarro et al., 2014) and depend on uncertain cloud microphysical properties (Navarro et al., 2014). The derived low-to-mid latitude changes in Mars water vapor vertical distributions should reduce current model- data disagreements in column O3 and H2O2 abundances over low-to-mid latitudes (e.g., within the ACB; Lefevre et al., 2008; Encrenaz et al., 2015; Clancy et al., 2016). Lastly, the global/seasonal average com- parison of CRISM and LMDGCM O2 (1 delta(sub g)) VER below 20 km altitudes indicates a factor of approx. 3 times lower value (0.25 x 10(exp -20) cu cm sec(exp -1)) for the CO2 collisional de-excitation rate coefficient of O2 (1 delta(sub g)) than derived recently by Guslyakova et al. (2016).

Clancy, R. Todd↗

Space-Based Lidar Observations of the 3D Structure of the Earth System

Lidar provides precise measurements of the three-dimensional structure of the clouds, aerosols, ocean/land/snow/ice surfaces, as well as ocean subsurface. Lidar also provides unique information about physical propertiesof particulates in the atmosphere for both radiative transfer and air quality applications.In this talk, I will present an overview of our recent studies of aerosols, clouds, ocean and snow using space-based lidar measurements (e.g., LITE, CALIPSO and ICESat-2), such as classifications of aerosols and thermodynamics phase of clouds, cloud microphysical properties, snow depths and phytoplankton biomass. I will also introduce a new concept of 3D Earth system observations with data fusion though combined active/passive remote sensing and machine learning. The new concept aims to reveal vertical structure of the aerosols/clouds/surfaces/subsurface from passive sensors by taking advantage of lidar measurements to effectively resolve the vertical structureby unscrambling the highly convoluted multi-angle, spectral and polarization information from passive sensors and apply the knowledge to a large swath where lidar measurements are not available.

Ali Omar↗

Towards an Optimal Estimation Retrieval of Cirrus Cloud Optical and Microphysical Properties Using Hyperspectral Shortwave Instruments and A Fast Radiative Transfer Algorithm

Cirrus cloud retrieval products (here, cloud optical depth, effective particle size, and cloud top height) are important inputs into numerical weather and climate models. Uncertainties in such retrieval products, as a matter of course, propagate downstream, impacting model calculations. Improvements in high-quality global cirrus cloud optical and microphysical data products from satellite observations are needed to understand and reduce retrieval uncertainties. Hyperspectral instruments produce high-resolution and information-dense radiance spectra, thus offering the opportunity to reduce uncertainties in retrieval products. An optimal estimation-based cirrus cloud optical and microphysical product retrieval is under development for the NASA Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) and the Earth Surface Mineral Dust Source Investigation (EMIT) instruments, and the forthcoming Climate Absolute Radiance and Refractivity Observatory Pathfinder (CLARREO-Pathfinder). The spectral coverage of all three instruments includes the ultraviolet, visible, and near-infrared. In this study a very fast radiative transfer model, the Principal Component-based Radiative Transfer Model in the solar spectral region (PCRTM-Solar), is used for forward modeling computations. This will reduce the computational burden in the forward radiance and Jacobian calculations as the cost function is minimized, enabling the entire AVIRIS, EMIT, and CLARREO-Pathfinder spectral range to be used in the optimal estimation framework. Using the entire spectrum will maximize the information content, resulting in a more robust and more accurate retrieval. As a first step, the retrieval is being designed for single layer ice clouds over open ocean water. Preliminary results will be shown.

Jeffrey Mast↗

Towards an Optimal Estimation Retrieval of Cirrus Cloud Optical and Microphysical Properties Using Hyperspectral Shortwave Instruments and A Fast Radiative Transfer Algorithm

Cirrus cloud retrieval products (here, cloud optical depth, effective particle size, and cloud top height) are important inputs into numerical weather and climate models. Uncertainties in such retrieval products, as a matter of course, propagate downstream, impacting model calculations. Improvements in high-quality global cirrus cloud optical and microphysical data products from satellite observations are needed to understand and reduce retrieval uncertainties. Hyperspectral shortwave instruments produce high-resolution and information-dense spectra, thus offering the opportunity to reduce uncertainties in retrieval products. We are in the process of developing a retrieval that uses the very fast Principal Component Radiative Transfer Model in the solar spectral region (PCRTM-Solar) in the forward model calculations. This retrieval will use measured reflectances from the NASA Earth Surface Mineral Dust Source Investigation (EMIT) and the forthcoming Climate Absolute Radiance and Refractivity Observatory Pathfinder (CLARREO-Pathfinder) instruments. In this manuscript we present progress towards a reference retrieval employing a widely used, verified, accurate, yet computationally slower radiative transfer modeling technique. The reference retrieval, while too slow for using the complete hyperspectral measurement, will allow us to study the behavior of retrieval products and help us verify results from our in-development fast retrieval. Both retrievals will use the optimal estimation retrieval framework. In this manuscript we present results from an uncertainty analysis considering three uncertainty sources for a cirrus cloud retrieval in the form of error covariance matrices: reflectance uncertainty due to water vapor, the reflectance uncertainty due to ice crystal scattering assumptions, and the instrument measurement uncertainty. Results show that the uncertainty due to habit selection is the largest, while that due to water vapor is at most 0.6% relative to channel reflectance. As a first step, the retrieval is being designed for single layer ice clouds over open ocean water.

Cirrus cloud↗

A Climatology of Midlatitude Continental Clouds from the ARM SGP Site: Low-Level Cloud Macrophysical, Microphysical, and Radiative Properties - Part I

A record of single-layer and overcast low cloud (stratus) properties has been generated using approximately 4000 hours of data collected from January 1997 to December 2002 at the Atmospheric Radiation Measurement (ARM) Southern Great Plains Central Facility (SCF). The cloud properties include liquid-phase and liquid-dominant, mixed-phase, low cloud macrophysical, microphysical, and radiative properties including cloud-base and -top heights and temperatures, and cloud physical thickness derived from a ground-based radar and lidar pair, and rawinsonde sounding; cloud liquid water path (LWP) and content (LWC), and cloud-droplet effective radius (r(sub e)) and number concentration (N) derived from the macrophysical properties and radiometer data; and cloud optical depth (tau), effective solar transmission (gamma), and cloud/top-of-atmosphere albedos (R(sub cldy)/R(sub TOA)) derived from Eppley precision spectral pyranometer measurements. The cloud properties were analyzed in terms of their seasonal, monthly, and hourly variations. In general, more stratus clouds occur during winter and spring than in summer. Cloud-layer altitudes and physical thicknesses were higher and greater in summer than in winter with averaged physical thicknesses of 0.85 km and 0.73 km for day and night, respectively. The seasonal variations of LWP, LWC, N. tau, R(sub cldy), and R(sub TOA) basically follow the same pattern with maxima and minima during winter and summer, respectively. There is no significant variation in mean r(sub e), however, despite a summertime peak in aerosol loading, Although a considerable degree of variability exists, the 6-yr average values of LWP, LWC, r(sub e), N, tau, gamma, R(sub cldy) and R(sub TOA) are 150 gm(exp -2) (138), 0.245 gm(exp -3) (0.268), 8.7 micrometers (8.5), 213 cm(exp -3) (238), 26.8 (24.8), 0.331, 0.672, 0.563 for daytime (nighttime). A new conceptual model of midlatitude continental low clouds at the ARM SGP site has been developed from this study. The low stratus cloud amount monotonically increases from midnight to early morning (0930 LT), and remains large until around local noon, then declines until 1930 LT when it levels off for the remainder of the night. In the morning, the stratus cloud layer is low, warm, and thick with less LWC, while in the afternoon it is high, cold, and thin with more LWC. Future parts of this series will consider other cloud types and cloud radiative forcing at the ARM SCF.

Dong, Xiquan↗

Understanding Ice Supersaturation, Particle Growth, and Number Concentration in Cirrus Clouds

Many factors control the ice supersaturation and microphysical properties in cirrus clouds. We explore the effects of dynamic forcing, ice nucleation mechanisms, and ice crystal growth rate on the evolution and distribution of water vapor and cloud properties in nighttime cirrus clouds using a one-dimensional cloud model with bin microphysics and remote sensing measurements obtained at the Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility located near Lamont, OK. We forced the model using both large-scale vertical ascent and, for the first time, mean mesoscale velocity derived from radar Doppler velocity measurements. Both heterogeneous and homogeneous nucleation processes are explored, where a classical theory heterogeneous scheme is compared with empirical representations. We evaluated model simulations by examining both bulk cloud properties and distributions of measured radar reflectivity, lidar extinction, and water vapor profiles, as well as retrieved cloud microphysical properties. Our results suggest that mesoscale variability is the primary mechanism needed to reproduce observed quantities. Model sensitivity to the ice growth rate is also investigated. The most realistic simulations as compared with observations are forced using mesoscale waves, include fast ice crystal growth, and initiate ice by either homogeneous or heterogeneous nucleation. Simulated ice crystal number concentrations (tens to hundreds particles per liter) are typically two orders of magnitude smaller than previously published results based on aircraft measurements in cirrus clouds, although higher concentrations are possible in isolated pockets within the nucleation zone.

Comstock, Jennifer M.↗

Investigation of the effects of the macrophysical and microphysical properties of cirrus clouds on the retrieval of optical properties: Results for FIRE 2

Due to the prevalence and persistence of cirrus cloudiness across the globe, cirrus clouds are believed to have an important effect on the climate. Stephens et al., (1990) among others have shown that the important factor determining how cirrus clouds modulate the climate is the balance between the albedo and emittance effect of the cloud systems. This factor was shown to depend in part upon the effective sizes of the cirrus cloud particles. Since effective sizes of cirrus cloud microphysical distributions are used as a basis of parameterizations in climate models, it is crucial that the relationships between effective sizes and radiative properties be clearly established. In this preliminary study, the retrieval of cirrus cloud effective sizes are examined using a two dimensional radiative transfer model for a cirrus cloud case sampled during FIRE Cirrus 11. The purpose of this paper is to present preliminary results from the SHSG model demonstrating the sensitivity of the bispectral relationships of reflected radiances and thus the retrieval of effective sizes to phase function and dimensionality.

Stackhouse, Paul W., Jr.↗

Remote Sensing of Cloud, Aerosol, and Water Vapor Properties from MODIS

MODIS is an earth-viewing cross-track scanning spectroradiometer launched on the Terra satellite in December 1999. MODIS scans a swath width sufficient to provide nearly complete global coverage every two days from a polar orbiting, sun-synchronous, platform at an altitude of 705 kilometers, and provides images in 36 spectral bands between 0.415 and 14.235 micrometers with spatial resolutions of 250 meters (2 bands), 500 meters (5 bands) and 1000 meters (29 bands). These bands have been carefully selected to enable advanced studies of land, ocean, and atmospheric processes. In this presentation we review the comprehensive set of remote sensing algorithms that have been developed for the remote sensing of atmospheric properties using MODIS data, placing primary emphasis on the principal atmospheric applications of (i) developing a cloud mask for distinguishing clear sky from clouds, (ii) retrieving global cloud radiative and microphysical properties, including cloud top pressure and temperature, effective emissivity, cloud optical thickness, thermodynamic phase, and effective radius, (iii) monitoring tropospheric aerosol optical thickness over the land and ocean and aerosol size distribution over the ocean, (iv) determining atmospheric profiles of moisture and temperature, and (v) estimating column water amount. The physical principles behind the determination of each of these atmospheric products will be described, together with an example of their application using MODIS observations. All products are archived into two categories: pixel-level retrievals (referred to as Level-2 products) and global gridded products at a latitude and longitude resolution of 1 degree (Level-3 products). An overview of the MODIS atmosphere algorithms and products, status, validation activities, and early level-2 and -3 results will be presented.

King, Michael D.↗

Remote Sensing of Cloud, Aerosol, and Land Properties from MODIS: Applications to the East Asia Region

MODIS is an earth-viewing cross-track scanning spectroradiometer launched on the Terra satellite in December 1999. MODIS scans a swath width sufficient to provide nearly complete global coverage every two days from a polar-orbiting, sun-synchronous platform at an altitude of 705 km, and provides images in 36 spectral bands between 0.415 and 14.235 microns with spatial resolutions of 250 m (two bands), 500 m (five bands) and 1000 m (29 bands). These bands have been carefully selected to enable advanced studies of land, ocean, and atmospheric processes. In this presentation we review the comprehensive set of remote sensing algorithms that have been developed for the remote sensing of atmospheric properties using MODIS data, placing primary emphasis on the principal atmospheric applications of (i) developing a cloud mask for distinguishing clear sky from clouds, (ii) retrieving global cloud radiative and microphysical properties, including cloud top pressure and temperature, effective emissivity, cloud optical thickness, thermodynamic phase, and effective radius, (iii) monitoring tropospheric aerosol optical thickness over the land and ocean and aerosol size distribution over the ocean, (iv) determining atmospheric profiles of moisture and temperature, and (v) estimating column water amount. The physical principles behind the determination of each of these atmospheric products will be described, together with an example of their application using MODIS observations to the east Asian region in Spring 2001. All products are archived into two categories: pixel-level retrievals (referred to as Level-2 products) and global gridded products at a latitude and longitude resolution of 1 degree (Level-3 products). An overview of the MODIS atmosphere algorithms and products, status, validation activities, and early level-2 and -3 results will be presented.

King, Michael D.↗