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At least 91 records · Page 5

Distribution and Sources of Tropospheric Aerosols Over the Western North Atlantic During ACTIVATE (February-March 2020)

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) is a five-year (2019-2023) NASA Earth-Venture Suborbital-3 (EVS-3) mission to robustly characterize aerosol-cloud-meteorology interactions during February-June, with a focus on marine boundary layer clouds. This characterization requires understanding of aerosol composition, distribution, transport pathways, and sources. Here we use the GEOS-Chem chemical transport model driven by the MERRA-2 reanalysis to simulate tropospheric carbon monoxide (CO) and aerosols over the western North Atlantic Ocean (WNAO) during the first field deployment of ACTIVATE (February-March 2020). CO is used as a tracer to diagnose transport pathways for continental pollution outflow to the WNAO. The aerosol simulation represents all major aerosols including sulfate-nitrate-ammonium (SNA), mineral dust, sea salt, black and organic carbon aerosols. Model-simulated mixing ratios of SNA and organic carbon are compared with aircraft observations. We show that intensive aerosol mass measurements in the lower troposphere over the North American outflow region during ACTIVATE provide strong constraints on model aerosol wet scavenging. Comparisons of model aerosol extinctions with the airborne High Spectral Resolution Lidar-2 (HSRL-2) measurements indicate that the model generally captures continental outflow of aerosols and enhanced extinctions associated with sea salt. Simulated aerosol optical depths (AODs) and extinction vertical profiles are also compared with satellite retrievals from MODIS/Aqua and CALIOP/CALIPSO, respectively. CALIOP sometimes observes enhanced aerosol extinction at altitudes between ~1.5km and ~2.0km south of 32°N. The model reproduces this enhancement and attributes it to coarse-mode sea salt associated with high relative humidity. The relative contributions of continental and oceanic sources to the aerosol loading, AOD, and their distributions over the study domain will also be discussed.

aerosols↗

Spectral absorption of solar radiation in cloudy atmospheres A 20/cm model

A radiative transfer model based on both LOWTRAN transmission functions (at a 20/cm resolution), and Monte Carlo simulations of wavelength distributions, is used to determine the spectral absorption of solar radiation in typical water clouds. This yields the relative absorption by the vapor and droplets within each cloud. The results obtained indicate a slightly lower absorption than had previously been found, with boundary layer clouds typically absorbing 9 percent of the terrestrial insolation for an overhead sun. This absorption is strongly dependent on the presence of water vapor above the cloud top and solar zenith angle. Droplets, rather than vapor, are shown to be the dominant absorbers within the cloud except in the absence of water vapor above the cloud top.

Davies, R.↗

Extending 3D Near-Cloud Corrections from Shorter to Longer Wavelengths

Satellite observations have shown a positive correlation between cloud amount and aerosol optical thickness (AOT) that can be explained by the humidification of aerosols near clouds, and/or by cloud contamination by sub-pixel size clouds and the cloud adjacency effect. The last effect may substantially increase reflected radiation in cloud-free columns, leading to overestimates in the retrieved AOT. For clear-sky areas near boundary layer clouds the main contribution to the enhancement of clear sky reflectance at shorter wavelengths comes from the radiation scattered into clear areas by clouds and then scattered to the sensor by air molecules. Because of the wavelength dependence of air molecule scattering, this process leads to a larger reflectance increase at shorter wavelengths, and can be corrected using a simple two-layer model. However, correcting only for molecular scattering skews spectral properties of the retrieved AOT. Kassianov and Ovtchinnikov proposed a technique that uses spectral reflectance ratios to retrieve AOT in the vicinity of clouds; they assumed that the cloud adjacency effect influences the spectral ratio between reflectances at two wavelengths less than it influences the reflectances themselves. This paper combines the two approaches: It assumes that the 3D correction for the shortest wavelength is known with some uncertainties, and then it estimates the 3D correction for longer wavelengths using a modified ratio method. The new approach is tested with 3D radiances simulated for 26 cumulus fields from Large-Eddy Simulations, supplemented with 40 aerosol profiles. The results showed that (i) for a variety of cumulus cloud scenes and aerosol profiles over ocean the 3D correction due to cloud adjacency effect can be extended from shorter to longer wavelengths and (ii) the 3D corrections for longer wavelengths are not very sensitive to unbiased random uncertainties in the 3D corrections at shorter wavelengths.

aerosol optical depth↗

Long-Term Trends in Aerosols, Low Clouds, and Large-scale Meteorology over the Western North Atlantic from 2003 to 2020

A continuous decrease of aerosol over the western North Atlantic Ocean (WNAO) on decadal timescales provides a long-term experiment to evaluate how other natural and anthropogenic processes affect the manifestation of aerosol-cloud interactions in this region. Furthermore, the WNAO is a natural laboratory with diverse aerosol sources, marine boundary layer clouds that are more variable than marine stratocumulus deck regions, and unique flow regimes set up by the Gulf Stream and semi-permanent Bermuda High. We investigate how satellite-retrieved macrophysical and microphysical properties of low clouds and the surface shortwave irradiance changed from 2003 to 2020, in tandem with this aerosol decrease. The decadal changes in large-scale meteorology relating to the North Atlantic Oscillation (NAO) are also examined. We find no significant changes in low-cloud fraction but a widespread reduction in low-cloud optical depth attributed to fewer and larger cloud droplets with almost no change in cloud liquid water path. Despite robust signals in low-cloud optical properties together with aerosol decrease, a corresponding increase in the surface shortwave irradiance trends, also called surface brightening, is lacking. This absence of brightening is potentially due to concomitant changes found in large-scale meteorology associated with NAO— a Bermuda High strengthening, sea surface warming, and atmospheric moistening— as well as an increase in high cloud fraction that can counteract the surface brightening. Ultimately, our findings suggest that spatial patterns in the decadal meteorological variability, likely set up by NAO, contribute more to the surface cloud radiative effect over the WNAO than aerosol-cloud interactions.

J Minnie Park↗

Evaluation of Low Altitude Cloud Amount Using CALIPSO Observations

Clouds strongly modulate the transfer of solar and thermal radiation within the atmosphere. Changes in the distribution and properties of clouds in a changing climate represent climate feedbacks affecting climate sensitivity, but the predicted responses of clouds from current climate models are inconsistent. Of particular concern is the response of low clouds, and it is recognized that proper representation of low clouds in global models is in need of improvement. Accurate satellite cloud climatologies are necessary to evaluate model performance, but existing climatologies require validation and are inadequate in some respects for model evaluation. CALIPSO and CloudSat have been acquiring high vertical resolution cloud profiles since launch in 2006. These global cloud datasets represent a new tool for evaluation of both models and existing satellite climatologies. While a recently available merged CALIPSO-CloudSat cloud climatology provides the most comprehensive view of global 3-D cloud distribution, the CALIPSO dataset set on its own has several unique characteristics, including profiles of the atmospheric boundary layer with 30 meter vertical resolution. In this paper we investigate the use of CALIPSO data to characterize boundary layer clouds, looking toward the development of a reliable global dataset suitable for evaluation of model performance.

Winker, Dave↗

Overview of ACTIVATE’s First Year of Flights Targeting Aerosol-Cloud-Meteorology Interactions

The Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) included 40 research flights in the winter and summer months of 2020 using a two-aircraft approach to simultaneously obtain in situ and remote sensing data of regions below, inside, and above boundary layer clouds. This presentation will summarize early findings from the first year of ACTIVATE flights with focus on aerosol and cloud droplet number concentration behavior, formation and evolution of clouds, and analysis of remote sensing retrievals of aerosol and cloud properties. There is a clear annual cycle in cloud droplet number concentration suggesting a marked annual cycle in aerosol-cloud interactions. Although aerosol particles are more abundant in spring and summer, the conditions needed to activate those particles into cloud droplets are weaker than in other colder months. Several flights targeted post-frontal clouds associated with cold air outbreaks pointing to enhanced levels of nucleated particles immediately above such clouds, and that ice formation hastens the transition from closed to open cloud structures in the sampled CAO events. Also observed in the marine boundary layer during CAOs is the frequent occurrence of non-spherical sea salt particles, which has significant implications for remote sensing retrievals.

Taylor Shingler↗

On the determination of cloud cover from satellite sensors - The effect of sensor spatial resolution

The effect of sensor spatial resolution on satellite-derived estimates of cloud fractional coverage is quantified on the basis of Landsat satellite radiance data. Cloud fraction is found to depend on cloud algorithm as much as it depends on sensor spatial resolution. Even for 28.5-m spatial resolution data, large cloud fraction differences exist between algorithms. Satellite cloud retrieval algorithms depend strongly on sensor spatial resolution and/or on the optical depth of the cloud field. When present, spatial resolution effects are small (less than 0.01) for pixel diameter less than 1/4 km and are large for pixel diameter larger than 1 km. The International Satellite Cloud Climatology Project bispectral threshold gives an increase in cloud fraction of 0.11 as spatial resolution degrades from 20 m to 8 km. The spatial coherence algorithm underestimates boundary layer cloud fraction by 0.18. The use of functional box counting and an assumption of fractal scale invariance overestimates the dependence of cloud fraction for spatial scales below 1 km.

Wielicki, Bruce A.↗

Independent Pixel and Two Dimensional Estimates of LANDSAT-Derived Cloud Field Albedo

A theoretical study has been conducted on the effects of cloud horizontal inhomogeneity on cloud albedo bias. A two-dimensional (2D) version of the Spherical Harmonic Discrete Ordinate Method (SHDOM) is used to estimate the albedo bias of the plane parallel (PP-IPA) and independent pixel (IPA-2D) approximations for a wide range of 2D cloud fields obtained from LANDSAT. They include single layer trade cumulus, open and closed cell broken stratocumulus, and solid stratocumulus boundary layer cloud fields over ocean. Findings are presented on a variety of averaging scales and are summarized as a function of cloud fraction, mean cloud optical depth, cloud aspect ratio, standard deviation of optical depth, and the gamma function parameter Y (a measure of the width of the optical depth distribution). Biases are found to be small for small cloud fraction or mean optical depth, where the cloud fields under study behave linearly. They are large (up to 0.20 for PP-IPA bias, -0.12 for IPA-2D bias) for large v. On a scene average basis PP-IPA bias can reach 0.30, while IPA-2D bias reaches its largest magnitude at -0.07. Biases due to horizontal transport (IPA-2D) are much smaller than PP-IPA biases but account for 20% RMS of the bias overall. Limitations of this work include the particular cloud field set used, assumptions of conservative scattering, constant cloud droplet size, no gas absorption or surface reflectance, and restriction to 2D radiative transport. The LANDSAT data used may also be affected by radiative smoothing.

Chambers, L. H.↗

Comparison of Cloud Resolving Model Simulations to Remote Sensing Data

The purpose of this research was to evaluate the ability of a cloud-resolving model (CRM) to simulate the dynamical, radiative, and microphysical properties of deep convective cloud objects identified using CERES (Clouds and the Earth s Radiant Energy System) on board the Tropical Rainfall Measuring Mission (TRMM) satellite platform, for many cases. A deep convective cloud object is a contiguous region that is composed of satellite footprints that fulfill the following selection criteria: 100% cloud fraction, cloud optical depth > 10, and a cloud top height of at least 10 km. Selection criteria have also been formed for different types of boundary-layer clouds, as described in Xu et al. (2005). The purpose of the cloud object approach is to identify specific areas of where the cloud properties simulated by the CRM systematically differ from the observed cloud properties. Where these systematic differences exist, concrete steps can be made to improve the CRM s simulation of an entire class of clouds, rather than by tuning the model to correctly simulate a single case study, as is often done. Additional information regarding detailed approaches and findings are presented.

Randall, David A.↗

Spatially-Coordinated Airborne Data and Complementary Products for Aerosol, Gas, Cloud, and Meteorological Studies: the Nasa Activate Dataset

The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions, with applications extending from process-based studies to multi-scale model intercomparison and improvement as well as to remote-sensing algorithm assessments and advancements. ACTIVATE used two NASA Langley Research Center aircraft, a HU-25 Falcon and King Air, to conduct systematic and spatially coordinated flights over the northwest Atlantic Ocean, resulting in 162 joint flights and 17 other single-aircraft flights between 2020 and 2022 across all seasons. Data cover 574 and 592 cumulative flights hours for the HU-25 Falcon and King Air, respectively. The HU-25 Falcon conducted profiling at different level legs below, in, and just above boundary layer clouds (< 3 km) and obtained in situ measurements of trace gases, aerosol particles, clouds, and atmospheric state parameters. Under cloud-free conditions, the HU-25 Falcon similarly conducted profiling at different level legs within and immediately above the boundary layer. The King Air (the high-flying aircraft) flew at approximately ∼ 9 km and conducted remote sensing with a lidar and polarimeter while also launching dropsondes (785 in total). Collectively, simultaneous data from both aircraft help to characterize the same vertical column of the atmosphere. In addition to individual instrument files, data from the HU-25 Falcon aircraft are combined into “merge files” on the publicly available data archive that are created at different time resolutions of interest (e.g., 1, 5, 10, 15, 30, 60 s, or matching an individual data product's start and stop times). This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes. The data are publicly accessible through https://doi.org/10.5067/SUBORBITAL/ACTIVATE/DATA001 (ACTIVATE Science Team, 2020).

Aerosol Cloud meTeorology Interactions oVer the we↗

FIRE Arctic Clouds Experiment

An overview is given of the First ISCCP Regional Experiment (FIRE) Arctic Clouds Experiment that was conducted in the Arctic during April through July, 1998. The principal goal of the field experiment was to gather the data needed to examine the impact of arctic clouds on the radiation exchange between the surface, atmosphere, and space, and to study how the surface influences the evolution of boundary layer clouds. The observations will be used to evaluate and improve climate model parameterizations of cloud and radiation processes, satellite remote sensing of cloud and surface characteristics, and understanding of cloud-radiation feedbacks in the Arctic. The experiment utilized four research aircraft that flew over surface-based observational sites in the Arctic Ocean and Barrow, Alaska. In this paper we describe the programmatic and science objectives of the project, the experimental design (including research platforms and instrumentation), conditions that were encountered during the field experiment, and some highlights of preliminary observations, modelling, and satellite remote sensing studies.

Curry, J. A.↗

Aerosol Radiative Effects over Ascension Island Using LASIC Observations and MERRA-2

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Thermodynamic profiles will be analyzed through the unique combination of sounding data from radiosonde launches and microwave profiling radiometers, giving observations of additional quantities important for cloud development such as CAPE and CIN at a fine temporal resolution. The thermodynamic profiles will be presented in conjunction with detailed observations of the cloud structure over the site from a K-band cloud radar, micropulse lidar, and laser ceilometer. Finally, the observed thermodynamic and cloud profiles will be used as input forcing, alongside aerosols from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), for the Rapid Radiative Transfer Model (RRTM) to gain information regarding the radiative heating profiles. Idealized experiments using RRTM with and without aerosols will be used to quantify the impact of biomass burning carbonaceous aerosol plumes as they pass over the site.

Collow, Allie↗

An Estimate of Low-Cloud Feedbacks from Variations of Cloud Radiative and Physical Properties with Sea Surface Temperature on Interannual Time Scales

Simulations of climate change have yet to reach a consensus on the sign and magnitude of the changes in physical properties of marine boundary layer clouds. In this study, the authors analyze how cloud and radiative properties vary with SST anomaly in low-cloud regions, based on five years (March 2000 - February 2005) of Clouds and the Earth s Radiant Energy System (CERES) -- Terra monthly gridded data and matched European Centre for Medium-Range Weather Forecasts (ECMWF) meteorological reanalaysis data. In particular, this study focuses on the changes in cloud radiative effect, cloud fraction, and cloud optical depth with SST anomaly. The major findings are as follows. First, the low-cloud amount (-1.9% to -3.4% /K) and the logarithm of low-cloud optical depth (-0.085 to -0.100/K) tend to decrease while the net cloud radiative effect (3.86 W/m(exp 2)/ K) becomes less negative as SST anomalies increase. These results are broadly consistent with previous observational studies. Second, after the changes in cloud and radiative properties with SST anomaly are separated into dynamic, thermodynamic, and residual components, changes in the dynamic component (taken as the vertical velocity at 700 hPa) have relatively little effect on cloud and radiative properties. However, the estimated inversion strength decreases with increasing SST, accounting for a large portion of the measured decreases in cloud fraction and cloud optical depth. The residual positive change in net cloud radiative effect (1.48 W/m(exp 2)/ K) and small changes in low-cloud amount (-0.81% to 0.22% /K) and decrease in the logarithm of optical depth (-0.035 to -0.046/ K) with SST are interpreted as a positive cloud feedback, with cloud optical depth feedback being the dominant contributor. Last, the magnitudes of the residual changes differ greatly among the six low-cloud regions examined in this study, with the largest positive feedbacks (approximately 4 W/m(exp 2)/ K) in the southeast and northeast Atlantic regions and a slightly negative feedback (-0.2 W/m(exp 2)/ K) in the south-central Pacific region. Because the retrievals of cloud optical depth and/or cloud fraction are difficult in the presence of aerosols, the transport of heavy African continental aerosols may contribute to the large magnitudes of estimated cloud feedback in the two Atlantic regions.

Eitzen, Zachary A.↗

Structures observed on the spot radiance fields during the FIRE experiment

Three Spot images taken during the FIRE experiment on stratocumulus are analyzed. From this high resolution data detailed observations of the true cloud radiance field may be made. The structure and inhomogeneity of these radiance fields hold important implications for the radiation budget, while the fine scale structure in radiance field provides information on cloud dynamics. Wieliki and Welsh, and Parker et al., have quantified the inhomogeneities of the cumulus clouds through a careful examination of the distribution of cloud (and hole) size as functions of an effective cloud diameter and radiance threshold. Cahalan (1988) has compared for different cloud types of (stratocumulus, fair weather cumulus, convective clouds in the ITCZ) the distributions of clouds (and holes) sizes, the relation between the size and the perimeter of these clouds (and holes), and examining the possibility of scale invariance. These results are extended from LANDSAT resolution (57 m and 30 m) to the Spot resolution (10 m) resolution in the case of boundary layer clouds. Particular emphasis is placed on the statistics of zones of high and low reflectivity as a function of a threshold reflectivity.

Seze, Genevieve↗

Computation of the Effects of Inhomogeneous Clouds on Retrieval of Remotely Sensed Properties

Current and future earth observation programs depend on satellite measurements of radiance to retrieve the properties of clouds on a global basis. At present, this retrieval is made assuming that the clouds in the instrument field of view are plane parallel and independent of adjacent pixels. While this assumption is known to be false except in very limited cases, its impact can be evaluated, and if possible corrected, based on emerging theoretical techniques. In this study, the Spherical Harmonic Discrete Ordinate Method (SHDOM, Evans, 1996) has been used to assess the sensitivity of the retrieval to a variety of cloud parameters. SHDOM allows the plane parallel assumption to be relaxed and makes 2D and even 3D radiative solutions practical. A previous study (Chambers et al., 1996) assessed the effect of horizontal inhomogeneity in 45 LANDSAT scenes of boundary layer clouds over ocean. The four scenes studied here represent overcast, broken, scattered and strongly thermally forced cloud fields and are used to perform sensitivity studies to a wider variety of parameters. Comparisons are made at three solar zenith angles (theta (sub 0) = 0, 49, and 63 degrees) to avoid ambiguity in the results due to solar zenith angle.

Chambers, Lin H.↗

UV 380 nm Reflectivity of the Earth's Surface

The 380 nm radiance measurements of TOMS (Total Ozone Mapping Spectrometer) have been converted into a global data set of daily (1979 to 1992) Lambert equivalent reflectivities R of the Earth's surface and boundary layer (clouds, aerosols, surface haze, and snow/ice). Since UV surface reflectivity is between 2 and 8% for both land and water during all seasons of the year (except for ice and snow cover), reflectivities larger than the surface value indicates the presence of clouds, haze, or aerosols in the satellite field of view. Statistical analysis of 14 years of daily data show that most snow/ice-free regions of the Earth have their largest fraction of days each year when the reflectivity is low (R less than 10%). The 380 nm reflectivity data shows that the true surface reflectivity is 2 to 3% lower than the most frequently occurring reflectivity value for each TOMS scene. The most likely cause of this could be a combination of frequently occurring boundary-layer water or aerosol haze. For most regions, the observation of extremely clear conditions needed to estimate the surface reflectivity from space is a comparatively rare occurrence. Certain areas (e.g., Australia, southern Africa, portions of northern Africa) are cloud-free more than 80% of the year, which exposes these regions to larger amounts of UV radiation than at comparable latitudes in the Northern Hemisphere. Regions over rain-forests, jungle areas, Europe and Russia, the bands surrounding the Arctic and Antarctic regions, and many ocean areas have significant cloud cover (R greater than 15%) more than half of each year. In the low to middle latitudes, the areas with the heaviest cloud cover (highest reflectivity for most of the year) are the forest areas of northern South America, southern Central America, the jungle areas of equatorial Africa, and high mountain regions such as the Himalayas or the Andes. The TOMS reflectivity data show the presence of large nearly clear ocean areas and the effects of the major ocean currents on cloud production.

Herman, J. R.↗

Observed Differences in Spectral Microphysical Retrievals from MODIS

The microphysical structure of clouds is of fundamental importance for understanding a variety of cloud radiation and physical processes. With the advent of MODIS (Moderate Resolution Imaging Spectroradiometer) on the NASA EOS Terra and Aqua platforms, simultaneous global/daily 1km retrievals of cloud effective particle size are available using the heritage 3.7 an band from AVHRR as well as the 1.6 and 2.1 m shortwave IR bands. The MODIS cloud product (MOD06/MYD06 for MODIS Terra and Aqua, respectively) provides separate effective radii results using each of these spectral bands. It has been found that significant differences can occur between the three size retrievals, mainly for liquid water marine boundary layer clouds and especially in broken (low cloud fraction) regimes. In particular, for such regimes, effective radii derived from the MODIS 2.1 lim band can be substantially larger than retrievals from the Heritage 3.7 lam band. In this paper, we present global and regional results of the differences, including correlations, view angle dependencies, and algorithm sensitivities for the existing MODIS Collection 5 product.

Platnick, Steven E.↗

The North Atlantic Aerosol and Marine Ecosystem Study (NAAMES): Science Motive and Mission Overview

The North Atlantic Aerosols and Marine Ecosystems Study (NAAMES) is an interdisciplinary investigation to improve understanding of Earth's ocean ecosystem-aerosol-cloud system. Specific overarching science objectives for NAAMES are to (1) characterize plankton ecosystem properties during primary phases of the annual cycle and their dependence on environmental forcings, (2)determine how these phases interact to recreate each year the conditions for an annual plankton bloom, and (3) resolve how remote marine aerosols and boundary layer clouds are influenced by plankton ecosystems. Four NAAMES field campaigns were conducted in the western subarctic Atlantic between November 2015 and April 2018, with each campaign targeting specific seasonal events in the annual plankton cycle. A broad diversity of measurements were collected during each campaign, including ship, aircraft, autonomous float and drifter, and satellite observations. Here, we present an overview of NAAMES science motives, experimental design, and measurements. We then briefly describe conditions and accomplishments during each of the four field campaigns and provide information on how to access NAAMES data. The intent of this manuscript is to familiarize the broad scientific community with NAAMES and to provide a common reference overview of the project for upcoming publications.

Behrenfeld, Michael J.↗