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At least 91 records · Page 5

How Representative Are Uncrewed Aircraft System Measurements of the Convective Boundary Layer?

Abstract Uncrewed aircraft systems (UAS) demonstrate significant potential for filling data gaps in the atmospheric boundary layer. However, the extent to which UAS observations—typically vertical profiles taken over 15 min—are representative of the boundary layer as a whole remains poorly characterized. Using large eddy simulations (LES) of the daytime convective boundary layer (CBL), we quantify random errors in UAS measurements that occur due to insufficient statistical convergence of the time average to the true ensemble mean. Random errors in first‐order moments increase as the CBL becomes increasingly unstable, and are largest near the surface for most quantities. Errors are on the order of 2–6 m for wind speed, 15–60 for wind direction, 0.2–3 K for potential temperature, and 0.1–1 g for specific humidity, with errors in turbulent fluxes on the order of 50%–100%. Sampling strategies that mitigate random errors are discussed in light of our results.

Greene, Brian R. [Now at Verisk Extreme Event Solu↗

Impact of Seasonal Snow-Cover Change on the Observed and Simulated State of the Atmospheric Boundary Layer in a High-Altitude Mountain Valley

The structure and evolution of the atmospheric boundary layer (ABL) under clear-sky fair weather conditions over mountainous terrain is dominated by the diurnal cycle of the surface energy balance and thus strongly depends on surface snow cover. We use data from three passive ground-based infrared spectrometers deployed in the East River Valley in Colorado's Rocky Mountains to investigate the response of the thermal ABL structure to changes in surface energy balance during the seasonal transition from low to high snow cover. Temperature profiles were retrieved from the infrared radiances using the optimal estimation physical retrieval Tropospheric Remotely Observed Profiling via Optimal Estimation. A nocturnal surface inversion formed in the valley during clear-sky days, which was subsequently mixed out during daytime with the development of a convective boundary layer when snow cover was low. Over high snow cover, a very shallow convective boundary layer formed, above which the inversion persisted through the daytime hours. We compare these observations to NOAA's operational High-Resolution-Rapid-Refresh model and find large warm biases on clear-sky days resulting from the model's inability to form strong nocturnal inversions and to maintain the stable stratification in the valley during daytime when there was snow on the ground. We suggest several factors contributing to the large model errors. These are (a) the inability of the model to represent well-developed thermally driven flows likely due to the too coarse horizontal grid spacing (3 km), (b) too much convective mixing during daytime, and (c) too strong vertical coupling between the valley atmosphere and the free troposphere.

54 ENVIRONMENTAL SCIENCES↗

Neural operator prediction of linear instability waves in high-speed boundary layers

Here, we investigate if neural operators can predict the linear evolution of instability waves in high-speed boundary layers. To this end, we extend the design of the DeepOnet to ensure accurate and robust predictions, and also to perform data assimilation. In particular, we train DeepONet to take as inputs an upstream disturbance and a downstream location of interest, and to provide as output the perturbation field downstream in the boundary layer. DeepONet thus approximates the linearized and parabolized Navier-Stokes operator for this flow. For successful application to the high-speed boundary layer problem, we add sample weighting and Fourier input features to the regular DeepONet formulation. Once trained, the DeepOnet can perform fast and accurate predictions of the downstream disturbances within the range of training frequencies (inside the distribution). In addition, we show that DeepONet can solve the inverse problem, where downstream wall measurements are adopted as input, and a trained network can predict the upstream disturbances that led to these observations. This capability, along with the forward predictions, allows us to perform a full data assimilation cycle efficiently: starting from wall-pressure data, we predict the upstream disturbance using the inverse DeepONet and its evolution using the forward DeepONet. Finally, we introduce three new metrics to benchmark the training, evaluation and break-even cost of neural operators.

42 ENGINEERING↗

Boundary-Layer-Coupled and Decoupled Clouds in Global Storm-Resolving Models: Comparisons With the ARM Observations

The accurate representation of interactions between clouds and planetary boundary layer (PBL) is a persistent challenge in climate models, critical for simulating surface energy budget. The emergence of kilometer-grid-scale global storm resolving models (GSRMs) offers the potential for enhanced details of PBL processes in these complex interactions. This study evaluates the representation of PBL-coupled and decoupled clouds in nine GSRM simulations against extensive ground-based observations by the Department of Energy Atmospheric Radiation Measurement (ARM) program, across six sites encompassing diverse regimes such as marine and continental environments in tropics and midlatitude. By differentiating coupling based on the relative positions between cloud bases and PBL tops, our analysis focuses on the simulation of PBL height, cloud frequency, position and vertical extent. The GSRMs generally exhibit commendable agreements with observed cloud structures and PBL diurnal cycles across different ARM sites. In contrast to the relatively consistent representation of decoupled clouds, discrepancies exist between the simulated and the observed coupled clouds, particularly in areas of intense convection, for example, over tropical rainforests and mountainous regions. These biases are probably associated with the models' tendency to underestimate the boundary layer humidity and the frequency of coupled clouds within different ranges of PBL heights. This study underscores the importance for continuous improvements in the representation of boundary layer and convection within these global kilometer-grid-scale models.

54 ENVIRONMENTAL SCIENCES↗

Deep-learning-derived planetary boundary layer height from conventional meteorological measurements

Abstract. The planetary boundary layer (PBL) height (PBLH) is an important parameter for various meteorological and climate studies. This study presents a multi-structure deep neural network (DNN) model, which can estimate PBLH by integrating the morning temperature profiles and surface meteorological observations. The DNN model is developed by leveraging a rich dataset of PBLH derived from long-standing radiosonde records augmented with high-resolution micro-pulse lidar and Doppler lidar observations. We access the performance of the DNN with an ensemble of 10 members, each featuring distinct hidden-layer structures, which collectively yield a robust 27-year PBLH dataset over the southern Great Plains from 1994 to 2020. The influence of various meteorological factors on PBLH is rigorously analyzed through the importance test. Moreover, the DNN model's accuracy is evaluated against radiosonde observations and juxtaposed with conventional remote sensing methodologies, including Doppler lidar, ceilometer, Raman lidar, and micro-pulse lidar. The DNN model exhibits reliable performance across diverse conditions and demonstrates lower biases relative to remote sensing methods. In addition, the DNN model, originally trained over a plain region, demonstrates remarkable adaptability when applied to the heterogeneous terrains and climates encountered during the GoAmazon (Green Ocean Amazon; tropical rainforest) and CACTI (Cloud, Aerosol, and Complex Terrain Interactions; middle-latitude mountain) campaigns. These findings demonstrate the effectiveness of deep learning models in estimating PBLH, enhancing our understanding of boundary layer processes with implications for improving the representation of PBL in weather forecasting and climate modeling.

54 ENVIRONMENTAL SCIENCES↗

Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic

Abstract. Warm boundary layer clouds in the eastern North Atlantic region exhibit significant diurnal variations in cloud properties. However, the diurnal cycle of the aerosol indirect effect (AIE) for these clouds remains poorly understood. This study takes advantage of recent advancements in the spatial resolution of geostationary satellites to explore the daytime variation in the AIE by estimating the cloud susceptibilities to changes in cloud droplet number concentration (Nd). Cloud retrievals for the month of July over 4 years (2018–2021) from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) on Meteosat-11 over this region are analyzed. Our results reveal a significant “U-shaped” daytime cycle in susceptibilities of the cloud liquid water path (LWP), cloud albedo, and cloud fraction. Clouds are found to be more susceptible to Nd perturbations at noon and less susceptible in the morning and evening. The magnitude and sign of cloud susceptibilities depend heavily on the cloud state defined by cloud LWP and precipitation conditions. Non-precipitating thin clouds account for 44 % of all warm boundary layer clouds in July, and they contribute the most to the observed daytime variation. Non-precipitating thick clouds are the least frequent cloud state (10 %), and they exhibit more negative LWP and albedo susceptibilities compared to thin clouds. Precipitating clouds are the dominant cloud state (46 %), but their cloud susceptibilities show minimal variation throughout the day. We find evidence that the daytime variation in LWP and albedo susceptibilities for non-precipitating clouds is influenced by a combination of the diurnal transition between non-precipitating thick and thin clouds and the “lagged” cloud responses to Nd perturbations. The daytime variation in cloud fraction susceptibility for non-precipitating thick clouds can be attributed to the daytime variation in cloud morphology (e.g., overcast or broken). The dissipation and development of clouds do not adequately explain the observed variation in cloud susceptibilities. Additionally, daytime variation in cloud susceptibility is primarily driven by variation in the intensity of cloud response rather than the frequency of occurrence of cloud states. Our results imply that polar-orbiting satellites with an overpass time at 13:30 LT underestimate daytime mean values of cloud susceptibility, as they observe susceptibility daily minima in the study region.

54 ENVIRONMENTAL SCIENCES↗

“Gray Zone” Simulations Using a Three-Dimensional Planetary Boundary Layer Parameterization in the Weather Research and Forecasting Model

Abstract Generating accurate weather forecasts of planetary boundary layer (PBL) properties is challenging in many geographical regions, oftentimes due to complex topography or horizontal variability in, for example, land characteristics. While recent advances in high-performance computing platforms have led to an increase in the spatial resolution of numerical weather prediction (NWP) models, the horizontal gridcell spacing (Δ x ) of many regional-scale NWP models currently fall within or are beginning to approach the gray zone (i.e., Δ x ≈ 100–1000 m). At these gridcell spacings, three-dimensional (3D) effects are important, as the most energetic turbulent eddies are neither fully parameterized (as in traditional mesoscale simulations) nor fully resolved [as in traditional large-eddy simulations (LES)]. In light of this modeling challenge, we have implemented a 3D PBL parameterization for high-resolution mesoscale simulations using the Weather Research and Forecasting Model. The PBL scheme, which is based on the algebraic model developed by Mellor and Yamada, accounts for the 3D effects of turbulence by calculating explicitly the momentum, heat, and moisture flux divergences in addition to the turbulent kinetic energy. In this study, we present results from idealized simulations in the gray zone that illustrate the benefit of using a fully consistent turbulence closure framework under convective conditions. While the 3D PBL scheme reproduces the evolution of convective features more appropriately than the traditional 1D PBL scheme, we highlight the need to improve the turbulent length scale formulation. Significance Statement The spatial resolution of weather models continues to increase at a rapid rate in accordance with the enhancement of computing power. As a result, smaller-scale atmospheric features become more explicitly resolved. However, most numerical models still ignore the impact of horizontal weather variations on boundary layer flows, which becomes more important at these smaller spatial scales. To address this issue, we have implemented a new modeling approach, using fundamental principles, which accounts for horizontal variability. Our results show that including three-dimensional effects of turbulence is necessary to achieve realistic boundary layer characteristics. This novel technique may be useful for many applications including complex terrain flows, pollutant dispersion, and surface–atmosphere interaction studies.

Juliano, Timothy W.↗

SST ..kappa..-..omega.. Simulations of the Atmospheric Boundary Layer Including the Coriolis Effect

For large-scale structures in the atmospheric boundary layer (ABL), the Coriolis effect and near-wall behavior can have a meaningful impact. For example, both the Coriolis effect and blade boundary layer impact how muchpower wind farms produce. RANS simulations of the ABL typically use the ..kappa..-epsilon turbulence model, which has been developed to accurately capture the Coriolis effect but typically does not perform well near walls. The SST ..kappa..-..omega.. turbulence model performs well near walls but does not accurately capture the Coriolis effect. This work modifies SST ..kappa..-..omega.. to accurately model the Coriolis effect. We discuss the similarities and differences in how to modify ..kappa..-epsilon and SST ..kappa..-..omega.. for the Coriolis effect. Finally, we compare ..kappa..-epsilon and SST ..kappa..-..omega.. simulations of the ABL, including the Coriolis effect, with large eddy simulations and measurements.

atmospheric boundary layer↗

Boundary layer moisture variability at the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic observatory during marine conditions

Abstract. Boundary layer moisture variability at the Eastern North Atlantic (ENA) site during marine conditions is examined at monthly and daily timescales using 5 years of ground-based observations and output from the European Center for Medium range Weather Forecast (ECMWF) reanalysis model. The annual cycle of the mixed-layer total water budgets is presented to estimate the relative contribution of large-scale advection, local moisture tendency, entrainment, and precipitation to balance the moistening due to surface latent heat flux on monthly timescales. When marine conditions prevail, advection of colder and dry air from the north acts as an important moisture sink (∼ 50 % of the overall budget) during fall and winter driving the seasonality of the budget. Entrainment and precipitation contribute to the drying of the boundary layer (∼ 25 % and ∼ 15 % respectively), and the local change in moisture contributes to a small residual part. On a daily temporal scale, moist and dry mesoscale columns of vapor (∼ 10 km) are analyzed during 10 selected days of precipitating stratocumulus clouds. Adjacent moist and dry columns present distinct mesoscale features that are strongly correlated with clouds and precipitation. Dry columns adjacent to moist columns have more frequent and stronger downdrafts immediately below the cloud base. Moist columns have more frequent updrafts, stronger cloud-top cooling, and higher liquid water path and precipitation compared to the dry columns. This study highlights the complex interaction between large-scale and local processes controlling the boundary layer moisture and the importance of spatial distribution of vapor to support convection and precipitation.

54 ENVIRONMENTAL SCIENCES↗

Insights of Boundary Layer Turbulence Over the Complex Terrain of Central Himalaya from GVAX Field Campaign

Limited observations hinder understanding of turbulent characteristics in mountainous terrain resulting from heating or cooling of slopes, wind, vertical motions, and heat or moisture advection, which disperse aerosols and other pollutants over the region. In this study, the 1290 MHz radar wind profiler data are utilized to compute the boundary layer height (BLH), the refractive index structure constant (C n 2 ), and the energy dissipation rate (ε) over the central Himalayan site for the period of November 2011 to March 2012, from the intense Ganges Valley Aerosol Experiment (GVAX) field measurements. The radar wind profiler (RWP) based estimation of BLH and ε is validated against the radiosonde, representing the effectiveness of the datasets for further investigation. The strong seasonal variation of log C n 2 and log ε, with average values of ≈ -12 m -2/3 and -2 m 2 s -3 , respectively, is associated with the mountain-induced local circulations and stability in the atmospheric boundary layer. The weak stratification during weak flow is found to be responsible for deep mixing, particularly in the nocturnal boundary layer in spring. Furthermore, the level of cloud cover significantly impacts the strength of turbulence, with the highest cloud cover resulting in a substantial increase in log C n 2 (approximately -11 m -2/3 ) due to intense updraft and downdraft motions compared to clear skies. Additionally, the distribution of aerosol loading across the site, coupled with the behavior of BLH, atmospheric stability, and orographic-induced circulations, implies distinctive seasonal mechanisms for transporting aerosols toward the mountains. This study offers valuable insights into the diurnal and seasonal patterns of turbulent mixing and the mechanisms behind the transport of pollutants through boundary layer processes over the region.

54 ENVIRONMENTAL SCIENCES↗

Refining Planetary Boundary Layer Height Retrievals From Micropulse‐Lidar at Multiple ARM Sites Around the World

Abstract Knowledge of the planetary boundary layer height (PBLH) is crucial for various applications in atmospheric and environmental sciences. Lidar measurements are frequently used to monitor the evolution of the PBLH, providing more frequent observations than traditional radiosonde‐based methods. However, lidar‐derived PBLH estimates have substantial uncertainties, contingent upon the retrieval algorithm used. In addressing this, we applied the Different Thermo‐Dynamic Stabilities (DTDS) algorithm to establish a PBLH data set at five separate Department of Energy's Atmospheric Radiation Measurement sites across the globe. Both the PBLH methodology and the products are subject to rigorous assessments in terms of their uncertainties and constraints, juxtaposing them with other products. The DTDS‐derived product consistently aligns with radiosonde PBLH estimates, with correlation coefficients exceeding 0.77 across all sites. This study delves into a detailed examination of the strengths and limitations of PBLH data sets with respect to both radiosonde‐derived and other lidar‐based estimates of the PBLH by exploring their respective errors and uncertainties. It is found that varying techniques and definitions can lead to diverse PBLH retrievals due to the inherent intricacy and variability of the boundary layer. Our DTDS‐derived PBLH data set outperforms existing products derived from ceilometer data, offering a more precise representation of the PBLH. This extensive data set paves the way for advanced studies and an improved understanding of boundary‐layer dynamics, with valuable applications in weather forecasting, climate modeling, and environmental studies.

54 ENVIRONMENTAL SCIENCES↗

Detection of Extreme Phenomena in the Stable Boundary Layer over the Amazonian Forest

We apply different methods for detection of extreme phenomena (EP) in air-turbulent time series measured in the nocturnal boundary layer above the Amazon forest. The methods used were: (a) a Morlet complex wavelet transform, which is often used in analysis of non-linear application processes. Through the use of the wavelet, it is possible to observe a phase singularity that involves a strong interaction between an extensive range of scales; (b) recurrence plot tests, which were used to identify a sudden change between different stable atmospheric states. (c) statistical analysis of early-warning signals, which verify simultaneous increases in the autocorrelation function and in the variance in the state variable; and (d) analysis of wind speed versus turbulent kinetic energy to identify different turbulent regimes in the stable boundary layer. We found it is adequate to use a threshold to classify the cases of strong turbulence regime, as a result of the occurrence of EP in the tropical atmosphere. All methods used corroborate and indicate synergy between events that culminate in what we classify as EP of the stable boundary layer above the tropical forest.

54 ENVIRONMENTAL SCIENCES↗

Transducer Resolution Effect on Pressure Fluctuations Beneath Hypersonic Turbulent Boundary Layers

The size of a pressure transducer is known to affect the accuracy of measurements of wall-pressure fluctuations beneath a turbulent boundary layer because of spatial averaging over the sensing area of the transducer. In this paper, the effect of finite transducer size is investigated by applying spatial averaging or wavenumber filters to a database of hypersonic wall pressure generated from a direct numerical simulation (DNS) that simulates the turbulent portion of the boundary layer over a sharp 7° half-angle cone at nominally Mach 8. Here, a good comparison between the DNS and the experiment in the Sandia Hypersonic Wind Tunnel at Mach 8 is achieved after spatial averaging is applied to the DNS data over an area similar to the sensing area of the transducer. The study shows that a finite sensor size similar to that of the PCB132 transducer can cause significant attenuation in the root-mean-square and power spectral density (PSD) of wall-pressure fluctuations, and the attenuation effect is identical between cone and flat plate configurations at the same friction Reynolds number. The Corcos theory is found to successfully compensate for the attenuated high-frequency components of the wall-pressure PSD.

42 ENGINEERING↗

Coupling Between Alfvén Wave and Kelvin–Helmholtz Waves in the Low Latitude Boundary Layer

The Kelvin–Helmholtz (KH) instability of magnetohydrodynamic surface waves at the low latitude boundary layer is examined using both an eigenfrequency analysis and a time-dependent wave simulation. The analysis includes the effects of sheared flow and Alfvén velocity gradient. When the magnetosheath flows are perpendicular to the ambient magnetic field direction, unstable KH waves that propagate obliquely to the sheared flow direction occur at the sheared flow surface when the Alfvén Mach number is higher than an instability threshold. Including a shear transition layer between the magnetosphere and magnetosheath leads to secondary KH waves (driven by the sheared flow) that are coupled to the resonant surface Alfvén wave. There are remarkable differences between the primary and the secondary KH waves, including wave frequency, the growth rate, and the ratio between the transverse and compressional components. The secondary KH wave energy is concentrated near the shear Alfvén wave frequency at the magnetosheath with a lower frequency than the primary KH waves. Although the growth rate of the secondary KH waves is lower than the primary KH waves, the threshold condition is lower, so it is expected that these types of waves will dominate at a lower Mach number. Because the transverse component of the secondary KH waves is stronger than that of the primary KH waves, more efficient wave energy transfer from the boundary layer to the inner magnetosphere is also predicted.

79 ASTRONOMY AND ASTROPHYSICS↗

Scientific challenges to characterizing the wind resource in the marine atmospheric boundary layer

Abstract. With the increasing level of offshore wind energy investment, it is correspondingly important to be able to accurately characterize the wind resource in terms of energy potential as well as operating conditions affecting wind plant performance, maintenance, and lifespan. Accurate resource assessment at a particular site supports investment decisions. Following construction, accurate wind forecasts are needed to support efficient power markets and integration of wind power with the electrical grid. To optimize the design of wind turbines, it is necessary to accurately describe the environmental characteristics, such as precipitation and waves, that erode turbine surfaces and generate structural loads as a complicated response to the combined impact of shear, atmospheric turbulence, and wave stresses. Despite recent considerable progress both in improvements to numerical weather prediction models and in coupling these models to turbulent flows within wind plants, major challenges remain, especially in the offshore environment. Accurately simulating the interactions among winds, waves, wakes, and their structural interactions with offshore wind turbines requires accounting for spatial (and associated temporal) scales from O(1 m) to O(100 km). Computing capabilities for the foreseeable future will not be able to resolve all of these scales simultaneously, necessitating continuing improvement in subgrid-scale parameterizations within highly nonlinear models. In addition, observations to constrain and validate these models, especially in the rotor-swept area of turbines over the ocean, remains largely absent. Thus, gaining sufficient understanding of the physics of atmospheric flow within and around wind plants remains one of the grand challenges of wind energy, particularly in the offshore environment. This paper provides a review of prominent scientific challenges to characterizing the offshore wind resource using as examples phenomena that occur in the rapidly developing wind energy areas off the United States. Such phenomena include horizontal temperature gradients that lead to strong vertical stratification; consequent features such as low-level jets and internal boundary layers; highly nonstationary conditions, which occur with both extratropical storms (e.g., nor'easters) and tropical storms; air–sea interaction, including deformation of conventional wind profiles by the wave boundary layer; and precipitation with its contributions to leading-edge erosion of wind turbine blades. The paper also describes the current state of modeling and observations in the marine atmospheric boundary layer and provides specific recommendations for filling key current knowledge gaps.

17 WIND ENERGY↗

Coupling between Alfven wave and Kelvin-Helmholtz waves in the low latitude boundary layer

The Kelvin-Helmholtz (KH) instability of magnetohydrodynamic surface waves at the low latitude boundary layer is examined using both an eigenfrequency analysis and a time-dependent wave simulation. The analysis includes the effects of sheared flow and Alfven velocity gradient. When the magnetosheath flows are perpendicular to the ambient magnetic field direction, unstable KH waves that propagate obliquely to the sheared flow direction occur at the sheared flow surface when the Alfv\'en Mach number is higher than an instability threshold. Including a shear transition layer between the magnetosphere and magnetosheath leads to secondary KH waves (driven by the sheared flow) that are coupled to the resonant surface Alfven wave. There are remarkable differences between the primary and the secondary KH waves including wave frequency, the growth rate, and the ratio between transverse and the compressional component. The secondary KH wave energy is concentrated near the shear Alfven wave frequency at the magnetosheath with a lower frequency than the primary KH waves. Although the growth rate of the secondary KH waves is lower than the primary KH waves, the threshold condition is lower, so it is expected that these types of waves will dominate at lower Mach number. Because the transverse component of the secondary KH waves is stronger than the primary KH waves, more efficient wave energy transfer from the boundary layer to the inner magnetosphere is also predicted.

Alfven wave↗

Turbulence in The Marine Boundary Layer and Air Motions Below Stratocumulus Clouds at the ARM Eastern North Atlantic Site

Marine stratocumulus clouds are intimately coupled to the turbulence in the boundary layer and drizzle is known to be ubiquitous within them. Six years of data collected at the Atmospheric Radiation Measurement (ARM)’s Eastern North Atlantic site are utilized to characterize turbulence in the marine boundary layer and air motions below stratocumulus clouds. Profiles of variance of vertical velocity binned by wind direction (wdir) yielded that the boundary layer measurements are affected by the island when the wdir is between 90° and 310° (measured clockwise from North where air is coming from). Data collected during the marine conditions (wdir<90 or wdir>310) showed that the variance of vertical velocity was higher during the winter months than during the summer months due to higher cloudiness, wind speeds, and surface fluxes. Furthermore, during marine conditions the variance of vertical velocity and cloud fraction exhibited a distinct diurnal cycle with higher values during the nighttime than during the daytime. Detailed analysis of 32 cases of drizzling marine stratocumulus clouds showed that for a similar amount of radiative cooling at the cloud top, within the sub-cloud layer 1) drizzle increasingly falls within downdrafts with increasing rain rates, 2) the strength of the downdrafts increases with increasing rain rates, and 3) the correlation between vertical air motion and rain rate is highest in the middle of the sub-cloud layer. The results presented herein have implications for climatological and model evaluation studies conducted at the ENA site, along with efforts of accurately representing drizzle-turbulence interactions in a range of atmospheric models.

54 ENVIRONMENTAL SCIENCES↗

The significant impact of aerosol vertical structure on lower atmosphere stability and its critical role in aerosol–planetary boundary layer (PBL) interactions

The aerosol–planetary boundary layer (PBL) interaction was proposed as an important mechanism to stabilize the atmosphere and exacerbate surface air pollution. Despite the tremendous progress made in understanding this process, its magnitude and significance still have large uncertainties and vary largely with aerosol distribution and meteorological conditions. In this study, we focus on the role of aerosol vertical distribution in thermodynamic stability and PBL development by jointly using micropulse lidar, sun photometer, and radiosonde measurements taken in Beijing. Despite the complexity of aerosol vertical distributions, cloud-free aerosol structures can be largely classified into three types: well-mixed, decreasing with height, and inverse structures. The aerosol–PBL relationship and diurnal cycles of the PBL height and PM 2.5 associated with these different aerosol vertical structures show distinct characteristics. The vertical distribution of aerosol radiative forcing differs drastically among the three types, with strong heating in the lower, middle, and upper PBL, respectively. Such a discrepancy in the heating rate affects the atmospheric buoyancy and stability differently in the three distinct aerosol structures. Absorbing aerosols have a weaker effect of stabilizing the lower atmosphere under the decreasing structure than under the inverse structure. As a result, the aerosol–PBL interaction can be strengthened by the inverse aerosol structure and can be potentially neutralized by the decreasing structure. Moreover, aerosols can both enhance and suppress PBL stability, leading to both positive and negative feedback loops. This study attempts to improve our understanding of the aerosol–PBL interaction, showing the importance of the observational constraint of aerosol vertical distribution for simulating this interaction and consequent feedbacks.

54 ENVIRONMENTAL SCIENCES↗