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An overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) project: aerosol–cloud–radiation interactions in the southeast Atlantic basin

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles, yet the fate of these particles and their influence on regional and global climate is poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA EVS-2 (Earth Venture Suborbital-2) investigation with three intensive observation periods designed to study key atmospheric processes that determine the climate impacts of these aerosols. During the Southern Hemisphere winter and spring (June-October), aerosol particles reaching 3-5 km in altitude are transported westward over the southeast Atlantic, where they interact with one of the largest subtropical stratocumulus (Sc) cloud decks in the world. The representation of these interactions in climate models remains highly uncertain in part due to a scarcity of observational constraints on aerosol and cloud properties, as well as due to the parameterized treatment of physical processes. Three ORACLES deployments by the NASA P-3 aircraft in September 2016, August 2017, and October 2018 (totaling ~350 science flight hours), augmented by the deployment of the NASA ER-2 aircraft for remote sensing in September 2016 (totaling ~100 science flight hours), were intended to help fill this observational gap. ORACLES focuses on three fundamental science themes centered on the climate effects of African BB aerosols: (a) direct aerosol radiative effects, (b) effects of aerosol absorption on atmospheric circulation and clouds, and (c) aerosol–cloud microphysical interactions. This paper summarizes the ORACLES science objectives, describes the project implementation, provides an overview of the flights and measurements in each deployment, and highlights the integrative modeling efforts from cloud to global scales to address science objectives. Significant new findings on the vertical structure of BB aerosol physical and chemical properties, chemical aging, cloud condensation nuclei, rain and precipitation statistics, and aerosol indirect effects are emphasized, but their detailed descriptions are the subject of separate publications. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project and the dataset it produced.

54 ENVIRONMENTAL SCIENCES↗

Cloud drop number concentrations over the western North Atlantic Ocean: seasonal cycle, aerosol interrelationships, and other influential factors

Cloud drop number concentrations (N d ) over the western North Atlantic Ocean (WNAO) are generally highest during the winter (DJF) and lowest in summer (JJA), in contrast to aerosol proxy variables (aerosoloptical depth, aerosol index, surface aerosol mass concentrations, surface cloud condensation nuclei (CCN) concentrations) that generally peak inspring (MAM) and JJA with minima in DJF. Using aircraft, satellite remote sensing, ground-based in situ measurement data, and reanalysis data, we characterize factors explaining the divergent seasonal cycles and furthermore probe into factors influencing N d on seasonal timescales. The results can be summarized well by features most pronounced in DJF, including features associated with cold-air outbreak (CAO) conditions such as enhanced values of CAO index, planetary boundary layer height (PBLH),low-level liquid cloud fraction, and cloud-top height, in addition to winds aligned with continental outflow. Data sorted into high- and low-N d days in each season, especially in DJF, revealed that all of these conditions were enhanced on the high-N d days, including reduced sea level pressure and stronger wind speeds. Although aerosols may be more abundant in MAM and JJA, the conditions needed to activate those particles into cloud droplets are weaker than in colder months, which is demonstrated by calculations of the strongest (weakest) aerosol indirect effects in DJF (JJA) based on comparing N d to perturbations in four different aerosol proxy variables (total and sulfate aerosol optical depth, aerosol index, surface mass concentration of sulfate). We used three machine learning models and up to 14 input variables to infer about most influential factors related to N d for DJF and JJA, with the best performance obtained with gradient-boosted regression tree (GBRT) analysis. The model results indicated that cloud fraction was the most important input variable, followed by some combination (depending on season) of CAO index and surface mass concentrations of sulfate and organic carbon. Future work is recommended to further understand aspects uncovered here such as impacts of free tropospheric aerosol entrainment on clouds, degree of boundary layer coupling, wet scavenging, and giant CCN effects on aerosol–N d relationships, updraft velocity, and vertical structure of cloud properties such as adiabaticity that impact the satellite estimation of N d .

54 ENVIRONMENTAL SCIENCES↗

Impact of Aerosol and Cloud on the Solar Energy Potential over the Central Gangetic Himalayan Region

We examine the impact of atmospheric aerosols and clouds on the surface solar radiation and solar energy at Nainital, a high-altitude remote location in the central Gangetic Himalayan region (CGHR). For this purpose, we exploited the synergy of remote-sensed data in terms of ground-based AERONET Sun Photometer and satellite observations from the MODerate Resolution Imaging Spectroradiometer (MODIS) and the Meteosat Second Generation (MSG), with radiative transfer model (RTM) simulations and 1 day forecasts from the Copernicus Atmosphere Monitoring Service (CAMS). Clouds and aerosols are one of the most common sources of solar irradiance attenuation and hence causing performance issues in the photovoltaic (PV) and concentrated solar power (CSP) plant installations. The outputs of RTM results presented with high accuracy under clear, cloudy sky and dust conditions for global horizontal (GHI) and beam horizontal irradiance (BHI). On an annual basis the total aerosol attenuation was found to be up to 105 kWh m –2 for the GHI and 266 kWh m –2 for BHI, respectively, while the cloud effect is much stronger with an attenuation of 245 and 271 kWh m –2 on GHI and BHI. The results of this study will support the Indian solar energy producers and electricity handling entities in order to quantify the energy and financial losses due to cloud and aerosol presence.

54 ENVIRONMENTAL SCIENCES↗

Improved constraints on hematite refractive index for estimating climatic effects of dust aerosols

Abstract Uncertainty in desert dust composition poses a big challenge to understanding Earth’s climate across different epochs. Of particular concern is hematite, an iron-oxide mineral dominating the solar absorption by dust particles, for which current estimates of absorption capacity vary by over two orders of magnitude. Here, we show that laboratory measurements of dust composition, absorption, and scattering provide valuable constraints on the absorption potential of hematite, substantially narrowing its range of plausible values. The success of this constraint is supported by results from an atmospheric transport model compared with station-based measurements. Additionally, we identify substantial bias in simulating hematite abundance in dust aerosols with current soil mineralogy descriptions, underscoring the necessity for improved data sources. Encouragingly, the next-generation imaging spectroscopy remote sensing data hold promise for capturing the spatial variability of hematite. These insights have implications for enhancing dust modeling, thus contributing to efforts in climate change mitigation and adaptation.

Environmental Sciences & Ecology↗

Virtual tower measurements during the American WAKE ExperimeNt (AWAKEN)

Dual-Doppler lidar measurements were made during the American WAKE ExperimeNt to provide height-resolved measurements of wind speed and direction at multiple locations immediately south of the leading row turbines in the King Plains wind farm in Oklahoma. These so-called virtual tower measurements were performed to characterize the inflow into the wind farm and to assess possible upwind blockage effects due to the collective action of the wind farm. The campaign was conducted from 12 November 2022 to 17 October 2023, during which time 14 unique virtual tower locations were sampled with heights ranging from 240 to 490 m AGL. The wind retrieval algorithm provided estimates of the horizontal winds and their uncertainties with a vertical resolution of about 10 m, while also accounting for the tilt of the lidar platform. The virtual tower results are compared to collocated lidar wind profiling data at the A1 site, which was located roughly 2.4 rotor diameters south of the nearest turbine. The wind speed difference between the wind profiler and the virtual tower was found to be quite sensitive to atmospheric stability and wind direction below 250 m AGL. The largest differences were observed for inflow under stable conditions, where the profiler wind speeds were observed to be about 22% lower than the virtual tower near hub height. These results suggest that there are persistent horizontal gradients in the flow upwind of the wind farm which result in biased estimates using standard ground-based lidar wind profiling methods.

17 WIND ENERGY↗

Utilizing a Storm-Generating Hotspot to Study Convective Cloud Transitions: The CACTI Experiment

The Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign was designed to improve understanding of orographic cloud life cycles in relation to surrounding atmospheric thermodynamic, flow, and aerosol conditions. The deployment to the Sierras de Córdoba range in north-central Argentina was chosen because of very frequent cumulus congestus, deep convection initiation, and mesoscale convective organization uniquely observable from a fixed site. The C-band Scanning Atmospheric Radiation Measurement (ARM) Precipitation Radar was deployed for the first time with over 50 ARM Mobile Facility atmospheric state, surface, aerosol, radiation, cloud, and precipitation instruments between October 2018 and April 2019. An intensive observing period (IOP) coincident with the RELAMPAGO field campaign was held between 1 November and 15 December during which 22 flights were performed by the ARM Gulfstream-1 aircraft. A multitude of atmospheric processes and cloud conditions were observed over the 7-month campaign, including numerous orographic cumulus and stratocumulus events; new particle formation and growth producing high aerosol concentrations; drizzle formation in fog and shallow liquid clouds; very low aerosol conditions following wet deposition in heavy rainfall; initiation of ice in congestus clouds across a range of temperatures; extreme deep convection reaching 21-km altitudes; and organization of intense, hail-containing supercells and mesoscale convective systems. These comprehensive datasets include many of the first ever collected in this region and provide new opportunities to study orographic cloud evolution and interactions with meteorological conditions, aerosols, surface conditions, and radiation in mountainous terrain.

54 ENVIRONMENTAL SCIENCES↗

Multiscale Wildfire Simulation Framework and Remote Sensing

Wildfire as one type of climate extreme events causes huge socioeconomic losses and damages. Large wildfires (i.e., generated pyrocumulonimbus (PyroCb)) can inject tremendous amounts of smoke into the stratosphere, where black carbon and organic carbon aerosols can persist months to years and influence climate by imposing a significant reduction in the radiative forcing like that associated with large volcanic eruptions or proposed via climate interventions such as geoengineering. Both observations and numerical modeling results clearly indicate an increasing trend in wildfire frequency and intensity in many regions during the recent decades with climate change. However, current understanding of wildfire remains largely uncertain owing to limitations of modeling capabilities in representing the multiscale wildfire physics and dynamics and a scarcity of observations constraining important wildfire and environmental variables. This study primarily aims to improve the wildfire simulation capabilities in the state-of-the-art climate model by filling in two major gaps: (1) model resolution is typically too coarse to resolve fine scale processes associated with fires, and (2) chemistry and aerosol processes in fire smoke are poorly represented.

54 ENVIRONMENTAL SCIENCES↗

Cloud micro- and macrophysical properties from ground-based remote sensing during the MOSAiC drift experiment

In the framework of the Multidisciplinary drifting Observatory for the Study of Arctic Climate Polarstern expedition, the Leibniz Institute for Tropospheric Research, Leipzig, Germany, operated the shipborne OCEANET-Atmosphere facility for cloud and aerosol observations throughout the whole year. OCEANET-Atmosphere comprises, amongst others, a multiwavelength Raman lidar, a microwave radiometer, and an optical disdrometer. A cloud radar was operated aboard Polarstern by the US Atmospheric Radiation Measurement program. These measurements were processed by applying the so-called Cloudnet methodology to derive cloud properties. To gain a comprehensive view of the clouds, lidar and cloud radar capabilities for low- and high-altitude observations were combined. Cloudnet offers a variety of products with a spatiotemporal resolution of 30 s and 30 m, such as the target classification, and liquid and ice microphysical properties. Additionally, a lidar-based low-level stratus retrieval was applied for cloud detection below the lowest range gate of the cloud radar. Based on the presented dataset, e.g., studies on cloud formation processes and their radiative impact, and model evaluation studies can be conducted.

54 ENVIRONMENTAL SCIENCES↗

dlppi2 (b1)

The Doppler lidar (DL) is an active remote-sensing instrument that provides range- and time-resolved measurements of the line-of-sight component of air velocity (i.e., radial velocity) and attenuated aerosol backscatter. The DL operates in the near-infrared and is sensitive to backscatter from atmospheric aerosol, which are assumed to be ideal tracers of atmospheric wind fields. The DL works by transmitting short pulses of infrared laser light into the atmosphere. Atmospheric aerosols scatter a small fraction of that light energy back to the transceiver, where it is collected and recorded as a time-resolved signal. From the delay between the outgoing pulse and the backscattered signal, the instrument infers the distance to the scattering volume. Coherent detection is used to measure the Doppler frequency shift of the backscatter signal. This is accomplished by mixing the backscatter signal with a reference laser beam (i.e., local oscillator) of known frequency. The onboard signal processor then determines the Doppler frequency shift from the spectrum of the mixed signal. The Doppler frequency shift and thus the radial air velocity is determined from the peak of the Doppler spectrum. The attenuated backscatter is determined from the energy content of the Doppler spectra. The DL provides accurate measurements of radial velocity in regions of the atmosphere where aerosol concentrations are high enough to ensure good signal-to-noise ratio. Thus, valid data are usually limited to the atmospheric boundary layer where aerosol is ubiquitous. Valid measurements can also be obtained in elevated aerosol layers or in optically thin clouds above the boundary layer. Most of the ARM DLs have full upper-hemispheric scanning capability, enabling 3D mapping of turbulent flows in the atmospheric boundary layer. With the scanner pointed vertically, the DL provides height- and time-resolved measurements of vertical velocity.

54 ENVIRONMENTAL SCIENCES↗

Shallow cloud variability in Houston, Texas, during the ESCAPE and TRACER field experiments

Shallow convection plays an important role in Earth's climate system by regulating the vertical transport of heat, moisture, and momentum in the lower troposphere. Aerosols, large-scale meteorology, and low-level convergence influence the spatiotemporal variability in shallow convection, and the coastal urban area of Houston, Texas, is an ideal laboratory to investigate these complex interactions. Here, geostationary satellite and ground-based radar observations from June to September 2022 during the TRacking Aerosol Convection interactions ExpeRiment (TRACER) and Experiment of Sea Breeze Convection, Aerosols, Precipitation, and Environment (ESCAPE) field campaigns are used to characterize the spatial coverage, vertical extent, and precipitation fraction of shallow convective clouds. The fused operational remote sensing datasets over a 250 km × 250 km domain are evaluated against profiling observations. The domain-wide diurnal shallow cloud fractions are used to identify four distinct modes of shallow convection. In all clusters, the domain-wide cloud fractions are consistently higher than the domain-wide precipitation fractions, and shallow cloud fractions are higher over water than they are over land, while the shallow precipitation fractions show the opposite behavior. In the two modes with minimal deep cloud activity, shallow cloud frequency is highest over ocean in the early morning, and there is a transition to higher shallow cloud frequency over land by the afternoon in one cluster or to high shallow cloud frequencies everywhere by the afternoon in the other. Lastly, we find regions with higher shallow cloud top heights and a large region along the coastline where shallow clouds are more likely to precipitate.

54 ENVIRONMENTAL SCIENCES↗

Measurement report: Vertically resolved atmospheric properties observed over the Southern Great Plains with the ArcticShark uncrewed aerial system

Abstract. This study presents the unique capability of the Department of Energy (DOE) ArcticShark – a mid-size fixed-wing uncrewed aerial system (UAS) – for measuring vertically resolved atmospheric properties over the Southern Great Plains (SGP) of the United States. Focusing on atmospheric states, such as ambient temperature, wind, and aerosol properties, we overview measurements from 32 research flights (∼ 97 flight hours) in 2023. The August operations, aided by a visual observer on a chase plane, allowed for extensive UAS coverage, surpassing typical UAS operation envelopes. Our data from March, June, and August 2023 reveal distinctive seasonal patterns within the atmospheric column through unique chemical composition measurements. In situ measurements combined with remote sensing retrievals and radiosonde measurements provided valuable insights into their consistency and complementarity. Furthermore, we demonstrate the capabilities of the ArcticShark through several case studies, including the analyses of correlations between UAS-derived atmospheric profiles and conventional radiosonde measurements, as well as the derivation of vertically resolved profiles of aerosol chemical, optical, and microphysical properties. These case studies highlight the versatility of the ArcticShark UAS as a powerful tool for comprehensive atmospheric research, effectively bridging data gaps and enhancing our understanding of vertical atmospheric structures in the region.

54 ENVIRONMENTAL SCIENCES↗

An Algorithm to Retrieve Total Precipitable Water Vapor in the Atmosphere from FengYun 3D Medium Resolution Spectral Imager 2 (FY-3D MERSI-2) Data

The atmosphere has substantial effects on optical remote sensing imagery of the Earth’s surface from space. These effects come through the functioning of atmospheric particles on the radiometric transfer from the Earth’s surface through the atmosphere to the sensor in space. Precipitable water vapor (PWV), CO 2 , ozone, and aerosol in the atmosphere are very important among the particles through their functioning. This study presented an algorithm to retrieve total PWV from the Chinese second-generation polar-orbiting meteorological satellite FengYun 3D Medium Resolution Spectral Imager 2 (FY-3D MERSI-2) data, which have three near-infrared (NIR) water vapor absorbing channels, i.e., channel 16, 17, and 18. The algorithm was improved from the radiance ratio technique initially developed for Moderate-Resolution Imaging Spectroradiometer (MODIS) data. MODTRAN 5 was used to simulate the process of radiant transfer from the ground surfaces to the sensor at various atmospheric conditions for estimation of the coefficients of ratio technique, which was achieved through statistical regression analysis between the simulated radiance and transmittance values for FY-3D MERSI-2 NIR channels. The algorithm was then constructed as a linear combination of the three-water vapor absorbing channels of FY-3D MERSI-2. Measurements from two ground-based reference datasets were used to validate the algorithm: the sun photometer measurements of Aerosol Robotic Network (AERONET) and the microwave radiometer measurements of Energy’s Atmospheric Radiation Measurement Program (ARMP). The validation results showed that the algorithm performs very well when compared with the ground-based reference datasets. The estimated PWV values come with root mean square error (RMSE) of 0.28 g/cm 2 for the ARMP and 0.26 g/cm 2 for the AERONET datasets, with bias of 0.072 g/cm 2 and 0.096 g/cm 2 for the two reference datasets, respectively. The accuracy of the proposed algorithm revealed a better consistency with ground-based reference datasets. Thus, the proposed algorithm could be used as an alternative to retrieve PWV from FY-3D MERSI-2 data for various remote sensing applications such as agricultural monitoring, climate change, hydrologic cycle, and so on at various regional and global scales.

54 ENVIRONMENTAL SCIENCES↗

Light transport with weak angular dependence in fog

Random scattering and absorption of light by tiny particles in aerosols, like fog, reduce situational awareness and cause unacceptable down-time for critical systems or operations. Computationally efficient light transport models are desired for computational imaging to improve remote sensing capabilities in degraded optical environments. To this end, we have developed a model based on a weak angular dependence approximation to the Boltzmann or radiative transfer equation that appears to be applicable in both the moderate and highly scattering regimes, thereby covering the applicability domain of both the small angle and diffusion approximations. An analytic solution was derived and validated using experimental data acquired at the Sandia National Laboratory Fog Chamber facility. The evolution of the fog particle density and size distribution were measured and used to determine macroscopic absorption and scattering properties using Mie theory. A three-band (0.532, 1.55, and 9.68 µ m) transmissometer with lock-in amplifiers enabled changes in fog density of over an order of magnitude to be measured due to the increased transmission at higher wavelengths, covering both the moderate and highly scattering regimes. The meteorological optical range parameter is shown to be about 0.6 times the transport mean free path length, suggesting an improved physical interpretation of this parameter.

74 ATOMIC AND MOLECULAR PHYSICS↗

Highly supercooled riming and unusual triple-frequency radar signatures over McMurdo Station, Antarctica

Abstract. Riming of ice crystals by supercooled water droplets is an efficient ice growth process, but its basic properties are still poorly known. While it has been shown to contribute significantly to surface precipitation at mid-latitudes, little is known about its occurrence at high latitudes. In Antarctica, two competing effects can influence the occurrence of riming: (i) the scarcity of supercooled liquid water clouds due to the extremely low tropospheric temperatures and (ii) the low aerosol concentration, which may lead to the formation of fewer and larger supercooled drops potentially resulting in an enhanced riming efficiency. In this work, by exploiting the deployment of an unprecedented number of multiwavelength remote sensing systems (including triple-frequency radar measurements) in West Antarctica, during the Atmospheric Radiation Measurements West Antarctic Radiation Experiment (AWARE) field campaign, we evaluate the riming incidence at McMurdo Station and find that riming occurs at much lower temperatures when compared to previous results in the mid-latitudes. This suggests the possible occurrence of a common atmospheric state over Antarctica that includes a rather stable atmosphere inhibiting turbulent mixing, and a high riming efficiency driven by large cloud droplets. We then focus on a peculiar case study featuring a persistent layer with a particularly pronounced riming signature in triple-frequency radar data but only a relatively modest amount of supercooled liquid water. In-depth analysis of the radar observations suggests that such signatures can only be explained by the combined effects of moderately rimed aggregates or similarly shaped florid polycrystals and a narrow particle size distribution (PSD). Simulations of this case study performed with a one-dimensional bin model indicate that similar triple-frequency radar observations can be reproduced when narrow PSDs are simulated. Such narrow PSDs can in turn be explained by two key factors: (i) the presence of a shallow homogeneous droplet or humidified aerosol freezing layer aloft seeding an underlying supercooled liquid layer, and (ii) the absence of turbulent mixing throughout a stable polar atmosphere that sustains narrow PSDs, as hydrometeors grow from the nucleation region aloft to ice particles of several millimeters in size, by vapor deposition and then riming.

54 ENVIRONMENTAL SCIENCES↗

MODIS Aerosol and Low‐Cloud Retrievals: Orographic Effects in the Wake of Macquarie Island

Abstract Visible/infrared imagery from passive satellites is commonly relied upon to study low cloud microphysics over oceanic regions, including for the Southern Ocean (SO), but relatively little validation has been undertaken for the SO. In this article, we compare low‐cloud effective radius ( r e ), cloud droplet number concentration ( N d ) and cloud liquid water path (LWP) retrievals from the NASA Moderate Imaging Spectroradiometer (MODIS) with surface measurements collected during the Macquarie Island Cloud and Radiation Experiment (MICRE). MODIS 3.7‐μm band retrievals show little bias and moderately good correlation relative to MICRE retrievals for liquid‐phase low clouds when restricted to Solar Zenith Angles <65° on spatial scales of 50–100 km. However, the low overall bias in 3.7‐μm band effective radius ( r e 3.7 ) retrievals partly results from cancellation of errors: r e 3.7 is overestimated for non‐to‐lightly precipitating clouds, and underestimated for heavier drizzling clouds by ∼1–1.5 μm. 1.6‐μm and 2.1‐μm band r e retrievals are biased high. N d may likewise be slightly under‐ or overestimated depending on the concentration, but there is insufficient data to provide confidence in this result. Interestingly, a composite of MODIS retrievals from 2002 to 2020 show a distinct region of enhanced cloud cover and N d (and lower r e ) in the wake of Macquarie Island associated with orographic cloud formation. MODIS retrievals of aerosol optical depth (AOD) and Angstrom Exponent (AE) upwind and downwind of the island do not differ significantly. Comparison with MICRE measurements suggests that MODIS Collection 6 AOD retrievals are reasonable, while AE is problematically large.

54 ENVIRONMENTAL SCIENCES↗

SCOPE: Spectral cloud optical property estimation using real-time GOES-R longwave imagery

The output of ground-based, solar power generation systems is strongly dependent on cloud cover, which is the main contributor to solar power variability and uncertainty. Cloud optical properties are typically over-simplified in forecasting applications due to the lack of realtime, accurate estimates. In this work, we introduce a method, the Spectral Cloud Optical Property Estimation (SCOPE), for estimating cloud optical properties directly from high-resolution (5-min, 2 km) imagery from Geostationary Operational Environmental Satellite (GOES)-R, which is the newest generation of the GOES system. The SCOPE method couples a two-stream, spectrally resolved radiative model with the longwave GOES-R sensor output to simultaneously estimate the cloud optical depth, cloud top height, and cloud thickness during both day and night at 5-min intervals. The accuracy of SCOPE is evaluated using one year (2018) of downwelling longwave (DLW) radiation measurements from the Surface Radiation Budget Network, which consists of seven sites spread across climatically diverse regions of the contiguous United States. During daytime clear-sky periods, SCOPE predicts DLW within instrument uncertainty (10 W m -2 ) for four of the seven locations, with the remaining locations yielding errors of the order of 11.2, 17.7, and 20.2 W m -2 . For daytime cloudy-sky, daytime all-sky (clear or cloudy), and nighttime all-sky periods, SCOPE achieves root mean square error values of 23.0–34.5 W m -2 for all seven locations. These results, together with the low-latency of the method (1 s per sample), show that SCOPE provides a viable solution to real-time, accurate estimation of cloud optical properties for both day and night.

42 ENGINEERING↗

Three-Channel Sunphotometer Cloud Mode Value-Added Product Report

A primary source of uncertainty in Earth system model (ESM) predictions is the representation of cloud processes and associated cloud feedback. Several fundamental cloud properties critical to the understanding of aerosol-cloud interactions are poorly constrained by observations, with key deficiencies in our observations of cloud and precipitation droplet sizes and cloud optical depth. Observations of these cloud properties are often challenging to estimate from remote-sensing platforms and costly to obtain from in situ aircraft. Nevertheless, observations of boundary-layer clouds, and improved knowledge of stratocumulus cloud (Sc) processes, are especially important to ESM advancement. This is because these clouds have extensive coverage and exert controls on boundary-layer dynamics and the global radiative energy balance.

54 ENVIRONMENTAL SCIENCES↗

Deep-learning-derived planetary boundary layer height from conventional meteorological measurements

Abstract. The planetary boundary layer (PBL) height (PBLH) is an important parameter for various meteorological and climate studies. This study presents a multi-structure deep neural network (DNN) model, which can estimate PBLH by integrating the morning temperature profiles and surface meteorological observations. The DNN model is developed by leveraging a rich dataset of PBLH derived from long-standing radiosonde records augmented with high-resolution micro-pulse lidar and Doppler lidar observations. We access the performance of the DNN with an ensemble of 10 members, each featuring distinct hidden-layer structures, which collectively yield a robust 27-year PBLH dataset over the southern Great Plains from 1994 to 2020. The influence of various meteorological factors on PBLH is rigorously analyzed through the importance test. Moreover, the DNN model's accuracy is evaluated against radiosonde observations and juxtaposed with conventional remote sensing methodologies, including Doppler lidar, ceilometer, Raman lidar, and micro-pulse lidar. The DNN model exhibits reliable performance across diverse conditions and demonstrates lower biases relative to remote sensing methods. In addition, the DNN model, originally trained over a plain region, demonstrates remarkable adaptability when applied to the heterogeneous terrains and climates encountered during the GoAmazon (Green Ocean Amazon; tropical rainforest) and CACTI (Cloud, Aerosol, and Complex Terrain Interactions; middle-latitude mountain) campaigns. These findings demonstrate the effectiveness of deep learning models in estimating PBLH, enhancing our understanding of boundary layer processes with implications for improving the representation of PBL in weather forecasting and climate modeling.

54 ENVIRONMENTAL SCIENCES↗