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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Experimental and Theoretical Comparison of Potential-dependent Methylation on Chemically Exfoliated WS 2 and MoS 2
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High-Frequency Sheet Conductance of Nanolayered WS 2 Crystals for Two-Dimensional Nanodevices
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Factors Controlling Intercalation of Metal Atoms into WS 2 : Implications for Electronically Tunable Semiconductors
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Solution-Phase Activation and Functionalization of Colloidal WS[subscript 2] Nanosheets with Ni Single Atoms
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Unraveling the Effect of Stacking Configurations on Charge Transfer in WS 2 and Organic Semiconductor Heterojunctions
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Twist-angle dependence of moiré excitons in WS 2 /MoSe 2 heterobilayers
Moiré lattices formed in twisted van der Waals bilayers provide a unique, tunable platform to realize coupled electron or exciton lattices unavailable before. While twist angle between the bilayer has been shown to be a critical parameter in engineering the moiré potential and enabling novel phenomena in electronic moiré systems, a systematic experimental study as a function of twist angle is still missing. Here we show that not only are moiré excitons robust in bilayers of even large twist angles, but also properties of the moiré excitons are dependant on, and controllable by, the moiré reciprocal lattice period via twist-angle tuning. From the twist-angle dependence, we furthermore obtain the effective mass of the interlayer excitons and the electron inter-layer tunneling strength, which are difficult to measure experimentally otherwise. These findings pave the way for understanding and engineering rich moiré-lattice induced phenomena in angle-twisted semiconductor van der Waals heterostructures.
Interlayer exciton landscape in WS 2 /tetracene heterostructures
The vertical stacking of two-dimensional materials into heterostructures gives rise to a plethora of intriguing optoelectronic properties and presents an unprecedented potential for technological development. While much progress has been made combining different monolayers of transition metal dichalcogenides (TMDs), little is known about TMD-based heterostructures including organic layers of molecules. In this work, we present a joint theory–experiment study on a TMD/tetracene heterostructure demonstrating clear signatures of spatially separated interlayer excitons in low temperature photoluminescence spectra. Here, the Coulomb-bound electrons and holes are localized either in the TMD or in the molecule layer, respectively. We reveal both in theory and experiment signatures of the entire intra- and interlayer exciton landscape in the photoluminescence spectra. In particular, we find both in theory and experiment a pronounced transfer of intensity from the intralayer TMD exciton to a series of energetically lower interlayer excitons with decreasing temperature. In addition, we find signatures of phonon-sidebands stemming from these interlayer exciton states. Our findings shed light on the microscopic nature of interlayer excitons in TMD/molecule heterostructures and could have important implications for technological applications of these materials.
Intervalley electron-hole exchange interaction and impurity-assisted recombination of indirect excitons in WS 2 and WSe 2 monolayers
The variety of excitonic states in tungsten-based dichalcogenide monolayers stems from unique interplay between the spin and valley degrees of freedom. One of the exciton species is the indirect exciton (momentum or valley dark), which is responsible for a series of resonances when the monolayer is charge neutral. We investigate the short-range electron-hole exchange interaction of the indirect exciton, as well as its recombination mechanism mediated by impurities. The analysis provides thorough understanding of the energy and polarization of the zero-phonon indirect exciton resonance in the emission spectrum.
Brightening of dark excitons in WS 2 via tensile strain-induced excitonic valley convergence
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First-principles study on the electronic properties and Schottky barrier of WC/ W S 2 and WC/ WS e 2 heterostructures
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Visualizing electron localization of WS 2 /WSe 2 moiré superlattices in momentum space
The search for materials with flat electronic bands continues due to their potential to drive strong correlation and symmetry breaking orders. Electronic moirés formed in van der Waals heterostructures have proved to be an ideal platform. However, there is no holistic experimental picture for how superlattices modify electronic structure. By combining spatially resolved angle-resolved photoemission spectroscopy with optical spectroscopy, we report the first direct evidence of how strongly correlated phases evolve from a weakly interacting regime in a transition metal dichalcogenide superlattice. By comparing short and long wave vector moirés, we find that the electronic structure evolves into a highly localized regime with increasingly flat bands and renormalized effective mass. The flattening is accompanied by the opening of a large gap in the spectral function and splitting of the exciton peaks. These results advance our understanding of emerging phases in moiré superlattices and point to the importance of interlayer physics.
Technoeconomic Analysis of Dye Sensitized Solar Cells (DSSCs) with WS 2 /Carbon Composite as Counter Electrode Material
Exploration of clean and renewable energy materials is necessary due to the coming energy crisis and environmental problems. Solar energy is one of the favorable energy sources because of the continuous energy reservoir and its affluence. Silicon-based solar devices are expensive due to their complicated production process, which limits this technology for urban and other commercial applications. Among the third generation of solar cells, Dye-Sensitized Solar Cells (DSSCs) have attracted widespread attention as potential cost-effective alternatives to silicon-based solar cells. In this paper, the commercializing potential of the DSSCs is investigated. A module is introduced where the materials, equipment, and distribution of direct manufacturing costs are calculated. The manufacturing costs and the Levelized Cost of Energy (LCOE) of these DSSCs for a system lifetime of 25 years were determined to be USD 22.40 per m 2 and USD 0.0438 per kWh and the module price of this technology is USD 0.18 per W and the total installed system cost is USD 0.88 per W in Kansas which suggest that this PV technology could challenge other leading PV technologies.
An Investigation of the Pressure Distribution on a 1/15-Scale Model of the Lockheed WS-117L Vehicle Plus Booster "B" at Mach Numbers from 1.55 to 2.35
Pressure coefficients were measured over the vehicle and over the forward part of the booster at Reynolds numbers of 3.0 x 10(exp 6) per foot. Tabular results are presented for two nose shapes at Mach numbers of 1.55, 1.75, 2.00, and 2.35, at angles of attack from -4 deg to +10 deg, and at 0 deg sideslip.
An Experimental Investigation of the Pressure Distribution on A 1/15-Scale Model of the Lockheed WS-117L Vehicle Plus Booster "B" at Mach Numbers from 0.70 to 1.45
Results obtained with two nose shapes tested at a Reynolds number per foot of 5 x 10(exp 6) at angles of attack from -4 deg to +10 deg at 0 deg angle of sideslip are presented in tabulated pressure coefficient form without analysis.