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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Analysis of the Reactive CO 2 Surface Flux in Electrocatalytic Aqueous Flow Reactors

We study how the mass transfer of a chemical species in shear flow is suppressed by the production of a second species that partially reacts away the first species. The second species is produced at the surface with the first species as a reactant. Our work is directly motivated by electrochemical CO 2 reduction in aqueous flow reactors, where OH– molecules generated by the CO evolution reaction react away CO 2 molecules, ultimately inhibiting the mass transfer of CO 2 to the cathode surface. We derive a simple approximation of the Sherwood number, a dimensionless measure of the mass flux into the surface, as a function of the Péclet number, surface Damköhler number, and bulk Damköhler number, and we compare our approximation to numerical solutions of the governing equations. We find that in the diffusion-limited regime, the Sherwood number is well described by the classical Graetz-Lévêque result reduced by a reaction factor due to the competing bulk reaction; with the stoichiometry relevant to electrochemical CO 2 reduction, this reaction factor is 1/2. While the model problem we solve provides insight into how OH– production affects CO 2 mass transfer, experimental systems often involve more complex chemistry. We thus also show how a common buffered electrolyte, KHCO 3 , affects our results.

30 DIRECT ENERGY CONVERSION↗
NASA NTRS2010

Investigation of Surface Flux Feedbacks for Coupled Atmosphere-Ocean Anomalies

The use of "dynamical coupling" rules allows for identifying coupled vs. uncoupled anomalies and one-way interaction. Results of this study are consistent with those of Pena et al. (2003,2004) although using a more recent reanalysis at higher resolution. Find more atmosphere-forcing coupled anomalies in the extratropics and ocean-forcing anomalies in the tropics. The LHF and SWR show the largest magnitude anomalies in the composite analysis. The turbulent flux responses are due to interactions between the differing responses in wind speed and near-surface gradients. The radiative fluxes responses are primarily tied to changes in cloud fraction, as expected, though longwave response can be tied more to changes in the upwelling component.

Roberts, J. Brent↗
NASA NTRS1992

Area-averaged surface fluxes and their time-space variability over the FIFE experimental domain

The underlying mean and variance properties of surface net radiation, sensible-latent heat fluxes and soil heat flux are studied over the densely instrumented grassland region encompassing FIFE. Flux variability is discussed together with the problem of scaling up to area-averaged fluxes. Results are compared and contrasted for cloudy and clear situations and examined for the influence of surface-induced biophysical controls (burn and grazing treatments) and topographic controls (aspect ratios and slope factors).

Smith, E. A.↗
DOE OSTI2021

Bridging Land-Surface Fluxes and Aerosol Concentrations to Triggering Convective Rainfall

During the period August 24-28, 2016, a delayed component the GO-Amazon Project, we launched nine altitude-controlled free balloons (CMET). Smaller than typical rawinsondes, CMET are equipped with altitude control, global communication via Iridium satellite, and aspirated sensors. The aims of our effort were to examine the interactions among convective boundary layer and dual river breeze circulations near the confluence of the Tapajos and Amazon Rivers in the eastern Basin. The week-long field campaign was timed to examine the reestablishment of the breeze circulations shortly after the passage of a strong instability line on August 22. Nine CMET were launched at the Curua-Una hydroelectric dam (2.8S; 54.3W), timed to encounter the Tapajos river breeze front by late afternoon. Soundings were made to establish the thickness of interface between the easterly trade and westerly Tapajos breeze circulation. Careful use of sounding strategies allowed these free balloons to track along the northerly channeled flow in the lowest 300 m above the River. Following the river encounter, balloons tracked to the west, sounding to describe the diurnal course of boundary layer in the forest west of the Tapajos River. The longest flight traveled more than 770 km over three days and twice rested overnight in the rain forest canopy. Ancillary data from surface climate and flux stations as well as the Santarem radiosonde, satellite images will be used to illustrate how the breeze circulations are seen near the surface and how they were disrupted by larger-scale events. Comparisons with HYSPLIT trajectories illustrate how sensitive real trajectories are to the refraction that the encounter with the breeze effects. A second effort was intensive analyses of data from the eddy flux tower at the Tapajós National Forest near Santarém Pará Brazil, with special emphasis on the role of clouds and canopy presence on light absorbance and photosynthetic activity.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1991

A bulk similarity approach in the atmospheric boundary layer using radiometric skin temperature to determine regional surface fluxes

Profiles of wind velocity and temperature in the outer region of the atmospheric boundary layer (ABL) were used together with surface temperature measurements, to determine regional shear stress and sensible heat flux by means of transfer parameterizations on the basis of bulk similarity. The profiles were measured by means of radiosondes and the surface temperatures by infrared radiation thermometry over hilly prairie terrain in northeastern Kansas during the First ISLSCP Field Experiment (FIFE). In the analysis, the needed similarity functions were determined and tested.

Brutsaert, Wilfried↗
NASA NTRS2004

The WCRP/GEWEX Surface Radiation Budget Project Release 2: An Assessment of Surface Fluxes at 1 Degree Resolution

The U.S. National Aeronautics and Space Administration (NASA) based Surface Radiation Budget (SRB) Project in association with the World Climate Research Programme Global Energy and Water Cycle Experiment (WCRP/GEWEX) is preparing a new 1 deg x 1 deg horizontal resolution product for distribution scheduled for release in early 2001. The new release contains several significant upgrades from the previous version. This paper summarizes the most significant upgrades and presents validation results as an assessment of the new data set.

Stackhouse, P. W., Jr.↗
NASA NTRS2009

Assessing the Uncertainty of Land Surface Fluxes Derived from Operational Analyses

Operational numerical weather prediction systems assimilate tremendous amounts of observations to produce global analyses of the atmospheric states. Since the systems include significant contributions from the model components, physical fields, such as the turbulent heat fluxes, can also be derived. However, the physical fields are indirectly constrained by the data assimilation, and so subject to uncertainty in the model parameterizations. Recently, 10 international operational analyses have been collected and reprocessed through the Coordinated Enhanced. Observing Period (CEOP). Comparisons against independent observations (global precipitation and outgoing longwave radiation) show that while there is significant range of the individual analyses, the ensemble of analyses provide data closest the observations. Here, we evaluate the collection of land surface turbulent heat fluxes. The data are available for Oct 2002 - Dec 2004, at 6 hourly, daily and monthly intervals. An ensemble mean and its variance have been computed. we will analyze the range of analysis results at daily and seasonal time scales, and where possible compare with existing observations.

Bosilovich, Michael G.↗
DOE OSTI2024

Three Decades of Wetland Methane Surface Flux Modeling by Earth System Models–Advances, Applications, and Challenges

Earth System Models (ESMs) simulate the exchange of mass and energy between the land surface and the atmosphere, with a key focus on modeling natural greenhouse gas feedbacks. Methane is the second most important greenhouse gas after carbon dioxide. There are growing concerns over the rapidly increasing methane concentration in the atmosphere, underscoring the need for accurate global modeling of its emissions using ESMs. Of the multitude of sources of methane globally, wetlands are the largest natural emitters for methane, leading to significant efforts targeting their representation in ESMs with a special focus on their methane emissions. In this review, we first provide a historical overview of including wetland–methane components in ESMs and how methane modeling approaches have evolved over time. Second, we discuss recent modeling advancements that show promise for improvements in methane emissions predictions, namely the coupling of surface and atmospheric modules of ESMs, the representation of microtopography and transport mechanisms, the resolution of microbial processes at different spatial–temporal scales, and the improved mapping of wetland area extent across the different wetland types. Third, we shed light on the different challenges hindering accurate estimations of wetland–methane emissions, as shown by the consistent discrepancy between bottom–up and top–down models' predictions. Finally, we emphasize that more detailed representation of biogeochemistry and dynamic hydrology while resolving the within–wetland vegetation heterogeneity should improve model predictions, especially when coupled with expanding ground–based measurement networks and high–resolution remote sensing mapping of methane–relevant variables, such as water elevation, water table depth, and methane concentration.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1999

Seasonal-to-Interannual Variability in Antarctic Sea-Ice Dynamics, and Its Impact on Surface Fluxes and Water Mass Production

Strong seasonal and interannual signals in Antarctic bottom-water outflow remain unexplained yet are highly correlated with anomalies in net sea-ice growth in coastal polynyas. The mechanisms responsible for driving salination and replenishment and rejuvenation of the dense shelf "source" waters likely also generate pulses of bottom water outflow. The objective of this research is to investigate time-scales of variability in the dynamics of sea-ice in the Southern Ocean in order to determine the primary sites for production of dense shelf waters. We are using a merged satellite/buoy sea-ice motion data set for the period 1978-present day to compute the dynamics of opening and closing of coastal polynyas over the continental shelf. The Ocean Circulation and Climate Advanced Model (OCCAM) ocean general circulation model with coupled sea-ice dynamics is presently forced using National Center for Environmental Prediction (NCEP) data to simulate fluxes and the salination impact of the ocean shelf regions. This work is relevant in the context of measuring the influence of polar sea-ice dynamics upon polar ocean characteristics, and thereby upon global thermohaline ocean circulation. Interannual variability in simulated net freezing rate in the Southern Weddell Sea is shown for the period 1986-1993. There is a pronounced maximum of ice production in 1988 and minimum in 1991 in response to anomalies in equatorward meridional wind velocity. This follows a similar approximate 8-year interannual cycle in Sea Surface Temperature (SST) and satellite-derived ice-edge anomalies reported elsewhere as the "Antarctic Circumpolar Wave." The amplitude of interannual fluctuations in annual net ice production are about 40% of the mean value, implying significant interannual variance in brine rejection and upper ocean heat loss. Southward anomalies in wind stress induce negative anomalies in open water production, which are observed in passive microwave satellite images. Thus, cycles of enhanced poleward wind stress reduce ice growth by compacting the ice along the coastline and closing open water in leads and polynyas. Model simulations confirm that years of low ice production, such as 1991, coincide with years of lower than normal bottom water outflow. Future plans include the assimilation of satellite ice concentrations and ice drift dynamics to more accurately constrain boundary conditions in the model.

Drinkwater, Mark R.↗
NASA NTRS1999

Soil Surface Runoff Scheme for Improving Land-Hydrology and Surface Fluxes in Simple SiB (SSiB)

Evapotranspiration on land is hard to measure and difficult to simulate. On the scale of a GCM grid, there is large subgrid-scale variability of orography, soil moisture, and vegetation. Our hope is to be able to tune the biophysical constants of vegetation and soil parameters to get the most realistic space-averaged diurnal cycle of evaporation and its climatology. Field experiments such as First ISLSCP Field Experiment (FIFE), Boreal Ecosystem-Atmosphere Study (BOREAS), and LBA help a great deal in improving our evapotranspiration schemes. However, these improvements have to be matched with, and coupled to, consistent improvement in land-hydrology; otherwise, the runoff problems will intrinsically reflect on the soil moisture and evapotranspiration errors. Indeed, a realistic runoff simulation also ensures a reasonable evapotranspiration simulation provided the precipitation forcing is reliable. We have been working on all of the above problems to improve the simulated hydrologic cycle. Through our participation in the evaluation and intercomparison of land-models under the behest of Global Soil Wetness Project (GSWP), we identified a few problems with Simple SiB (SSIB; Xue et al., 1991) hydrology in regions of significant snowmelt. Sud and Mocko (1999) show that inclusion of a separate snowpack model, with its own energy budget and fluxes with the atmosphere aloft and soil beneath, helps to ameliorate some of the deficiencies of delayed snowmelt and excessive spring season runoff. Thus, much more realistic timing of melt water generation was simulated with the new snowpack model in the subsequent GSWP re-evaluations using 2 years of ISLSCP Initiative I forcing data for 1987 and 1988. However, we noted an overcorrection of the low meltwater infiltration of SSiB. While the improvement in snowmelt timing was found everywhere, the snowmelt infiltration has became excessive in some regions, e.g., Lena river basin. This leads to much reduced runoff in many basins as compared to observations. We believe this is a consequence of neglect of the influence of subgrid-scale variations in orography that affects the production of surface runoff.

Sud, Y. C.↗
DOE OSTI2021

Vacuum magnetic fields with exact quasisymmetry near a flux surface. Part 1. Solutions near an axisymmetric surface

While several results have pointed to the existence of exactly quasisymmetric fields on a surface (Garren & Boozer, Phys. Fluids B, vol. 3, 1991, pp. 2805–2821; 2822–2834; Plunk & Helander, J. Plasma Phys. , vol. 84, 2018, 905840205), we have obtained the first such solutions using a vacuum surface expansion formalism. We obtain a single nonlinear parabolic partial differential equation for a function $\eta$ such the field strength satisfies $B = B(\eta )$ . Closed-form solutions are obtained in cylindrical, slab and isodynamic geometries. Numerical solutions of the full nonlinear equations in general axisymmetric toroidal geometry are obtained, resulting in a class of quasihelical local vacuum equilibria near an axisymmetric surface. The analytic models provide additional insight into general features of the nonlinear solutions, such as localization of the surface perturbations on the inboard side. The local solutions thus obtained can be continued globally only for special initial surfaces.

Physics↗
DOE OSTI2020

Full-orbit simulations of fast-ion charge-exchange losses induced by neutral particles outside the plasma last closed flux surface

The interaction between neutrals outside tokamak plasmas and fast ions that are generated by neutral beam injection and pass outside the plasma is studied. It is shown that at beam energies (up to ~100~keV) fast-ion losses are significant, up to 20% in the studied case, because of charge exchange reactions between the neutrals and the fast ions. About half of the fast ions that neutralize outside the plasma get lost to the wall while the other half re-enter the plasma and ionize again, often on better confined orbits which is visible as an enhanced beam power deposition in the plasma core (rho ~< 0.7). As a result, the the plasma performance as measured from the beam-thermal neutrons is hardly changed despite the significant fast-ion losses toward the plasma edge.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗