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At least 91 records · Page 5

Shielding development for the spallation neutron source VENUS instrument

VENUS is a neutron imaging instrument that will use a broad range of neutron wavelengths, from epithermal to cold energies, and will include enhanced contrast mechanisms. It will offer novel energy-selective imaging techniques directly connecting complex engineering materials and systems’ structures, properties, and functions to reveal practical and fundamental answers about their real-world performance. Here, the instrument will be built at SNS beamline 10, facing the decoupled poisoned hydrogen moderator. The driving cost for the instrument is the beamline and instrument cave shielding. Final analyses were performed to evaluate the thickness and composition of shielding materials for the instrument cave and beamline to meet radiation safety criteria for the instrument to start up in 2024 after completing the SNS proton power upgrade.

43 PARTICLE ACCELERATORS

Machine learning at the Spallation Neutron Source accelerator and target

We describe the ongoing efforts to apply Machine Learning techniques to improve the performance of our accelerator and target. Specially, we are looking to minimize halo beam losses in the absence of a proper physics model, automatically detect and log anomalies in the target support systems such as cooling, and detect and prevent errant beam pulses in the linac. We also describe the infrastructure we use to acquire and stream data to the GPU cluster for training, our code development cycle, and edge computing for model inference. To minimize halo beam losses, we use a Reinforcement Learning technique tested on a virtual accelerator. The target anomaly detection is trained on archived data using incomplete physics models and is made part of the existing target reporting system. The errant beam prevention analyzes beam current and beam phase waveforms as well as accelerator configuration data to predict errant pulses. We also develop continual learning to adapt to changes in the accelerator.

Accelerator Physics

Actinides and Neutron Scattering at the Spallation Neutron Source and High Flux Isotope Reactor

The importance of actinides for science, technology, and medicine is widely recognized and does not require a lengthy introduction. However, the fundamental understanding of actinides and their chemical and physical properties lags behind the knowledge of most other elements in the periodic table. Most actinides (89 ≤ Z ≤ 103) are man-made and were produced in particle accelerators or nuclear reactors in the second half of the 20th century. Although trends in bonding and electronic structure are well characterized and documented across the periodic table, fundamental questions remain regarding the chemistry and physics of the actinides. This lack of knowledge is largely because most isotopes of actinides are intensely radioactive, which greatly increases the difficultly in handling them.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS

Spallation Neutron Source Proton Power Upgrade (PPU) Project: Lessons Learned for CD-4

The SNS PPU project goals were to design, build, install and test the equipment necessary to double the accelerator power from 1.4 MW to 2.8 MW and to deliver a 2.0 MW qualified target. PPU also included the provision of a stub-out in the SNS accumulator-ring-to-target tunnel to facilitate a rapid connection to a new proton beamline for the Second Target Station (STS) project. The power capability was doubled by increasing the proton beam energy by 33% and the peak beam current by 50%, relative to pre-PPU accelerator performance. The project also included modifications to some buildings and services. The PPU project accomplished the energy upgrade by fabricating and installing new superconducting radiofrequency (RF) cryomodules, with supporting RF equipment, in the existing linac tunnel and klystron gallery, respectively. The High Voltage Converter Modulators (HVCM) and klystrons for some of the existing installed RF equipment were upgraded to handle the higher beam current. The increased beam power of 2 MW on the First Target Station (FTS) was enabled by the addition of a new high-volume gas injection system for pressure pulse and cavitation mitigation in the mercury target and a redesigned mercury target vessel.

43 PARTICLE ACCELERATORS

Harvesting Isotopically Pure Ac-225 from Ra-225 Produced in Thorium Target Spallation Reaction

A method for isolating Ra-225 from linear accelerator irradiated Th metal chemical processing waste streams has been established. Separating Ra-225 from the complex matrix following proton irradiation of Th metal provides a source of isotopically pure Ac-225 free of the Ac-227 impurity that is present in accelerator-produced Ac-225. Ra isotopes are first separated from the irradiated Th target via cation exchange methods. Importantly, the Ra-containing fraction is cleaned from residual citrate via dilute nitric acid washes (0.5 M) on AG50W-X8 resin. The mixed Ra isotopes are then further purified from Ba-140 impurity using a Sr resin column. Ra elutes through the resin with successive washes of 2.5 M HNO 3 while Ba-140 is retained. Ac-225 is then harvested by loading the Ra content onto an AG50W-X8 cation exchange column where the Ra-225 parent is eluted with 2.5 M HNO 3 before the Ac-225 daughter is eluted with 8 M HNO 3 .

07 ISOTOPE AND RADIATION SOURCES

Elastic plate spallation

The dynamic finite element method was used to investigate elastic stress waves in a plate. Strain displacement and stress strain relations are discussed along with the stiffness and mass matrix. The results of studying point load, and distributed load over small, intermediate, and large radii are reported. The derivation of finite element matrices, and the derivation of lumped and consistent matrices for one dimensional problems with Laplace transfer solutions are included. The computer program JMMSPALL is also included.

Oline, L.

Barites - Anomalous xenon from spallation and neutron-induced reactions

Sedimentary barites from South Africa and Western Australia (about 3 billion years old) contain spallogenic Xe isotopes produced by reactions of Ba with nuclear-active particles in cosmic rays. 'Surface residence time' of these samples was calculated from the observed concentrations of spallogenic Xe-126. Comparison of spallogenic ratios of Xe-131/Xe-126 in the two samples provides evidence for the reaction Ba-130(n, gamma) yields Xe-131, which is characterized by a large number of resonances for neutron absorption in the epithermal region. This observation lends additional support to the conclusions already reached regarding the origin of anomalous Xe-131 in lunar samples.

Srinivasan, B.

Galileo probe thermal protection: Entry heating environments and spallation experiments design

A valid procedure was developed for predicting wall heating and ablation rates about the probe forebody. Entropy layer effects on convective heating rate were analyzed and the computed results are given. A feasibility study to perform an experiment, the selection of a candidate test facility, and the definition of a test matrix are described. The material selection, fabrication, and evaluation of the metal containing carbon-carbon composites for use on the Galileo probe are summarized. The effect of various Jovian atmospheric models on entry heating environment is considered as well as the effect of the nonspherical shape of the planet on entry trajectory.

Balakrishnan, A.

Impact ejection, spallation, and the origin of meteorites

A model for the ejection of material from an impact crater which links ejection velocity, fragment size, and shock pressure through a simplified stress-wave propagation and reflection scheme is presented. It is shown that a small amount of material (0.01 to 0.05 projectile mass) may be ejected at high velocity without suffering petrologically detectable shock pressures. The largest fragments ejected at any velocity are spalls that originate from the target planet's surface. The spall size is proportional to the radius of the primary impactor and the target tensile strength and inversely proportional to ejection velocity. The shock level in the spalls is low, typically half of the dynamic crushing strength of the rock. The model also predicts the aspect ratio of the spalled fragments, the angle of ejection, and the sizes and shock level of other fragments originating deeper in the target. Comparison with observational and experimental data shows generally good agreement.

Melosh, H. J.

Impact spallation experiments - Fracture patterns and spall velocities

The spall velocities produced by nine experimental impacts of 1 to 6.5 km/sec into San Marcos gabbro targets, using projectiles of Fe, Al, Pb, and basalt of various sizes, have been measured in conjunction with fragment-velocity high-speed filmings of the events. A detailed comparison is made between measured spall velocities and those predicted by the model of Melosh (1984), with a view to the compatibility of small-scale results and large planetary impacts. Attention is also given to the patterns of internal fracture generated by impact within the targets.

Polanskey, Carol A.