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At least 91 records · Page 5

Radiation driven Hohlraum using 2 ω for ICF implosions at the NIF

Radiation flux symmetry in laser-irradiated Hohlraum environments is difficult to model and control and relies on the details of plasma evolution and laser energy deposition in the harsh plasma-filled Hohlraum over the duration of the laser pulse. This study presents a conceptual design and assesses the feasibility of using lasers to create a radiation drive where the implosion symmetry relies mainly on radiation transport. In this design, the ends of a capsule containing Hohlraum are irradiated by drive laser beams that are shielded from the view of the capsule. This configuration enables the use of frequency doubled light that has a higher power and energy threshold for the current capability of NIF, up to 670 TW and ∼3.5 MJ. We estimate, using VISRAD benchmarked against HYDRA calculations, that the same drive conditions that are currently being achieved in hybridE experiments at the NIF 270–290 at the equator can be reached in this new geometry and large 6.4 mm diameter Hohlraums. The radiation drive asymmetries in this design can be mitigated by shimming the capsule ablator thickness or through tailoring the shape of the shielding to the laser spots.

Kritcher, A. L. (ORCID:0000000296941088)↗

Multiscale ACI Satellite Database

The SATELLITE_EAGLES_PNNL NetCDF dataset contains a suite of satellite- and reanalysis-derived atmospheric and surface parameters on a regular latitude–longitude grid. The dataset includes core geophysical fields such as land fraction, aerosol optical depth at multiple wavelengths (465, 550, 667, and 865 nm), sea surface temperature, estimated inversion strength, and various thermodynamic and dynamic quantities (e.g., relative humidity, vertical velocity, boundary-layer height, and surface fluxes) from both MERRA and ERA reanalysis products, provided as daily-mean and instantaneous values. A major component of the dataset consists of MODIS-retrieved cloud microphysical properties, including cloud droplet number concentration, cloud effective radius, optical thickness, and liquid water path, provided for three compositing regimes (“All,” “Q06,” and “G18”). Corresponding cloud-top parameters—temperature, height, and pressure—along with total and domain-mean cloud fraction fields are also included. The file further integrates additional satellite data from AMSR-E (for cloud water, rain water, and surface precipitation retrievals) and CERES (for top-of-atmosphere radiative fluxes, cloud fractions, and albedo). This dataset is designed to evaluate aerosol–cloud interactions in warm clouds, emphasizing the use of MODIS for deriving cloud droplet number concentration and liquid water path statistics. The complementary satellite and reanalysis fields are co-located and time-matched to the same instantaneous MODIS observations, enabling consistent comparisons between cloud properties, aerosol loading, and large-scale meteorological conditions. The dataset is recently featured in Christensen et al. (2025), Machine Learning Reveals Strong Grid-Scale Dependence in the Satellite Nd–LWP Relationship, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2025-3850, 2025.

Christensen, Matthew [Pacific Northwest National L↗

Multiscale ACI Satellite Database

The SATELLITE_EAGLES_PNNL NetCDF dataset contains a suite of satellite- and reanalysis-derived atmospheric and surface parameters on a regular latitude–longitude grid. The dataset includes core geophysical fields such as land fraction, aerosol optical depth at multiple wavelengths (465, 550, 667, and 865 nm), sea surface temperature, estimated inversion strength, and various thermodynamic and dynamic quantities (e.g., relative humidity, vertical velocity, boundary-layer height, and surface fluxes) from both MERRA and ERA reanalysis products, provided as daily-mean and instantaneous values. A major component of the dataset consists of MODIS-retrieved cloud microphysical properties, including cloud droplet number concentration, cloud effective radius, optical thickness, and liquid water path, provided for three compositing regimes (“All,” “Q06,” and “G18”). Corresponding cloud-top parameters—temperature, height, and pressure—along with total and domain-mean cloud fraction fields are also included. The file further integrates additional satellite data from AMSR-E (for cloud water, rain water, and surface precipitation retrievals) and CERES (for top-of-atmosphere radiative fluxes, cloud fractions, and albedo). This dataset is designed to evaluate aerosol–cloud interactions in warm clouds, emphasizing the use of MODIS for deriving cloud droplet number concentration and liquid water path statistics. The complementary satellite and reanalysis fields are co-located and time-matched to the same instantaneous MODIS observations, enabling consistent comparisons between cloud properties, aerosol loading, and large-scale meteorological conditions. The dataset is recently featured in Christensen et al. (2025), Machine Learning Reveals Strong Grid-Scale Dependence in the Satellite Nd–LWP Relationship, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2025-3850, 2025.

54 ENVIRONMENTAL SCIENCES↗

Graphite Licensing (ASME) and Testing (ASTM) Technical Assistance

DOE ART Graphite R&D program is currently involved in developing the structural code for licensing the new High Temperature Reactor (HTR) designs through the ASME Boiler Pressure Vessel Code (BPVC). The basic structural design code for graphite core components has been written, approved, and within the BPVC since 2012. However, several areas within the graphite code remain to be improved, specifically the addition of material property changes resulting from environmental degradation (neutron flux and oxidation). The incorporation of this data, which can significantly affect the graphite components and alter the structural integrity of the core during operation, is proving to be an important activity. How this data will be incorporated within the code and how it will be used for license applications will be critical to a number of HTR applicants in the future. These modifications to the code must take into account the unique irradiation and oxidation response of the wide spectrum of available nuclear graphite grades currently under consideration for HTR applications. Additionally, the ASME BPVC requires material property testing within the expected operational conditions of the HTR core including neutron radiation flux, elevated temperatures, and after chronic/acute oxidation of the graphite components. Currently, no standardized graphite testing methods are approved for these environmental conditions. New American Society for Testing and Materials (ASTM) standardized tests for elevated temperature testing, small sample testing, and testing after oxidation must be developed to support the requirements within the ASME code.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Machine learning in nuclear materials research

Nuclear materials are often demanded to function for extended time in extreme environments, including high radiation fluxes with associated transmutations, high temperature and temperature gradients, mechanical stresses, and corrosive coolants. They also have a wide range of microstructural and chemical makeups, resulting in multifaceted and often out-of-equilibrium interactions. Machine learning (ML) is increasingly being used to tackle these complex time-dependent interactions and aid researchers in developing models and making predictions, sometimes with better accuracy than traditional modeling that focuses on one or two parameters at a time. Conventional practices of acquiring new experimental data in nuclear materials research are often slow and expensive, limiting the opportunity for data-centric ML, but new methods are changing that paradigm. Here we review high-throughput computational and experimental data approaches, especially robotic experimentation and active learning that is based on Gaussian process and Bayesian optimization. We show ML examples in structural materials (e.g., reactor pressure vessel (RPV) alloys and radiation detecting scintillating materials) and highlight new techniques of high-throughput sample preparation and characterizations, and automated radiation/environmental exposures and real-time online diagnostics. Herein, this review suggests that ML models of material constitutive relations in plasticity, damage, and even electronic and optical responses to radiation are likely to become powerful tools as they develop. Finally, we speculate on how the recent trends of using natural language processing (NLP) to aid the collection and analysis of literature data, interpretable artificial intelligence (AI), and the use of streamlined scripting, database, workflow management, and cloud computing platforms that will soon make the utilization of ML techniques as commonplace as the spreadsheet curve-fitting practices of today.

36 MATERIALS SCIENCE↗

X-Ray Spectra from General Relativistic Radiation Magnetohydrodynamic Simulations of Thin Disks

We compare X-ray emission from several general relativistic, multifrequency, radiation magnetohydrodynamic simulations of thin black hole accretion disks with different accretion rates and spins. The simulations were performed using the M1 closure scheme, resolved with 12 frequency (energy) bins logarithmically spaced from 5 × 10 −3 to 5 × 10 3 ​​​ keV. We apply a general relativistic Monte Carlo transport code to postprocess the simulation data with greater fidelity in frequency resolution and Compton scattering treatment. Despite the relatively few energy bins and Kompaneets approximation to Compton scattering utilized in the M1 method, we find generally good agreement between the methods. Both produce prominent thermal profiles with peaks around 2–2.5 keV, where agreement is particularly strong and representative of the soft state. Both also find weaker (lower-luminosity) thermally sourced emission extending out to 100 keV due to the hotter innermost regions of the disks. Inverse Compton scattering becomes increasingly effective at hardening spectral outputs with increasing black hole spin, and becomes the dominant mechanism for photons that escape with energies between 10 to several hundred keV. At very high rates of spin, the radiation flux in this upscattered component becomes comparable to the thermal flux, a phenomenon typically associated with intermediate states. Beyond 10 4 keV, we observe faint, free–free emission from hot, optically thin coronal regions developing near the horizon, common to both spinning and nonspinning black holes.

79 ASTRONOMY AND ASTROPHYSICS↗

Examining Cloud Feedback Components in the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM)

Cloud feedback remains the main source of uncertainty in climate sensitivity estimated by global climate models (GCMs), largely because subgrid cloud responses are parameterized in GCMs due to their coarse resolution. Here, this study examines cloud feedback in the global 3.25-km Simple Cloud-Resolving Energy Exascale Earth System Model (E3SM) Atmosphere Model (SCREAM 3 km) through a pair of 1-yr atmosphere-only simulations with control and +4-K sea surface temperature perturbations. SCREAM 3 km produces a positive cloud feedback that falls within but at the upper end of the range of Coupled Model Intercomparison Project phase 5 (CMIP5) and CMIP phase 6 (CMIP6) models and expert judgment. The positive cloud feedback arises from positive contributions from both high- and low-level clouds, with increases in high-cloud altitude and decreases in low-cloud amount and optical depth playing key roles. The stronger-than-CMIP-average feedback is mainly attributable to the high-cloud altitude feedback, owing to cloud tops rising nearly isothermally in SCREAM 3 km. The positive low-cloud amount feedback is weaker in SCREAM than in GCMs because estimated inversion strength (EIS) increases more dramatically with warming. A coarser 12-km resolution version of SCREAM exhibits a weaker positive cloud feedback than SCREAM 3 km, mainly because its low-cloud-radiative flux is more sensitive to EIS, leading to a stronger negative low-cloud amount feedback. With this process-level assessment of cloud feedback, this study reveals where SCREAM aligns with and diverges from conventional GCMs and expert assessment, providing insights to inform further model improvement and future expert assessment.

Cloud radiative effects↗

Improvements to a class of hybrid methods for radiation transport: Nyström reconstruction and defect correction methods

In this study, two modifications are introduced for improving the accuracy, versatility, and robustness of a class of hybrid methods for radiation transport. In general, such methods are constructed by splitting the radiative flux into collided and uncollided components to which low- and high-resolution angular approximations are applied, respectively. In this work we focus on discrete ordinates discretizations of high and low order. The first modification we introduce changes the way in which the collided component is mapped into the uncollided component at the end of each time step in a simulation. The new mapping is a Nyström-type reconstruction that is applicable to arbitrary discrete ordinates quadratures, is guaranteed to preserve positivity of the solution provided that all ordinate weights are positive, is significantly more accurate than previous methods, and can be readily extended to other discretizations such as moment methods, finite element methods, and diffusion approximations. The second modification leverages integral deferred correction (IDC) to iteratively correct for the splitting error introduced by the inconsistency in angular discretization between the collided and uncollided components, in addition to improving the accuracy of the low-order temporal error that is treated by traditional IDC methods. Numerical tests in one- and two-dimensional geometries are used to demonstrate the increased accuracy and efficiency of the proposed modifications. It is found that the two techniques combined yield methods with solution accuracy and memory requirements comparable to that of monolithic discrete ordinates methods while reducing runtime by as much as a factor of between two and ten, depending on the problem.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photochemical reactions on aerosols at West Antarctica: A molecular case-study of nitrate formation among sea salt aerosols

Environmental implications of climate change are complex and exhibit regional variations both within and between the polar regions. The increase of solar UV radiation flux over Antarctica due to stratospheric ozone depletion creates the optimal conditions for photochemical reactions on the snow. Modeling, laboratory, and indirect field studies suggest that snowpack process release gases to the atmosphere that can react on sea salt particles in remote regions such as Antarctica, modifying aerosol composition and physical properties of aerosols. Here, we present evidence of photochemical processing in West Antarctica aerosols using microscopic and chemical speciation of individual atmospheric particles. Individual aerosol particles collected at the Brazilian module Criosfera 1 were analyzed by scanning transmission X-ray microscopy with near edge X-ray absorption fine structure spectroscopy (STXM/NEXAFS) combined with computer controlled scanning electron microscopy (CCSEM) with energy-dispersive X-ray (EDX) microanalysis. The displacement of chlorine relative to sodium was observed over most of the sea salt particles. Particles with a chemical composition consistent with NaCl-NO3 contributed up to 30% of atmospheric particles investigated. Overall, this study provides evidence that the snowpack and particulate nitrate photolysis should be considered in dynamic partition equilibrium in the troposphere. Finally, these findings may assist in reducing modeling uncertainties and present new insights into the aerosol chemical composition in the polar environment.

54 ENVIRONMENTAL SCIENCES↗

Development and Evaluation of Chemistry‐Aerosol‐Climate Model CAM5‐Chem‐MAM7‐MOSAIC: Global Atmospheric Distribution and Radiative Effects of Nitrate Aerosol

Abstract An advanced aerosol treatment, with a focus on semivolatile nitrate formation, is introduced into the Community Atmosphere Model version 5 with interactive chemistry (CAM5‐chem) by coupling the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC) with the 7‐mode Modal Aerosol Module (MAM7). An important feature of MOSAIC is dynamic partitioning of all condensable gases to the different fine and coarse mode aerosols, as governed by mode‐resolved thermodynamics and heterogeneous chemical reactions. Applied in the free‐running mode from 1995 to 2005 with prescribed historical climatological conditions, the model simulates global distributions of sulfate, nitrate, and ammonium in good agreement with observations and previous studies. Inclusion of nitrate resulted in ∼10% higher global average accumulation mode number concentrations, indicating enhanced growth of Aitken mode aerosols from nitrate formation. While the simulated accumulation mode nitrate burdens are high over the anthropogenic source regions, the sea‐salt and dust modes respectively constitute about 74% and 17% of the annual global average nitrate burden. Regional clear‐sky shortwave radiative cooling of up to −5 W m −2 due to nitrate is seen, with a much smaller global average cooling of −0.05 W m −2 . Significant enhancements in regional cloud condensation nuclei (at 0.1% supersaturation) and cloud droplet number concentrations are also attributed to nitrate, causing an additional global average shortwave cooling of −0.8 W m −2 . Taking into consideration of changes in both longwave and shortwave radiation under all‐sky conditions, the net change in the top of the atmosphere radiative fluxes induced by including nitrate aerosol is −0.7 W m −2 .

54 ENVIRONMENTAL SCIENCES↗

Reconstructing High Resolution ESM Data Through a Novel Fast Super Resolution Convolutional Neural Network (FSRCNN)

In this work, we present the first application of a fast super resolution convolutional neural network (FSRCNN) based approach for downscaling earth system model (ESM) simulations. Unlike other SR approaches, FSRCNN uses the same input feature dimensions as the low resolution input. This allows it to have smaller convolution layers, avoiding over-smoothing, and reducing computational costs. We adapt the FSRCNN to improve reconstruction on ESM data, we term the FSRCNN-ESM. We use high-resolution (~0.25°) monthly averaged model output of five surface variables over North America from the US Department of Energy's Energy Exascale Earth System Model's control simulation. These high-resolution and corresponding coarsened low-resolution (~1°) pairs of images are used to train the FSRCNN-ESM and evaluate its use as a downscaling approach. We find that FSRCNN-ESM outperforms FSRCNN and other super-resolution methods in reconstructing high resolution images producing finer spatial scale features with better accuracy for surface temperature, surface radiative fluxes, and precipitation.

58 GEOSCIENCES↗

On the Effect of Historical SST Patterns on Radiative Feedback

Here, we investigate the dependence of radiative feedback on the pattern of sea-surface temperature (SST) change in fourteen Atmospheric General Circulation Models (AGCMs) forced with observed variations in SST and sea-ice over the historical record from 1871 to near-present. We find that over 1871-1980, the Earth warmed with feedbacks largely consistent and strongly correlated with long term climate sensitivity feedbacks (diagnosed from corresponding atmosphere-ocean GCM abrupt 4xCO2 simulations). Post 1980 however, the Earth warmed with unusual trends in tropical Pacific SSTs (enhanced warming in the west, cooling in the east) and cooling in the Southern Ocean that drove climate feedback to be uncorrelated with – and indicating much lower climate sensitivity than – that expected for long-term CO 2 increase. We show that these conclusions are not strongly dependent on the AMIP II SST dataset used to force the AGCMs, though the magnitude of feedback post 1980 is generally smaller in nine AGCMs forced with alternative HadISST1 SST boundary conditions. We quantify a ‘pattern effect’ (defined as the difference between historical and longterm CO 2 feedback) equal to 0.48 ± 0.47 [5-95%] W m -2 K -1 for the time-period 1871-2010 when the AGCMs are forced with HadISST1 SSTs, or 0.70 ± 0.47 [5-95%] W m -2 K -1 when forced with AMIP II SSTs. Assessed changes in the Earth’s historical energy budget agree with the AGCM feedback estimates. Furthermore satellite observations of changes in top-of-atmosphere radiative fluxes since 1985 suggest that the pattern effect was particularly strong over recent decades but may be waning post 2014.

54 ENVIRONMENTAL SCIENCES↗

Regime-specific Cloud Vertical Overlap Characteristics from Radar and Lidar Observations at the ARM sites

Climate and numerical weather prediction models require assumptions to represent the vertical distribution of subgrid-scale clouds, which have radiative transfer implications. In this study, nearly 25 years of ground-based radar and lidar observations of vertical cloud profiles at the Atmospheric Radiation Measurement Program (ARM) Southern Great Plains (SGP) site are utilized to derive cloud vertical overlap characteristics from the Cloud Type (CLDTYPE) data product. Here, the cloud vertical overlap characteristics are further separated by cloud regime by considering seven cloud types (i.e., low cloud, congestus, deep convection, altocumulus, altostratus, cirrostratus, and cirrus) as well as periods of shallow cumulus. The decorrelation length scale (i.e., exponential transition from maximum to random overlap with layer separation) is found to vary by cloud regime, ranging between 0.04 km for cirrostratus paired with cirrus to 4.58 km for low cloud paired with cirrus at SGP. Cloud vertical overlap characteristics are also considered for other ARM sites including the Tropical Western Pacific (TWP), North Slope of Alaska (NSA), and Eastern North Atlantic (ENA) sites amongst other shorter term ARM deployments globally. The decorrelation length scale ranged globally from 1.03 km in the Arctic Ocean to 3.06 km in Manacapuru, Brazil. Globally, the decorrelation length scale by cloud regime exhibited similarities (e.g., for cirrus paired with cirrus) and differences (e.g., congestus paired with cirrus). The results could help inform development of cloud vertical overlap assumptions within operational numerical weather prediction models and potentially improve prediction of radiative fluxes for weather, climate, and renewable energy forecasting.

54 ENVIRONMENTAL SCIENCES↗

Simulating Atmospheric Processes in Earth System Models and Quantifying Uncertainties With Deep Learning Multi‐Member and Stochastic Parameterizations

Abstract Deep learning is a powerful tool to represent subgrid processes in climate models, but many application cases have so far used idealized settings and deterministic approaches. Here, we develop stochastic parameterizations with calibrated uncertainty quantification to learn subgrid convective and turbulent processes and surface radiative fluxes of a superparameterization embedded in an Earth System Model (ESM). We explore three methods to construct stochastic parameterizations: (a) a single Deep Neural Network (DNN) with Monte Carlo Dropout; (b) a multi‐member parameterization; and (c) a Variational Encoder Decoder with latent space perturbation. We show that the multi‐member parameterization improves the representation of convective processes, especially in the planetary boundary layer, compared to individual DNNs. The respective uncertainty quantification illustrates that methods (b) and (c) are advantageous compared to a dropout‐based DNN parameterization regarding the spread of convective processes. Hybrid simulations with our best‐performing multi‐member parameterizations remained challenging and crash within the first days. Therefore, we develop a pragmatic partial coupling strategy relying on the superparameterization for condensate emulation. Partial coupling reduces the computational efficiency of hybrid Earth‐like simulations but enables model stability over 5 months with our multi‐member parameterizations. However, our hybrid simulations exhibit biases in thermodynamic fields and differences in precipitation patterns. Despite this, the multi‐member parameterizations enable improvements in reproducing tropical extreme precipitation compared to a traditional convection parameterization. Despite these challenges, our results indicate the potential of a new generation of multi‐member machine learning parameterizations leveraging uncertainty quantification to improve the representation of stochasticity of subgrid effects.

Behrens, Gunnar [Deutsches Zentrum für Luft‐ und R↗

Exposing and Reducing Biases of Simulating Mixed-Phase Clouds in the Convection-Permitting E3SM Atmosphere Model: Lessons From an Arctic Cold-Air Outbreak

Mixed-phase clouds modulate the water and energy cycles of high-latitude regions, yet their liquid-ice phase partitioning has long been poorly simulated in climate models. Here, simulations of Arctic mixed-phase clouds by the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM) are assessed against large-eddy simulations, satellite data, and ground-based observations during the Cold-Air Outbreaks in the Marine Boundary Layer Experiment field campaign. SCREAM simulates nearly completely frozen clouds, which is attributed largely to the unreasonably strong Wegener–Bergeron–Findeisen (WBF) process that converts liquid to ice excessively and partly to the early over-abundant ice production at cold temperatures from a temperature-deterministic deposition ice nucleation scheme. Assuming no subgrid variation for the WBF process in the original formulation particularly conflicts with the instantaneous saturation adjustment assumption in the condensation scheme that assumes subgrid variability, leading to exaggerated WBF process rates. A proposed simple physically-based improvement on the treatment of subgrid cloud overlap substantially increases supercooled liquid water content and notably improves cloud-top phase partitioning, aligning better with observations. Improvement of supercooled liquid water content also converges with increasing horizontal resolution. The deposition ice nucleation scheme is found responsible for a falsely-produced ice cloud aloft that is not observed, biasing the simulated cloud radiative effects and top-of-atmosphere radiative fluxes. This study identifies key deficiencies in cloud parameterizations that continue to challenge convection-permitting models.

Geosciences↗

Symmetric fielding of the largest diamond capsule implosions on the NIF

We present results for the largest diamond capsule implosions driven symmetrically on the National Ignition Facility (NIF) (inner radius of ~1050 μm) without the use of cross beam transfer in cylindrical Hohlraums. We show that the methodology of designing Hohlraum parameters in a semi-empirical way using an extensive database resulted in a round implosion. In addition, we show that the radiation flux symmetry is well controlled during the foot of the pulse and that swings in P2 symmetry between the inflight dense shell and hot spot are within ±4 μm and that swings around peak compression are also within the symmetry specification of ±4 μm. We observed a stronger dependence of symmetry on the capsule scale than previously observed and also observed enhanced inner beam propagation for experiments using a gas fill density of 0.3 mg/cm 3 and 1000 μm inner radius capsules. We have observed sufficient symmetry and mass remaining at near full NIF power and energy, up to 480 TW and 1.9 MJ, with little laser–plasma interactions (low laser backscattered light) and predict that this design could support extended NIF energy of up to 2.1 MJ.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Evaluation of the Rapid Refresh Numerical Weather Prediction Model over Arctic Alaska

Abstract Despite a need for accurate weather forecasts for societal and economic interests in the U.S. Arctic, thorough evaluations of operational numerical weather prediction in the region have been limited. In particular, the Rapid Refresh Model (RAP), which plays a key role in short-term forecasting and decision-making, has seen very limited assessment in northern Alaska, with most evaluation efforts focused on lower latitudes. In the present study, we verify forecasts from version 4 of the RAP against radiosonde, surface meteorological, and radiative flux observations from two Arctic sites on the northern Alaskan coastline, with a focus on boundary layer thermodynamic and dynamic biases, model representation of surface inversions, and cloud characteristics. We find persistent seasonal thermodynamic biases near the surface that vary with wind direction, and may be related to the RAP’s handling of sea ice and ocean interactions. These biases seem to have diminished in the latest version of the RAP (version 5), which includes refined handling of sea ice, among other improvements. In addition, we find that despite capturing boundary layer temperature profiles well overall, the RAP struggles to consistently represent strong, shallow surface inversions. Further, while the RAP seems to forecast the presence of clouds accurately in most cases, there are errors in the simulated characteristics of these clouds, which we hypothesize may be related to the RAP’s treatment of mixed-phase clouds.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Characterizing the Variation and Covariation of Cloud Microphysical Properties and Implications for Simulation of Subgrid-scale Warm-Rain Processes in Earth System Models (Final DOE-ASR Report)

Warm marine boundary layer (MBL) clouds constitute an important component in the global climate system, and precipitation plays a central role in controlling the water budget, radiative effects, and lifetime of these MBL clouds. Unfortunately, because of the relatively coarse effective grid resolution of the current generation of Earth system models (ESMs), the variety of cloud microphysical processes occurring inside an ESM grid cell are often oversimplified or unconstrained by observations. For example, the warm rain processes (e.g., autoconversion and accretion) are usually parameterized as nonlinear functions of grid-mean cloud properties. Because of the nonlinear nature of these functions, neglecting variability within the ESM grid volume can lead to substantial biases in precipitation production, cloud cover, and surface radiative fluxes. In state-of-the art ESMs, the influence of subgrid-scale variability is represented as an enhancement factor (EF) coefficient to the autoconversion, and accretion rates calculated from the model variables. However, EF is typically taken to be a constant or even used as a knob to tune model cloud properties to match observations, an ad hoc approach that may yield a desired cloud outcome yet introduce compensating errors. In this project, we used the combination of in situ cloud microphysics measurements from the ACE-ENA field campaign and large-eddy simulations (LES) to characterize and understand subgrid-scale variations and co-variations of cloud microphysical properties and use the results to evaluate and improve the representation of subgrid warm-rain processes in ESMs, in particular the EF used to tune the autoconversion and accretion processes. In this final report, we summarize our research activities and main findings in Section 2, provide a list of publications (Section 3) and presentations (Section 4) resulted from our research, and briefly discuss the student activities supported by this project.

54 ENVIRONMENTAL SCIENCES↗