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At least 91 records · Page 5

Inductive Measurement of Plasma Jet Electrical Conductivity (MSFC Center Director's discretionary Fund)

Measurement of plasma jet electrical conductivity has utility in the development of explosively driven magnetohydrodynamic (MHD) energy converters as well as magnetic flux compression reaction chambers for nuclear/chemical pulse propulsion and power. Within these types of reactors, the physical parameter of critical importance to underlying MHD processes is the magnetic Reynolds number, the value of which depends upon the product of plasma electrical conductivity and velocity. Therefore, a thorough understanding of MHD phenomena at high magnetic Reynolds number is essential, and methods are needed for the accurate and reliable measurement of electrical conductivity in high-speed plasma jets. It is well known that direct measurements using electrodes suffer from large surface resistance, and an electrodeless technique is desired. To address this need, an inductive probing scheme, originally developed for shock tube studies, has been adapted. In this method, the perturbation of an applied magnetic field by a plasma jet induces a voltage in a search coil, which, in turn, can be used to infer electrical conductivity through the inversion of a Fredholm integral equation of the first kind. A 1-in.-diameter probe using a light-gas gun. Exploratory laboratory experiments were carried out using plasma jets expelled from 15-g shaped charges. Measured conductivities were in the range of 4 kS/m for unseeded octol charges and 26 kS/m for seeded octol charges containing 2-percent potassium carbonate by mass.

Turner, M. W.↗

DNA damage in oral cancer cells induced by nitrogen atmospheric pressure plasma jets

The nitrogen atmospheric pressure plasma jet (APPJ) was applied to induce DNA damage of SCC-25 oral cancer cells. Optical emission spectra were taken to characterize the reactive species produced in APPJ. In order to explore the spatial distribution of plasma effects, cells were placed onto photo-etched grid slides and the antibody H2A.X was used to locate double strand breaks of DNA inside nuclei using an immunofluorescence assay. The number of cells with double strand breaks in DNA was observed to be varied due to the distance from the irradiation center and duration of plasma treatment.

60 APPLIED LIFE SCIENCES↗

Nanosecond pulsed humid Ar plasma jet in air: shielding, discharge characteristics and atomic hydrogen production

Gas phase non-equilibrium plasmas jets containing water vapor are of growing interest for many applications. In this work, we report a detailed study of an atmospheric pressure nanosecond pulsed Ar + 0.26% H 2 O plasma jet. The plasma jet operates in an atmospheric pressure air surrounding but is shielded with a coaxial argon flow to limit the air diffusion into the jet effluent core. The jet impinges on a metal plate electrode and produces a stable plasma filament (transient spark) between the needle electrode in the jet and the metal plate. The stable plasma filament is characterized by spatially and time resolved electrical and optical diagnostics. This includes Rayleigh scattering, Stark broadening of the hydrogen Balmer lines and two-photon absorption laser induced fluorescence (TaLIF) to obtain the gas temperature, the electron density and the atomic hydrogen density respectively. Electron densities and atomic hydrogen densities up to $5 \times 10^{22}$ ${\rm m}^{-3}$ and $2 \times 10^{22}$ ${\rm m}^{-3}$ have been measured. This shows that atomic hydrogen is one of the main species in high density Ar-H 2 O plasmas. The gas temperature does not exceed 550 K in the core of the plasma. To enable in situ calibration of the H TaLIF at atmospheric pressure a previously published O density calibration scheme is extended to include a correction for the line profiles by including overlap integrals as required by H TaLIF. The line width of H TaLIF, due to collision broadening has the same trend as the neutral density obtained by Rayleigh scattering. This suggests the possibility to use this technique to in situ probe neutral gas densities.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Optical properties of the atmospheric pressure helium plasma jet generated by alternative current (a.c.) power supply

In this work, an atmospheric pressure plasma jet (APPJ) was produced to generate cold flowing post-discharge plasma of pure helium gas. The main aim of this study was to generate cold flowing APPJ of pure helium gas and to determine how their optical emission spectrum change influences varying different flow rates. Lengths of early, middle, and late post-discharge plasma (jet) regions and their fluctuations were determined, respectively. Then, ignition condition dependence of the post-discharge plasma for flow rate was specified at a constant voltage. Spectroscopic studies of an atmospheric pressure plasma jet of helium were presented via analyzing OH, N{sub 2}, N{sub 2}{sup +}, oxygen, and helium intensities for various flow rates.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Atmospheric pressure He-air plasma jet: Breakdown process and propagation phenomenon

In this paper He-discharge (plasma jet/bullet) in atmospheric pressure air and its progression phenomenon has been studied experimentally using ICCD camera, optical emission spectroscopy (OES) and calibrated dielectric probe measurements. The repetitive nanosecond pulse has applied to a plasma pencil to generate discharge in the helium gas channel. The discharge propagation speed was measured from the ICCD images. The axial electric field distribution in the plasma jet is inferred from the optical emission spectroscopic data and from the probe measurement. The correlation between the jet velocities, jet length with the pulse duration is established. It shows that the plasma jet is not isolated from the input voltage along its propagation path. The discharge propagation speed, the electron density and the local and average electric field distribution along the plasma jet axis predicted from the experimental results are in good agreement with the data predicted by numerical simulation of the streamer propagation presented in different literatures. The ionization phenomenon of the discharge predicts the key ionization parameters, such as speed, peak electric field in the front, and electron density. The maximum local electric field measured by OES is 95 kV/cm at 1.3 cm of the jet axis, and average EF measured by probe is 24 kV/cm at the same place of the jet. The average and local electron density estimated are in the order of 10{sup 11} cm{sup -3} and it reaches to the maximum of 10{sup 12} cm{sup -3}.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Characteristics of atmospheric-pressure non-thermal N{sub 2} and N{sub 2}/O{sub 2} gas mixture plasma jet

An atmospheric-pressure non-thermal plasma jet driven by high frequency alternating current and operating on N{sub 2} and N{sub 2}/O{sub 2} gas mixture is investigated. The plasma jet can reach 55 mm in length at a gas flow rate of 2500 l/h. The gas temperature at a distance of 4 mm from the nozzle is close to room temperature. Optical emission spectroscopy is employed to investigate the important plasma parameters such as the excited species, rotational temperature, vibrational temperature, and excitation temperature under different discharge conditions. The results show that the plasma source operates under non-equilibrium conditions. The absolute irradiance intensity of the vibrational band N{sub 2}(C-B) in the active region is measured. Taking into account the irradiance intensity of N{sub 2}(C-B,0-0) and N{sub 2}(B-X,0-0) as well as measured current, the electron density, which is determined by considering direct and step-wise electron impact excitation of nitrogen emission, reaches a maximum value of 5.6 × 10{sup 20}/m{sup 3}.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Magnetized Plasma Target for Plasma-Jet-Driven Magneto-Inertial Fusion

Here, we identify the desired characteristics and parameters of a β>1 magnetized plasma, possibly with highly tangled, open field lines, that could be a suitable target to be compressed to fusion conditions by a spherically imploding plasma liner (Hsu et al. in IEEE Trans Plasma Sci 40:1287, 2012) formed by merging hypersonic plasma jets. This concept is known as plasma-jet-driven magneto-inertial fusion (PJMIF). We set requirements on the target and liner such that (a) compressional heating dominates over thermal transport in the target, and (b) magnetic amplification due to compression dominates over dissipation over the entire implosion. We also evaluate the requirements to avoid drift-instability-induced anomalous transport and current-driven anomalous resistivity in the target. Next, we describe possible approaches to create such a magnetized, β>1 plasma target. Finally, assuming such a target can be created, we evaluate the feasibility of a proof-of-concept experiment using presently achievable plasma jets to demonstrate target compressional heating at a plasma-liner kinetic energy of ≲100kJ (a few hundred times below that needed in a PJMIF reactor).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Temporal and spatial profiles of emission intensities in atmospheric pressure helium plasma jet driven by microsecond pulse: Experiment and simulation

A needle-circular electrode structure helium plasma jet driven by microsecond pulsed power is studied. Spatially resolved emission results show that the emission intensity of He(3{sup 3}S{sub 1}) line decreases monotonically along the axial direction, while those of N{sub 2}(C{sup 3}Π{sub u}), N{sub 2}{sup +}(B{sup 2}∑{sup +}{sub u}), and O(3p{sup 5}P) reach their maxima at 3 cm, 2.6 cm, and 1.4 cm, respectively. The plasma plume of the four species shows different characteristics: The N{sub 2} emission plume travels at a fast speed along the entire plasma jet; the N{sub 2}{sup +} emission plume is composed of a bright head and relatively weak tail and travels a shorter distance than the N{sub 2} emission plume; the He emission plume travels at a slower speed for only a very short distance; propagation of the O emission plume is not observed. Results of calculation of radiation fluxes emitted by positive streamers propagating along helium plasma jets are presented. It is shown, in agreement with the results of the present experiment and with other available experimental data, that the intensities of radiation of N{sub 2}(C{sup 3}Π{sub u}) molecules and He(3{sup 3}S{sub 1}) atoms vary with time (along the plasma jet) quite differently. The factors resulting in this difference are discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Particle-in-cell modeling of plasma jet merging in the large-Hall-parameter regime

The merging process of magnetized plasma jets with parameters relevant to the plasma-jet-driven magneto-inertial fusion (PJMIF) design and the plasma liner experiment (PLX) is modeled by fully kinetic particle-in-cell (PIC) simulations in one and two spatial dimensions. Here, the modified two-stream instability is identified to be the main mechanism responsible for stopping the plasma jets and preventing species interpenetration. The electron and ion Hall parameters of the merged plasma are greater than unity, and the plasma β is close to unity, which is the desired characteristic of planned experiments at PLX. Our 2D PIC simulations validate the results of the radiation magneto-hydrodynamics code FLASH, which will be the primary tool for modeling various stages of future PJMIF experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Role of ambient dielectric in propagation of Ar atmospheric pressure nonequilibrium plasma jets

A single-electrode atmospheric pressure nonequilibrium plasma jet surrounded with different ambient dielectrics is investigated driven by AC power supply. Another three ambient dielectrics, distilled water, ethanol, and carbon tetrachloride, are adopted to compare with air. By examining electrical and optical characteristics, it was found that the molecular polarity of ambient dielectrics had its significant effect on the propagation of atmospheric pressure nonequilibrium plasma jets. When the polarization of molecules was enhanced, the discharge current and the bullet velocity were also increased. For nonpolar dielectric of carbon tetrachloride, this was mainly resulted from the electron polarization in the built-in electric field. For polar dielectrics of ethanol and distilled water, in addition to the electron polarization, orientation polarization was the main cause for the further increase in discharge current and bullet velocity.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Plasma‐driven biocatalysis: In situ hydrogen peroxide production with an atmospheric pressure plasma jet increases the performance of OleT JE when compared to adding the same molar amount of hydrogen peroxide in bolus

Abstract Enzymes like fatty acid peroxygenase OleT JE are desirable enzymes for the industry. While they require inexpensive hydrogen peroxide for activity, the same hydrogen peroxide also causes overoxidation of their reactive heme center. Here, we generate hydrogen peroxide slowly in situ using the Cooperation in Science and Technology (COST)‐Jet, an atmospheric pressure plasma jet, to avoid overoxidizing OleT JE . The COST‐Jet was operated in helium with a water admixture to provide hydrogen peroxide for OleT JE activity. This helium/water admixture produced the highest enzyme turnover numbers after 2 min of treatment. These turnover numbers were even superior to using an equimolar amount of hydrogen peroxide to treat the enzymes exogenously, showing that this plasma source can provide a reliable amount of reaction mediator to support OleT JE activity.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Effects of irradiation distance on supply of reactive oxygen species to the bottom of a Petri dish filled with liquid by an atmospheric O{sub 2}/He plasma jet

The impact of irradiation distances on plasma jet-induced specific effects on the supply of reactive oxygen species (ROS) to the bottom of a Petri dish filled with liquid was investigated using a KI-starch gel reagent that can be employed as a ROS indicator even in water. O{sub 3} exposure experiments without plasma irradiation were also performed to elucidate the specific effects of the plasma jet. Relative concentrations of ROS transported to the bottom were evaluated using absorbance measurements. The results indicated that ROS supply to the bottom is markedly enhanced by the plasma jet irradiation at shorter irradiation distances, whereas similar results could not be obtained for the O{sub 3} exposure. In these cases, the liquid mixing in the depth direction was also enhanced by the plasma jet irradiation only, and the supply of reactive atomic oxygen to the liquid surface was markedly increased as well.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ionization wave propagation in a He plasma jet in a controlled gas environment

Characterizing ionization wave propagation in low temperature plasma jets is critical to predicting production of reactive species and plasma–surface interactions for biomedical applications and surface functionalization. In this work, results from optical emission and laser induced fluorescence measurements of the ionization wave in a He plasma jet operating in a controlled gas environment are discussed and used for comparison with numerical modeling. Additionally, the ionization wave was observed using ICCD (Intensified Charge Coupled Device) imaging and characterized by time and spatially resolved electron density measurements using laser-collision-induced fluorescence. The plasma jet was initially characterized using pure He (nominally at 200 Torr), while varying pressure and voltage. When operating in pure He, the ionization wave broadly expands exiting the plasma tube. Increasing the operating pressure reduces the speed and isotropic expansion of the ionization wave. Furthermore, the jet operated with a humid He shroud was also studied. The humid He shroud results in the electron density increasing and having an annular profile due to the lower ionization potential of H2O compared to He and localized photoionization in the mixing region. Numerical modeling highlighted the importance of resonance radiation emitted by excited states of He, photoelectron emission from the quartz tube, and the kinetic behavior of the electrons produced by photoionization ahead of the ionization front.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The impact of Hall physics on magnetized high energy density plasma jets

Hall physics is often neglected in high energy density plasma jets due to the relatively high electron density of such jets (n{sub e} ∼ 10{sup 19} cm{sup −3}). However, the vacuum region surrounding the jet has much lower densities and is dominated by Hall electric field. This electric field redirects plasma flows towards or away from the axis, depending on the radial current direction. A resulting change in the jet density has been observed experimentally. Furthermore, if an axial field is applied on the jet, the Hall effect is enhanced and ignoring it leads to serious discrepancies between experimental results and numerical simulations. By combining high currents (∼1 MA) and magnetic field helicity (15° angle) in a pulsed power generator such as COBRA, plasma jets can be magnetized with a 10 T axial field. The resulting field enhances the impact of the Hall effect by altering the density profile of current-free plasma jets and the stability of current-carrying plasma jets (e.g., Z-pinches)

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Electrical studies and plasma characterization of an atmospheric pressure plasma jet operated at low frequency

Low-temperature, high-pressure plasma jets have an extensive use in medical and biological applications. Much work has been devoted to study these applications while comparatively fewer studies appear to be directed to the discharge itself. In this work, in order to better understand the kind of electrical discharge and the plasma states existing in those devices, a study of the electrical characteristics of a typical plasma jet, operated at atmospheric pressure, using either air or argon, is reported. It is found that the experimentally determined electrical characteristics are consistent with the model of a thermal arc discharge, with a highly collisional cathode sheet. The only exception is the case of argon at the smallest electrode separation studied, around 1 mm in which case the discharge is better modeled as either a non-thermal arc or a high-pressure glow. Also, variations of the electrical behavior at different gas flow rates are interpreted, consistently with the arc model, in terms of the development of fluid turbulence in the external jet.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Development of a dielectric barrier discharge enhanced plasma jet in atmospheric pressure air

A plasma jet equipped with dielectric barrier discharge (DBD) is developed to generate diffuse air plasma with fairly large gap and cross sectional area. The diffuse air plasma has two discharge modes under different gap widths from the nozzle to the ground plate electrode. For large gap width, a diffuse plume fills the whole space between the nozzle and the plate electrode after coaxial DBD is ignited when the applied voltage reaches a certain value. Rather than diffuse plasma plume, a bright plasma column bridges the nozzle and the plate electrode with further increasing the applied voltage under small gap width. By optical and electrical measurement, results show that the macroscopically diffuse discharge in air is obtained by the superimposition of radially distributed streamers that appear at different cycles of the applied voltage, and the bright plasma column belongs to atmospheric pressure glow discharge. The molecular vibrational temperature and the gas temperature are given as functions of the peak value of the applied voltage.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Electrical and optical properties of Ar/NH{sub 3} atmospheric pressure plasma jet

Inspired by the Penning effect, we obtain a glow-like plasma jet by mixing ammonia (NH{sub 3}) into argon (Ar) gas under atmospheric pressure. The basic electrical and optical properties of an atmospheric pressure plasma jet (APPJ) are investigated. It can be seen that the discharge mode transforms from filamentary to glow-like when a little ammonia is added into the pure argon. The electrical and optical analyses contribute to the explanation of this phenomenon. The discharge mode, power, and current density are analyzed to understand the electrical behavior of the APPJ. Meanwhile, the discharge images, APPJ's length, and the components of plasma are also obtained to express its optical characteristics. Finally, we diagnose several parameters, such as gas temperature, electron temperature, and density, as well as the density number of metastable argon atoms of Ar/NH{sub 3} APPJ to help judge the usability in its applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Time resolved optical emission images of an atmospheric pressure plasma jet with transparent electrodes

We study development of plasma packages in atmospheric pressure plasma jet from their formation as a discharge close to the instantaneous cathode, following their motion between and inside the electrodes up to their emergence at the edge of the glass tube and formation of a plasma bullet. Inside both electrodes, plasma is concentrated close to the walls and is bright, while outside it is located at the axis. This paper opens issues of the geometry of electrodes, fields, and atomic processes, allowing some predictions to be made about pertinent mechanisms.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗