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At least 91 records · Page 5

Zirconium and hafnium in meteorites

The abundances of zirconium and hafnium have been determined in nine stony meteorites by a new, precise neutron-activation technique. The Zr/Hf abundance ratios for the chondrites vary in a rather narrow range, consistent with previously published observations from our group. Replicate analyses of new, carefully selected clean interior samples of the Cl chondrite Orgueil yield mean zirconium and hafnium abundances of 5.2 and 0.10 ppm, respectively. These abundances are lower than we reported earlier for two Cl chondrite samples which we now suspect may have suffered contamination. The new Cl zirconium and hafnium abundances are in closer agreement with predictions based on theories of nucleosynthesis than the earlier data.

Ehmann, W. D.↗

Estimate of contribution of jet aircraft operations to trace element concentration at or near airports

Samples of ASTM type A jet fuel were analyzed for trace element content by instrumental neutron activation techniques. Forty-nine elements were sought. Only ten, aluminum, gold, indium, lanthanum, titanium, vanadium, barium, dysprosium, tellurium, and uranium, were observed at levels above the detection limits encountered; of these only aluminum, titanium, and barium were present at concentrations greater than 0.1 ppm. Estimates of exhaust gas concentrations are made, and the ambient contribution at or near airports is calculated by using the Los Angeles International Airport dispersion model. It is shown that the ambient contribution is about an order of magnitude below typical urban levels for virtually all elements sought.

Fordyce, J. S.↗

Total body calcium analysis using the Ca-12(n, alpha) Ar-37 reaction

A low dose neutron activation technique was developed to measure total body calcium in vivo. The effort had included development of irradiation and processing facilities and conduction of human studies to determine the accuracy and precision of measurement attainable with the systems.

Lewellen, T. K.↗

Derivation of a heterogeneous lithic fragment in the Bovedy L-group chondrite from impact-melted porphyritic chondrules

Results are presented of petrographic, compositional and dating analyses of a light-colored lithic fragment in the L-group Bovedy meteorite that has a composition different from that of the host chondrite. Polished thin sections of the lithic fragment, host, and the fragment-host boundary were examined microscopically and analyzed by electron microprobe, metallic Ni-Fe, and instrumental neutron activation techniques; chips of the fragment were also used for Ar-39/Ar-40 dating and oxygen isotope analyses. The poikilitic textures, olivine, low-Ca pyroxene and kamacite composition and low Na2O, K2O and P2O5 contents of the fragment indicate that it represents a solidified, slightly fractionated impact melt formed from a source rich in porphyritic chondrules. A progressive increase on MgO content across the fragment is accounted for by the heterogeneous nucleation of MgO-rich phases. The Ar data indicate that the Bovedy lithic fragment and its host were partly degassed of radiogenic Ar less than 0.94 billion years ago, probably due to shock. The data are consistent with a cooling rate of about 5 C/million years through 500 C, which must have resulted from the burial of the assemblage beneath insulating material on the parent body at depths of at least several km.

Rubin, A. E.↗

Locating Residual Wax In Coolant Channels

Neutron inspection finds deposits and defects invisible to x rays. Neutron radiography detects many low-density materials even when surrounded by larger quantities of denser materials. Materials with similar properties and densities often appear quite different when viewed by neutron radiography. Technique gives comprehensive view of hidden channels.

Guthrie, Douglas M.↗

Residual thermal strains and stresses in nickel aluminide matrix composites

Thermally induced residual strains and stresses developed during postfabrication cooling in Saphikon/NiAl and tungsten/NiAl high-temperature composites are investigated through three-dimensional elastoplastic finite-element analyses. Average axial and transverse strains in the matrix are found to be tensile and compressive, respectively, and similar for both Saphikon and W-fiber-reinforced NiAl composites. It is suggested that the residual matrix stresses and strains are controlled more by the low-matrix yield stress than by the fiber/matrix expansion mismatch. Residual thermal strains in the matrix of these composites are measured by using a neutron-diffraction technique; the measured axial and transverse strains in the matrix are found to be in agreement with the computed values.

Saigal, A.↗

Classification of mafic clasts from mesosiderites - Implications for endogenous igneous processes

Results are presented from an analysis of 13 igneous pebbles from the Vaca Muerta, EET87500, and Bondoc mesosiderites, using electron microprobe and instrumental neutron activation techniques. These data, combined with literature data on compositions of 43 mesosiderite clasts were used to compile a classification scheme for the various types of mafic silicate clasts that occur in mesosiderites. These clasts were classified into five principal groups: (1) polygenic and monogenic cumulates (30 percent); (2) polygenic basalts (30 percent); (3) quench-textured rocks, comprising two compositional subgroups (those which resemble basaltic eucrites (5 percent), and those which resemble cumulate eucrites (2 percent)); (4) monogenic basalts (11 percent); and (5) ultramafic rocks, consisting mainly of large crystals of orthopyroxene (9 percent) or olivine (4 percent). The conditions under which these clasts were formed are discussed.

Rubin, Alan E.↗

Diffusion model for lightning radiative transfer

A one-speed Boltzmann transport theory, with diffusion approximations, is applied to study the radiative transfer properties of lightning in optically thick thunderclouds. Near-infrared (lambda = 0.7774 micrometers) photons associated with a prominent oxygen emission triplet in the lightning spectrum are considered. Transient and spatially complex lightning radiation sources are placed inside a rectangular parallelepiped thundercloud geometry and the effects of multiple scattering are studied. The cloud is assumed to be composed of a homogeneous collection of identical spherical water droplets, each droplet a nearly conservative, anisotropic scatterer. Conceptually, we treat the thundercloud like a nuclear reactor, with photons replaced by neutrons, and utilize standard one-speed neutron diffusion techniques common in nuclear reactor analyses. Valid analytic results for the intensity distribution (expanded in spherical harmonics) are obtained for regions sufficiently far from sources. Model estimates of the arrival-time delay and pulse width broadening of lightning signals radiated from within the cloud are determined and the results are in good agreement with both experimental data and previous Monte Carlo estimates. Additional model studies of this kind will be used to study the general information content of cloud top lightning radiation signatures.

Koshak, William J.↗

Fabrication and Testing of Micro Flux Monitors in the High Flux Isotope Reactor

Neutron dosimetry is a critical technique to measure the neutron flux, fluence, and energy spectrum of nuclear reactors and can be used to indicate fuel reloading, high-power operations, or changes in cycle length. This work presents results of a novel device named the micro flux monitor, which is a miniaturized neutron dosimeter made from small quantities (100s of nanograms) of Ti, Al, Ni, and Au metals deposited on Si and high-purity fused silica substrates using standard semiconductor fabrication techniques. Approximately 1,250 of these devices were produced, and 40 were irradiated in the pneumatic tube facility of the Neutron Activation Analysis Laboratory at the High Flux Isotope Reactor. Testing demonstrated that dosimeter metals can be deposited predictably and repeatedly in multiple geometries, including as quick response (QR) codes. Neutron flux measurements with these devices were within 3% of measurements made using standard flux monitors, demonstrating the efficacy of these devices. Devices were also tested at 500°C under a N2 atmosphere and showed minimal degradation, suggesting they could be deployed for neutron dosimetry measurements in high-temperature advanced reactors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Survey of in-situ and remote sensing methods for soil moisture determination

General methods for determining the moisture content in the surface layers of the soil based on in situ or point measurements, soil water models and remote sensing observations are surveyed. In situ methods described include gravimetric techniques, nuclear techniques based on neutron scattering or gamma-ray attenuation, electromagnetic techniques, tensiometric techniques and hygrometric techniques. Soil water models based on column mass balance treat soil moisture contents as a result of meteorological inputs (precipitation, runoff, subsurface flow) and demands (evaporation, transpiration, percolation). The remote sensing approaches are based on measurements of the diurnal range of surface temperature and the crop canopy temperature in the thermal infrared, measurements of the radar backscattering coefficient in the microwave region, and measurements of microwave emission or brightness temperature. Advantages and disadvantages of the various methods are pointed out, and it is concluded that a successful monitoring system must incorporate all of the approaches considered.

Schmugge, T. J.↗

Exotic Uses of Neutrons an X-rays as Probes for Chiral Magnets (Early Career Award) (Final Report)

This is the final report for Exotic Uses of Neutrons an X-rays as Probes for Chiral Magnets, an Early Career award to Prof. Dustin Gilbert, University of Tennessee, running 09/01/2020 - 08/31/2025. This project used neutron scattering as a unique tool to investigate magnetic chiral structures. Neutron scattering is a powerful technique in which the neutron wavepacket scatters from nuclear or magnetic structures, providing insight into the structure of a material and its magnetic features. In this work, we focused on chiral magnetic structures. Most magnetic materials are colinear ferro- or antiferromagnets, where the spin moments align parallel or anti-parallel with their neighbors. In some materials, the magnetic moments instead curl and can form closed loops. These structures, with the additional feature that the core and perimeter are oriented in opposite out-of-plane directions, exhibit a property called topology; these structures are known as skyrmions. Topology is a broadly used term, but here it refers to a magnetic configuration that cannot be created or destroyed through any continuous transformation. For these looped structures, the closed loop cannot be destroyed continuously, giving rise to unique properties such as collective dynamics and particle-like behavior. This also raises fundamental questions about how such structures form and evolve.

36 MATERIALS SCIENCE↗

Extrapolation techniques applied to matrix methods in neutron diffusion problems

A general matrix method is developed for the solution of characteristic-value problems of the type arising in many physical applications. The scheme employed is essentially that of Gauss and Seidel with appropriate modifications needed to make it applicable to characteristic-value problems. An iterative procedure produces a sequence of estimates to the answer; and extrapolation techniques, based upon previous behavior of iterants, are utilized in speeding convergence. Theoretically sound limits are placed on the magnitude of the extrapolation that may be tolerated. This matrix method is applied to the problem of finding criticality and neutron fluxes in a nuclear reactor with control rods. The two-dimensional finite-difference approximation to the two-group neutron fluxes in a nuclear reactor with control rods. The two-dimensional finite-difference approximation to the two-group neutron-diffusion equations is treated. Results for this example are indicated.

Mccready, Robert R↗

Observational techniques for solar flare gamma-rays, hard X-rays, and neutrons

The development of new instrumentation and techniques for solar hard X-ray, gamma ray and neutron observations from spacecraft and/or balloon-borne platforms is examined. The principal accomplishments are: (1) the development of a two segment germanium detector which is near ideal for solar hard X-ray and gamma ray spectroscopy; (2) the development of long duration balloon flight techniques and associated instrumentation; and (3) the development of innovative new position sensitive detectors for hard X-ray and gamma rays.

Lin, Robert P.↗

Oscillations of rotating neutron stars

A perturbation technique is used to compute the rotational corrections to the nonradial oscillation spectrum of a realistic neutron star model. The l = l(0) oscillations are coupled to l = l(0) + or - 1 oscillations by the Coriolis force. To calculate the rotational corrections to the quadrupole, l(0) = 2, oscillation modes, previous calculations of the nonradial oscillation spectrum of this neutron star model are extended to include l(0) = 1 and l(0) = 3 modes, as well as many higher overtones at each value of l(o). As an example of this technique, the rotational corrections to two quadrupole toroidal modes are computed. For these modes the coupling to the spheroidal class of oscillations produced by the Coriolis force introduces a nonzero radial component to the velocity field, as well as a nonvanishing Lagrangian density perturbation. This result is used to compute the neutrino damping rates for these toroidal modes of a rotating neutron star. The neutrino damping time can approach the gravitational radiation damping time in rotating neutron stars if the central temperature is high enough. The rotationally induced coupling of spheroidal oscillations to toroidal modes can also produce significant displacements at the stellar surface in some of the toroidal modes. The damping rates due to this process for the rotationally corrected toroidal modes are estimated. The coupling of surface motions to the toroidal modes also have interesting implications for channeling energy, e.g., that associated with a glitch in the crust, to the surface of the star. Perhaps this might produce observable effects in the pulsar emission process or a gamma-ray burst event.

Strohmayer, Tod E.↗

Observation of a Giant Goos-Hänchen Shift for Matter Waves

The Goos-Hänchen (GH) shift describes a phenomenon in which a specularly reflected beam is translated along the reflecting surface such that the incident and reflected rays no longer intersect at the surface. Using a neutron spin-echo technique and a specially designed magnetic multilayer mirror, we have measured the relative phase between the reflected up and down neutron spin states in total reflection. The relative GH shift calculated from this phase shows a strong resonant enhancement at a particular incident neutron wave vector, which is due to a waveguiding effect in one of the magnetic layers. Calculations based on the observed phase difference between the neutron states indicate a propagation distance along the waveguide layer of 0.65 mm for the spin-down state, which we identify with the magnitude of the giant GH shift. The existence of a physical GH shift is confirmed by the observation of neutron absorption in the waveguide layer. Here, we propose ways in which our experimental method may be exploited for neutron quantum-enhanced sensing of thin magnetic layers.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Nuclear activation analysis of zirconium-90 isomeric and ground-state reactions at the OMEGA Laser Facility

Nuclear activation is a well-established technique for inferring neutron yields in laser direct-drive deuterium–tritium (DT) and deuterium–deuterium (D 2 ) implosions at the OMEGA Laser Facility. Zirconium has long been considered an excellent candidate for measuring DT neutron fusion yields by observing decays of the 90 Zr(n,2n) 89 Zr ground-state reaction. As it has a higher energy threshold than present activation detectors utilizing copper, zirconium provides a means to infer primary neutron yields that are less susceptible to being skewed due to neutron scattering within the experimental environment. However, with a 78.41-h half-life, it is not operationally practical to utilize this reaction for OMEGA experiments, which have a 1-h shot cycle. Zirconium’s 90 Zr(n,2n) 89 mZr reaction presents itself as a viable candidate to infer neutron yields within a shot cycle, given its half-life of 4.16 min. Here, we present an overview of the approach and methodology, utilizing first principles techniques, to infer the primary neutron yields from OMEGA DT fusion experiments by using both the isomeric and the ground-state reaction. Yields inferred from both reactions are compared, which are in good agreement between the two.

Activation analysis↗