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DOE OSTI2020

Neutrino signal from proto-neutron star evolution: Effects of opacities from charged-current–neutrino interactions and inverse neutron decay

In this work, we investigate the impact of charged-current–neutrino processes on the formation and evolution of neutrino spectra during the deleptonization of proto-neutron stars. To this end we develop the full kinematics of these reaction rates consistent with the nuclear equation of state, including weak magnetism contributions. This allows us to systematically study the impact of inelastic contributions and weak magnetism on the $ν_e$ and $\bar{ν}_e$ luminosities and average energies. Furthermore, we explore the role of the inverse neutron decay, also known as the direct Urca process, on the emitted spectra of $\bar{ν}_e$. This process is commonly considered in the cooling scenario of cold neutron stars but has so far been neglected in the evolution of hot proto-neutron stars. We find that the inverse neutron decay becomes the dominating opacity source for low-energy $\bar{ν}_e$. Accurate three-flavor Boltzmann neutrino transport enables us to relate the magnitude of neutrino fluxes and spectra to details of the treatment of weak processes. This allows us to quantify the corresponding impact on the conditions relevant for the nucleosynthesis in the neutrino-driven wind, which is ejected from the proto-neutron star surface during the deleptonization phase.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Resolving Neutron Transport with the CoGNAC Neutron Scattering Program at LANSCE [Poster]

Neutron Scattering Defines Neutron Transport. Elastic (n,n) and inelastic (n,n'γ) reactions dictate the neutronic energy flow. Each scattering reaction changes neutron direction $\vartheta$ and energy E. Scattering cross sections and angular distributions are essential for neutron transport. Uncertainties on scattering evaluations and measurements dominate total uncertainties. New, high-precision neutron scattering measurements and evaluations are needed from light elements to actinides

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

239 Pu R -matrix Analysis and Neutron Multiplicities in the Neutron Energy Region up to a few keVs [Abstract]

The evaluation of 239 Pu neutron resonance parameters coupled to neutron multiplicities $\overline{v}_p$ is of particular importance to investigate the ($\mathcal{n, γf}$) reaction in which a $\mathcal{γ}$-ray emission occurs before the scission of the compound nuclear. This reaction has offered one explanation for the fluctuations in the measured values of $\overline{v}_p$ In this regard, the competition between ($\mathcal{n, γf}$) reaction and the direct fission process can be also included in the R matrix analysis of fission and capture measured data. The goal of this work is the coupled evaluation of the $\mathcal{n}$+ 239 Pu resonance parameters and related neutron multiplicities by ensuring the adoption of thermal neutron constants recently evaluated at the International Atomic Nuclear Energy as well as the recommended (thermal-neutron) induced prompt neutron fission spectrum (PFNS). Moreover, this new set of physical evaluated quantities should also guarantee the agreement for high-leakage solution benchmarks while keeping the good performance of large thermal solution assemblies.

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2022

Two bright, optically clear, intrinsic fast-neutron and charged-particle detector materials for neutron imaging and other applications

Two optically clear, bright, scintillating ZnS materials have been identified that, like previous opaque ZnS scintillators, are excellent charged particle detectors. We show that ZnS is a good fast-neutron-to charged-particle converter making optically clear ZnS an intrinsic fast-neutron detector that does not require layering or mixing of converter materials and scintillator materials, and removes the limitations imposed by opaque ZnS scintillator materials used for more than a century. Thermal neutron detection using optically clear 6 LiF or 10 BN and clear ZnS may benefit from improved spatial resolution and light transmission. Properties and tests of clear scintillating ZnS are described. Fast-neutron imaging applications benefit from increased efficiency of these scintillators, minimal scattering in the scintillator, and increased useful detector volume. Charged particle and fast-neutron detectors have numerous applications in nuclear non-proliferation and security, nuclear and particle physics, and non-destructive testing and environmental measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2021

Verification and Validation Tests of Gamma Library of MC2-3 for Coupled Neutron and Gamma Heating Calculation

For the accurate assessment of the heat generation rate in fast reactors, the gamma library of MC2 -3 and the MC2 -3 + GAMSOR procedure employing the coupled neutron and gamma heating calculation has been thoroughly verified against Monte Carlo results and validated using the ZPPR-15D gamma dose measurement data. NJOY outputs are post-processed in a consistent way with the NJOY procedure to avoid any missing data or double counting of data. Prompt heating for 379 out of 391 isotopes in the gamma library was verified against MCNP6.2 to within 1% relative error in total heating for most isotopes. For both a simple one-dimensional slab problem representing a sodium cooled fast reactor and the Experimental Breeder Reactor II (EBR-II) benchmark problem, the root-mean-square values of assembly power error were less than 0.5% for fuel assemblies, ~1% in blankets and ~1 to ~3% in reflectors compared to MCNP6.2 results. The most plausible cause for the 3% error in a reflector assembly is believed to be the error in the multigroup neutron cross sections for the reflector assembly. For validation, gamma doses measured with thermoluminiscent dosimeters (TLDs) in the ZPPR-15D experiment were calculated using GAMSOR. Due to the uncertainty in the TLD measurement with regards to the energy deposition of photons and neutrons, the validation data leads to a 12.7% uncertainty on the experimental measurement. With this uncertainty bound, the calculated doses all fell within one standard deviation of the measured value. Combined with the accurate calculation of reaction rate distributions and neutron spectrum measurements, these results indicate good agreement for the neutron and gamma heating calculations that were performed.

coupled neutron and gamma heating↗

DOE OSTI2026

Effect of a transparent water-cooled cathode on the neutron production rate in the glow discharge-type fusion neutron source

In glow discharge-type deuterium–deuterium fusion neutron sources, fusion reactions occurring on the cathode surface contribute significantly to the neutron production rate (NPR); therefore, cathode design plays a crucial role in enhancing NPR. Although the NPR generally increases with discharge current, deuterium desorption caused by cathode heating tends to stagnate it in the high-current regime. Water cooling has been shown to mitigate this stagnation for nontransparent cathodes, but its effectiveness for transparent cathodes has not been experimentally clarified. Here, in this study, a transparent cathode with active water cooling and a spherical geometry was designed and fabricated using stainless steel tubing. Neutron production experiments were conducted with and without water cooling: with water cooling, applied voltages of 20–40 kV were investigated, while without water cooling, the applied voltage was limited to 25 kV. The results showed that the NPR increased continuously with discharge current without stagnation when water cooling was applied. A maximum NPR of (1.8 ± 0.02) × 10 6 n/s was achieved at 40 kV and 50 mA. Compared with our previously reported disk cathode and nontransparent water-cooled cathode of the same diameter, the transparent water-cooled cathode exhibited a significantly enhanced NPR. These findings indicate that combining cathode transparency with active cooling is an effective strategy for improving neutron production in glow discharge-type fusion neutron sources.

43 PARTICLE ACCELERATORS↗

DOE OSTI2021

Understanding the effects of neutron scattering for neutron-yield-isotropy measurements at the NIF

Neutron-yield diagnostics at the NIF have been upgraded to include 48 detectors placed around the NIF target chamber to assess the DT-neutron-yield isotropy for inertial confinement fusion experiments. Real-time neutron-activation detectors are used to understand yield asymmetries due to Doppler shifts in the neutron energy attributed to hotspot motion, variations in the fuel and ablator areal densities, and other physics effects. In order to isolate target physics effects, we must understand the contribution due to neutron scattering associated with the different hardware configurations used for each experiment. Here, we present results from several calibration experiments that demonstrate the ability to achieve our goal of 1% or better precision in determining the yield isotropy.

47 OTHER INSTRUMENTATION↗

DOE OSTI2022

CENTAUR - The small- and wide-angle neutron scattering diffractometer/spectrometer for the Second Target Station of the Spallation Neutron Source

CENTAUR has been selected as one of the eight initial instruments to be built at the Second Target Station (STS) of the Spallation Neutron Source at Oak Ridge National Laboratory. It is a small-angle neutron scattering (SANS) and wide-angle neutron scattering (WANS) instrument with diffraction and spectroscopic capabilities. This instrument will maximally leverage the high brightness of the STS source, the state-of-the-art neutron optics, and a suite of detectors to deliver unprecedented capabilities that enable measurements over a wide range of length scales with excellent resolution, measurements on smaller samples, and time-resolved investigations of evolving structures. Notably, the simultaneous WANS and diffraction capability will be unique among neutron scattering instruments in the United States. This instrument will provide much needed capabilities for soft matter and polymer sciences, geology, biology, quantum condensed matter, and other materials sciences that need in situ and operando experiments for kinetic and/or out-of-equilibrium studies. Beam polarization and a high-resolution chopper will enable detailed structural and dynamical investigations of magnetic and quantum materials. CENTAUR’s excellent resolution makes it ideal for low-angle diffraction studies of highly ordered large-scale structures, such as skyrmions, shear-induced ordering in colloids, and biomembranes. Additionally, the spectroscopic mode of this instrument extends to lower momentum transfers than are currently possible with existing spectrometers, thereby providing a unique capability for inelastic SANS studies.

47 OTHER INSTRUMENTATION↗

DOE OSTI2023

Characterization of D-T Generator Neutron Flux Spectrum for Cyclic Neutron Activation Analysis Experiments

Improving nuclear data for short-lived fission product yields will further our fundamental understanding of fission, which is needed across various scientific fields and applications. One method of attaining the needed product yield data is through cyclic neutron activation, which allows a target to be irradiated in a neutron environment and then transported for counting of the radionuclides produced, typically via g spectroscopy. Recently, such a system has been constructed and commissioned at Pacific Northwest National Laboratory. Targets are shuttled between the head of a D-T neutron generator and a counting station with a transit time of 2 seconds. As part of the characterization of this system, the neutron flux was studied using two activation targets. The neutron flux from the deuterium-tritium fusion generator was determined to be 9.95(33) x10^8 n/cm2-s with a peak energy of 14.9 MeV and a spread of approximately 4 decades between the epithermal and 14 MeV peak group flux.

cyclic neutron activation, gamma-ray spectroscopy,↗

DOE OSTI2026

Neutron skins probed in proton knockout from neutron-rich nuclei

Proton-induced quasifree knockout reactions provide a powerful probe of nuclear single-particle structure and reaction dynamics in both stable and neutron-rich nuclei. Here, in this work, we develop a unified theoretical framework for the calculation of inclusive (𝑝, 2⁢𝑝) and sequential (𝑝, 3⁢𝑝) reaction cross sections and fragment momentum distributions at intermediate and relativistic energies. The approach is based on a probabilistic extension of Glauber multiple-scattering theory combined with microscopic nuclear densities obtained from Hartree-Fock-Bogoliubov calculations using Skyrme energy-density functionals. We focus in particular on the sensitivity of total cross sections and longitudinal momentum dispersions to neutron-skin thickness along isotopic chains. Our results indicate that both (𝑝, 2⁢𝑝) and (𝑝, 3⁢𝑝) reactions exhibit a systematic decrease of cross section and momentum width with increasing neutron excess, reflecting enhanced attenuation and surface bias induced by neutron skins. The effect is significantly stronger for two-proton removal, suggesting that (𝑝, 3⁢𝑝) reactions may offer enhanced sensitivity to isovector nuclear structure. These findings establish proton-induced knockout reactions as complementary hadronic probes of neutron skins and the density dependence of the nuclear symmetry energy.

direct reactions↗

DOE OSTI2025

Performance Characterization of FB-Line Neutron Multiplicity Counter and Large Neutron Multiplicity Counter

Savanah River National Laboratory’s (SRNL) Nuclear Measurements group was tasked with characterizing the performance of two neutron multiplicity counters located at SRNL. Characterization measurements were made to determine the gate width, pre-delay, deadtime parameters, triples and doubles gate fractions, detector efficiency, and operating high voltage for the Large Neutron Multiplicity Counter (LNMC) and the FB Line Neutron Multiplicity Counter (FBLNMC). The parameters were determined, shown below, and were, as to be expected, slightly different than the previous calibrations, which were performed over 20 years ago. Several Pu samples were measured to validate the characterizations of the FBLNMC and LNMC. The measurements determined the sample Pu-240 mass within <2% deviation for the pure plutonium samples and ~8% for the mixed oxide sample. The pure Pu samples had significantly better accuracy compared with the impure mixed oxide sample due to the lack of induced fission or alpha,n neutrons from impurities. Overall, the characterization of the neutron multiplicity counters, and the determination of their operability has been completed successfully.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2021

Damage development in neutron-irradiated concrete in a test reactor: Hygro-thermal and mechanical simulations

This paper reports the development of a 3D mesoscale hygro-thermal-mechanical simulation approach to predict damage in concrete irradiated in a test reactor. This framework, developed in MOOSE, considers the effects of elevated temperature, moisture content, and high neutron fluence (energy threshold, E > 0.1 MeV) on the mortar and aggregates separately. The first-stage simulation implements hygro-thermal analysis to determine the temperature and RH inside the specimen as a function of imposed radiation energy. These are used as inputs to the second stage, which considers radiation-induced volumetric expansion (RIVE) of aggregates, and creep, shrinkage, and stress-strain response of mortar to predict the expansion, stresses, and damage in specimens made using different coarse aggregates and subjected to different irradiation times. The irradiation time-dependent damage in the mortar is expressed using an isotropic damage parameter. This multi-physics model serves as a predictive tool for damage quantification in concrete due to neutron irradiation.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Microgravity crystallization of perdeuterated tryptophan synthase for neutron diffraction

Abstract Biologically active vitamin B 6 -derivative pyridoxal 5′-phosphate (PLP) is an essential cofactor in amino acid metabolic pathways. PLP-dependent enzymes catalyze a multitude of chemical reactions but, how reaction diversity of PLP-dependent enzymes is achieved is still not well understood. Such comprehension requires atomic-level structural studies of PLP-dependent enzymes. Neutron diffraction affords the ability to directly observe hydrogen positions and therefore assign protonation states to the PLP cofactor and key active site residues. The low fluxes of neutron beamlines require large crystals (≥0.5 mm 3 ). Tryptophan synthase (TS), a Fold Type II PLP-dependent enzyme, crystallizes in unit gravity with inclusions and high mosaicity, resulting in poor diffraction. Microgravity offers the opportunity to grow large, well-ordered crystals by reducing gravity-driven convection currents that impede crystal growth. We developed the Toledo Crystallization Box (TCB), a membrane-barrier capillary-dialysis device, to grow neutron diffraction-quality crystals of perdeuterated TS in microgravity. Here, we present the design of the TCB and its implementation on Center for Advancement of Science in Space (CASIS) supported International Space Station (ISS) Missions Protein Crystal Growth (PCG)-8 and PCG-15. The TCB demonstrated the ability to improve X-ray diffraction and mosaicity on PCG-8. In comparison to ground control crystals of the same size, microgravity-grown crystals from PCG-15 produced higher quality neutron diffraction data. Neutron diffraction data to a resolution of 2.1 Å has been collected using microgravity-grown perdeuterated TS crystals from PCG-15.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2026

Collision Tracking in OpenMC: Methods and Applications in Neutron Noise, Neutron Imaging, Time-of-Flight, and Multiplicity Counting

We present the development and application of a collision tracking feature within the OpenMC Monte Carlo particle transport code, designed for diverse applications such as neutron spectroscopy, scatter camera system, neutron noise, and multiplicity counting simulations. This feature enables the tracking of individual particle collisions, with potential applications in nuclear nonproliferation, reactor physics, and nuclear security. Additionally, the feature holds potential for the calibration of neutron detectors, specifically in converting light output into energy deposited within the detectors. The implementation consists of a set of filters—such as reaction type, energy, cell, and material—that constrain the set of collisions that are tracked, extensions to the Python API to enable simple input specification, and support for writing either OpenMC’s native HDF5-based format or the Monte Carlo particle list format. This feature was added to the official OpenMC release in version 0.15.3. In this work, the feature will be applied to showcase scenarios such as time-of-flight simulations, scatter-camera imaging for neutron source localization, neutron-noise analysis to extract integral kinetic parameters such as the prompt decay constant α, and multiplicity counting to estimate the mass of special nuclear materials. Ultimately, this feature aims to expand the application scope of open-source Monte Carlo particle transport codes such as OpenMC.

Monte Carlo code↗

DOE OSTI2025

Model Development and Analysis of a High-Fidelity Neutron Transport Sensor: The Quadrupole Detector Concept for Measurement of the Neutron Flux Gradient

Accurate reconstruction of the neutron flux distribution within a reactor core is essential for safe and efficient reactor operation. Traditional power shape synthesis in Light Water Reactors relies on hundreds of in-core detectors. However, this approach becomes impractical for Advanced Reactors and Microreactors due to limited space and harsh environments. To address this challenge, we propose a data-driven methodology that combines high-fidelity modeling with real-time ex-core sensor measurements, enabling the reconstruction of core power distribution while minimizing the reliance on intrusive in-core instrumentation. This project began in FY24 and achieved two initial milestones: (1) the definition of a three-year development plan for a Digital Twin framework and (2) the development of high-fidelity neutronics models of the Purdue University Reactor One (PUR-1) using both MCNP6 and OpenMC. The PUR-1 reactor, a zero-power facility, was selected due to its suitability for neutronics-focused modeling and the availability of experimental data for validation. Both models were benchmarked using neutron flux measurements obtained from irradiated gold foils, which were strategically placed within the core during a dedicated campaign in July 2024. This report marks the continuation and completion of those foundational tasks. The OpenMC model has been refined (improved geometric accuracy, expanded cross-section libraries, and refined sampling) and validated using additional experimental data. An updated sensor design—based on quadrupole configuration—was designed to measure both ex-core flux and its spatial gradient. These measurements will serve as inputs to a neural network-based reconstruction algorithm. Finally, the methodology was demonstrated on a two-dimensional test case representative of the heterogeneous material composition of the PUR-1 reactor core. A neural network implementation of the Kirchhoff-Helmholtz integral equation was employed to solve the boundary value problem using peripheral sensor measurements. The preliminary results confirm the strong potential of the proposed approach for accurate and minimally invasive neutron flux reconstruction.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2021

The Relative Contribution to Heavy Metals Production from Binary Neutron Star Mergers and Neutron Star–Black Hole Mergers

The origin of the heavy elements in the universe is not fully determined. Neutron star–black hole (NSBH) and binary neutron star (BNS) mergers may both produce heavy elements via rapid neutron-capture (r-process). We use the recent detection of gravitational waves from NSBHs, improved measurements of the neutron star equation of state (EoS), and the most modern numerical simulations of ejected material from binary collisions to measure the relative contribution of NSBHs and BNSs to the production of heavy elements. As the amount of r-process ejecta depends on the mass and spin distribution of the compact objects, as well as on the EoS of the neutron stars, we consider various models for these quantities, informed by gravitational-wave and pulsar data. We find that in most scenarios, BNSs have produced more r-process elements than NSBHs over the past 2.5 billion years. If black holes have preferentially small spins, BNSs can produce at least twice the amount of r-process elements than NSBHs. If black hole spins are small and there is a dearth of low-mass (<5M ⊙ ) black holes within NSBH binaries, BNSs can account for the near totality of the r-process elements from binaries. For NSBH to produce a large fraction of r-process elements, black holes in NSBHs must have small masses and large aligned spins, which is disfavored by current data.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Development of Large-Volume-Diamond Anvil Cell for Neutron Diffraction: The Neutron Diamond Anvil Cell Project at ORNL

10 years ago, Dave Mao, director of EFree (energy frontier research in extreme environments), a DOE energy frontier recognized the importance of neutron science for energy research. The subsequent establishment of a neutron group within EFree lead to the establishment of an “Instrument Development Team” for SNAP, the High-Pressure beamline at the Spallation Neutron Source at Oak Ridge National Laboratory in Tennessee. The idea was to develop novel high pressure techniques to expand the pressure range for neutron diffraction. A goal was set to reach half megabar levels (50 GPa), which at the time was considered as extremely challenging. Here we will give a brief overview of the developments during the last decade in this novel area of research. Fortunately, during this period multi carat diamond anvils have become available mainly by the chemical vapor deposition process (CVD), making research in this pressure range and beyond rather routine. This paper shows the latest developments in large anvil designs, compact multiple ton diamond cells and some examples of high-quality neutron diffraction patterns of sample sizes far below conventional levels.

Boehler, Reinhard↗

DOE OSTI2021

Microstructure and water absorption of ancient concrete from Pompeii: An integrated synchrotron microtomography and neutron radiography characterization

There is renewed interest in using advanced techniques to characterize ancient Roman concrete due to its exceptional durability and low-carbon footprint. In the present work, samples were drilled from the “Hospitium” in Pompeii and were analyzed by synchrotron microtomography (μCT) and neutron radiography to study how the microstructure, including the presence of induced cracks, affects their water adsorption. The water distribution and absorptivity were quantified by neutron radiography. The 3D crack propagation, pore size distribution and orientation, tortuosity, and connectivity were analyzed from μCT results using advanced imaging methods. Porosity was also measured by mercury intrusion porosimetry (MIP) as a reference. Ductile fracture patterns were observed once cracks were introduced. Compared to Portland cement mortar/concrete, the Pompeii samples had relatively high porosity, low connectivity, and a similar coefficient of capillary penetration. In addition, permeability was predicted from models based on percolation theory and pore structure data to evaluate the fluid transport properties. Understanding the microstructure of ancient Pompeii concrete is important because it could inspire the development of modern concrete with high durability.

36 MATERIALS SCIENCE↗