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At least 91 records · Page 5
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Comparison of the Distribution of the In Situ Ring Current Density Based on Magnetic Field Observations From THEMIS, MMS and Cluster

Abstract We review and extend previous work on the ring current density distribution by applying the curlometer technique to multi‐spacecraft magnetic field data on different spatial scales, directly comparing the results of three space missions: Time History of Events and Macroscale Interactions during Substorms (THEMIS), The Magnetospheric Multiscale (MMS) and Cluster, that have so far accrued decades of data on a range of spatial separation scales. We suggest that the statistical results of Cluster data over two decades can illustrate well the overall form of the ring current (in the ring plane), but can underestimate the current density, while THEMIS (partially) and MMS are able to observe the detailed structure of the ring current and indeed show different behavior on some (smaller) spatial scales. These results suggest that, in addition to the local time and radial form, reported previously, the morphology of the ring current may also depend on magnetic latitude, as influenced by the tilt angle between the inner and outer magnetic fields.

Tan, X. [School of Space and Earth Sciences Beihan↗
DOE OSTI2020

Logical gates embedding in artificial spin ice

The realization and study of arrays of interacting magnetic nanoislands, such as artificial spin ices, have reached mature levels of control that allow design and demonstration of exotic, collective behaviors not seen in natural materials. Advances in the direct manipulation of their local, binary moments also suggest a use as nanopatterned, interacting memory media, for computation within a magnetic memory. Recent experimental work has demonstrated the possibility of building logic gates from clusters of interacting magnetic domains, and yet the possibility of large scale integration of such gates can prove problematic even at the theoretical level. Here we introduce theoretically complete sets of logical gates, in principle realizable in an experiment, and we study the feasibility of their integration into tree-like circuits. By evaluating the fidelity control parameter between their collective behavior and their expected logic functionality we determine conditions for integration. Also, we test our numerical results against the presence of disorder in the couplings, showing that the design gate structure is robust to small coupling perturbations, and thus possibly to small imperfections in the fabrication of the islands.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Long-range three-dimensional magnetic structures of the spin S =1 hexamer cluster fedotovite-like A 2 Cu 3 O ( SO 4 ) 3 ( A 2 = K 2 , NaK, Na 2 ): A neutron diffraction study

The crystal and magnetic structures of the spin S = 1 hexamer cluster fedotovite-like A 2 Cu 3 O(SO 4 ) 3 (A 2 = K 2 , NaK, Na 2 ) were studied by neutron powder diffraction at temperatures 1.6–290 K. The crystal structures in all compounds are well refined in the monoclinic space group C2/c. The basic magnetic units of the compounds are copper hexamers, which are coupled by weak superexchange interactions giving rise to three-dimensional long-range magnetic order below 3.0 < T N < 4.7 K. We have found that for A 2 = K 2 and NaK the propagation vector of the magnetic structure is k = [0,0,0], and the coupling of the Cu hexamers is ferromagnetic (FM) along the ab diagonal and antiferromagnetic along the bc diagonal. In contrast, for A = Na the propagation vector is k = [0,1,0], and the Cu hexamers are coupled antiferromagnetically (AFM) along the ab diagonal. Further, the hexamers are formed by three Cu pairs arranged along the b axis. The calculated spin expectation values $\langle s \rangle$ for the simplest symmetric spin Hamiltonian (obtained from inelastic neutron spectroscopy) of the isolated hexamers in the mean field amounted to $\langle s \rangle$ = 3/8 for the side spins Cu1 and Cu2 and $\langle s \rangle$ = 1/4 for Cu3 in the middle. The Cu spins are FM coupled in pairs and AFM between neighboring pairs. The experimental magnetic moments of the Cu 2+ ions turn out to be not completely collinear due to spin frustrations within the weak interhexamer interactions. The sizes of magnetic moments of Cu in the hexamers determined from the diffraction data are in fair agreement with the calculated values.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Filaments in and between galaxy clusters at low and mid-frequency with the SKA

Context. Understanding the magnetised Universe is a major challenge in modern astrophysics, and cosmic magnetism has been acknowledged as one of the key scientific drivers of the most ambitious radio instrument ever planned, the Square Kilometre Array. Aims. With this work, we aim to investigate the potential of the Square Kilometre Array and its precursors and pathfinders in the study of magnetic fields in galaxy clusters and filaments through diffuse synchrotron radio emission. Galaxy clusters and filaments of the cosmic web are indeed unique laboratories in which to investigate turbulent fluid motions and large-scale magnetic fields in action, and much of what is known about magnetic fields in galaxy clusters comes from sensitive radio observations. Methods. Based on cosmological magneto-hydrodynamic simulations, we predict radio properties (total intensity and polarisation) of a pair of galaxy clusters connected by a cosmic-web filament. Results. We use our theoretical expectations to explore the potential of polarimetric observations to study large-scale structure magnetic fields in the frequency ranges 50–350 MHz and 950–1760 MHz. We also present predictions for galaxy cluster polarimetric observations with the Square Kilometre Array precursors and pathfinders, such as the LOw frequency ARray 2.0 and the MeerKAT+ telescope. Conclusions. Our findings point out that polarisation observations are particularly powerful for the study of large-scale magnetic fields, since they are not significantly affected by confusion noise. The unprecedented sensitivity and spatial resolution of the intermediatefrequency radio telescopes make them the favourite instruments for the study of these sources through polarimetric data, potentially allowing us to understand if the energy density of relativistic electrons is in equipartition with the magnetic field or rather coupled with the thermal gas density. Our results show that low-frequency instruments also represent a precious tool to study diffuse synchrotron emission in total intensity and polarisation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Evolution of 1 / f Flux Noise in Superconducting Qubits with Weak Magnetic Fields

The microscopic description of 1/f magnetic flux noise in superconducting circuits has remained an open question for several decades despite extensive experimental and theoretical investigation. Recent progress in superconducting devices for quantum information has highlighted the need to mitigate sources of qubit decoherence, driving a renewed interest in understanding the underlying noise mechanism(s). Though a consensus has emerged attributing flux noise to surface spins, their identity and interaction mechanisms remain unclear, prompting further study. Here, we apply weak in-plane magnetic fields to a capacitively shunted flux qubit (where the Zeeman splitting of surface spins lies below the device temperature) and study the flux-noise-limited qubit dephasing, revealing previously unexplored trends that may shed light on the dynamics behind the emergent 1/f noise. Notably, we observe an enhancement (suppression) of the spin-echo (Ramsey) pure-dephasing time in fields up to B = 100 G. With direct noise spectroscopy, we further observe a transition from a 1/f to approximately Lorentzian frequency dependence below 10 Hz and a reduction of the noise above 1 MHz with increasing magnetic field. Here, we suggest that these trends are qualitatively consistent with an increase of spin cluster sizes with magnetic field. These results should help to inform a complete microscopic theory of 1/f flux noise in superconducting circuits.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2008

Four Point Measurements of the Foreshock

Hybrid code numerical simulations accurately predict the properties of the Earth's foreshock, a region populated by solar wind particles heated and reflected by their interaction with the bow shock. The thermal pressures associated with the reflected population suffice to substantially modify the oncoming solar wind, substantially reducing densities, velocities, and magnetic field strengths, but enhance temperatures. Enhanced thermal pressures cause the foreshock to expand at the expense of the ambient solar wind, creating a boundary that extends approx.10 RE upstream which is marked by enhanced densities and magnetic field strengths, and flows deflected away from the foreshock. We present a case study of Cluster plasma and magnetic field observations of this boundary.

Sibeck, D. G.↗
NASA NTRS1979

On the angle between the average interplanetary magnetic field and the propagation direction of plane large amplitude Alfven waves

The paper shows that the experimentally observed close alignment of magnetic field minimum variance direction with the average magnetic field for Alfven waves in the solar wind is consistent with theoretically predicted properties of plane large amplitude Alfven waves in the MHD approximation. The theoretical properties of these Alfven waves constrain the time averaged magnetic field to cluster around the direction of minimum variance, which is aligned with the wave normal. Thus, spacecraft magnetometer observations in the solar wind of minimum variance directions strongly peaked about the average magnetic field direction are consistent with plane large amplitude Alfven waves which have wave normals aligned with the directions of minimum variance. This does not imply that geometrical hydromagnetic calculations for Alfven wave propagation direction in the solar wind are incorrect, but there is a discrepancy between geometrical hydromagnetics theory and observations that IMF minimum variance directions tend to be aligned with the ideal Parker spiral instead of the radial direction.

Lichtenstein, B. R.↗
DOE OSTI2025

Theory meets experiment: Insights into structure and magnetic properties of Fe 1-x Ni x B alloy

Here, we studied the structural and magnetic properties of the solid solution Fe 1-x Ni x B through theoretical and experimental approaches. Powder X-ray diffraction, X-ray Pair Distribution Function analysis, and energy dispersive X-ray spectroscopy reveal that the Fe 1-x Ni x B solid solution crystallizes in the β-FeB structure type up to x = 0.6–0.7 and exhibits anisotropic unit cell volume contraction with increasing Ni concentration. Magnetic measurements showed a transition from ferromagnetism to paramagnetism around x = 0.7. For x = 0.5, the low (< 0.3 μ B ) magnetic moments suggest itinerant magnetism despite the relatively high Curie temperature (up to 225 K). Theoretical calculations indicated different types of magnetic orderings depending on the Fe/Ni atomic order, with the antiferromagnetic state being stable for ordered FeNiB 2 , whereas the ground state is ferromagnetic for the disordered alloy. Calculations also predicted the coexistence of low- and high-spin states in Fe atoms around the composition with x = 0.5, in line with the experimental evidence from 57 Fe Mössbauer spectroscopy. The two magnetically distinct Fe sites for x = 0.3, 0.4, and 0.5 observed by 57 Fe Mössbauer spectroscopy can also be interpreted as two magnetically different regions or clusters. The formation of these clusters could affect the critical behavior near a quantum magnetic transition based on a potential ferromagnetic quantum critical point identified computationally and experimentally near x = 0.64. This work highlights the complex interplay between structure and magnetism in Fe 1-x Ni x B alloys, suggesting areas for future research on quantum critical behavior.

Bhaskar, Gourab [Iowa State Univ., Ames, IA (Unite↗
NASA NTRS1994

Merged interaction regions and large-scale magnetic field fluctuations during 1991: Voyager 2 observations

This paper analyzes Voyager 2 observations of the magnetic field between 33.6 AU and 36.2 AU during 1991 when extraordinary events were observed on the Sun and in the heliosphere. The magnetic field strength signal B(t) has the unusual form of two large transient merged interaction regions (MIRs) on a fluctuating background. The two MIRs moved past the spacecraft in 32 days and 18 days, respectively. The mean field strength in each transient MIR was approx. equals 2.6 times the mean field during the remaining part of the year (0.11 nT). Each of the MIRs is related to a fast stream. The magnetic field is strong throughout each stream, suggesting that the strong fields are carried by the streams as well as produced by shock and stream compression. The fluctuations in B(t) during 1991 are not multifractal, and the MIRs cannot be approximated as multifractal clusters of intense magnetic fields. The distribution of the hour-averaged magnetic field strengths is approximately lognormal over 90% of its intermediate range, and it has an exponential tail for B greater than the average magnetic field strength. The elevation angles of B have a normal distribution with a standard deviation of 16 deg +/- 4 deg. The distributions of the azimuthal angles of B in the ranges 1 deg - 180 deg and 180 deg - 360 deg are approximately normal over a more limited range, and non-Gaussian tails associated with nearly radial magnetic fields; the standard deviations are approx. equal to 40 deg. Individual sectors are present throughout most of the interval, even in the MIRs, but there is no recurrent sector pattern. A model of the large-scale fluctuations in 1991 will have to include both determinaistic and statistical factors.

Burlaga, L. F.↗
DOE OSTI2023

Magnetic Properties of Tetravalent Pu in the Perovskites BaPuO 3 and SrPuO 3

BaPuO 3 and SrPuO 3 were synthesized, and their structures were refined in the orthorhombic space group Pbnm , a common distortion from the classic $Pm\bar{3}$m over barm cubic perovskite. Magnetic-susceptibility measurements, obtained as a function of temperature over the range of 1.8-320 K, exhibit temperature-dependent behavior, with evidence of long-range magnetic order at temperatures higher than their lanthanide and actinide analogues: BaPuO 3 below 164(1) K and SrPuO 3 below 76(1) K. Effective moments of 1.66(10)μ B for BaPuO 3 and 1.84(8)μ B for SrPuO 3 were obtained by fitting their paramagnetic susceptibilities using the Curie-Weiss law. Further, both are below the free-ion value of 2.68 μ B expected for a Pu 4+ 5 $\mid$ 4 ground level. Ab initio wave function calculations, performed at the relativistic complete active space level including spin-orbit coupling and with an embedded cluster approach that neglects interactions between Pu centers, were used to generate embedded-cluster Pu 4+ magnetic susceptibilities. The calculations agree well with experimental data at higher temperatures, providing evidence that a single-ion representation is sufficient to account for the observed paramagnetic behavior without the need to invoke charge transfer, disproportionation, strong covalent bonding, or other more complex electronic behavior.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Structure and magnetism across the Sr 2- x Ba x NiOsO 6 phase diagram: Understanding magnetic superexchange between first and third row transition metal ions

The crystal chemistry and magnetism of compositions in the Sr 2-x Ba x NiOsO 6 phase diagram have been investigated to better understand the superexchange interactions between 3d and 5d transition metal ions. Compositions with x ​< ​1.35 crystallize with the double perovskite structure, while those with x ​> ​1.83 crystallize in a trigonal structure that is a cation ordered variant of the 6H hexagonal perovskite structure. The Sr-rich double perovskites undergo a cubic to tetragonal distortion upon cooling that is driven by out-of-phase octahedral tilting. The tetragonal distortion occurs upon cooling below 650 ​K in Sr 2 NiOsO 6 . The temperature of this transition decreases as the barium content increases and is completely suppressed for x ​≥ ​1.2. All compositions in the double perovskite region become spin glasses below T g ​≈ ​40 ​K, due to the competition between ferromagnetic Ni–Os and antiferromagnetic Ni–Ni and Os–Os superexchange interactions. The double perovskite compositions that are rich in barium, like Sr 0.8 Ba 1.2 NiOsO 6 show some signs of magnetic ordering in small clusters, but the presence of Ba/Sr disorder inhibits long-range magnetic order. Trigonal Ba 2 NiOsO 6 orders ferrimagnetically below T C ​= ​108 ​K. In conclusion, the magnetic structure of this compound contains ferromagnetic ~180° Ni–O–Os interactions and antiferromagnetic ~90° Ni–O–Os interactions, both in agreement with the Goodenough-Kanamori rules.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Ion-rich Acceleration during an Eruptive Flux Rope Event in a Multiple Null-point Configuration

We report on the γ-ray emission above 100 MeV from the GOES M3.3 flare SOL2012-06-03. The hard X-ray (HXR) and microwave emissions have typical time profiles with a fast rise to a well-defined peak followed by a slower decay. The >100 MeV emission during the prompt phase displayed a double-peaked temporal structure with the first peak following the HXR and microwaves, and the second one, about 3 times stronger, occurring 17 ± 2 s later. The time profiles seem to indicate two separate acceleration mechanisms at work, where the second γ-ray peak reveals a potentially pure or at least largely dominant ion acceleration. The Atmospheric Imaging Assembly imaging shows a bright elliptical ribbon and a transient brightening in the northwestern (NW) region. Nonlinear force-free extrapolations at the time of the impulsive peaks show closed field lines connecting the NW region to the southeastern part of the ribbon, and the magnetic topology revealed clusters of nulls. These observations suggest a spine-and-fan geometry, and based on these observations, we interpret the second γ-ray peak as being due to the predominant acceleration of ions in a region with multiple null points. The >100 MeV emission from this flare also exhibits a delayed phase with an exponential decay of roughly 350 s. We find that the delayed emission is consistent with ions being trapped in a closed flux tube with gradual escape via their loss cone to the chromosphere.

Pesce-Rollins, Melissa [Istituto Nazionale di Fisi↗
NASA NTRS2011

Observations of Electron Vorticity in the Inner Plasmasheet and Its Relationship to Reconnection

Spatial derivatives of the electron moments can be estimated using data from the four Cluster spacecraft. Using spatial derivatives of the velocity we have computed the vorticity in the plasmasheet for several crossings. What we have found is that vorticity appears to be a common feature in the inner plasmasheet. We will show a number of examples. In at least some of the observations the vorticity is well correlated with the passage of Cluster through the ion diffusion region of known reconnection events. That most of the vorticity events observed are reconnection related cannot be dismissed and in fact observations of vorticity may provide a means to locate times when the Cluster spacecraft are magnetically connected to regions where reconnection is taking place. Understanding the role and source of the vorticity should advance our understanding of the dissipation of the turbulence associated with reconnection. In the course of the presentation we will also touch on the methods used to estimate the spatial derivatives as well as the limitations and assumptions involved.

Gurgiolo, Chris A.↗
NASA NTRS1986

Magnetic nonequilibrium and current sheet formation

This paper investigates the equilibrium of a cluster of long, straight, twisted magnetic flux tubes extending in the z-direction in a highly conducting fluid, subject to the boundary condition that the cluster is surrounded by a uniform pressure P. It is shown that there is equilibrium only for axial symmetry, i.e., only for a single twisted flux tube. Any more complicated cluster of twisted tubes is subject to nonequilibrium reconnection of the transverse component of the field. The example provides another perspective on the general absence of equilibrium, and consequent rapid dissipation, of any magnetic field subject to random small-scale internal strains, such as the fields extending outward from the convective zones of stars.

Vainshtein, S. I.↗
DOE OSTI2021

Paramagnetic Mn 8 Fe 4 -co-Polystyrene Nanobeads as a Potential T 1 –T 2 Multimodal Magnetic Resonance Imaging Contrast Agent with In Vivo Studies

In developing a cluster-nanocarrier design, as a magnetic resonance imaging contrast agent, we have investigated the enhanced relaxivity of a manganese and iron-oxo cluster grafted within a porous polystyrene nanobead with increased relaxivity due to a higher surface area. The synthesis of the cluster-nanocarrier for the cluster Mn 8 Fe 4 O 12 (O 2 CC 6 H 4 CH=CH 2 ) 16 (H 2 O) 4 , cross-linked with polystyrene (the nano-carrier), under miniemulsion conditions is described. By including a branched hydrophobe, iso-octane, the resulting nanobeads are porous and similar to 70 nm in diameter. The increased surface area of the nanobeads compared to nonporous nanobeads leads to an enhancement in relaxivity; r 1 increases from 3.8 to 5.2 ± 0.1 mM -1 s -1 , and r 2 increases from 11.9 to 50.1 ± 4.8 mM -1 s -1 , at 9.4 teslas, strengthening the potential for T 1 and T 2 imaging. Several metrics were used to assess stability, and the porosity produced no reduction in metal stability. Synchrotron X-ray fluorescence microscopy was used to demonstrate that the nanobeads remain intact in vivo . In depth, physicochemical characteristics were determined, including extensive pharmacokinetics, in vivo imaging, and systemic biodistribution analysis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Novel Co 5 Cluster Based Triazole Bridged Cobalt-Fluorophosphate: Synthesis, Structure, Magnetic and Heterogeneous Catalytic Epoxidation Studies

A novel triazole bridged cobalt fluorophosphate coordination polymer with the formula {Co 5 (1,2,4-triazole) 2 (OH) 2 (PO 3 F) 4 } n has been synthesized. Single crystal X-ray studies reveal that the compound comprises of Co 5 clusters which ultimately build the whole framework, here all cobalt centers are in octahedral geometry established from continuous shape analysis. All the cobalt centers are in Co(II) oxidation state and the results are supported by the bond valence sum (BVS) calculation. The sample has been characterized by single crystal X-ray, powder X-ray, FTIR and TGA analysis. The compound was tested for olefin catalysis performance and magnetism. Magnetization measurements reveal overall antiferromagnetic interactions among the Co(II) ions. The compound is very active in the catalytic transformation of olefins to their corresponding epoxides. In conclusion, catalytic epoxidation studies reveal that cyclohexene and styrene can be converted up to 97% with almost 65% selectivity of products with higher TON numbers.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1998

Large-Scale Coronal Heating, Clustering of Coronal Bright Points, and Concentration of Magnetic Flux

By combining quiet-region Fe XII coronal images from SOHO/EIT with magnetograms from NSO/Kitt Peak and from SOHO/MDI, we show that on scales larger than a supergranule the population of network coronal bright points and the magnetic flux content of the network are both markedly greater under the bright half of the quiet corona than under the dim half. These results (1) support the view that the heating of the entire corona in quiet regions and coronal holes is driven by fine-scale magnetic activity (microflares, explosive events, spicules) seated low in the magnetic network, and (2) suggest that this large-scale modulation of the magnetic flux and coronal heating is a signature of giant convection cells.

Falconer, D. A.↗