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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 883 records · Page 49

Hanford Low-Activity Waste Glass Minor Component Concentration Boundary Expansion

This study investigated the effects of increasing concentrations of minor components on simulated Hanford low-activity waste (LAW) glass properties to allow for LAW glass composition envelope expansion. A test matrix of ten glasses was generated by spiking three previously studied simulated Hanford LAW glass compositions with increasing concentrations of minor component mixes up to a total concentration of 2 wt%. In this study, the ten glasses were fabricated, and key properties were measured including crystal formation after canister centerline cooling (CCC), crystallinity as a function of temperature, density, viscosity, electrical conductivity, glass durability using the Vapor Hydration Test (VHT), product consistency using the Product Consistency Test (PCT), and sulfur solubility. The data from these tests are presented in this report.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Design and Scoping Tests on Alloy 617 Using Notched Specimen Geometry to Validate Methods for Multiaxial Stress Relaxation

In FY 2022, a development effort was initiated at the US Department of Energy’s Oak Ridge National Laboratory (ORNL) to examine the multiaxial stress-relaxation behavior and multiaxial stress-state effect on the creep-fatigue (CF) performance for Alloy 617 at elevated temperatures. This effort supported the development of the design rules in the American Society of Mechanical Engineers (ASME) Boiler and Pressure Vessel Code (BPVC), Section III, Division 5. In this work, two types of the notch specimen geometries were designed. An inelastic constitutive model was used to investigate the stress triaxiality and elastic follow-up effects on the notch specimens under CF deformation in the finite element (FE) simulations. The numerical study demonstrated that the stress triaxiality and elastic follow-up caused by the notches both play significant roles in the stress-relaxation behavior. In addition, Alloy 617 CF experiments were designed, and the testing on the notch specimens is ongoing. CF test failure data will be generated on the specimens with notches under various conditions in FY 2023, and the results will be used to validate methods for accounting for the multiaxial stress relaxation effect in the design code.

36 MATERIALS SCIENCE↗

Hydraulic Testing of the Lost Lake Aquifer Near Recovery Wells RWM 6 and RWM 7

Hydrologic tests were conducted on the Lost Lake Aquifer Zone (LLAZ) at recovery wells RWM 6 and RWM 7 in accordance with the approved test plan (Dixon, 2023). The objective of the testing was to determine well performance parameters of RWM 6 and aquifer hydraulic properties near RWM 6 and RWM 7. Tests at RWM 6 consisted of a step-drawdown test to determine well performance parameters, a constant rate pump test to determine aquifer hydraulic properties, and an aquifer recovery test also used to determine aquifer hydraulic properties. Well performance parameters determined included specific capacity, well efficiency, and head loss coefficients. Prior to testing at RWM 6, a constant rate pump test was conducted at RWM 7. Data from this testing was used to determine aquifer hydraulic properties near RWM 7.

42 ENGINEERING↗

Status of Measuring Cross Sections of Hadrons on Argon with ProtoDUNE-SP

ProtoDUNE Single-Phase is a 700-ton liquid argon detector operated in the CERN Neutrino Platform from 2018 to 2020. It is part of the Deep Underground Neutrino Experiment (DUNE), a long-baseline neutrino oscillation experiment with a 40 kT liquid argon far detector to be built at the Sanford Underground Research Facility and a near detector, with both argon and non-argon detector technologies, to be hosted at the Fermi National Accelerator Laboratory. A critical uncertainty to understand in the neutrino oscillation program of DUNE is the uncertainty on final state interactions, either reaction or elastic, of various hadrons on argon since the scattering of neutrino-induced hadrons off argon bias the hadron's measured energy. It can also prevent algorithms from identifying the hadron's particle type. Protons, kaons, and pions from the beam are especially important for the DUNE neutrino program as they represent common final state particles in neutrino interactions off a nucl eus. Therefore, ProtoDUNE is analyzing the test beam data to measure cross sections of pions, protons, and kaons on argon, aiming to tune parameters that model charged particle scattering off argon. This talk will discuss the data-taking program for ProtoDUNE and an overview of the status and results of measuring cross sections of pions, protons, and kaons on argon. It will conclude with a brief overview of how these measurements can be used for future liquid argon neutrino detectors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Engineering Scale Testing of Transformational Non-Aqueous Solvent-Based CO 2 Capture Process at Technology Center Mongstad

Progress is reported for the period from August 8, 2018 to June 30, 2023. This final report involves work performed under ten tasks spanning two budget periods. The tasks are Task 1 Project Management, Task 2 TCM EH&S Risk Evaluation and Permitting, Task 3 Solvent Qualification, Task 4 Preliminary Design of NAS Optimized System, Task 5 TCM Amine Plant Equipment Procurement, Modification and Commissioning, Task 6 Solvent Production, Task 7 NAS Modified Amine Plant Test Plan Development, Testing, and Data Analysis, Task 8 Decommissioning and Waste Handling, Task 9 Final Techno-Economic Assessment and EH&S Risk Assessment, and Task 10 Cost Benefit Analysis and Technology Maturation Planning.

01 COAL, LIGNITE, AND PEAT↗

Methodological guidelines on concrete degradation based on predictive models and the release of MOSAIC for industry use

In light-water reactors (LWRs), the concrete biological shield (CBS) designates the concrete structure directly facing the reactor pressure vessel (RPV). The primary function of the CBS is to protect equipment and personnel from the neutron and gamma radiation exiting the RPV. Most CBSs in operation in the United States also provide structural support to the RPV. Based on a long-term structural analysis, the structural integrity of the CBS to transfer the in-service passive load to the foundation, dynamic loading during an earthquake, and thermal loading during a loss-of-coolant accident (LOCA) must be maintained. Based on test reactor data for accelerated conditions, the mechanical properties of irradiated concrete are affected when exposed to neutron fluence higher than ≈ 10 19 n.cm -2 (E > 0.1 MeV). At 80 years of operation, the fluence estimates at the surface of the CBS range between 1×10 19 and 7×10 19 n.cm -2 (E > 0.1 MeV): the fluence value depends mostly on the design. Although fluence attenuates through the CBS by virtue of the shielding properties of concrete, about 5% to 10% of the CBS wall depth is affected by high fluence. The main degradation mechanism is the so-called radiation-induced volumetric expansion (RIVE) caused by the amorphization of aggregate-forming minerals. RIVE causes large deformation of up to 18% in pure quartz, and it also reduces the structural properties of concrete. The structural effects of long-term exposure to fast neutron irradiation in LWRs was studied in the report entitled “Assessment of the Effect of the Irradiation-Induced Degradation on the In-Service Structural Performance of the Concrete Biological Shields” (M3LW-23OR0403013). This report illustrates that (1) irradiation-induced damage expands further than the region subject to a cumulative fluence of 10 19 n.cm -2 (E > 0.1 MeV) to reach the steel reinforcement location, and (2) the irradiation-induced damage region shows no substantial residual bearing capacity and should not be accounted for in the integrity assessment of the CBS.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Lost and Found Opportunities Around the Chlorine Worth Study [Slides]

This presentation begins with an Introduction and models and sensitivity results. Included within this lecture is a chlorine gap assessment discussion. referenced is an opportunity to test covariance data. This presentation wraps up with some conclusions and thoughts.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Methodology for Digital Image Correlation and Infrared Measurement of Melting Aluminum Bars

Ultimately, our experiment measures two quantities on an aluminum bar: motion (which modeling must predict) and temperature (which sets thermal boundary conditions). For motion, stereo DIC is a technique to use imaging data to provide displacements relative to a reference image down to 1/100th of a pixel. We use a calibrated infrared imaging method for accurate temperature measurements. We will be capturing simultaneous data and then registering temperature data in space to the same coordinate system as the displacement data. While we will later show that our experiments are repeatable, indicating that separate experiments for motion and temperature would provide similar data, the simultaneous and registered data removes test to test variability as a source of uncertainty for model calibration and reduces the number of time-consuming tests that must be performed.

36 MATERIALS SCIENCE↗

Integrated Off-Gas System Tests on the DM1200 Melter with RPP-WTP LAW Sub-Envelope C1 Simulants (Final Report)

The report documents melter and off-gas performance results obtained on the DM1200 during processing of LAW Sub-Envelope Cl feed. The principal objectives of the DM1200 melter testing were to demonstrate suitable processing and production rates for LAW Cl feed; characterize the glass product for elemental composition, the presence of organic compounds, and TCLP response for metals; and measure destruction and removal efficiencies (DREs) for organic compounds across the melter and off-gas treatment components. The feed was spiked with organic compounds for part of the testing duration. Data were collected for both process engineering needs and to support regulatory activities. The data needed for regulatory support were collected using EPA methods and independent data analyses and data checking were performed.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Setup and Testing of the RS105 Wire Array Pulser

The report covers the RS105 Wire Array Pulser testbed. The setup of the wire array at Reapplication, building 996, is laid out. Setup instructions are provided. Details of the commissioning test are given. Measurement data from the commissioning test shows the field output of the array exceeds 50 kV/m and that tuning the pulser output with a peaking switch can provide a rise time of ~2.3 ns and a pulse width of ~23 ns. The field levels and timeframes shown are within the tolerance conditions of

42 ENGINEERING↗

Gamma and Neutron Measurement and Modeling of Irradiated TRISO Fuel

Given the unique characteristics of the PBR fuel cycle, both gamma and neutron measurements are expected to play important roles in performing and maintaining nuclear material control and accounting for spent pebbles to safeguard the fuel cycle. Given the lack of irradiated pebbles in the US, a variety of irradiated TRISO fuel samples with wide ranges of burnups and cooling times available at ORNL were used in this work. A large number of gamma and neutron measurements have been performed on these samples to collect data to test the various detectors and to benchmark the computer models to simulate the depletion and decay of the fuel and the measurements themselves. Two neutron detectors, including a custom-made detector and the Very High-Performance Neutron Multiplicity Counting, were used to measure the neutrons emitted by these TRISO samples. Three gamma spectrometry detectors, including an HPGe and the M400 CZT detector, were used to measure gamma-ray emissions from these samples. The M400 was recently adopted by the IAEA for fresh uranium measurements, but it was tested for spent fuel measurements prior to this project. Detailed MCNP models were developed to simulate these neutron and gamma measurements. Some GADRAS models were also developed to cross check the MCNP models for the gamma measurements. It was found challenging to perform neutron measurements in the hot cell due to the high background counts. Close agreements were observed between the simulated and measured neutron count rates in both detectors’ measurements of californium calibration sources. Both the HPGe and M400 detectors were able to measure the 604 and 662 keV peaks from these samples, which are the two most important peaks used to infer fuel burnup. Although the M400 detector did not have nearly good energy resolution and did not detect some of the minor peaks as the HPGe detector, it was found to be capable of handling significantly higher dose rates than HPGe. Given the complexities in the TRISO samples (e.g., different samples sizes) and uncertainties in the alignments between the detector and the TRISO fuel inside the containers, large scatters were found between the peak area rates and the samples’ burnups. However, the 604/662 peak ratios were found to trend well with the samples’ burnups among most samples in both measured and simulated results.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of a Framework and Methodology for an Advanced Reactor Materials Environmental Effects Design Guide

Advanced non-light-water reactor components may operate at elevated temperature while experiencing cyclic loading, significant neutron irradiation, and exposure to reactor coolant. ASME Boiler and Pressure Vessel Code, Section III, Division 5, provides design rules for elevated-temperature service but does not include specific procedures to account for environmental effects on material properties. This report develops an initial framework and methodology for an Environmental Effects Design Guide (EEDG) focused on neutron irradiation; coolant-environment effects are reserved for future work. The proposed approach treats irradiation as a property-based overlay on the existing Division 5 design process, with two routes: a sparse-data route applying two reduction factors — FCR on creep-rupture strength and FF on fatigue life — for the creep-fatigue evaluations that typically control the design of advanced high-temperature reactor components, and a fuller framework developing the property-to-rule chain across the four Division 5 checks (primary load, strain limits and ratcheting, creep-fatigue, and buckling), together with swelling and weldments as scope items. Both routes are scoped by an in-pile qualification that restricts the use of post-irradiation-examination-derived properties in regimes where an in-pile mechanism could control the design outcome. Illustrative outputs derived on a compiled annealed Type 316 database — FCR ≈ 0.78–0.86 and FF ≈ 0.4 — demonstrate the calculation method within that specific dataset. The framework is an initial, testable design-rule concept; it identifies a practical path for preliminary design evaluations under sparse data and the material data and testing needed to develop the framework further.

Barua, Bipul (ORCID:0000000247184113)↗