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At least 883 records · Page 49

Low spin spectroscopy of neutron-rich Cl 43 , 44 , 45 via β - and β n decay

In this article, β - decay studies of neutron-rich isotopes 43,45 S performed at the National Superconducting Cyclotron Laboratory are reported. β -delayed $\gamma$ transitions were detected by an array of 16 clover detectors surrounding the Beta Counting Station, which consists of a 40×40 double-sided silicon strip detector followed by a single-sided silicon strip detector. β -decay half-lives were extracted for 43,45 S by correlating implants and decays in the pixelated implant detector and by considering further coincidences with $\gamma$ transitions in the daughter nuclei. Further, the level structures of 43,45 Cl are expanded by the addition of 20 and 8 new $\gamma$ transitions in 43 Cl and 45 Cl respectively, and core-excited negative-parity states were observed in both nuclei for the first time. For 45 S, a large fraction of the β -decay strength was observed feeding neutron-unbound states in 45 Cl, which, decaying by delayed neutrons, populated excited states in the β ⁢1⁢ n daughter, 44 Cl. Experimental observations were compared to detailed shell-model calculations using the SDPFSDG-MU interaction to highlight the role of the diminished N = 28 neutron shell gap and the near degeneracy of the proton s 1/2 and d 3/2 orbitals in the structure of the neutron-rich Cl isotopes. The current work also provides further support to a ground-state spin-parity assignment of 3/2 + in 45 Cl.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

One-neutron transfer study of Xe 137 and systematics of 13 / 2 1 + and 13 / 2 2 + levels in N = 83 nuclei

Excited states in 137 Xe have been studied by using the near-barrier single-neutron transfer reactions 13 C( 136 Xe, 12 C ) 137 Xe and 9 Be( 136 Xe, 8 Be ) 137 Xe in inverse kinematics.Particle- and particle- coincidence measurements have been performed with the Phoswich Wall and Digital Gammasphere detector arrays. Evidence is found for a 13/2 + 2 level (E = 3137 keV) and for additional high-lying 3/2 – and 5/2 – states. The results are discussed in the framework of realistic shell-model calculations. These calculations are also extended to the 13/2 + 1 and 13/2 + 2 levels in the N = 83 isotonic chain. Furthermore, they indicate that there is a need for a value of the neutron 0i 13/2 single-particle energy (E SPE = 2366 keV) lower than the one proposed in the literature. It is also demonstrated that the population patterns of the j = l ± 1/2 single-particle states in 137 Xe are different for the two targets used in these measurements and the implications of this effect are addressed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

β decay of Si 38 , 40 ( T z = + 5 , + 6 ) to low-lying core excited states in odd-odd P 38 , 40 isotopes

Low-lying excited states in P 38,40 have been identified in the β decay of T z =+5,+6, Si 38,40 . Based on the allowed nature of the Gamow-Teller (GT) decay observed, these states are assigned spin and parity of 1 + and are core-excited 1p1h intruder states with a parity opposite to the ground state. The occurrence of intruder states at low energies highlights the importance of pairing and quadrupole correlation energies in lowering the intruder states despite the N=20 shell gap. Configuration interaction shell model calculations with the state-of-art SDPF-MU effective interaction were performed to understand the structure of these 1p1h states in the even-A phosphorus isotopes. States in P 40 with N=25 were found to have very complex configurations involving all the fp orbitals leading to deformed states as seen in neutron-rich nuclei with N≈28. The calculated GT matrix elements for the β decay highlight the dominance of the decay of the core neutrons rather than the valence neutrons.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Kaon mixing beyond the standard model with physical masses

We present nonperturbative results for beyond the standard model kaon mixing matrix elements in the isospin symmetric limit ( m u = m d ) of QCD, including a complete estimate of all dominant sources of systematic error. Our results are obtained from numerical simulations of lattice QCD with N f = 2 + 1 flavors of dynamical domain wall fermions. For the first time, these quantities are simulated directly at the physical pion mass m π ∼ 139 MeV for two different lattice spacings. We include data at three lattice spacings in the range a = 0.11 – 0.07 fm and with pion masses ranging from the physical value up to 450 MeV. Compared to our earlier work, we have added both direct calculations at physical quark masses and a third lattice spacing making the removal of discretization effects significantly more precise and eliminating the need for any significant mass extrapolation beyond the range of simulated data. We renormalize the lattice operators nonperturbatively using RI-SMOM off-shell schemes. These schemes eliminate the need to model and subtract nonperturbative pion poles that arises in the RI-MOM scheme and, since the calculations are performed with domain wall fermions, the unphysical mixing between chirality sectors is suppressed. Our results for the bag parameters in the MS ¯ scheme at 3 GeV are B K ≡ B 1 = 0.5240 ( 17 ) ( 54 ) , B 2 = 0.4794 ( 25 ) ( 35 ) , B 3 = 0.746 ( 13 ) ( 17 ) , B 4 = 0.897 ( 02 ) ( 10 ) and B 5 = 0.6882 ( 78 ) ( 94 ) , where the first error is from lattice uncertainties and the second is the uncertainty due to the perturbative matching to MS ¯ . Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurements of ionization states in warm dense aluminum with betatron radiation

Time-resolved measurements of the ionization states of warm dense aluminum via K-shell absorption spectroscopy are demonstrated using betatron radiation generated from laser wakefield acceleration as a probe. The warm dense aluminum is generated by irradiating a free-standing nanofoil with a femtosecond optical laser pulse and was heated to an electron temperature of ~20–25 eV at a close-to-solid mass density. Absorption dips in the transmitted x-ray spectrum due to the Al 4+ and Al 5+ ions are clearly seen during the experiments. The measured absorption spectra are compared to simulations with various ionization potential depression models, including the commonly used Stewart-Pyatt model and an alternative modified Ecker-Kröll model. Furthermore, the observed absorption spectra are in approximate agreement with these models, though indicating a slightly higher state of ionization and closer agreement for simulations with the modified Ecker-Kröll model.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Chlorine and potassium enrichment in the Cassiopeia A supernova remnant

The elements in the Universe are synthesized primarily in stars and supernovae, where nuclear fusion favours the production of even-Z elements. In contrast, odd-Z elements are less abundant and their yields are highly dependent on detailed stellar physics, making theoretical predictions of their cosmic abundance uncertain. In particular, the origin of odd-Z elements such as phosphorus (P), chlorine (Cl) and potassium (K), which are important for planet formation and life, is poorly understood. While the abundances of these elements in Milky Way stars are close to solar values, supernova explosion models systematically underestimate their production by up to an order of magnitude, indicating that key mechanisms for odd-Z nucleosynthesis are currently missing from theoretical models. Here we report the observation of P, Cl and K in the Cassiopeia A supernova remnant using high-resolution X-ray spectroscopy with X-Ray Imaging and Spectroscopy Mission data, with the detection of K at above the 6σ level being the most significant finding. Supernova explosion models of normal massive stars cannot explain the element abundance pattern, especially the high abundances of Cl and K, while models that include stellar rotation, binary interactions or shell mergers agree closely with the observations. Our observations suggest that such stellar activity plays an important role in supplying these elements to the Universe.

Astronomy and AstroPhysics↗

Octupole correlations near Te 110

The lifetime of the 2 + and 9 – , 11 – , 13 – , 15 – states in the neutron-deficient 110 Te was measured for the first time using the recoil distance Doppler shift technique. The reported value of the reduced transition probability B(E2; $0$$^{+}_{g.s}$ → 2 + ) = 4.3(8) × 10 3 e 2 fm 4 supports the systematic for even-mass Te isotopes and was interpreted in the framework of the large-scale shell model and cranked shell model calculations. The measured reduced transition probabilities in the negative-parity yrast band revealed the upward trend towards the high spins. Furthermore, the enhanced collectivity is discussed in terms of the tilted axis cranking approach and the symmetry configuration mixing method with the Gogny D1S interaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Origin of the Low-Energy Enhancement of the γ-Ray Strength Function

The low-energy enhancement (LEE) in γ-ray strength functions has been experimentally identified in a large number of nuclei during the past two decades; however, the origin of the enhancement is not fully understood. Building on previous theoretical work, we investigate the LEE and its relation to the scissors mode (SM) with an independent theoretical approach. We apply a novel angular-momentum-projected shell-model method that explicitly endows degrees of freedom to describe the scissors motion. Taking the recently measured γ-ray strength functions in Neodymium isotopes as examples, we find that the LEE arises from a quasi-free scissors motion appearing only in weakly-deformed nuclei, which can be viewed as an approximate free-rotation of neutrons with respect to protons. This leads us to propose a new type of collective motion, scissors rotation, to contrast the scissors vibration widely known in well-deformed nuclei. The observed LEE is naturally interpreted as the first evidence for this collective excitation mode.

Collective models↗

Application of an ab initio S matrix to data analysis of transfer reactions to the continuum populating Be 11

Recently, the bound and continuum spectrum of 11 Be has been calculated within the ab initio no-core shell model with continuum (NCSMC) method, with the parity inversion in the ground state successfully reproduced. Here, the continuum spectrum obtained is in agreement with known experimental levels. The S matrix contained in the NCSMC continuum wave functions of the n + 10 Be system is used in this work for the first time in a transfer-to-the-continuum (TC) reaction calculation. The TC approach is applied to study the excitation energy spectrum of 11 Be measured in the 9 Be( 18 O, 16 O) 11 Be reaction at 84 MeV. Previously known levels are confirmed and theoretical and experimental evidence for a 9/2 + state at E x = 5.8 MeV is given, whose configuration is thought to be 10 Be(2 + )+n( d 5/2 ).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Observation of the near-threshold intruder 0 – resonance in 12 Be

A resonant state at $3.21^{+0.12}_{–0.04}$ MeV, located just above the one-neutron separation threshold, was observed for the first time in 12 Be from the 11 Be(d,p) 12 Be one-neutron transfer reaction in inverse kinematics. This state is assigned a spin-parity of 0 – according to the systematics of the level scheme of the N=8 isotones and decay-width analysis. Gamow coupled-channel and Gamow shell-model calculations show the importance of the continuum coupling, which dramatically influences the excitation energy and ordering of low-lying states. Various exotic structures associated with cross-shell intruding configurations in 12 Be and in its isotonic nucleus 11 Li are comparably discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Excited states in the neutron-rich nucleus $\mathrm{^{25}F}$

The structure of the nucleus $^{25}_{9}$F was investigated through in-beam $γ$ -ray spectroscopy of the fragmentation of $\mathrm{^{26}Ne}$ and $\mathrm{^{27, 28}Ne}$ ion beams. Based on the particle-$γ$ and particle-$γγ$ coincidence data, a level scheme was constructed and compared with shell model and coupled-cluster calculations. Some of the observed states were interpreted as quasi-single-particle states built on top of the closed-shell nucleus $\mathrm{^{24}O}$, while the others were described as states arising from coupling of a single proton to the $\mathrm{2^+}$ core excitation of $\mathrm{^{24}O}$.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Supplemental Structural Analyses Used in Support of Certification of the Defense Programs Package 3

The Defense Programs Package (DPP)-3 is to be certified by the National Nuclear Security Administration (NNSA) Packaging and Transportation Division (PTD). Certification is based on successful physical testing of the package, and six certification test units (CTUs) have been subjected to the normal conditions of transport (NCT) and hypothetical accident conditions (HAC) outlined in Title 10 of the Code of Federal Regulations Part 71 (10 CFR 71). During regulatory testing of one of the CTUs, the drum lid closure bolt closest to the impact surface failed during the HAC 30-ft side drop. One of the testing goals for this CTU was to minimize the thermal pathway from the drum exterior shell to the containment vessel (CV) flange and O-rings, leading to the maximum damage scenario in preparation for thermal testing at 1475 °F. Therefore, the puncture bar impact proceeded as originally planned by striking the side wall of the package exterior closest to the location of the CV flange. This puncture bar impact did not attempt to exploit the region of the failed drum lid closure bolt to potentially cause more damage to the package. After the conclusion of regulatory testing, the DPP-3 package finite element model was used to numerically evaluate the effects of puncture bar impacts to the drum exterior in the vicinity of the failed drum lid closure bolt to further demonstrate the robustness of the DPP-3 design. Three alternate puncture bar impact locations and orientations were evaluated to demonstrate that these puncture bar impacts would not substantially reduce the effectiveness of the DPP-3 packaging. This paper describes the supplemental finite element models performed and structural analysis results that demonstrate the alternate HAC 40-in. puncture bar impact tests would have no deleterious effect on the performance of the DPP-3.

Sakalaukus Jr., Peter J.↗

Direct lifetime measurements of the excited states in Ni 72

The lifetimes of the first excited 2 + and 4 + states in 72 Ni were measured at the National Superconducting Cyclotron Laboratory with the recoil-distance Doppler-shift method, a model-independent probe to obtain the reduced transition probability. Excited states in 72 Ni were populated by the one-proton knockout reaction of an intermediate energy 73 Cu beam. γ-ray-recoil coincidences were detected with the γ-ray tracking array GRETINA and the S800 spectrograph. Our results provide evidence of enhanced transition probability B(E2;2 + → 0 + ) as compared to 68 Ni, but do not confirm the trend of large B(E2) values reported in the neighboring isotope 70 Ni obtained from Coulomb excitation measurement. The results are compared to shell model calculations. Here, the lifetime obtained for the excited 4 + 1 state is consistent with models showing decay of a seniority ν = 4, 4 + state, which is consistent with the disappearance of the 8+ isomer in 72 Ni.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Symmetry tuning of a near one-dimensional 2-shock platform for code validation at the National Ignition Facility

Here, we introduce a new quasi 1-D implosion experimental platform at the National Ignition Facility designed to validate physics models as well as to study various Inertial Confinement Fusion aspects such as implosion symmetry, convergence, hydrodynamic instabilities, and shock timing. The platform has been developed to maintain shell sphericity throughout the compression phase and produce a round hot core at stagnation. This platform utilizes a 2-shock 1 MJ pulse with 340 TW peak power in a near-vacuum AuHohlraum and a CH ablator capsule uniformly doped with 1% Si. We also performed several inflight radiography, symmetry capsule, and shock timing experiments in order to tune the symmetry of the capsule to near round throughout several epochs of the implosion. Finally, adjusting the relative powers of the inner and outer cones of beams has allowed us to control the drive at the poles and equator of the capsule, thus providing the mechanism to achieve a spherical capsule convergence. Details and results of the tuning experiments are described.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Engineering defect energy landscape of CoCrFeNi high-entropy alloys by the introduction of additional dopants

The concept of high-entropy alloys (HEAs) focusing on tuning the overall chemical complexity represents a novel alloy design strategy. In contrast, alloying of a metallic matrix with minor doping elements with limited and localized tunability has been a common practice to improve material performance. Combining the idea of globally engineering defect energy landscape in HEAs and the localized doping strategy in dilute alloys, in this work, we explore doping effects of minor elements in a HEA matrix to further enhance the overall and localized chemical tunability, aiming to improve its irradiation resistance. Specifically, we study the influence of minor Al, Cu, Ti, and Pd substitutional doping elements on defect energetics in a CoCrFeNi model HEA based on density-functional theory (DFT) calculations. The DFT results indicate that the formation and migration energies of vacancies can be strongly influenced when a dopant is introduced at the first nearest neighbor shells around a vacancy. On the other hand, interstitial energetics are only slightly affected. Among the four elements, Ti and Pd generally decrease vacancy formation energies and increase vacancy migration energies more significantly than Al and Cu. The doping effects become more pronounced when the concentration of the substitutional dopants increases. Based on the energy distributions obtained from DFT, we build a kinetic Monte Carlo (kMC) model to assess the impact of dopants on vacancy-mediated diffusivity in the doped HEAs. Our results suggest that Ti and Pd can lower the tracer diffusivity in the considered HEAs and act as trapping sites, whereas Cu may enhance the atomic transport. This work indicates that substitutional doping in HEAs is an effective strategy in metallurgy to further tune the defect and transport properties of complex alloys.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Relativistic Iron K Emission and Absorption in the Seyfert 1.9 Galaxy MCG-05-23-16

We present the results of the simultaneous deep XMM-Newton and Chandra observations of the bright Seyfert 1.9 galaxy MCG-5-23-16, which is thought to have one of the best known examples of a relativistically broadened iron Kalpha line. We detected a narrow sporadic absorption line at 7.7 keV which appears to be variable on a time-scale of 20 ksec. If associated with FeXXVI this absorption is indicative of a possible variable high ionization, high velocity outflow. The time averaged spectral analysis shows that the iron K-shell complex is best modeled with an unresolved narrow emission component (FWHM less than 5000 kilometers per second, EW approx. 60 eV) plus a broad component. This latter component has FWHM approx. 44000 kilometers per second, an EW approx. 50 eV and its profile is well described with an emission line originating from the accretion disk viewed with an inclination angle approx. 40 deg. and with the emission arising from within a few tens of gravitational radii of the central black hole. The time-resolved spectral analysis of the XMM-Newton EPIC-pn spectrum shows that both the narrow and broad components of the Fe K emission line appear to be constant within the errors. The analysis of the XMM-Newton/RGS spectrum reveals that the soft X-ray emission of MCG-5-23-16 is likely dominated by several emission lines superimposed on an unabsorbed scattered power-law continuum. The lack of strong Fe L shell emission together with the detection of a strong forbidden line in the O VII triplet supports a scenario where the soft X ray emission lines are produced in a plasma photoionized by the nuclear emission.

Braito, V.↗

$\mathrm{^{12}C}$ properties with evolved chiral three-nucleon interactions

In this research, we investigate selected static and transition properties of $\mathrm{^{12}C}$ using ab initio no-core shell model (NCSM) methods with chiral two- and three-nucleon interactions. We adopt the similarity renormalization group (SRG) to assist convergence including up to three-nucleon ($3N$) contributions. We examine the dependencies of the 12 C observables on the SRG evolution scale and on the model-space parameters. We obtain nearly converged low-lying excitation spectra. We compare results of the full NCSM with the importance truncated NCSM in large model spaces for benchmarking purposes. We highlight the effects of the chiral $3N$ interaction on several spectroscopic observables. The agreement of some observables with experiment is improved significantly by the inclusion of $3N$ interactions, e.g., the $B(M1)$ from the first $J^πT = 1^+1$ state to the ground state. However, in some cases the agreement deteriorates, e.g., for the excitation energy of the first $1^+0$ state, leaving room for improved next-generation chiral Hamiltonians.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Improved Tensor Current Limit from 8 B 𝛽 Decay Including New Recoil-Order Calculations

A precision measurement of the 𝛽 + decay of 8 B was performed using the Beta-decay Paul Trap to determine the 𝛽−𝜈 angular correlation coefficient 𝑎 𝛽⁢𝜈 . The experimental results were combined with new ab initio symmetry-adapted no-core shell-model calculations to yield the second-most precise measurement from Gamow-Teller decays, 𝑎 𝛽⁢𝜈 = −0.3345 ± 0.001⁢9 stat ± 0.002⁢1 syst . This value agrees with the standard model value of −1/3 and improves uncertainties in 8 B by nearly a factor of 2. By combining results from 8 B and 8 Li , a tight limit on tensor current coupling to right-handed neutrinos was obtained. A recent global evaluation of all other precision 𝛽 decay studies suggested a nonzero value for right-handed neutrino coupling in contradiction with the standard model at just above 3⁢𝜎. Finally, the present results are of comparable sensitivity and do not support this finding.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗