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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 883 records · Page 49
All sourcesNASA NTRSDOE OSTI
NASA NTRS1973

An efficient algorithm for calculation of the Luenberger canonical form.

A new algorithm is presented to obtain the Luenberger canonical form for multivariable systems. A distinct feature of the method is that the canonical form is obtained directly and, if necessary, the similarity transformation can be computed. There is a substantial reduction in the amount of computation compared to Luenberger's method. The reduced computations along with Gaussian techniques lend greater inherent accuracy and the ability to refine the solution with additional computations. An example is presented to illustrate the technique.

Jordan, D.↗
NASA NTRS2012

A Large-Scale Design Integration Approach Developed in Conjunction with the Ares Launch Vehicle Program

This paper presents a method for performing large-scale design integration, taking a classical 2D drawing envelope and interface approach and applying it to modern three dimensional computer aided design (3D CAD) systems. Today, the paradigm often used when performing design integration with 3D models involves a digital mockup of an overall vehicle, in the form of a massive, fully detailed, CAD assembly; therefore, adding unnecessary burden and overhead to design and product data management processes. While fully detailed data may yield a broad depth of design detail, pertinent integration features are often obscured under the excessive amounts of information, making them difficult to discern. In contrast, the envelope and interface method results in a reduction in both the amount and complexity of information necessary for design integration while yielding significant savings in time and effort when applied to today's complex design integration projects. This approach, combining classical and modern methods, proved advantageous during the complex design integration activities of the Ares I vehicle. Downstream processes, benefiting from this approach by reducing development and design cycle time, include: Creation of analysis models for the Aerodynamic discipline; Vehicle to ground interface development; Documentation development for the vehicle assembly.

Redmon, John W.↗
NASA NTRSDate not supplied

Tail Sizing Considerations for Wingtip Propulsor Driven Aircraft Applied to the Parallel Electric-Gas Architecture with Synergistic Utilization Scheme (PEGASUS) Concept

This research focuses on the vertical tail sizing implications of a single propulsion system fault when using wingtip propulsors as applied to the PEGASUS concept. PEGASUS is a conceptual regional aircraft featuring wingtip propulsors, an aft boundary layer ingestion propulsor, and inboard propulsors. Using four propulsors on the wing, rather than the typical two, enables a reduction in the vertical tail size needed in the event of a single fault in the propulsion system. Achieving a reduction in vertical tail size, and its associated reduction in drag, is dependent on splitting the takeoff thrust appropriately between the inboard and wingtip propulsors. At takeoff, the wingtip propulsors can only provide a small portion of the takeoff thrust. Compared with a conventional baseline vehicle employing only inboard propulsors, the increased wetted area from the wingtip nacelles outweighs the cruise drag benefits obtained from the reduced tail size and the reduction in wingtip vortices due to the wingtip propellers. The research highlights the need for aggressive cruise drag reductions on PEGASUS, possibly through increased use of the boundary layer ingestion propulsor. By lowering the wingtip propulsor power at cruise, the propulsors would be better sized for takeoff and have smaller nacelles with lower drag.

Nathaniel J Blaesser↗
NASA NTRS2023

Direct Measurement of the Cosmic-Ray Helium Spectrum from 40 GeV to 250 TeV with the Calorimetric Electron Telescope on the International Space Station

We present the results of a direct measurement of the cosmic-ray helium spectrum with the CALET instrument in operation on the International Space Station since 2015. The observation period covered by this analysis spans from October 13, 2015, to April 30, 2022 (2392 days). The very wide dynamic range of CALET allowed for the collection of helium data over a large energy interval, from ∼40 GeV to ∼250 TeV, for the first time with a single instrument in low Earth orbit. The measured spectrum shows evidence of a deviation of the flux from a single power law by more than 8σ with a progressive spectral hardening from a few hundred GeV to a few tens of TeV. This result is consistent with the data reported by space instruments including PAMELA, AMS-02, and DAMPE and balloon instruments including CREAM. At higher energy we report the onset of a softening of the helium spectrum around 30 TeV (total kinetic energy). Though affected by large uncertainties in the highest energy bins, the observation of a flux reduction turns out to be consistent with the most recent results of DAMPE. A double broken power law is found to fit simultaneously both spectral features: the hardening (at lower energy) and the softening (at higher energy). A measurement of the proton to helium flux ratio in the energy range from 60 GeV=n to about 60 TeV=n is also presented, using the CALET proton flux recently updated with higher statistics.

O Adriani↗
DOE OSTI2019

An Analysis on Cost Reduction Potential of Vertical Bore Ground Heat Exchangers Used for Ground Source Heat Pump Systems

The cost for installing ground heat exchangers (GHXs) used for ground source heat pump (GSHP) systems usually accounts for more than 30% of the total cost of a GSHP system and it is the biggest contributor to the cost premium of GSHPs compared with conventional HVAC systems. This study evaluates the cost reduction potential of several possible improvements in borehole heat transfer and bore field layout. A detailed cost model for GHX installation was updated and new features were added to account for various GHX designs, geological conditions, and drilling technologies. Coupled with a well-established GHX sizing program, a systematic study was conducted to assess the impacts of these improvements on the needed total drilling length and resulting cost under various geological and loading conditions. Finally, improvements with significant potential to reduce GHX installation cost are recommended.

Liu, Xiaobing↗
DOE OSTI2018

Development of Advanced T-OZON{sup TM} for PWR Decommissioning (2) - 18170

The number of aging nuclear power plants (NPPs) slated for closure around the world has increased. The majority of them are PWRs. Minimization of radiation exposure for PWR decommissioning workers is one of the key factors in decommissioning in order to apply the as low as reasonably achievable (ALARA) principle. To this end, it is desirable to establish a chemical decontamination method to reduce the exposure of PWR decommissioning workers. Toshiba developed T-OZON{sup TM}, a chemical decontamination method for BWRs [1, 2, 3]. To date, the method has been applied more than 90 times in Japanese BWR plants. The reduction in radiation exposure of workers achieved by applying T-OZON{sup TM} is estimated at about 300-2700 man mSv [4]. A major feature of T-OZON{sup TM} is the reduced amount of radioactive waste produced when compared to other decontamination processes. Oxide films on PWR wetted surfaces are harder to decontaminate than those in a BWR due to their chemical composition. To apply T-OZON{sup TM} to PWR oxide films, it is necessary to modify the process conditions. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2018

Numerical Analysis of Fatigue Behavior of ITER-Like Monoblock Divertor Interlayer Under Coupled Heat Loads

High-confinement mode is a very prominent operation style for future fusion device due to its unique advantages. However, the conjuncted edge localized modes (ELMs) are very difficult to control so that divertor plates are very prone to suffer both stationary high heat flux (HHF) loads of long-pulse operating mode and transient shock loads of ELMs. Most previous researches focus on degradation of plasma facing material (PFM), however, as a layer joining PFM and cooling tube, the soft copper interlayer suffers concentrated thermal stress loads due to mismatched thermal expansion of PFM and cooling tube. Its thermal fatigue behavior under such coupled loads is also of great significance to structural safety of divertor component. With such a motivation, the reduction effects on fatigue life time of a typical interlayer of monoblock divertor under series of coupled HHF and ELMs shock loading conditions are investigated. It is found that: (1) The transient shock feature of ELMs loading is propagated into interlayer with less sharp pattern. The increase of damage induced by coupled ELMs loading is limited in single cycle, while the accumulated damage of multiple consecutive coupled loading cycles is increased nonlinearly. (2) Under the coupled HHF and ELMs loading, the fatigue life time of interlayer is generally decreasing. The magnitude of decrease is increasing nonlinearly with the magnitude of ELMs peak and averaged heat flux. (3) For three characteristic parameters of ELMs shock loading such as frequency, duration and peak heat flux, the peak heat flux and frequency are two parameters more sensitive to determine coupled reduction effects on fatigue lifetime of the interlayer, while for high frequency case, time averaged heat flux takes the lead.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Optimizing Catalysis by Combining Molecular Scaling Relationships: Iron Porphyrin-Catalyzed Electrochemical Oxygen Reduction as a Case Study

Here, the present work demonstrates the generality of molecular scaling relationships toward achieving faster catalysis at lower overpotentials. In iron porphyrin-catalyzed oxygen reduction, independent tuning of the catalyst E 1/2 and buffer pK a resulted in improvement of both the maximum turnover frequency (TOF max ) and the effective overpotential (η eff ). Interestingly, the most optimal system is achieved with the most reducing catalyst and a weak buffered acid—a perhaps counterintuitive conclusion. More generally, this study illustrates a path to optimization of catalytic systems through their differing responses to changes in the intrinsic features of the system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2013

Development of a Universal Waste Management System

NASA is working with a number of commercial companies to develop the next low Earth orbit spacecraft. The hardware volume and weight constraints are similar to or greater than those of the Apollo era. This, coupled with the equally demanding cost challenge of the proposed commercial vehicles, causes much of the Environmental Control and Life Support System (ECLSS) designs to be reconsidered. The Waste Collection System (WCS) is within this group of ECLSS hardware. The development to support this new initiative is discussed within. A WCS concept - intended to be common for all the vehicle platforms currently on the drawing board - is being developed. The new concept, referred to as the Universal Waste Management System (UWMS), includes favorable features from previous designs while improving on other areas on previous Space Shuttle and the existing International Space Station (ISS) WCS hardware, as needed. The intent is to build a commode that requires less crew time, improved cleanliness, and a 75% reduction in volume and weight compared to the previous US ISS/Extended Duration Orbitor WCS developed in the 1990s. The UWMS is most similar to the ISS Development Test Objective (DTO) WCS design. It is understood that the most dramatic cost reduction opportunity occurs at the beginning of the design process. To realize this opportunity, the cost of each similar component between the UWMS and the DTO WCS was determined. The comparison outlined were the design changes that would result with the greatest impact. The changes resulted in simplifying the approach or eliminating components completely. This initial UWMS paper will describe the system layout approach and a few key features of major components. Future papers will describe the UWMS functionality, test results, and components as they are developed.

Stapleton, Thomas J.↗
DOE OSTI2014

Genome analyses of the carboxydotrophic sulfate-reducers Desulfotomaculum nigrificans and Desulfotomaculum carboxydivorans and reclassification of Desulfotomaculum caboxydivorans as a later synonym of Desulfotomaculum nigrificans

Desulfotomaculum nigrificans and D. carboxydivorans are moderately thermophilic members of the polyphyletic spore-forming genus Desulfotomaculum in the family Peptococcaceae. They are phylogenetically very closely related and belong to ‘subgroup a’ of the Desulfotomaculum cluster 1. D. nigrificans and D. carboxydivorans have a similar growth substrate spectrum; they can grow with glucose and fructose as electron donors in the presence of sulfate. Additionally, both species are able to ferment fructose, although fermentation of glucose is only reported for D. carboxydivorans. D. nigrificans is able to grow with 20% carbon monoxide (CO) coupled to sulfate reduction, while D. carboxydivorans can grow at 100% CO with and without sulfate. Hydrogen is produced during growth with CO by D. carboxydivorans. Here we present a summary of the features of D. nigrificans and D. carboxydivorans together with the description of the complete genome sequencing and annotation of both strains. Moreover, we compared the genomes of both strains to reveal their differences. This comparison led us to p

Peptococcaceae↗
DOE OSTI2023

Hierarchically Templated Synthesis of 3D‐Printed Crosslinked Cyclodextrins for Lycopene Harvesting

Abstract Plants produce a wide range of bioactive phytochemicals, such as antioxidants and vitamins, which play crucial roles in aging prevention, inflammation reduction, and reducing the risk of cancer. Selectively harvesting these phytochemicals, such as lycopene, from tomatoes through the adsorption method is cost‐effective and energy efficient. In this work, a templated synthesis of 3D‐printed crosslinked cyclodextrin polymers featuring nanotubular structures for highly selective lycopene harvesting is reported. Polypseudorotaxanes formed by triethoxysilane‐based telechelic polyethylene glycols and α‐cyclodextrins (α‐CDs) are designed as the template to (1) synthetically access urethane‐based nanotubular structures at the molecular level, and (2) construct 3D‐printed architectures with designed macroscale voids. The polypseudorotaxane hydrogels showed good rheological properties for direct ink writing, and the 3D‐printed hydrogels were converted to the desired α‐CD polymer network through a three‐step postprinting transformation. The obtained urethane‐crosslinked α‐CD monoliths possess nanotubular structures and 3D‐printed voids. They selectively adsorb lycopene from raw tomato juice, protecting lycopene from photo‐ or thermo‐degradations. This work highlights the hierarchically templated synthesis approach in developing functional 3D‐printing materials by connecting the bottom‐up molecular assembly and synthesis with the top‐down 3D architecture control and fabrication.

Chemistry↗
DOE OSTI2018

Abrupt cloud clearing of marine stratocumulus in the subtropical southeast Atlantic

We document rapid and abrupt clearings of large portions of the subtropical marine low cloud deck that have implications for the global radiation balance and climate sensitivity. Over the southeast Atlantic, large areas of stratocumulus are quickly eroded, yielding partial or complete clearing along sharp transitions hundreds to thousands of kilometers in length that move westward at 8 to 12 meters per second and travel as far as 1000+ kilometers from the African coast. The westward-moving cloudiness reductions have an annual peak in occurrence in the period from April through June. The cloud erosion boundaries reduce cloud at ≈10-kilometer scale in less than 15 minutes, move approximately perpendicular to the mean flow, and are often accompanied by small-scale wave features. Observations suggest that the cloud erosion is caused by atmospheric gravity waves.

Science & Technology - Other Topics↗
DOE OSTI2025

Mechanical properties, strain hardening, and fracture behavior of ultrasonic additively manufactured Zircaloy-4 after low-temperature neutron irradiation

Ultrasonic additive manufacturing (UAM) is a solid-state, layer-by-layer advanced manufacturing process that has the potential to create custom spatially controlled composites with embedded wires and sensors for nuclear component manufacture. For this work, to assess the feasibility of using UAM for nuclear-relevant materials research, the technique was used to produce a 3.5-mm-thick Zircaloy-4 plate for irradiation testing. The UAM Zircaloy-4 specimens were irradiated in the High Flux Isotope Reactor at a target irradiation temperature of 117 °C to 2.9 displacements per atom (dpa) to assess differences in irradiation-hardening behavior as a function of alloy processing path. The UAM and reference baseplate (BP) materials increased in yield strength by 372±27 MPa and 346±21 MPa, respectively, and both suffered significant reductions in uniform and total elongation attributed to irradiation hardening at low-temperature. Although the materials had similar nanoscale defect structures, including nanoscale black dot/loop features and strain-induced dislocation channels, the UAM material’s processing-related defects resulted in accelerated strain localization and failure as demonstrated by lower post-irradiation uniform elongation of UAM specimens (0.5 %) compared to BP (1.5 %) material. The UAM material also showed considerable anisotropy in mechanical response due to crack propagation along weld boundaries, resulting in differences in strength & ductility when tested parallel and perpendicular to the prior UAM build orientation. Therefore, although the fundamental irradiation response of UAM-processed Zircaloy-4 was phenomenologically comparable to that of BP reference material, additional optimization of the UAM processing is needed to produce irradiation-resistant and nuclear-relevant materials.

Digital image correlation↗
DOE OSTI2024

A flexible class of priors for orthonormal matrices with basis function-specific structure

Statistical modeling of high-dimensional matrix-valued data motivates the use of a low-rank representation that simultaneously summarizes key characteristics of the data and enables dimension reduction. Low-rank representations commonly factor the original data into the product of orthonormal basis functions and weights, where each basis function represents an independent feature of the data. However, the basis functions in these factorizations are typically computed using algorithmic methods that cannot quantify uncertainty or account for basis function correlation structure a priori. While there exist Bayesian methods that allow for a common correlation structure across basis functions, empirical examples motivate the need for basis function-specific dependence structure. We propose a prior distribution for orthonormal matrices that can explicitly model basis function-specific structure. The prior is used within a general probabilistic model for singular value decomposition to conduct posterior inference on the basis functions while accounting for measurement error and fixed effects. We discuss how the prior specification can be used for various scenarios and demonstrate favorable model properties through synthetic data examples. Finally, we apply our method to two-meter air temperature data from the Pacific Northwest, enhancing our understanding of the Earth system’s internal variability.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2019

Iodosylbenzene Coordination Chemistry Relevant to Metal–Organic Framework Catalysis

Hypervalent iodine compounds formally feature expanded valence shells at iodine. These reagents are broadly used in synthetic chemistry due to the ability to participate in well-defined oxidation-reduction processes and because the ligand-exchange chemistry intrinsic to the hypervalent center allows hypervalent iodine compounds to be applied to a broad array of oxidative substrate functionalization reactions. We have recently developed methods to generate these compounds from O 2 that are predicated on diverting reactive intermediates of aldehyde autoxidation towards the oxidation of aryl iodides. Coupling the aerobic oxidation of aryliodides with catalysts that effect C–H bond oxidation would provide a strategy to achieve aerobic C–H oxidation chemistry. In this Forum article we discuss the aspects of hypervalent iodine chemistry and bonding that render this class of reagents attractive lynchpins for aerobic oxidation chemistry. We then discuss the oxidation processes relevant to the aerobic preparation of 2-(tertbutylsulfonyl) iodosylbenzene, which is a popular hypervalent iodine reagent for use with porous metal-organic framework-based catalysts because it displays significantly enhanced solubility as compared with unsubstituted iodosylbenzene. We demonstrate that popular synthetic methods to this reagent often provide material that displays unpredictable disproportionation behavior due to the presence of trace impurities. We provide a revised synthetic route that avoids impurities common in the reported methods and provides access to material that displays predictable stability. Lastly, we describe the coordination chemistry of hypervalent iodine compounds with metal clusters relevant to MOF chemistry and discuss the potential implications of this coordination chemistry to catalysis in MOF scaffolds.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Synergistic Solvent-Surface Interactions Enable Alkyne Semihydrogenation at Palladium

Enabling higher yield and better selectivity for fine-chemical synthesis through heterogeneous catalysis is intricately linked to the interplay of active sites, reaction conditions, and mass transfer influence provided by the catalyst. Alkyne semihydrogenation is ubiquitous in the production of bulk chemicals in the pharmaceutical, polymer, or fine-chemical industries, but product selectivity remains a major challenge. Here, in this study, we demonstrate that the design of catalysts encompassing nickel (Ni) foams as contiguous monolith supports, decorated with ultralow loading of Pd/PdO x nanoparticles on a carbonized polydopamine interface and tuned with a thin layer of Al 2 O 3 , in conjunction with an optimized reaction environment leads to highly selective alkyne semihydrogenation. The reactions demonstrate good functional group tolerance and applicability to flow reactor systems. Combined computational and experimental studies are presented to describe the synergistic effect between the solvent-surface interaction and the degree of Pd surface reduction that are necessary to promote this selectivity. The system highlights the opportunity for catalyst-solvent codesign as a benign alternative to more complex reactants featuring extrinsic poisons or less-favored dopants.

atomic layer deposition↗
DOE OSTI2017

Platinum–nickel nanowire catalysts with composition-tunable alloying and faceting for the oxygen reduction reaction

The ability to tune the alloying properties and faceting characteristics of bimetallic nanocatalysts is essential for designing catalysts with enhanced activity and stability through optimizing strain and ligand effects, which is an important frontier for designing advanced materials as catalysts for fuel cell applications. This report describes composition-controlled alloying and faceting of platinum–nickel nanowires (PtNi NWs) for the electrocatalytic oxygen reduction reaction. The PtNi NWs are synthesized by a surfactant-free method and are shown to display bundled morphologies of nano-tetrahedra or nanowires, featuring an ultrathin and irregular helix morphology with composition-tunable facets. Using high-energy synchrotron X-ray diffraction coupled with atomic pair distribution function analysis, lattice expansion and shrinking are revealed, with the Pt : Ni ratio of ~3 : 2 exhibiting a clear expansion, which coincides with the maximum electrocatalytic activity for the ORR. In comparison with PtNi nanoparticles (NPs), the PtNi NWs display remarkably higher electrocatalytic activity and stability as a result of the composition dependent atomic-scale alloying and faceting, demonstrating a new pathway to the design of alloy nanocatalysts with enhanced activity and durability for fuel cells.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Self-similar structure and experimental signatures of suprathermal ion distribution in inertial confinement fusion implosions

The distribution function of suprathermal ions is found to be self-similar under conditions relevant to inertial confinement fusion hot spots. By utilizing this feature, interference between the hydrodynamic instabilities and kinetic effects is for the first time assessed quantitatively to find that the instabilities substantially aggravate the fusion reactivity reduction. Thus, the ion tail depletion is also shown to lower the experimentally inferred ion temperature, a novel kinetic effect that may explain the discrepancy between the exploding pusher experiments and rad-hydro simulations and contribute to the observation that temperature inferred from DD reaction products is lower than from DT at the National Ignition Facility.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗