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At least 883 records · Page 49

Strengthening of tungsten by coherent rhenium precipitates formed during low fluence irradiation

Experimental data show that the accumulation of rhenium and osmium from transmutation reactions severely affect the microstructural evolution and property degradation of tungsten-based materials under neutron irradiation. Theory and modeling have confirmed that Re atom transport in W is by irradiation-produced migrating self-interstitial atoms. With this diffusion mode in operation, a specific microstructure evolution is realized when at relatively low neutron fluence the Re-rich precipitates are formed, while the void and interstitial loop population development is suppressed, affecting the mechanical properties. Here, this research shows the effect of small coherent Re-rich precipitates on the dislocation glide under stress, investigated using the molecular dynamics approach with empirical interatomic potentials. The results are compared with an earlier simulation of void hardening in W. It is demonstrated that small coherent Re-rich precipitates of less than 6 nm diameter represent relatively weak obstacles for moving edge dislocations. The implication of these results on the interpretation of experimental results is discussed.

36 MATERIALS SCIENCE↗

Lifetime measurements in the even-even Cd 102 – 108 isotopes

The heaviest T z = 0 doubly-magic nucleus, Sn 100 , and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction. For instance, the structure of light-Sn nuclei has been shown to be affected by the delicate balance between nuclear-interaction components, such as pairing and quadrupole correlations. From Cd to Te, many common features and phenomena have been observed experimentally along the isotopic chains, leading to theoretical studies devoted to a more general and comprehensive study of the region. In this context, having only two proton holes in the Z = 50 shell, the Cd isotopes are expected to present properties similar to those found in the Sn isotopic chain. The aim of this work was to measure lifetimes of excited states in neutron-deficient nuclei in the vicinity of Sn 100 . Here, the neutron-deficient nuclei in the N ≈ Z ≈ 50 region were populated using a multinucleon transfer reaction with a Cd 106 beam and a Mo 92 target. The beamlike products were identified by the VAMOS + + spectrometer, while the γ rays were detected using the AGATA array. Lifetimes of excited states were determined using the recoil distance Doppler-shift method, employing the Cologne differential plunger. Lifetimes of low-lying states were measured in the even-mass Cd 102 – 108 isotopes. In particular, multiple states with excitation energy up to ≈ 3 MeV, belonging to various bands, were populated in Cd 106 via inelastic scattering. The transition strengths corresponding to the measured lifetimes were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach. Conclusions: Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z = 48 and Z = 50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with β 2 ≈ 0.2 . At this deformation Z = 48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

(U) Energy-Dependent Perturbations of Scattering Cross Sections Using the PERT Card in MCNP6.2

The PERT card is used for first- and second-order perturbations of material densities, isotope densities, and isotope cross sections in the MCNP6.2 Monte Carlo code. Using the PERT card for firstand second-order sensitivities is straightforward. Reference 2 only looked at density perturbations with no energy dependence. This report looks at the sensitivity of a response to scattering cross sections as a function of energy and finds that there is a bug in the PERT capability. The SENSMG multigroup neutron sensitivity code was recently given the capability of computing sensitivities to user-specified reactions whose cross sections are available in a user-supplied NJOY output file. SENSMG uses the PARTISN multigroup discrete ordinates code for the transport. The NJOY-reaction capability is similar to that of SUSD3D, which also uses PARTISN for the multigroup transport. The PERT bug was identified by comparing MCNP6.2 outputs with SENSMG outputs. The next section of this report describes the test problem. Section III presents the MCNP6.2 PERT bug and proposes a solution. Section IV is a summary and conclusions. The SENSMG and MCNP input files are listed in the appendix.

07 ISOTOPE AND RADIATION SOURCES↗

Time-dependent 2.2 MeV and 0.5 MeV lines from solar flares

The time dependences of the 2.2 MeV and 0.51 MeV gamma ray lines from solar flares are calculated and the results are compared with observations of the 1972, August 4 and 7 flares. Time lag between the nuclear reactions and the formation of these two lines are caused, respectively, by capture of the neutrons, and by deceleration of the positrons and decay of the radioactive nuclei. Results show that the calculation is consistent with the observed rise of the 2.2 MeV line on August 4, and it does not require different time dependences for the accelerated protons and electrons in the flare region. The above lags can explain the delayed gamma ray emission observed on August 7. Positrons of energies greater than about 10 MeV could be detected in interplanetary space following large solar flares.

Wang, H. T.↗

X-ray bursts and neutron-star thermonuclear flashes

A description is presented of a model concerning the production of X-ray bursts by thermonuclear flashes in the freshly accreted matter near the surface of an accreting neutron star. An investigation is conducted regarding the physical processes relevant to such thermonuclear flashes. It is concluded that thermonuclear flashes may account for some, but not all, of the observed X-ray burst sources. Attention is given to a neutron star undergoing accretion of mass from a binary stellar companion, aspects of energetics, nuclear reactions, and heat transport mechanisms.

Joss, P. C.↗

Cosmogenic nuclides: Observable effects of Martian volatiles

Cosmic-ray produced (cosmogenic) nuclides in returned Martian samples could be used to study the amounts and distributions of volatiles in the recent past on Mars. In planning for the gamma-ray spectrometer experiment that is scheduled to fly on the Mars Observer, many calculations were done on the nuclear reactions that should occur in the Martian surface, studying especially the production and transport of neutrons. It is found that three aspects of Mars can very significantly affect the production of cosmogenic products in Mars: the Martian atmosphere and the presence of H2O in or CO2 on the surface of Mars. These volatile components can greatly affect the energy and spatial distributions of neutrons, expecially those with thermal or near thermal energies, in the surface of Mars. In turn, these neutrons produce many cosmogenic nuclides that can be observed in samples returned from Mars.

Reedy, R. C.↗

Apparatus and method for generating medical isotopes

An apparatus for generating medical isotopes provides an annular fissile solution vessel surrounding a neutron generator. The annular fissile solution vessel provides for good capture of the emitted neutrons and a geometry that provides enhanced stability in an aqueous reactor. A neutron multiplier and/or a neutron moderator may be used to improve the efficiency and control the criticality of the reaction in the annular fissile solution vessel.

Piefer, Gregory Richard↗

Configuration mixing in 28 Mg and the 26 Mg (t,p) 28 Mg reaction

We have studied the 26 Mg(t,p) 28 Mg reaction. The nucleus 28 Mg lies between 24 Mg and 32 Mg, the latter of which is central to the “island of inversion” characterized by low-lying neutron fp-shell configurations. The present results show that the second-excited 0 + state in 28 Mg contains large fp-shell occupation for the neutrons. The experiment was performed in inverse kinematics using the HELIcal Orbit Spectrometer (HELIOS) at Argonne National Laboratory. Shell-model calculations using the SDPF-MU interaction yielded level energies and two-neutron transfer amplitudes that were used in one-step distorted-wave Furthermore, born approximation calculations to provide theoretical predictions of the proton angular distributions. In many, but not all cases, the data were in good agreement with theoretical predictions.

20 ≤ A ≤ 38↗

Properties of hadron matter. II - Dense baryon matter and neutron stars.

In this article we have provided certain details of a nuclear-matter computation, based on the Brueckner-Bethe-Goldstone theory of nuclear reaction, which leads to an equation of state for matter in the density region of 10 to 500 trillion g/cu cm. We also explore the possibilities that at very high baryon densities or for very short baryon separations, the net baryon-baryon interaction may be negligible so that the results of dynamical models, like the statistical bootstrap model and the dual-resonance model, may be applicable to the study of dense baryon matter. Several plausible equations of state are constructed, and their effect on the limiting mass of the neutron star is examined.

Leung, Y. C.↗

(U) A Code System for Cross-Section Uncertainty Propagation for PARTISN

A rudimentary code system has been developed for propagating neutron cross-section uncertainties to response uncertainties using the PARTISN multigroup discrete-ordinates neutron transport code. The code system uses the first-order sandwich rule with sensitivities computed using SENSMG and covariances computed using NJOY. Databases of reaction cross sections and covariances using ENDF/B-VIII.0 data in the LANL standard 30-group structure have been precalculated. The final uncertainty in a k eff example problem compares well with the result from TOFFEE, a similar code that propagates neutron cross-section uncertainties to response uncertainties using the MCNP6 Monte Carlo neutron transport code. Presently, neither code system propagates uncertainties in $\overline{v}$, $\overline{μ}$, or χ, and neither code system propagates nuclide-nuclide covariances

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Ultrarelativistic Heavy-Ion Reactions at the LHC with the CMS Detector

This grant funded the travel to CERN to allow participation in the 2018 PbPb run as part of the Compact Muon Solenoid (CMS) detector collaboration. Among the activities performed were the testing and installation of the spectator reaction plane detector (SRPD). This detector was designed and constructed by the heavy ion group at the University of Maryland. Its purpose is to map the spacial distribution of the spectator neutrons that make it at zero degrees to the Zero Degree Calorimeter (ZDC), located 140 meters from the interaction point of CMS. This will be used to determine the spectator reaction plane for the PbPb collisions. During this heavy ion run at the LHC, there was also the opportunity to participate in a test beam at the CERN SPS. A duplicate copy of the SRPD was used in this test. This report focuses on the results from the test beam.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A revisitation of the ENEA TAPIRO Fast Source Reactor neutronic capabilities

This work is devoted to the analysis of the neutronic characterization of the ENEA-Casaccia center RSV TAPIRO fast neutrons source reactor performed during the 80's in the frame of a joint ENEA-SCK-CEN Mol collaboration. The Belgian scientist Albert Fabry, who was available to investigate a fast research reactor to perform a full characterization of the system neutron flux, led the TAPIRO experimental campaign. In particular, the paper is focused on the comparison between some 'recommended' Fabry experimental reaction rates traverses and nowadays MCNP Monte Carlo and ERANOS deterministic calculation results. It appears that the quality of the results depends on the penetration depth into the copper reflector. The influence of copper nuclear data are more evident in the ERANOS results. Massimo Salvatores has provided a great contribution to the interpretation of the TAPIRO neutronics: this humble work is dedicated to him.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Quantification of the 35 Cl($\textit{n, p}$) reaction channel

The evaluated 35 Cl($\textit{n, p}$) cross sections in the ENDF/B-VIII.0 nuclear data library remain uncertain because of the lack of measured data in the neutron energy range between 100-600 keV. In this energy region, the R-matrix analysis relies heavily on estimated ($\textit{n, p}$) partial widths and level density information. This resulted in significant differences of the evaluated cross sections and predicted reactivity in nuclear reactor applications with respect to previous nuclear data libraries. Here, we present a methodology to quantify the cross sections for the 35 Cl($\textit{n, p}$) reaction channel from the combination of measured total cross sections and model calculations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A STUDY OF SHORT-RANGE CORRELATED PAIR FORMATION MECHANISMS

Short-Range Correlations (SRCs) refers to pairs of nucleons that are temporary high density fluctuations with high relative momenta and lower center-of-mass momenta com pared to the nuclear Fermi momentum (kF). SRCs account for 20–25% of the nucleons in medium to heavy nuclei, make up essentially all nucleons with momentum greater than kF, and contribute most of the kinetic energy carried by nucleons in nuclei. The existing semi-inclusive and exclusive measurements only cover a handful of light nu clei or heavy elements. This does not allow for a systematic study of the dependence of SRC pairs on nuclear mass and proton-neutron asymmetry. It also does not allow for insights into SRC pairing mechanisms. Therefore, we systematically studied the individual probabilities for finding SRC protons in symmetric and neutron-rich asymmetric nuclei d, 9Be, 10B, 11B, 12C, 40Ca, 48Ca, 54Fe, and 197Au. We measured the (e,e'p) reaction in kinematics dominated by scattering off mean-field nucleons (k = kF) and nucleons in SRC pairs (k = kF) at the Thomas Jefferson National Accelerator Facility (JLab) in Hall C of the Continuous Electron Beam Accelerator Facility (CEBAF) in the Fall of 2022. The measured results were used to determine the SRC pairing probabilities for protons to examine how pairing depends on nuclear mass, proton-neutron asymmetry, and nuclear shell structure. The extracted cross-section ratios were also compared to theoretical calculations. We found that SRC pair formation depends more on the nuclear shell structure with sharp increases locally within the general trend of a slower increase with larger A. We also found that intra-shell pairing has a much larger influence than inter-shell pairing. Comparisons to theory suggest that angular momentum selection rules are important to SRC pair formation and can provide new constraints for new theoretical models.

Swan, Noah [Old Dominion Univ., Norfolk, VA (Unite↗

Lasers for the observation of multiple order nuclear reactions

Nuclear reaction rates become nonlinear with respect to flux (cm −2 s −1 ) in extreme environments such as those found during stellar nucleosynthesis and terrestrial nuclear detonations. To observe these effects directly in the laboratory, extremely high particle fluences (cm −2 ) are necessary but not sufficient. Reactor-based neutron sources, such as the Institut Laue-Langevin’s high-flux neutron reactor, were previously the closest to meeting this challenge, albeit over ∼hour time scales. In ultra-high flux environments, where multiple reactions occur on picosecond time scales, nuclei are unable to return to their ground states between reactions; consequently, reactions take place on excited nuclei. To accurately model high-flux environments, data on the cross-sections of excited nuclear states are required, which differ significantly from those of ground states due to spin/parity effects. In order to replicate these effects in the laboratory, short high-fluence pulses on the order of the lifetime of a typical nuclear excited state (generally ≲1 ns) are required. Particle beams generated by high-intensity lasers are uniquely positioned to meet this need with the potential to produce fluences of 10 17 protons/cm 2 and 10 22 neutrons/cm 2 over a few pico-seconds or less. In addition to providing a quantitative analysis of the rates of multiple rapid reactions in general, the present work examines a number of laser-based experiments that could be conducted in the near future to observe multiple rapid reactions for laboratory-based astrophysics and the measurement of exotic cross-sections.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Astrophysics through simulations of neutron star mergers using Monte‐Carlo neutrino radiation transport (DE-SC0020435 Final Technical Report)

Neutron star mergers are an important source of information for nuclear physics. Except for black holes, neutron stars are the densest macroscopic objects known to exist in the Universe. They provide us with a remarkable laboratory to study the poorly understood high-density states of matter, complementing the study of heavy nuclei performed by nuclear physics experiments on Earth. Collisions of neutron stars are of particular interest. They are among the most energetic events observable in the Universe, powering a broad range of signals across the electromagnetic spectrum as well as gravitational wave signals. These signals contain important information about the properties of extremely dense matter. Colliding neutron stars additionally eject large amounts of neutron-rich material into the surrounding interstellar medium -- material that then undergoes rapid neutron-capture (r-process) nucleosynthesis, the mechanism thought to be responsible for the production of about half of the heavy nuclei. In order to understand current and future observations of neutron star mergers, we need reliable models for the signals that they power. An important component in the construction of such models are numerical simulations of colliding neutron stars. These simulations are costly, running for multiple months on supercomputers, and require the inclusion of complex physics (general relativity, magnetohydrodynamics, neutrino physics, nuclear reactions). In this document, we describe the development of new methods for the treatment of neutrinos in merger simulations, as well as the first simulations capable of evolving the equations of neutrino radiation transport directly and their impact on our understanding of neutron star mergers and more broadly in nuclear astrophysics. We also discuss additional work performed in the study of nucleosynthesis and neutrino physics in neutron star mergers as part of Early Career Award DE-SC0020435.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Production of C-14 and neutrons in red giants

We have examined the effects of mixing various amounts of hydrogen-rich material into the intershell convective region of red giants undergoing helium shell flashes. We find that significant amounts of C-14 can be produced via the N-14(n, p)C-14 reaction. If substantial portions of this intershell region are mixed out into the envelopes of red giants, then C-14 may be detectable in evolved stars. We find a neutron flux many orders of magnitude above the flux required for the classical s-process, and thus an intermediate neutron process (i-process) may operate in evolved red giants. In all cases studied we find substantial enhancements of O-17. These mixing models offer a plausible explanation of the observations of enhanced O-17 in the carbon star IRC 10216. For certain physical conditions we find significant enhancements of N-15 in the intershell region.

Cowan, J. J.↗

GCR Transport in the Brain: Assessment of Self-Shielding, Columnar Damage, and Nuclear Reactions on Cell Inactivation Rates

Radiation shield design is driven by the need to limit radiation risks while optimizing risk reduction with launch mass/expense penalties. Both limitation and optimization objectives require the development of accurate and complete means for evaluating the effectiveness of various shield materials and body-self shielding. For galactic cosmic rays (GCR), biophysical response models indicate that track structure effects lead to substantially different assessments of shielding effectiveness relative to assessments based on LET-dependent quality factors. Methods for assessing risk to the central nervous system (CNS) from heavy ions are poorly understood at this time. High-energy and charge (HZE) ion can produce tissue events resulting in damage to clusters of cells in a columnar fashion, especially for stopping heavy ions. Grahn (1973) and Todd (1986) have discussed a microlesion concept or model of stochastic tissue events in analyzing damage from HZE's. Some tissues, including the CNS, maybe sensitive to microlesion's or stochastic tissue events in a manner not illuminated by either conventional dosimetry or fluence-based risk factors. HZE ions may also produce important lateral damage to adjacent cells. Fluences of high-energy proton and alpha particles in the GCR are many times higher than HZE ions. Behind spacecraft and body self-shielding the ratio of protons, alpha particles, and neutrons to HZE ions increases several-fold from free-space values. Models of GCR damage behind shielding have placed large concern on the role of target fragments produced from tissue atoms. The self-shielding of the brain reduces the number of heavy ions reaching the interior regions by a large amount and the remaining light particle environment (protons, neutrons, deuterons. and alpha particles) may be the greatest concern. Tracks of high-energy proton produce nuclear reactions in tissue, which can deposit doses of more than 1 Gv within 5 - 10 cell layers. Information on rates of cell killing from GCR, including patterns of cell killing from single particle tracks. can provide useful information on expected differences between proton and HZE tracks and clinical experiences with photon irradiation. To model effects on cells in the brain, it is important that transport models accurately describe changes in the GCR due to interactions in the cranium and proximate tissues. We describe calculations of the attenuated GCR particle fluxes at three dose-points in the brain and associated patterns of cell killing using biophysical models. The effects of the brain self-shielding and bone-tissue interface of the skull in modulating the GCR environment are considered. For each brain dose-point, the mass distribution in the surrounding 4(pi) solid angle is characterized using the CAM model to trace 512 rays. The CAM model describes the self-shielding by converting the tissue distribution to mass-equivalent aluminum, and nominal values of spacecraft shielding is considered. Particle transport is performed with the proton, neutron, and heavy-ion transport code HZETRN with the nuclear fragmentation model QMSFRG. The distribution of cells killed along the path of individual GCR ions is modeled using in vitro cell inactivation data for cells with varying sensitivity. Monte Carlo simulations of arrays of inactivated cells are considered for protons and heavy ions and used to describe the absolute number of cell killing events of various magnitude in the brain from the GCR. Included are simulations of positions of inactivated cells from stopping heavy ions and nuclear stars produced by high-energy ions most importantly, protons and neutrons.

Shavers, M. R.↗