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At least 883 records · Page 49
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Minimizing particle aggregation in Sm 2 Fe 17 N 3 powders: A CaO-assisted reduction-diffusion approach

We report a novel synthesis of Sm 2 Fe 17 N 3 powders using a CaO-assisted reduction-diffusion (RD) approach. CaO plays a crucial role during mechanochemical processing – acting both as a dispersant and a surface coating agent, which helps to prevent agglomeration due to sintering of Sm 2 Fe 17 particles during the RD step. Together with the added dispersant, the CaO by-product formed during RD can be easily removed in the washing step resulting in fewer aggregated Sm 2 Fe 17 N 3 particles and lower oxygen contamination in the final product. The impact of varying CaO amounts was examined, and synthesis conditions were optimized to achieve phase-pure Sm 2 Fe 17 N 3 powders with less aggregation of magnetic particles. The powders synthesized with addition of 1 wt% CaO as dispersant exhibited the highest hard-magnetic properties: a coercivity (H c ) of 10.7 kOe and a maximum energy product ((BH) max ) of 17.3 MGOe. By densifying the Sm 2 Fe 17 N 3 powders using high-pressure spark plasma sintering, a bulk magnet with a (BH) max of 21.1 MGOe with 88 % of theoretical density was produced. In conclusion, reducing aggregation of the Sm 2 Fe 17 N 3 increases coercivity and remanence of these magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Electromagnetic turbulence in increased β plasmas in the Large Plasma Device

The variation of pressure-gradient-driven turbulence with plasma $\beta$ (up to $\beta \approx 15\,\%$ ) is investigated in linear, magnetized plasma. The magnitude of magnetic fluctuations is observed to increase substantially with increasing $\beta$ . More importantly, parallel magnetic fluctuations are observed to dominate at higher $\beta$ values, with $\delta B_\parallel / \delta B_\perp \approx 2$ and $\delta B / B_0 \approx 1\,\%$ . Parallel magnetic fluctuations are strongly correlated with density fluctuations and the two are observed to be out of phase. The relative magnitude of and cross-phase between density and parallel magnetic field fluctuations are consistent with the dynamic pressure balance ( $P+{B_{0}^2}/{2\mu _0} = \textrm {constant}$ ). A local slab model theory for electromagnetic, modified drift Alfvén waves, including parallel magnetic fluctuations, shows partial agreement with experimental observations.

Physics↗
NASA NTRS1993

Magnetospheric response to solar wind dynamic pressure variations: Interaction of interplanetary tangential discontinuities with the bow shock

Some magnetic impulse events observed in the polar region are related to vortices associated with plasma convection in the ionosphere. Recent analyses of satellite and ground data suggest that the interaction of solar wind dynamic pressure pulses and the magnetosphere may lead to the formation of velocity vortices in the magnetopause boundary layer region. This can in turn lead to the presence of vortices in the polar ionosphere. However, before reaching the Earth's magnetopause, these interplanetary pressure pulses must interact with and pass through the bow shock. A variation of the solar wind dynamic pressure may be associated with shocks, magnetic holes, or tangential discontinuities (TDs) in the interplanetary medium. We study the interaction of interplanetary TDs with the Earth's bow shock (BS) using both theoretical analysis and MHD computer simulations. It is found that as a result of the collision between a TD and the BS, the jump in the solar wind dynamic pressure associated with the TD is significantly modified, the bow shock moves, and a new fast shock or fast rarefaction wave, which propagates in the downstream direction, is excited. Our theoretical analysis shows that the change in the plasma density across the interplanetary TD plays the most important role in the collision process. In the case with an enhanced dynamic pressure behind the interplanetary TD, the bow shock is intensified in strength and moves in the earthward direction. The dynamic pressure jump associated with the transmitted TD is generally reduced from the value before the interaction. A fast compressional shock is excited ahead of the transmitted TD and propagates toward the Earth's magnetosphere. For the case in which the dynamic pressure is reduced behind the interplanetary TD, the pressure jump across the transmitted TD is substantially weakened, the bow shock moves in the sunward direction, and a rarefaction wave which propagates downstream is excited. We also simulate and discuss the interaction of a pair of tangential discontinuities, which may correspond to a magnetic hole, with the BS.

Wu, Bor-Han↗
DOE OSTI2023

Electronic structure, dimer physics, orbital-selective behavior, and magnetic tendencies in the bilayer nickelate superconductor $\mathrm{La_3Ni_2O_7}$under pressure

Motivated by the recently reported high-temperature superconductivity in the bilayer La 3 Ni 2 O 7 (LNO) under pressure, we comprehensively study this system using ab initio techniques. The Ni 3d orbitals have a large bandwidth at ambient pressure, increasing by ~22% at 29.5 GPa. Without electronic interactions, the Ni d 3z 2 -r 2 orbitals form a bonding-antibonding molecular orbital state via the O p z inducing a “dimer” lattice in the LNO bilayers. The Fermi surface consists of two-electron sheets with mixed e g orbitals and a hole pocket defined by the d 3z 2 -r 2 orbital, suggesting a Ni two-orbital minimum model. Different from the infinite-layer nickelate, we obtained a large interorbital hopping between d 3z 2 -r 2 and d x 2 -y 2 states in LNO, caused by the ligand “bridge” of in-plane O p x or p y orbitals connecting those two orbitals, inducing d-p σ-bonding characteristics. The competition between the intraorbital and interorbital hoppings leads to an interesting dominant spin stripe (π,0) order because of bond ferromagnetic tendencies via the recently discussed “half-empty” mechanism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Pressure-induced shift of effective Ce valence, Fermi energy and phase boundaries in CeOs 4 Sb 12

Abstract CeOs 4 Sb 12 , a member of the skutterudite family, has an unusual semimetallic low-temperature L -phase that inhabits a wedge-like area of the field H —temperature T phase diagram. We have conducted measurements of electrical transport and megahertz conductivity on CeOs 4 Sb 12 single crystals under pressures of up to 3 GPa and in high magnetic fields of up to 41 T to investigate the influence of pressure on the different H – T phase boundaries. While the high-temperature valence transition between the metallic H -phase and the L -phase is shifted to higher T by pressures of the order of 1 GPa, we observed only a marginal suppression of the S -phase that is found below 1 K for pressures of up to 1.91 GPa. High-field quantum oscillations have been observed for pressures up to 3.0 GPa and the Fermi surface of the high-field side of the H -phase is found to show a surprising decrease in size with increasing pressure, implying a change in electronic structure rather than a mere contraction of lattice parameters. We evaluate the field-dependence of the effective masses for different pressures and also reflect on the sample dependence of some of the properties of CeOs 4 Sb 12 which appears to be limited to the low-field region.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Coupled Experimental/Computational Investigation of the Dynamics of Interacting Magnetized Plasmas

The interaction, or interpenetration, of magnetized plasmas of different density and/or pressure occurs in a wide variety of natural and man-made systems. Such systems include extragalactic jets propagating into the intergalactic medium, solar coronal mass ejections into background solar wind, compact toroid (CT) fueling of magnetic fusion plasmas, and jets of capsule shell impurities into DT fusion fuel, which can lead to enhanced impurity mix in inertial fusion implosions. These plasmas may take the form of jets, with open, helical magnetic structure, or plasma “bubbles” with closed magnetic fields (B-fields), such as spheromaks or CT’s. Such structures, both open and closed B-field cases, can transport heat, particles and magnetic flux or magnetic helicity into background plasma regions. For example, the origin of extragalactic magnetic fields may be due, at least in part, to transport by astrophysical jets. The goal of this proposed work was to elucidate the detailed plasma and magnetic field dynamics of high-density plasma jets (open B-field) and bubbles (closed B-field) propagating into lower density background magnetized plasma through controlled laboratory experiments and closely coupled nonlinear MHD modeling. These experiments were conducted in the HelCat (Helicon-Cathode) linear plasma device at the University of New Mexico (UNM). Plasma jets and bubbles were launched via an existing compact coaxial plasma gun, mounted on the HelCat device. This gun produced plasmas tens of cm in scale and lasting tens of microseconds, thereby allowing detailed multipoint, space- and time-resolved measurements to be made routinely. The experiments were directly modeled using the extended magnetohydrodynamic (XMHD) PERSEUS code, developed at Cornell University [23,24]. Both experimental and numerical modeling work are ongoing. The main results to date are reported here. Additional supplemental funding for one year (8/1/2019 – 7/31/2020) supported numerical investigation of photoionization processes important in many low temperature plasmas, including the HelCat device. Initial results of this modeling work is also reported.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1993

Energy storage and dissipation in the magnetotail during substorms. I - Particle simulations. II - MHD simulations

2D electromagnetic particle simulations are used to investigate the dynamics of the tail during development of substorms under the influence of the pressure in the magnetospheric boundary layer and the dawn-to-dusk electric field. It is shown that pressure pulses result in thinning of the tail current sheet as the magnetic field becomes pinched near the region where the pressure pulse is applied. The pinching leads to the tailward flow of the current sheet plasma and the eventual formation and injection of a plasmoid. Surges in the dawn-to-dusk electric field cause plasma on the flanks to convect into the center of the current sheet, thereby thinning the current sheet. The pressure in the magnetospheric boundary laser is coupled to the dawn-to-dusk electric field through the conductivity of the tail. Changes in the predicted evolution of the magnetosphere during substorms due to changes in the resistivity are investigated under the assumption that MHD theory provides a suitable representation of the global or large-scale evolution of the magnetotail to changes in the solar wind and to reconnection at the dayside magnetopause. It is shown that the overall evolution of the magnetosphere is about the same for three different resistivity distributions with plasmoid formation and ejection in each case.

Winglee, R. M.↗
DOE OSTI2020

Kinetic Simulations of Radiative Magnetic Reconnection in the Coronae of Accreting Black Holes

We perform 2D and 3D particle-in-cell simulations of reconnection in magnetically dominated e ± plasmas subject to strong Compton cooling. Magnetic reconnection under such conditions can operate in accretion disk coronae around black holes, which produce hard X-rays through Comptonization. Our simulations show that most of the plasma in the reconnection layer is kept cold by Compton losses and locked in magnetically dominated plasmoids with a small thermal pressure. Compton drag clears cavities inside plasmoids and also affects their bulk motions. These effects, however, weakly change the reconnection rate and the plasmoid size distribution from those in nonradiative reconnection. This demonstrates that the reconnection dynamics is governed by similar magnetic stresses in both cases and weakly affected by thermal pressure. We examine the energy distribution of particles energized by radiative reconnection and observe two distinct components: (1) A mildly relativistic peak, which results from bulk motions of cooled plasmoids. This component receives most of the dissipated reconnection power and dominates the output X-ray emission. The peak has a quasi-Maxwellian shape with an effective temperature of ~100 keV. Thus, it mimics thermal Comptonization used previously to fit hard-state spectra of accreting black holes. (2) A high-energy tail, which receives ~20% of the dissipated reconnection power. It is populated by particles accelerated impulsively at X-points or "picked up" by fast outflows from X-points. The high-energy particles immediately cool, and their inverse Compton emission explains the MeV spectral tail detected in the hard state of Cyg X-1. Our first-principle simulations support magnetic reconnection as a mechanism powering hard X-ray emission from magnetically dominated regions of accreting black holes.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2007

Effect of Shock on the Magnetic Properties of Pyrrhotite, the Martian Crust, and Meteorites

We performed planar shock recovery experiments on natural pyrrhotite at pressures up to 6.9 GPa. We find that high-field isothermal remanent magnetization in pyrrhotite is demagnetized up to 90% by shock due to preferential removal of low coercivity components of magnetization. Contrary to static experiments, we do not observe complete demagnetization. Post shock permanent changes in magnetic properties include increasing saturation isothermal remanent magnetization, bulk coercivity and lowtemperature memory, and changes in squareness of hysteresis. These changes are consistent with an increase in the volume fraction of single domain grains. The lack of magnetic anomalies over large Martian impact basins is not expected to be solely due to shock demagnetization of the crust. We find that pyrrhotite-bearing rocks and meteorites can retain records of Martian magnetic fields even if shocked to pressures approaching 7 GPa. However, some paleointensity techniques may underestimate this field.

Louzad, Karin L.↗
NASA NTRS2010

Electrical Switching of Perovskite Thin-Film Resistors

Electronic devices that exploit electrical switching of physical properties of thin films of perovskite materials (especially colossal magnetoresistive materials) have been invented. Unlike some related prior devices, these devices function at room temperature and do not depend on externally applied magnetic fields. Devices of this type can be designed to function as sensors (exhibiting varying electrical resistance in response to varying temperature, magnetic field, electric field, and/or mechanical pressure) and as elements of electronic memories. The underlying principle is that the application of one or more short electrical pulse(s) can induce a reversible, irreversible, or partly reversible change in the electrical, thermal, mechanical, and magnetic properties of a thin perovskite film. The energy in the pulse must be large enough to induce the desired change but not so large as to destroy the film. Depending on the requirements of a specific application, the pulse(s) can have any of a large variety of waveforms (e.g., square, triangular, or sine) and be of positive, negative, or alternating polarity. In some applications, it could be necessary to use multiple pulses to induce successive incremental physical changes. In one class of applications, electrical pulses of suitable shapes, sizes, and polarities are applied to vary the detection sensitivities of sensors. Another class of applications arises in electronic circuits in which certain resistance values are required to be variable: Incorporating the affected resistors into devices of the present type makes it possible to control their resistances electrically over wide ranges, and the lifetimes of electrically variable resistors exceed those of conventional mechanically variable resistors. Another and potentially the most important class of applications is that of resistance-based nonvolatile-memory devices, such as a resistance random access memory (RRAM) described in the immediately following article, Electrically Variable Resistive Memory Devices (MFS-32511-1).

Liu, Shangqing↗
DOE OSTI2023

Magnetic flux trapping in hydrogen-rich high-temperature superconductors

Recent discoveries of superconductivity in various hydrides at high pressures have shown that a critical temperature of superconductivity can reach near-room-temperature values. However, experimental studies are limited by high-pressure conditions, and electrical transport measurements have been the primary technique for detecting superconductivity in hydrides. Here we implement a non-conventional protocol for the magnetic measurements of superconductors in a SQUID magnetometer and probe the trapped magnetic flux in two near-room-temperature superconductors H 3 S and LaH 10 at high pressures. Contrary to traditional magnetic susceptibility measurements, the magnetic response from the trapped flux is almost unaffected by the background signal of the diamond anvil cell due to the absence of external magnetic fields. The behaviour of the trapped flux generated under zero-field-cooled and field-cooled conditions proves the existence of superconductivity in these materials. We reveal that the absence of a pronounced Meissner effect is associated with the very strong pinning of vortices inside the samples. This approach can also be a tool for studying multiphase samples or samples that have a low superconducting fraction at ambient pressure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1977

Global exospheric temperatures and densities under active solar conditions

Temperatures measured by the OGO-6 satellite using the 6300 A airglow spectrum are compared with temperatures derived from total densities and N2 densities. It is shown that while the variation of the total densities with latitude and magnetic activity agree well with values used for CIRA (1972), the temperature behavior is very different. While the temperatures derived from the N2 density were in much better agreement there were several important differences which radically affect the pressure gradients. The variation of temperature with magnetic activity showed seasonal and local time variations. Neutral temperature, density, pressure and boundary oxygen variations for the storm of 8 March 1970 are presented.

Nisbet, J. S.↗
NASA NTRS1971

Computer simulation for attitude disturbance torques for the Tiros-series.

Description of the Tiros-M Magnetic Attitude Prediction Program (TMMGAP), a simulation program designed to assist in the rotational motion control of the Tiros-series spacecraft. The subsystems of the program include input, attitude simulation, executive, attitude control and output components, simulating solar radiation pressure torque, gravity gradient torque, residual magnetic moment torque, and magnetic attitude control torques. The program provides data for prelaunch studies for launch window selection and mission planning, facilitates spacecraft spin axis reorientation after launch, provides spin axis control recommendations to meet mission constraints, and assists in the interpretation of cloud cover data. The program is characterized as effective in controlling spin axis and in processing picture data.

Sugai, I.↗
DOE OSTI2024

Valence instability and collapse of ferromagnetism in EuB 6 at high pressures

Despite the simplicity of their cubic crystal lattice, rare-earth hexaborides display complex physical properties including a (long debated) onset of metallization via magnetic polaron formation at T c1 approximate to 15 K preceding ferromagnetic ordering at T c2 approximate to 12 K. Here, in this work, we used applied pressure to tune the interplay between electronic structure and magnetism in EuB6. We probed the magnetism, valence, and structure of EuB 6 under quasi-hydrostatic pressures up to 30 GPa using X-ray techniques. Our findings show evidence for collapse of ferromagnetism above 20 GPa following a monotonic increase of mean Eu valence. While X-ray diffraction measurements in the paramagnetic state at room temperature show that the lattice retains cubic symmetry, a measurable quadrupole interaction seen by time-domain synchrotron Mössbauer spectroscopy suggests a lowering of symmetry associated with magnetic ordering, becoming more prominent across the magnetic transition. The interplay between conduction band electron count and magnetism observed under applied pressure in EuB 6 opens possibilities for fine-tuning metallization and magnetic properties of similar Eu-based semi-metal systems.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

First-principles calculation of Hubbard U for Terbium metal under high pressure

Abstract Using density functional theory (DFT) and linear response approaches, we compute the on-site Hubbard interaction U of elemental Terbium (Tb) metal in the pressure range ∼ 0–65 GPa. The resulting first-principles U values with experimental crystal structures enable us to examine the magnetic properties of Tb using a DFT+U method. The lowest-energy magnetic states in our calculations for different high-pressure Tb phases—including hcp, α -Sm, and dhcp—are found to be compatible with the corresponding magnetic ordering vectors reported in experiments. The result shows that the inclusion of Hubbard U substantially improves the accuracy and efficiency in modeling correlated rare-earth materials. Our study also provides the necessary U information for other quantum many-body techniques to study Tb under extreme pressure conditions.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Avoided ferromagnetic quantum critical point in pressurized La 5 Co 2 Ge 3

We present the pressure-temperature phase diagram La 5 Co 2 Ge 3 up to ~ 5 GPa, which was constructed from magnetization, resistivity, and specific heat measurements. At ambient pressure, La 5 Co 2 Ge 3 is an itinerant ferromagnet with a Curie temperature T C ~ 4 K. Upon increasing pressure up to ~ 1.7 GPa, T C is suppressed down to ~ 3 K. Upon further increasing pressure, our results suggest that La 5 Co 2 Ge 3 enters a different low-temperature ground state. The corresponding transition temperature T* has a nonmonotonic pressure dependence up to ~ 5 GPa. Our results demonstrate that the ferromagnetic quantum critical point in La 5 Co 2 Ge 3 is avoided by the appearance of a different, likely magnetically ordered, state that has an antiferromagnetic component.

36 MATERIALS SCIENCE↗
NASA NTRS1992

The Galactic center wind

The combined effect of winds from a cluster of stars in the central 0.8 pc of the Galaxy is modeled as uniform power and mass input over the central region. The flow becomes supersonic outside the central region, and the expected decrease in pressure is in approximate accord with observations. The pressure variations on a larger scale suggest that the Galactic center wind passes through a shock front at a radius of a few pc, leading to a shocked wind bubble on a scale of 100 pc. The tangential magnetic field can come to dominate the pressure in the shocked wind flow even if the energy density of the magnetic field in the initial wind is only 0.1 percent of the wind kinetic energy density. The magnetic region produced in this way may be related to some of the apparently magnetized structures observed in the central region of the Galaxy.

Chevalier, Roger A.↗
DOE OSTI2023

Topological features in the ferromagnetic Weyl semimetal CeAlSi: Role of domain walls

In the ferromagnetic (FM) Weyl semimetal CeAlSi both space-inversion and time-reversal symmetries are broken. Our quantum oscillation (QO) data indicate that the FM ordering modifies the Fermi-surface topology and also leads to an unusual drop in the QO amplitude. In the FM phase, we find a pressure-induced suppression of the anomalous and the loop Hall effects. This cannot be explained based on the electronic band structure or magnetic structure, both of which are nearly pressure independent. Instead, we show that a simplified model describing the scattering of Weyl fermions off FM domain walls can potentially explain the observed topological features. Our study highlights the importance of domain walls for understanding transport in FM Weyl semimetals.

36 MATERIALS SCIENCE↗