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At least 883 records · Page 49
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Features of Spin Waves Focusing in Ferromagnets

Abstract—Features of focusing spin waves in ferromagnets with magnetic moment exchange interaction with the closest neighbors and second neighbors are explored. It is shown that in the long-wave approximation, no spin wave focusing occurs: it is observed only in the wavevectors in the second half of the Brillouin zone (at aq ≥ π/2, where a is the lattice constant, q is the value of wavevector). Additionally, it is shown that magnons in such system are focused along directions [110], and are defocused in directions [100]. It is found that the external magnetic field and the magnetic anisotropy field do not cause changes in directions of magnon focusing. When the parameter of exchange interaction with the second neighbors near directions [110] and [111] is negative, magnons form a caustic, near which the intensity of the spin-wave field surges.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Thermal Expansion in Fe{sub 2}MAl (M = Ti, V, Cr, Mn, Fe, Co, and Ni) Band Ferromagnets

The linear thermal expansion coefficients (LTEC) of semimetallic Fe{sub 2}MAl (M = Ti, V, Cr, Mn, Fe, Co, and Ni) alloys have been measured in the temperature range 80–900 K. The magnetic-fluctuation contribution to LTEC α{sub m,} {sub sf}(T) = α{sub m}(T) + α{sub sf}(T) consisting of negative “Stoner” α{sub m}(T) and positive “spin-fluctuation” α{sub sf}(T) contributions. The α{sub m}(T) contribution is assumed to be proportional to the square of the spontaneous magnetization. The α{sub sf}(T) contribution, as is the case in paramagnetic and ferromagnetic states, is due to the effects of inducing local magnetic moments by spin fluctuations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Phase Transitions in Helicoidal Ferromagnets with Concentrational Fluctuations of Local Magnetization

A phenomenological approach to the theory of phase transitions induced by fluctuations in helicoidal ferromagnets with concentrational fluctuations is developed. For this purpose, random variables equal to one at a site ν occupied by a magnetic atom and zero otherwise are introduced into the Ginzburg–Landau functional. It is shown that, above the magnetic transition temperature (T{sub C}), due to concentrational effects, local magnetization is preserved, fluctuations of the helicoidal spin helix arise, and skyrmion states in the magnetic field are formed. The disappearance of the vortical states is due to the suppression of local magnetization by thermodynamic fluctuations at the temperature T{sub S} (>T{sub C}). The theoretical results explain the reasons for the significant expansion of the temperature range of skyrmion states in nonstoichiometric manganese monosilicide with manganese deficiency.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Semiconductor Behavior and Room Temperature Ferromagnetism in e-Beam Evaporated Co/TiO{sub 2} Multilayer Thin Films

The Co/TiO{sub 2} multilayer thin films have been deposited by e-beam evaporation method on glass substrates in vacuum and annealed in air at 773 K for 1 h. The crystal structure, surface morphology, optical properties, electrical properties and magnetic properties of Co/TiO{sub 2} multilayer thin films have been systematically investigated. The results showed that the particle sizes were significantly reduced when the samples are annealed and the enlargement of particle size occurred when the samples thickness is increased. The spectroscopic analysis exhibited enhanced transmittance and higher optical band gap of annealed sample than the as-deposited one and it was decreased with sample thickness. The resistivity measurement confirmed resistivity decreament with temperature. Furthermore, by investigating the magnetic properties, room temperature ferromagnetism was observed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

From vortex to bubble: Unraveling formation of merons and skyrmions in van der Waals ferromagnet $\textrm{Fe}_{5-\textrm{x}}\textrm{GeTe}_2$

Magnetic topology, such as merons and skyrmions, is important from the perspective of both fundamental physics and next-generation spintronic devices. We observe/demonstrate the coexistence of merons and skyrmions in the van der Waals ferromagnet Fe 5-x GeTe 2 . Merons remain stable across a wide temperature range, from 100 K to 290 K, whereas skyrmions are only present within a narrower range from 100 K to approximately 170 K. Our finding reveals that the formation of merons or skyrmions is governed by the local magnetocrystalline anisotropy. Furthermore, the spatial variations in local magnetic anisotropy are attributed to subtle fluctuations in Fe content.

2D materials↗
DOE OSTI2020

Perspective: Ferromagnetic Liquids

Mechanical jamming of nanoparticles at liquid–liquid interfaces has evolved into a versatile approach to structure liquids with solid-state properties. Ferromagnetic liquids obtain their physical and magnetic properties, including a remanent magnetization that distinguishes them from ferrofluids, from the jamming of magnetic nanoparticles assembled at the interface between two distinct liquids to minimize surface tension. This perspective provides an overview of recent progress and discusses future directions, challenges and potential applications of jamming magnetic nanoparticles with regard to 3D nano-magnetism. We address the formation and characterization of curved magnetic geometries, and spin frustration between dipole-coupled nanostructures, and advance our understanding of particle jamming at liquid–liquid interfaces.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Presence of Induced Weak Ferromagnetism in Fe-Substituted YFe x Cr 1–x O 3 Crystalline Compounds

Fe-substituted YFe x Cr 1–x O 3 crystalline compounds show promising magnetic and multiferroic properties. Here we report the synthesis and characterization of several compositions from this series. Using the autocombustion route, various compositions (x = 0.25, 0.50, 0.6, 0.75, 0.9, and 1) were synthesized as high-quality crystalline powders. In order to obtain microscopic and atomic information about their structure and magnetism, characterization was performed using room temperature X-ray diffraction and energy dispersion analysis as well as temperature-dependent neutron diffraction, magnetometry, and 57 Fe Mössbauer spectrometry. Rietveld analysis of the diffraction data revealed a crystallite size of 84 (8) nm for YFeO 3 , while energy dispersion analysis indicated compositions close to the nominal compositions. The magnetic results suggested an enhancement of the weak ferromagnetism for the YFeO 3 phase due to two contributions. First, a high magnetocrystalline anisotropy was associated with the crystalline character that favored a unique high canting angle of the antiferromagnetic phase (13°), as indicated by the neutron diffraction analysis. This was also evidenced by the high magnetic hysteresis curves up to 90 kOe by a remarkable high critical coercivity value of 46.7 kOe at room temperature. Second, the Dzyaloshinskii–Moriya interactions between homogenous and heterogeneous magnetic pairs resulted from the inhomogeneous distribution of Fe 3+ and Cr 3+ ions, as indicated by 57 Fe Mössbauer studies. Together, these results point to new methods of controlling the magnetic properties of these materials.

36 MATERIALS SCIENCE↗
DOE OSTI2016

FERROMAGNETISM AND PARTICLE COLLISIONS: APPLICATIONS TO PROTOPLANETARY DISKS AND THE METEORITICAL RECORD

The meteoritical record shows both iron partitioning and tungsten isotopic partitioning between the matrix and chondrules. Tungsten is not abundant enough to have driven its own isotopic partitioning, but if tungsten were correlated with iron then ferromagnetic interaction grains could help explain both observations. We derive a practical parameterization for the increase in particle–particle collision rates caused by mutually attracting particle magnetic dipole moments. While the appropriate magnetic parameters remain uncertain, we show that ambient magnetic fields in protoplanetary disks are expected to be strong enough to magnetize iron metal bearing dust grains sufficiently to drive large increases in their collision rates. Such increased collision rates between iron-metal-rich grains could help preserve primordial iron and W isotopic inhomogeneities, and would help explain why the meteoritical record shows their partitioning in the solar nebula. The importance of magnetic interactions for larger grains whose growth is balanced by fragmentation is less clear and will require future laboratory or numerical studies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Current-Induced Skyrmion Generation through Morphological Thermal Transitions in Chiral Ferromagnetic Heterostructures

Magnetic skyrmions promise breakthroughs in future memory and computing devices due to their inherent stability and small size. Their creation and current driven motion have been recently observed at room temperature, but the key mechanisms of their formation are not yet well-understood. Here it is shown that in heavy metal/ferromagnet heterostructures, pulsed currents can drive morphological transitions between labyrinth-like, stripe-like, and skyrmionic states. Using high-resolution X-ray microscopy, the spin texture evolution with temperature and magnetic field is imaged and it is demonstrated that with transient Joule heating, topological charges can be injected into the system, driving it across the stripe-skyrmion boundary. The observations are explained through atomistic spin dynamic and micromagnetic simulations that reveal a crossover to a global skyrmionic ground state above a threshold magnetic field, which is found to decrease with increasing temperature. It is demonstrated how by tuning the phase stability, one can reliably generate skyrmions by short current pulses and stabilize them at zero field, providing new means to create and manipulate spin textures in engineered chiral ferromagnets.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Spin–Phonon Coupling in Ferromagnetic Monolayer Chromium Tribromide

Novel 2D magnets exhibit intrinsic electrically tunable magnetism down to the monolayer limit, which has significant value for nonvolatile memory and emerging computing device applications. In these compounds, spin–phonon coupling (SPC) typically plays a crucial role in magnetic fluctuations, magnon dissipation, and ultimately establishing long-range ferromagnetic order. However, a systematic understanding of SPC in 2D magnets that combines theory and experiment is still lacking. Here in this work, monolayer chromium tribromide is studied to investigate SPC in 2D magnets via Raman spectroscopy and first principle calculations. The experimental Curie temperature and phonon shifts are found to be in good agreement with the numerical simulations. Specifically, it is demonstrated how magnetic exchange interactions affect phonon vibrations, which helps establish design fundamentals for 2D magnetic materials and other related devices.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Coexistence of Merons with Skyrmions in the Centrosymmetric Van Der Waals Ferromagnet Fe 5– x GeTe 2

Fe 5-x GeTe 2 is a centrosymmetric, layered van der Waals (vdW) ferromagnet that displays Curie temperatures T c (270–330 K) that are within the useful range for spintronic applications. However, little is known about the interplay between its topological spin textures (e.g., merons, skyrmions) with technologically relevant transport properties such as the topological Hall effect (THE) or topological thermal transport. Here, via high-resolution Lorentz transmission electron microscopy, it is shown that merons and anti-meron pairs coexist with Néel skyrmions in Fe 5-x GeTe 2 over a wide range of temperatures and probe their effects on thermal and electrical transport. A THE is detected, even at room T, that senses merons at higher T's, as well as their coexistence with skyrmions as T is lowered, indicating an on-demand thermally driven formation of either type of spin texture. Remarkably, an unconventional THE is also observed in absence of Lorentz force, and it is attributed to the interaction between charge carriers and magnetic field-induced chiral spin textures. Here these results expose Fe 5-x GeTe 2 as a promising candidate for the development of applications in skyrmionics/meronics due to the interplay between distinct but coexisting topological magnetic textures and unconventional transport of charge/heat carriers.

two-dimensional magnets↗
DOE OSTI2023

Room-Temperature, Current-Induced Magnetization Self-Switching in A Van Der Waals Ferromagnet

2D layered materials with broken inversion symmetry are being extensively pursued as spin source layers to realize high-efficiency magnetic switching. Such low-symmetry layered systems are, however, scarce. In addition, most layered magnets with perpendicular magnetic anisotropy show a low Curie temperature. Here, in this study, the experimental observation of spin–orbit torque magnetization self-switching at room temperature in a layered polar ferromagnetic metal, Fe 2.5 Co 2.5 GeTe 2 is reported. The spin–orbit torque is generated from the broken inversion symmetry along the c-axis of the crystal. These results provide a direct pathway toward applicable 2D spintronic devices.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Ferromagnetic–Antiferromagnetic Coupling by Distortion of Fe/Mn Oxygen Octahedrons in (BiFeO 3 ) m (La 0.7 Sr 0.3 MnO 3 ) n Superlattices

Interface enhanced magnetism attracts much attention due to its potential use in exploring novel structure devices. Nevertheless, the magnetic behavior at interfaces has not been quantitatively determined. In this study, abnormal magnetic moment reduction is observed in La 0.7 Sr 0.3 MnO 3 (LSMO)/BiFeO 3 (BFO) superlattices, which is induced by ferromagnetic (FM)/antiferromagnetic (AFM) coupling in the interface. With reduced repetition of the superlattice's unit cell [(LSMO) n /(BFO) n ] 60/ n ( n = 1, 2, 5, 10) on a SrTiO 3 substrate, magnetic moment reduction from 25.5 emu cc −1 ([(LSMO) 10 /(BFO) 10 ] 6 ) to 1.5 emu cc −1 ([(LSMO) 1 /(BFO) 1 ] 60 ) is obtained. Ab initio simulations show that due to the different magnetic domain formation energies, the magnetic moment orientation tends to be paramagnetic in the FM/AFM interface. The work focuses on the magnetic domain formation energy and provides a pathway to construct artificial heterostructures that can be an effective way to tune the magnetic moment orientation and control the magnetization of ultrathin films.

Xiong, Jie↗
DOE OSTI2023

Electrochemical Intercalation and Exfoliation of CrSBr into Ferromagnetic Fibers and Nanoribbons

Abstract Recent studies dedicated to layered van der Waals crystals have attracted significant attention to magnetic atomically thin crystals offering unprecedented opportunities for applications in innovative magnetoelectric, magneto‐optic, and spintronic devices. The active search for original platforms for the low‐dimensional magnetism study has emphasized the entirely new magnetic properties of two dimensional (2D) semiconductor CrSBr. Herein, for the first time, the electrochemical exfoliation of bulk CrSBr in a non‐aqueous environment is demonstrated. Notably, crystal cleavage governed by the structural anisotropy occurred along two directions forming atomically thin and few‐layered nanoribbons. The exfoliated material possesses an orthorhombic crystalline structure and strong optical anisotropy, showing the polarization dependencies of Raman signals. The antiferromagnetism exhibited by multilayered CrSBr gives precedence to ferromagnetic ordering in the revealed CrSBr nanostructures. Furthermore, the potential application of CrSBr nanoribbons is pioneered for electrochemical photodetector fabrication and demonstrates its responsivity up to 30 µA cm −2 in the visible spectrum. Moreover, the CrSBr‐based anode for lithium‐ion batteries exhibited high performance and self‐improving abilities. This anticipates that the results will pave the way toward the future study of CrSBr and practical applications in magneto‐ and optoelectronics.

Chemistry↗
DOE OSTI2024

Axion detection via superfluid 3 He ferromagnetic phase and quantum measurement techniques

We propose to use the nuclear spin excitation in the ferromagnetic A 1 phase of the superfluid 3 He for the axion dark matter detection. This approach is striking in that it is sensitive to the axion-nucleon coupling, one of the most important features of the QCD axion introduced to solve the strong CP problem. We review a quantum mechanical description of the nuclear spin excitation and apply it to the estimation of the axion-induced spin excitation rate. We also describe a possible detection method of the spin excitation in detail and show that the combination of the squeezing of the final state with the Josephson parametric amplifier and the homodyne measurement can enhance the sensitivity. It turns out that this approach gives good sensitivity to the axion dark matter with the mass of $\mathcal{O}$(1) μeV depending on the size of the external magnetic field. We estimate the parameters of experimental setups, e.g., the detector volume and the amplitude of squeezing, required to reach the QCD axion parameter space.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Critical Behavior Near the Paramagnetic-Ferromagnetic Phase Transition in La{sub 1−x}Sr{sub x}CoO{sub 3} (x = 0.3 and x = 0.5) Cobaltites

In this work, we present the study of structural, magnetic and critical behavior of La{sub 1−x}Sr{sub x}CoO{sub 3} (x = 0.3 and 0.5) cobaltites. X-ray diffraction analysis using the Rietveld refinement shows that the sample La{sub 0.7}Sr{sub 0.3}CoO{sub 3} crystallizes in a rhombohedral distorted perovskite structure with R3̄c space group, while La{sub 0.5}Sr{sub 0.5}CoO{sub 3} exhibits both phases rhombohedric and cubic, with R3̄c and Pm3̄m space groups. Our samples exhibit thermo-magnetic irreversibility behavior in the magnetization data under a magnetic applied field of 0.05 T. The temperature dependence of magnetic susceptibility at higher temperatures for La{sub 0.7}Sr{sub 0.3}CoO{sub 3} sample reveals the presence of the Griffiths’ phase above the Curie temperature, while it follows the Curie–Weiss law perfectly for La{sub 0.5}Sr{sub 0.5}CoO{sub 3}. Different techniques including the modified Arrott plot, the Kouvel-Fisher method and the critical isotherm analysis have been used to analyze the paramagnetic-ferromagnetic phase transition. The values of the critical exponents associated to this transition were close to those expected in the mean-field model. The validity of the calculated critical exponents has been confirmed by the scaling equation of state. The determined critical exponents using various methods are found to follow the scaling equation with the magnetization data scaled into two different curves below and above the critical temperature.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

First-Principles Calculations of Acoustic and Anharmonic Properties of Ferromagnetic Cu{sub 2}MnZ (Z = Al and In) Heusler Alloys

The acoustic and anharmonic properties of ferromagnetic Cu{sub 2}MnZ (Z = Al and In) Heusler alloys have been investigated by first-principles calculations method. The obtained lattice parameters, magnetic moments, elastic properties are found to be in good agreement with the available experimental values. From the elastic properties, the sound velocities and the related Debye temperatures and minimum thermal conductivities have been obtained for the two alloys. The sound velocities and thermal conductivities of both alloys are found to show significant anisotropy, and the Cu{sub 2}MnAl with small density and large elastic constants has large sound velocities, high Debye temperature, and large thermal conductivities. Also, the effective second-order elastic constants, generalized Grüneisen constants, and nonlinear ultrasonic parameters to characterize anharmonic properties have been studied for the two alloys. These predictions on the acoustic and anharmonic properties can provide a valuable guidance or reference for further related investigations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Revival of Metal-Insulator and Ferromagnetic-Paramagnetic Transitions by Ni Substitution at Mn Site in Charge-Ordered Monovalent Doped Nd{sub 0.75}Na{sub 0.25}MnO{sub 3} Manganites

Nd{sub 0.75}Na{sub 0.25}Mn{sub 1−x}Ni{sub x}O{sub 3} (x = 0 − 0.07) were synthesized using a conventional solid-state synthesis method to investigate the effect of Ni substitution on their magnetic and electrical transport properties. XRD analysis using the Rietvield refinement method showed an increase in unit cell volume with increasing Ni content, indicating the possibility of substituting Ni for the Mn site. For x = 0, magnetization measurements showed paramagnetic (PM) to antiferromagnetic (AFM) transition at the transition temperature, T{sub N} ∼ 185 K, which may be related to the presence of charge-ordering (CO) state. For Ni-substituted samples, ferromagnetic (FM) to PM transition was induced with Curie temperature (T{sub C}), increasing from 91 K (x = 0.01) to 115 K (x = 0.03), followed by decreases in T{sub C} to 60 K (x = 0.07). Electrical resistivity measurements showed that samples for x ≤ 0.01 exhibited insulator behavior while both x = 0.03 and 0.05 samples exhibited metal-insulator transition suggesting that the CO state is weakened. For x = 0.07, the sample shows re-entrant of insulating characteristic. Inducement of FM metallic (FMM) state, as well as increased of T{sub C} for x = 0.03 is suggested to be related to FM SE between Ni{sup 2+} and Mn{sup 4+}, which suppressed the CO state, hence inducing double-exchange (DE)-like mechanism. In addition, an increase in resistivity was observed as temperature decreased below the resistivity minimum (R{sub min}) at T{sub min} ∼ 40 K for x = 0.05 is possibly due to the Kondo-like effect mechanism. On one hand, the M(H) curve showed the presence of a hysteresis loop for x = 0 and 0.01 at T= 60 and 80 K, indicating the presence of an unstable phase, which may be related with the CO-AFM phase. For x = 0.03, no hysteresis loop was observed, indicating the suppression of the CO-AFM. Intriguingly, for x = 0.05 and 0.07, small hysteresis loop was observed, indicating the possible presence of a minor AFM component. Further, the observed MR behavior in present studies can be understood as a result of a decreased scattering mechanism in the presence of magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗