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NASA NTRS1994

Variability in daily, zonal mean lower-stratospheric temperatures

Satellite data from the microwave sounding unit (MSU) channel 4, when carefully merged, provide daily zonal anomalies of lower-stratosphere temperature with a level of precision between 0.01 and 0.08 C per 2.5 deg latitude band. Global averages of these daily zonal anomalies reveal the prominent warming events due to volcanic aerosol in 1982 (El Chichon) and 1991 (Mt. Pinatubo), which are on the order of 1 C. The quasibiennial oscillation (QBO) may be extracted from these zonal data by applying a spatial filter between 15 deg N and 15 deg S latitude, which resembles the meridional curvature. Previously published relationships between the QBO and the north polar stratospheric temperatures during northern winter are examined but were not found to be reproduced in the MSU4 data. Sudden stratospheric warmings in the north polar region are represented in the MSU4 data for latitudes poleward of 70 deg N. In the Southern Hemisphere, there appears to be a moderate relationship between total ozone concentration and MSU4 temperatures, though it has been less apparent in 1991 and 1992. In terms of empirical modes of variability, the authors find a strong tendency in EOF 1 (39.2% of the variance) for anomalies in the Northern Hemisphere polar regions to be counterbalanced by anomalies equatorward of 40 deg N and 40 deg S latitudes. In addition, most of the modes revealed significant power in the 15-20 day period band.

Christy, John R.↗
NASA NTRS1994

'Downward control' of the mean meridional circulation and temperature distribution of the polar winter stratosphere

According to the 'downward control' principle, the extratropical mean vertical velocity on a given pressure level is approximately proportional to the meridional gradient of the vertically integrated zonal force per unit mass exerted by waves above that level. In this paper, a simple numerical model that includes parameterizations of both planetary and gravity wave breaking is used to explore the influence of gravity wave breaking in the mesosphere on the mean meridional circulation and temperature distribution at lower levels in the polar winter stratosphere. The results of these calculations suggest that gravity wave drag in the mesosphere can affect the state of the polar winter stratosphere down to altitudes below 30 km. The effect is most important when planetary wave driving is relatively weak: that is, during southern winter and in early northern winter. In southern winter, downwelling weakens by a factor of 2 near the stratospause and by 20% at 30 km when gravity wave drag is not included in the calculations. As a consequence, temperatures decrease considerably throughout the polar winter stratosphere (over 20 K above 40 km and as much as 8 K at 30 km, where the effect is enhanced by the long radiative relaxation timescale). The polar winter states obtained when gravity wave drag is omitted in this simple model resemble the results of simulations with some general circulation models and suggest that some of the shortcomings of the latter may be due to a deficit in mesospheric momentum deposition by small-scale gravity waves.

Garcia, Rolando R.↗
NASA NTRS1994

Spread of denitrification from 1987 Antarctic and 1988-1989 Arctic stratospheric vortices

Vertical profiles of N2O and NO(y) taken by the ER-2 outside the vortex are used to construct average vertical profiles of F(NO(y)) = NO(y)/(A-N2O), where A is the tropospheric content of N2O three years prior to the measurements. The southern hemisphere had less nitrous oxide in the range 400 less than Theta less than 470 K, by up to 25% relative to the northern hemisphere. F(NO(y)) is the ratio of NOy produced to N2O lost in a stratospheric air mass since entry from the troposphere. The profiles of F(NO(y)) have the following characteristics: (1) Relative to 1991-1992, a year without denitrification inside or outside the vortex, the northern hemisphere in 1988-1989 showed denitrification outside the vortex ranging up to 25% and averaging 17% above Theta = 425 K. (2) Relative to the northern hemisphere in 1991-1992, the southern hemisphere in 1987 showed denitrification outside the vortex ranging up to 32% and averaging 20% above Theta = 400 K. (3) Below Theta = 400 K the southern hemisphere showed enhancements of F(NO(y)) relative to the northern hemisphere in 1991-1992 ranging up to 200% at Theta = 375 K, outside the vortex. Corresponding profiles of residual water, R(H2O) = H2O - 2(1.6 - CH4), are considered and shown to be consistent with those of F(NO(y)) in the sense that they show deficits outside the Antarctic vortex, which was both dehydrated and denitrified, but not outside the 1988-1989 Arctic vortex, which was denitrified but not dehydrated. R(H2O) is the water content of stratospheric air with the contribution from methane oxidation subtracted. Comparison of F(NO(y)) and R(H2O) below 400 K outside the Antarctic vortex leads to the suggetion that dehydration in the Antarctic vortex occurs by the sedimentation of ice crystals large enough to fall out of the stratosphere, whereas denitrification occurs mainly on mixed nitric acid-water crystals which evaporate below the base of the vortex at Theta = 400 K but above the tropopause.

Tuck, A. F.↗
NASA NTRS1994

The solar cycle variation of ozone in the stratosphere inferred from Nimbus 7 and NOAA 11 satellites

The combined Nimbus 7 solar backscattered ultraviolet (SBUV) and NOAA 11 SBUV/2 ozone data, covering a period of more than a solar cycle (about 15 years), are used to study the UV response of ozone in the stratosphere. The study shows that about 2% change in total column ozone and about 5-7% change in ozone mixing ratio in the upper stratosphere (0.7 to 2 hPa) may be attributed to the change in the solar UV flux over a solar cycle. In the upper stratosphere, where photochemical processes are expected to play a major role, the measured solar cycle variation of ozone is significantly larger than inferred either from the photochemical models or from the ozone response to the 27-day solar UV modulation. For example, the observed solar cycle related change in ozone mixing ratio at 2 hPa is about 1% for 1% change in the solar UV flux near 200 nm. The inferred change in ozone from either the photochemical models or from the 27-day ozone-UV response is about a factor of 2-3 lower than this value.

Chandra, S.↗
NASA NTRS1994

SAGE II observations of a previously unreported stratospheric volcanic aerosol cloud in the northern polar summer of 1990

Analysis of aerosol extinction profiles obtained by the spaceborne SAGE II sensor reveals that there was an anomalous increase of aerosol extinction below 18.5 km at latitudes poleward of 50 deg N from July 28 to September 9, 1990. This widespread increase of aerosol extinction in the lower stratosphere was apparently due to a remote high-latitude volcanic eruption that has not been reported to date. The increase in stratospheric optical depth in the northern polar region was about 50% in August and had diminished by October 1990. This eruption caused an increase in stratospheric aerosol mass of about 0.33 x 10(exp 5) tons, assuming the aerosol was composed of sulfuric acid and water.

Yue, Glenn K.↗
NASA NTRS1994

Spring dehydration in the Antarctic stratospheric vortex observed by HALOE

The distribution of dehydrated air in the middle and lower stratosphere during the 1992 Southern Hemisphere spring is investigated using Halogen Occultation Experiment (HALOE) observations and trajectory techniques. Comparisons between previously published Version 9 and the improved Version 16 retrievals on the 700-K isentropic surface show very slight (0.05 ppmv) increases in Version 16 CH4 relative to Version 9 within the polar vortex. Version 16 H2O mixing ratios show a reduction of 0.5 ppmv relative to Version 9 within the polar night jet and a reduction of nearly 1.0 ppmv in middle latitudes when compared to Version 9. The version 16 HALOE retrievals show low mixing ratios of total hydrogen (2CH4 + H2O) within the polar vortex on both 700 and 425 K isentropic surfaces relative to typical middle-stratospheric 2CH4 + H2O mixing ratios. The low 2CH4 + H2O mixing ratios are associated with dehydration. Slight reductions in total hydrogen, relative to typical middle-stratospheric values, are found at these levels throughout the Southern Hemisphere during this period. Trajectory calculations show that middle-latitude air masses are composed of a mixture of air from within the polar night jet and air from middle latitudes. A strong kinematic barrier to large-scale exchange is found on the poleward flank of the polar night jet at 700 K. A much weaker kinematic barrier is found at 425 K. The impact of the finite tangent pathlength of the HALOE measurements is investigated using an idealized tracer distribution. This experiment suggests that HALOE should be able to resolve the kinematic barrier, if it exists.

Pierce, R. Bradley↗
NASA NTRS1994

Isentropic mass exchange between the Tropics and extratropics in the stratosphere

The isentropic mass exchange between the Tropics and extratropics in the stratosphere is investigated with a semi-Lagrangian transport model for the periods from 1 June to 31 October 1992 and from 1 December 1992 to 30 April 1993 using winds from the U.K. Meteorological Office data assimilation system. Calculations with an idealized, initially zonally symmetric tracer show that in the middle and upper stratosphere the bulk of tropical air is transported into the midlatitudes of the winter hemisphere although there exist quasi-permeable barriers in the subtropics. The transport takes place in the form of planetary-scale 'tongues' of material that are drawn poleward in association with the episodic amplification of planetary-scale waves in high latitudes of the winter hemisphere. Once air of tropical origin is transported to the midlatitudes it is irreversibly mixed with the midlatitude air in the 'surf zone.' Air of tropical origin can, however, hardly penetrate into the interior of the winter polar vortex until the breakdown of the vortex. Transport of tropical air into the midlatitudes of the summer hemisphere is strongly inhibited. In the lower stratosphere, tropical air is transported into the northern and southern midlatitudes. During the period from 1 June to 31 October 1992, the amount of tropical air transported into the Northern Hemisphere is, however, much smaller than that transported into the Southern Hemisphere, and there exist strong gradients in the tracer field in the equatorial region, indicating that there is a quasi-permeable barrier to cross-equator mass exchange. During the period from 1 December 1992 to 30 April 1993, on the other hand, roughly the same amounts of tropical air are transported into the Southern Hemisphere, and there exist strong gradients in the tracer field in the equatorial region, indicating that there is a quasi-permeable barrier to cross-equator mass exchange. During the period from 1 December 1992 to 30 April 1993, on the other hand, roughly the same amounts of tropical air are transported into the northern midlatitudes and into the southern midlatitudes, and there exist no significant transport barriers in the equatorial area.

Chen, Ping↗
NASA NTRS1994

Spectral signatures of polar stratospheric clouds and sulfate aerosol

Multiwavelength observations of Antarctic and midlatitude aerosol by the Cryogenic Limb Array Etalon Spectrometer (CLAES) experiment on the Upper Atmosphere Research Satellite (UARS) are used to demonstrate a technique that identifies the location of polar stratospheric clouds. The technique discussed uses the normalized area of the triangle formed by the aerosol extinctions at 925, 1257, and 1605/cm (10.8, 8.0, and 6.2 micrometers) to derive a spectral aerosol measure M of the aerosol spectrum. Mie calculations for spherical particles and T-matrix calculations for spheriodal particles are used to generate theoretical spectral extinction curves for sulfate and polar stratospheric cloud particles. The values of the spectral aerosol measure M for the sulfate and polar stratospheric cloud particles are shown to be different. Aerosol extinction data, corresponding to temperatures between 180 and 220 K at a pressure of 46 hPa (near 21-km altitude) for 18 August 1992, are used to demonstrate the technique. Thermodynamic calculations, based upon frost-point calculations and laboratory phase-equilibrium studies of nitric acid trihydrate, are used to predict the location of nitric acid trihydrate cloud particles.

Massie, S. T.↗
NASA NTRS1994

The anomalous Arctic lower stratospheric polar vortex of 1992-1993

Potential vorticity (PV) gradients defining the lower stratospheric vortex during the 1992-1993 winter were anomalously strong and persistent compared to those during the last 16 Arctic winters. For approximately equal to 3 months PV gradients were closer to typical Antarctic values than to most Arctic values. Air motion diagnostics computed for 3-dimensional air parcels confirm that the 1992-1993 Arctic lower stratospheric vortex was substantially more isolated than is typical. Such isolation will delay and reduce the export of the higher ozone typical of the winter lower stratospheric vortex to mid-latitudes. This may have contributed to the record-low total ozone amounts observed in northern mid-latitudes in 1993.

Manney, G. L.↗
NASA NTRS1994

Radiatively forced dispersion of the Mt. Pinatubo volcanic cloud and induced temperature perturbations in the stratosphere during the first few months following the eruption

A combined 3-dimensional circulation model and aerosol microphysical/transport model is used to simulate the dispersion of the Mt. Pinatubo volcanic cloud in the stratosphere for the first few months following the eruption. Radiative heating of the cloud due to upwelling infrared radiation from the troposphere is shown to be an important factor affecting the transport. Without cloud heating, cloud material stays mostly north of the equator, whereas with cloud heating, the cloud is transported southward across the equator within the first two weeks following the eruption. Generally the simulations agree with Total Ozone Mapping Spectrometer (TOMS), Advanced Very High Resolution Radiometer (AVHRR), and Stratospheric Aerosol and Gas Experiment (SAGE) satellite observations showing the latitude distribution of cloud material to be between about 20 deg S and 30 deg N within the first few months. Temperature perturbations in the stratosphere induced by the aerosol heating are generally 1-4 K, in the range of those observed.

Young, Richard E.↗
NASA NTRS1994

Low-light video observations of frequent luminous structures in the stratosphere above thunderstorms

A new series of video measurements were made of the phenomenon provisionally termed the cloud-to-stratosphere (CS) event, an electrical discharge extending to great heights above thunderstorm tops. This new series of measurements were accomplished by properly positioning a sensor, the Xybion model ISS 225 low-light monochrome imaging system with a C-mount fl.8 manual zoom lens, and training it on the appropriate portion of the sky above a distant thunderstorm complex mean Fort Collins, Colorado. The resulting images are currently undergoing intensive analysis. Some tentative conclusions are given. Cloud-to-stratosphere events occur far more frequently than previously suspected and are perhaps a ubiquitous aspect of many larger convective systems. Cloud-to-stratosphere events are also of substantial horizontal extent, on the order of tens of kilometers in some cases.

Lyons, Walter A.↗
NASA NTRS1995

Observations of lightning in the stratosphere

An examination and analysis of video images of lightning, captured by the payload bay TV cameras of the space shuttle, provided a variety of examples of lightning in the stratosphere above thunderstorms. These images were obtained on several recent shuttle flights while conducting the Mesoscale Lightning Experiment (MLE). The images of stratospheric lightning illustrate the variety of filamentary and broad vertical discharges in the stratosphere that may accompany a lightning flash. A typical event is imaged as a single or multiple filament extending 30 to 40 km above a thunderstorm that is illuminated by a series of lightning strokes. Examples are found in temperate and tropical areas, over the oceans, and over the land.

Boeck, William L.↗
NASA NTRS1993

In situ measurements of the ClO/HCl ratio: Heterogeneous processing on sulfate aerosols and polar stratospheric clouds

Simultaneous in situ measurements of stratospheric ClO and HCl have been made for the first time, during numerous flights of the ER-2 aircraft covering latitudes 24-90 deg N from October 1991 through March 1992. The ClO/HCl ratio is identified as a key indicator of heterogeneous processing both outside and within the Arctic polar vortex. For ClO mixing ratios below about 120 pptv, remarkably constant ClO/HCl values of about 15% characterize the lower stratosphere. The observed values are significantly higher than those derived from a 2-D model using either gas phase photochemistry alone (2%), or including heterogeneous sulfate chemistry (5-10%). During the Arctic early spring, after conversion of HCl into reactive chlorine has taken place, the vortex edge is poorly defined by ClO levels. Loss of HCl and its slow recovery following low-temperature polar heterogeneous chemistry distinguishes HCl as a new and unique dynamical tracer of polar stratospheric clouds (PSC)-processed air.

Webster, C. R.↗
NASA NTRS1993

In-situ measurements of changes in stratospheric aerosol and the N2O-aerosol relationship inside and outside of the polar vortex

Two optical particle counters on the ER-2, together covering a particle size diameter range from 0.1 microns to 23 microns, were used to measure the aerosol bulk quantities integral number, aerosol surface and volume, as well as detailed size distributions inside and outside of the polar vortex in the lower stratosphere. While AAES I (Arctic Airborne Stratospheric Expedition, (Dec. 88 - Feb. 89) was conducted in a period of relative volcanic quiescence, enhancements in aerosol number, surface and volume of factors around 10, 25 and 100 were observed during AASE 2 (Aug. 91 - Mar. 92) due to the eruption of Mt. Pinatubo. The changes in these bulk quantities as well as in the size distributions measured both outside and inside the polar vortex are presented and compared with those obtained in polar stratospheric cloud events (AASE I). Except for a shift towards larger aerosol mixing ratios the general shape of correlograms between the measured N2O and particle mixing ratios remain similar before and after the eruption. Similar correlograms are used to interpret data from vertical profiles inside and outside of the polar vortex.

Borrmann, S.↗
NASA NTRS1995

Sensitivity of two-dimensional model predictions of ozone response to stratospheric aircraft: An update

The Goddard Space Flight Center (GSFC) two-dimensional model of stratospheric photochemistry and dynamics has been used to calculate the O3 response to stratospheric aircraft (high-speed civil transport (HSCT)) emissions. The sensitivity of the model O3 response was examined for systematic variations of five parameters and two reaction rates over a wide range, expanding on calculations by various modeling groups for the NASA High Speed Research Program and the World Meteorological Organization. In all, 448 model runs were required to test the effects of variations in the latitude, altitude, and magnetitude of the aircraft emissions perturbation, the background chlorine levels, the background sulfate aerosol surface area densities, and the rates of two key reactions. No deviation from previous conclusions concerning the response of O3 to HSCTs was found in this more exhaustive exploration of parameter space. Maximum O3 depletions occur for high-altitude, low altitude HSCT perturbations. Small increases in global total O3 can occur for low-altitude, high-altitude injections. Decreasing aerosol surface area densities and background chlorine levels increases the sensitivity of model O3 to the HSCT perturbations. The location of the aircraft emissions is the most important determinant of the model response. Response to the location of the HSCT emissions is not changed qualitatively by changes in background chlorine and aerosol loading. The response is also not very sensitive to changes in the rates of the reactions NO + HO2 yields NO2 + OH and HO2 + O3 yields OH + 2O2 over the limits of their respective uncertainties. Finally, levels of lower stratospheric HO(sub x) generally decrease when the HSCT perturbation is included, even though there are large increases in H2O due to the perturbation.

Considine, David B.↗
NASA NTRS1995

Smithsonian stratospheric far-infrared spectrometer and data reduction system

The Smithsonian far-infrared spectrometer (FIRS) is a remote sensing Fourier transform spectrometer that measures the mid- and far-infrared thermal emission spectrum of the stratosphere from balloon and aircraft platforms. The spectrometer has had nine successful balloon flights from 1987 to 1994, flying at float altitudes of 36 - 39 km and collecting 131 hours of midlatitude stratospheric limb spectra. The spectrometer also flew on a NASA CD-8 aircraft, as part of the second Airborne Arctic Stratospheric Expedition (AASE-2), collecting 140 hours of overhead spectra at latitudes ranging from the equator to the north pole. We present here a brief description of the instrument, a discussion of data reduction procedures, an estimation of both random and systematic errors, an outline of the procedure for retrieving mixing ratio profiles, and an explanation of the method of deriving temperature and pressure from the far- and mid-infrared spectra.

Johnson, D. G.↗
NASA NTRS1995

Effect of stratospheric aerosol on ozone profile from BUV measurements

Results of a simulation study on the effects of optically thick stratospheric sulfate aerosol layers on the backscattered ultraviolet radiation (buv) in the range 256-340 nm are presented. In general, the increased Mie scattering produced by the aerosols results in an enhancement of the buv radiation. The increase is approximately linear with optical depth and strongly depends on solar zenith angle and aerosol layer altitude in relation to the ozone maximum. The effect is greatest at those wavelenghts whose contribution functions peak in the vicinity of the densest part of the aerosol layer. The aerosol induced perturbation of the buv field affects the ozone profile retrieval from space measurements by the Solar Backscatter Ultraviolet Experiment (SBUV) experiment. In the tropical stratosphere, the retrieved ozone between 25 and 45 km is underestimated as a result of increased Mie scattering. On the other hand, an algorithm related effect causes the retrieved ozone below 25 km to be overestimated by an amount similar to the stratospheric deficit.

Torres, Omar↗
NASA NTRS1994

An examination of the total hydrogen budget of the lower stratosphere

We analyze the hydrogen budget of the lower stratosphere using simultaneous in situ measurements of northern hemispheric water vapor (H2O) and methane (CH4) obtained during the spring Stratospheric Photochemistry, Aerosols, and Dynamics Expedition (SPADE), as well as previously published in situ H2 data. Based on this data, we conclude that approximately two H2O molecules are produced for each CH4 molecule destroyed. This implies that H2 production from CH4 oxidation is balanced by H2 oxidation. The uncertainty in this analysis is greatly reduced by the use of multiple data sets. Additionally, we infer that, on an annual and global average, H2O enters the stratosphere with a mixing ratio of 4.2 +/- 0.5 ppmv, and that the quasi-conserved quantity 2 x CH4 + H2O has a value of 7.6 +/- 0.6 ppmv in these northern hemishere air parcels (where xi denotes the mixing ratio of the constituent xi).

Dessler, A. E.↗