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At least 865 records · Page 48

Evaluation of Anodized and Electroplated Radioactive Check Sources for Radiological Monitoring Instruments

Radioactive check sources are often used for source checking calibrated instruments to confirm accurate readings are obtained from radiological monitoring instruments. Because of the importance of check sources and their application, PNNL conducted a study to evaluate the effectiveness and accuracy of active sources produced using different construction methods. Eleven, randomly selected check sources of both anodized (five) and electroplated (six) construction were evaluated, along with their calculated decay curves, to determine how well they withstand consistent, multi-year use in the field. Results show that the anodized and electroplated check sources evaluated hold up well enough to continue their use, regardless of wear and tear sustained over years of use. This report provides the source information, empirical data for the 11 anodized and electroplated check sources and their representative decay curves, and it documents the conclusion that anodized and electroplated check sources are reliable for routine use in the field over multiple years.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Radioactive Plume Avoidance and Aircraft Decontamination – Best Practices

Response to an incident involving the release of radioactive material will most likely involve aircraft for disaster relief and radiological monitoring. Aircraft flying into a radiologically contaminated area risk becoming contaminated, and in the worst cases having to be removed from service. Contamination is avoidable, and decontamination is possible, but both require planning and forethought.

61 RADIATION PROTECTION AND DOSIMETRY↗

Radioactive Cleaning Robot

Here at Fermi, work is centered around particle accelerators. With the functionality of these accelerators comes a small amount of radioactive dust. For the sake of all employees in this environment, a yearly deep clean is necessary. The aim of this robot is to save time by running an automated cleaning robot 24/7.

Stachowicz, Emily↗

Nevada National Security Site 2019 Waste Management Monitoring Report Area 3 and Area 5 Radioactive Waste Management Sites

Environmental monitoring data are collected at and around the Area 3 and Area 5 Radioactive Waste Management Sites (RWMSs) within the Nevada National Security Site (NNSS). This report summarizes the 2019 environmental data to provide an overall evaluation of RWMS performance and to support environmental compliance and performance assessment (PA) activities. Some of these data (e.g., radiation exposure, air, and groundwater) are presented in other reports (Mission Support and Test Services, LLC 2019, 2020a, 2020b). Direct radiation monitoring data indicate exposure levels at the Area 3 and Area 5 RWMSs are within the range of background levels measured at the NNSS. Slightly elevated exposure levels outside the Area 3 RWMS are attributed to nearby historical aboveground nuclear weapons tests. Air monitoring data at the Area 3 and Area 5 RWMSs show that tritium concentrations in water vapor and americium and plutonium concentrations in air particles are below Derived Concentration Standards for these radionuclides. Groundwater monitoring data indicate the groundwater in the uppermost aquifer beneath the Area 5 RWMS is not impacted by RWMS operations. Results of groundwater analysis from wells around the Area 5 RWMS are below established investigation levels. Leachate samples collected from the leachate collection systems at the Area 5 mixed low-level waste disposal unit are below established contaminant regulatory limits. During 2019, precipitation at the Area 3 RWMS was 77 percent above average, and precipitation at the Area 5 RWMS was 69 percent above average. Water balance measurements indicate that evapotranspiration from the vegetated weighing lysimeter at the Area 5 RWMS dries the soil and prevents downward percolation of precipitation more effectively than evaporation as measured from the bare-soil weighing lysimeter. Vadose zone monitoring in the Area 3 and Area 5 RWMS soil covers shows no evidence of precipitation percolating through the covers to the waste. Moisture from precipitation did not percolate below 120 centimeters (3.9 feet [ft]) in the vegetated final cover on the U-3ax/bl disposal unit at the Area 3 RWMS during 2019. There was no drainage through 2.4 meters (8 ft) of soil as indicated from the Area 3 drainage lysimeters that received only natural precipitation. At the Area 3 RWMS, which received three times the natural precipitation, 57 percent of the applied precipitation and irrigation drained from the bare-soil drainage lysimeter. All 2019 monitoring data indicate that the Area 3 and Area 5 RWMSs are performing within expectations of the model and parameter assumptions for the facilities’ PAs.

2019↗

Chapter 9. Control of Accountable Sealed Radioactive Sources (ASRSs) and Radioisotope Thermoelectric Generators (RTGs)

This chapter describes the processes that Members of the Workforce (MOW) follow to control Accountable Sealed Radioactive Sources (ASRSs) and Radioisotope Thermoelectric Generators (RTGs). It also describes the Sandia National Laboratories (SNL) program for implementing the ASRS requirements in 10 CFR 835.1202 and the ASRS and RTG requirements in DOE 0 231.1B.

07 ISOTOPE AND RADIATION SOURCES↗

Review of New or Modified Radioactive Air Emission Sources

This Environmental Protection and Compliance (EPC), Compliance Programs (CP) Quality Procedure (QP) describes the process for review and evaluation of new and modified sources of radioactive air emissions to determine the requirements for pre-construction approval, stack monitoring, stack sampling system upgrade, ambient air monitoring, and the implementation of As Low As Reasonably Achievable (ALARA) principles. These requirements are specified in 40 CFR 61 Subpart H and by DOE Order 458.1, Radiation Protection of the Public and the Environment.

61 RADIATION PROTECTION AND DOSIMETRY↗

Health effects of Radiation and Radioactivity + Historic Nuclear Accidents

The safety of nuclear energy technology goes hand in hand with a modern understanding of the health impacts and required precautions associated with radiation. This is because nuclear power plants require fuel sources like uranium, which is an element that is naturally radioactive.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Addendum to Capability Needs for Irradiated and Radioactive Materials Research (Ad Hoc Committee Summary Report)

Nuclear materials and fuels studies are challenging research and engineering targets because of their inherent radioactivity as well as their heterogeneous microstructure. Advanced light sources have made significant underpinning scientific contributions to the understanding of structural and fuel cladding material microstructure and properties and the development of structure-property relationships. These facilities have the potential to help advance the Department of Energy (DOE) Office of Nuclear Energy (DOE-NE) mission priorities providing underpinning understanding of technically important challenges, including: irradiation induced embrittlement and swelling; stress corrosion cracking and corrosion in extreme environments; ageing of reactor pressure vessels steels; nuclear fuel characterization; and nuclear waste form optimization as well as playing a major role in the development of a materials performance matrix to aid in the design of new materials to meet the needs of advanced reactor concepts. However, the delivery of underpinning understanding is the mission of DOE Office of Science (DOE-SC). While filling such knowledge gaps is important, efforts in this direction should not be confused with the strategic technology focused mission goals of DOE-NE to enable the continued operation of existing U.S. nuclear reactors, to enable the deployment of advanced nuclear reactors, to develop advanced nuclear fuel cycles, and to maintain U.S. leadership in nuclear energy technology.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessment of Naturally Occurring Radioactive Material (NORM) in Illicit Drugs Using High-Resolution Gamma Spectroscopy

This report documents results assessing the presence of Naturally Occurring Radioactive Material (NORM) in illicit drugs using high-resolution gamma spectroscopy. Specifically, high-purity germanium (HPGe) measurements were conducted at the Drug Enforcement Administration (DEA) South Central Laboratory on 11 samples (referred to as exhibits) including cocaine, fentanyl, heroin, ketamine, LSD, marijuana, methamphetamines, psilocybin mushrooms, and synthetic cannabinoids.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Late-time photometry of type IA supernova SN 2012cg reveals the radioactive decay of {sup 57}Co

Seitenzahl et al. have predicted that roughly three years after its explosion, the light we receive from a Type Ia supernova (SN Ia) will come mostly from reprocessing of electrons and X-rays emitted by the radioactive decay chain {sup 57}Co → {sup 57}Fe, instead of positrons from the decay chain {sup 56}Co → {sup 56}Fe that dominates the SN light at earlier times. Using the Hubble Space Telescope, we followed the light curve of the SN Ia SN 2012cg out to 1055 days after maximum light. Our measurements are consistent with the light curves predicted by the contribution of energy from the reprocessing of electrons and X-rays emitted by the decay of {sup 57}Co, offering evidence that {sup 57}Co is produced in SN Ia explosions. However, the data are also consistent with a light echo ∼14 mag fainter than SN 2012cg at peak. Assuming no light-echo contamination, the mass ratio of {sup 57}Ni and {sup 56}Ni produced by the explosion, a strong constraint on any SN Ia explosion models, is 0.043{sub −0.011}{sup +0.012}, roughly twice Solar. In the context of current explosion models, this value favors a progenitor white dwarf with a mass near the Chandrasekhar limit.

79 ASTRONOMY AND ASTROPHYSICS↗

Galactic Chemical Evolution of Short-lived Radioactive Isotopes Produced by Explosive Nucleosynthesis: 60 Fe and 53 Mn

Several short-lived radionuclides (SLRs) are know to have existed in the early solar system (ESS). These species, which typically decay with half-lives of the order of a few million years, can be used to probe the timescales of events preceding the birth of the Sun. We investigate the ESS origin of 53 Mn, produced by core-collapse supernovae (CCSNe) and Type Ia supernovae (SNe Ia), and 60 Fe, produced exclusively by CCSNe. We model the evolution of the radioactive-to-stable abundance ratios of these SLRs with a Galactic chemical evolution (GCE) framework accounting for different SN yields, SN Ia delay times, and other Galactic features (K). A further set of models is calculated assuming that SNe Ia did not contribute any 53 Mn to the ESS. The predicted ratios are compared to meteoritic ratios to derive a distribution of solar isolation times that includes uncertainties due to stochastic chemical enrichment and measurements of the ESS values. The isolation times are then compared to those of 107 Pd and 182 Hf calculated in previous work. A self-consistent solution can be found within the current uncertainties, especially when using the GCE setups with K = 1.6 and 2.3, although the maximum likelihood for the 60 Fe distribution is typically ∼4–5 Myr shorter than for 53 Mn. The predicted 60 Fe/ 53 Mn ratio, instead, is completely inconsistent with the ESS value; this could be resolved using a larger fraction of faint CCSNe than usually considered in GCE models.

79 ASTRONOMY AND ASTROPHYSICS↗

Pulsational Pair-instability Model for Superluminous Supernova PTF12dam:Interaction and Radioactive Decay

Being a superluminous supernova, PTF12dam can be explained by a {sup 56}Ni-powered model, a magnetar-powered model, or an interaction model. We propose that PTF12dam is a pulsational pair-instability supernova, where the outer envelope of a progenitor is ejected during the pulsations. Thus, it is powered by a double energy source: radioactive decay of {sup 56}Ni and a radiative shock in a dense circumstellar medium. To describe multicolor light curves and spectra, we use radiation-hydrodynamics calculations of the STELLA code. We found that light curves are well described in the model with 40 M {sub ⊙} ejecta and 20–40 M {sub ⊙} circumstellar medium. The ejected {sup 56}Ni mass is about 6 M {sub ⊙}, which results from explosive nucleosynthesis with large explosion energy (2–3)×10{sup 52} erg. In comparison with alternative scenarios of pair-instability supernova and magnetar-powered supernova, in the interaction model, all the observed main photometric characteristics are well reproduced: multicolor light curves, color temperatures, and photospheric velocities.

79 ASTRONOMY AND ASTROPHYSICS↗

Astromers in the Radioactive Decay of r-process Nuclei

Certain nuclear isomers are well known to affect nucleosynthesis with important observable consequences (e.g., 26 Al and 180 Ta). We study the impact of nuclear isomers in the context of rapid neutron capture process (r-process) nucleosynthesis. Here we demonstrate that nuclear isomers are dynamically populated in the r process and that some are populated far from thermal equilibrium; this makes them astrophysical isomers, or "astromers." We compute thermally mediated transition rates between long-lived isomers and the corresponding ground states in neutron-rich nuclei. We calculate the temperature-dependent β-decay feeding factors, which represent the fraction of material going to each of the isomer and ground state daughter species from the β-decay parent species. We simulate nucleosynthesis following the decay of a solar-like r-process composition and include as separate species nuclear excited states with measured terrestrial half-lives greater than 100 μs. We introduce a new metric to identify those astromers most likely to be influential and summarize them in a table. Notable entries include many second peak nuclei (e.g., the Te isotopic chain) and previously overlooked isomers in stable nuclei (e.g., 119 Sn, 131 Xe, and 195 Pt). Finally, we comment on the capacity of isomer production to alter radioactive heating in an r-process environment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multimessengers from the Radioactive Decay of r -process Nuclei

The radioactive β-decay of nuclei synthesized in the rapid neutron capture process (r-process) releases a variety of particles, including electrons, γ-rays, neutrinos, and neutrons. These particles provide a rich set of multimessenger signals that carry information about the astrophysical environments where neutron-rich nucleosynthesis occurs. In this work, we calculate from first principles the emission spectra resulting from the β-decay of r-process nuclei. Our approach incorporates detailed nuclear structure and decay data to model the energy distributions of each particle species. We couple the spectra with a nuclear reaction network simulation to obtain the temporal evolution of these distributions. We find that the emission distributions vary significantly in time and are nonthermal, with substantial average energies. We investigate these nuclear signals as a direct probe of heavy element formation and show that they are complementary observables to kilonova.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Recent Direct Reaction Experimental Studies with Radioactive Tin Beams

Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z = 50 proton shell closure, as well as the neutron shell closures lying in the neutron-rich, N = 82, and neutron-deficient, N = 50, regions. Here, we present two examples of direct reactions on exotic tin isotopes. The first uses a one-neutron transfer reaction and a low-energy reaccelerated ISOL beam to study states in Sn-131 from across the N = 82 shell closure. The second example utilizes a one-neutron knockout reaction on fragmentation beams of neutron-deficient Sn- 106,108 Sn. In conclusion, In both cases, measurements of γ rays in coincidence with charged particles proved to be invaluable.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗