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At least 865 records · Page 48

Performance Simulations for a Spaceborne Methane Lidar Mission

Future spaceborne lidar measurements of key anthropogenic greenhouse gases are expected to close current observational gaps particularly over remote, polar, and aerosol-contaminated regions, where actual in situ and passive remote sensing observation techniques have difficulties. For methane, a "Methane Remote Lidar Mission" was proposed by Deutsches Zentrum fuer Luft- und Raumfahrt and Centre National d'Etudes Spatiales in the frame of a German-French climate monitoring initiative. Simulations assess the performance of this mission with the help of Moderate Resolution Imaging Spectroradiometer and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations of the earth's surface albedo and atmospheric optical depth. These are key environmental parameters for integrated path differential absorption lidar which uses the surface backscatter to measure the total atmospheric methane column. Results showthat a lidar with an average optical power of 0.45W at 1.6 μm wavelength and a telescope diameter of 0.55 m, installed on a low Earth orbit platform(506 km), will measure methane columns at precisions of 1.2%, 1.7%, and 2.1% over land, water, and snow or ice surfaces, respectively, for monthly aggregated measurement samples within areas of 50 × 50 km2. Globally, the mean precision for the simulated year 2007 is 1.6%, with a standard deviation of 0.7%. At high latitudes, a lower reflectance due to snow and ice is compensated by denser measurements, owing to the orbital pattern. Over key methane source regions such as densely populated areas, boreal and tropical wetlands, or permafrost, our simulations show that the measurement precision will be between 1 and 2%.

methane↗

Highlights from 4STAR Sky-Scanning Retrievals of Aerosol Intensive Optical Properties from Multiple Field Campaigns with Detailed Comparisons of SSA Reported During SEAC4RS

The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument combines airborne sun tracking capabilities of the Ames Airborne Tracking Sun Photometer (AATS-14) with AERONET (Aerosol Robotic Network)-like sky-scanning capability and adds state-of-the-art fiber-coupled grating spectrometry to yield hyperspectral measurements of direct solar irradiance and angularly resolved sky radiance. The combination of sun-tracking and sky-scanning capability enables retrievals of wavelength-dependent aerosol optical depth (AOD), mode-resolved aerosol size distribution (SD), asphericity, and complex refractive index, and thus also the scattering phase function, asymmetry parameter, single-scattering albedo (SSA), and absorption aerosol optical thickness (AAOT). From 2012 to 2014 4STAR participated in four major field campaigns: the U.S. Dept. of Energy's TCAP (Two-Column Aerosol Project) I & II campaigns, and NASA's SEAC4RS (Studies of Emissions, Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) and ARISE (Arctic Radiation - IceBridge Sea & Ice Experiment) campaigns. Establishing a strong performance record, 4STAR operated successfully on all flights conducted during each of these campaigns. Sky radiance spectra from scans in either constant azimuth (principal plane) or constant zenith angle (almucantar) were interspersed with direct beam measurements during level legs. During SEAC4RS and ARISE, 4STAR airborne measurements were augmented with flight-level albedo from the collocated Shortwave Spectral Flux Radiometer (SSFR) providing improved specification of below-aircraft radiative conditions for the retrieval. Calibrated radiances and retrieved products will be presented with particular emphasis on detailed comparisons of ambient SSA retrievals and measurements during SEAC4RS from 4STAR, AERONET, HSRL2 (High Spectral Resolution Lidar), and from in situ measurements.

Radiance↗

4STAR Sky-Scanning Retrievals of Aerosol Intensive Optical Properties from Multiple Field Campaigns with Detailed Comparisons of SSA Reported During SEAC4RS

The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument combines airborne sun tracking capabilities of the Ames Airborne Tracking Sun Photometer (AATS-14) with AERONET-like sky-scanning capability and adds state-of-the-art fiber-coupled grating spectrometry to yield hyper spectral measurements of direct solar irradiance and angularly resolved sky radiance. The combination of sun-tracking and sky-scanning capability enables retrievals of wavelength-dependent aerosol optical depth (AOD), mode-resolved aerosol size distribution (SD), asphericity, and complex refractive index, and thus also the scattering phase function, asymmetry parameter, single-scattering albedo (SSA), and absorption aerosol optical thickness (AAOT).From 2012 to 2014 4STAR participated in four major field campaigns: the U.S. Dept. of Energy TCAP I II campaigns, and NASAs SEAC4RS and ARISE campaigns. Establishing a strong performance record, 4STAR operated successfully on all flights conducted during each of these campaigns. Sky radiance spectra from scans in either constant azimuth (principal plane) or constant zenith angle (almucantar) were interspersed with direct beam measurements during level legs. During SEAC4RS and ARISE, 4STAR airborne measurements were augmented with flight-level albedo from the collocated Shortwave Spectral Flux Radiometer (SSFR) providing improved specification of below-aircraft radiative conditions for the retrieval. Calibrated radiances and retrieved products will be presented with particular emphasis on detailed comparisons of ambient SSA retrievals and measurements during SEAC4RS from 4STAR, AERONET, HSRL2, and from in situ measurements.

Flynn, Connor↗

Day 640 infrared line and continuum measurements: Dust formation in SN 1987A

We have measured day 640-645 line and continuum spectra of (Ni II) 6.6 micrometer (Ne II) 12.8 micrometer (line emission was not detected), and (Fe II) 17.9 and 26.0 micrometer from SN 1987A. The high velocity feature at v(sub HVF) approximately 3900 km/sec found in both of our day 410 (Fe II) spectra is again detected in the day 640 (Ni II) spectrum, although the signal-to-noise of the day 640 (Fe II) spectra is insufficient to show this feature. The continuum fluxes provide clear evidence for the formation of dust between day 410 and day 640 and are best fitted by a graybody spectrum with a temperature of 342 +/- 17 K at day 640 and a surface area corresponding to a minimum dust velocity v(sub dust) = 1910 +/- 170 km/sec. Optically thin dust emissivity laws proportional to lambda(exp -1) or lambda(exp -2) are inconsistent with the data. Either the dust grains are large (radius a much greater than 4 micrometer and radiate like individual blackbodies, or else they are located in clumps optically thick in the 6-26 micrometer range. The (Ni II) 6.6 micrometer line flux yields a minimum Ni(+) mass of 5.8 +/- 1.6 x 10(exp -4) solar mass and a Ni/Fe abundance ratio of 0.06 +/- 0.02, equal to the solar value. The ratio of the two (Fe II) line profiles implies a gas temperature 2600 +/- 700 K, a drop of 1800 +/- 800 K from our day 410 measurement. The (Fe II) 26.0 micrometer line flux has decreased by a factor of 2 and the day 640 (Ni II) profile is blueshifted by -440 +/- 270 km/sec, relative to observations before day 500. We show that the decrease in the (Fe II) flux and the blueshift are not produced by a decrease in electron scattering optical depth, electron density, or temperature, but rather are probably due to obscuration by the same dust which produces the infrared continuum. This supports the interpretation that the dust spectrum is produced by optically thick clumps. We discuss possible explanations for the discrepancy between the mass of Fe(+) detected and the total iron mass required to power the light curve. The decrease in the (Fe II) fluxes relative to the decrease required to account for the blueshifts of optical lines from non-iron-group elements and the similarity between v(sub dust) and the Ni(+) expansion velocity imply a spatial association between the dust clumps and the iron-group elements. In addition, the larger blueshift observed for the near and far-infrared, heavy metal transitions relative to non-iron-group lines suggests that the iron-group elements are somewhat segregated from lighter elements such as the Mg(sup 0) and O(sup 0) responsible for shorter wavelength lines. We speculate that FeS may be an important constituent of the dust. A comparison of our line profiles with radiative transfer models shows that while power law and exponential density distributions yield reasonable fits to the data, polytrope distributions provided significantly worse agreement. The best fits require a substantial fraction of the iron to be undetectable, and are consistent with maximum expansion velocities of v(sub max) approximately 3000 km/sec.

Colgan, Sean W. J.↗

A Fast Hybrid (3-D/1-D) Model for Thermal Radiative Transfer in Cirrus via Successive Orders of Scattering

We investigate the impact of cirrus cloud heterogeneity on the direct emission by cloud or surface and on the scattering by ice particles in the thermal infrared (TIR). Realistic 3-D cirri are modeled with the 3DCLOUD code, and top-of-atmosphere radiances are simulated by the 3-D Monte Carlo radiative transfer (RT) algorithm 3DMCPOL for two (8.65 micrometers and 12.05 micrometers) channels of the Imaging Infrared Radiometer on CALIPSO. At nadir, comparisons of 1-D and 3-D RT show that 3-D radiances are larger than their 1-D counterparts for direct emission but smaller for scattered radiation. For our cirrus cases, 99% of the 3-D total radiance is computed by the third scattering order, which corresponds to 90% of the total computational effort, but larger optical thicknesses need more scattering orders. To radically accelerate the 3-D RT computations (using only few percent of 3-D RT time with a Monte Carlo code), even in the presence of large optical depths, we develop a hybrid model based on exact 3-D direct emission, the first scattering order from 1-D in each homogenized column, and an empirical adjustment linearly dependent on the optical thickness to account for higher scattering orders. Good agreement is found between the hybrid model and the exact 3-D radiances for two very different cirrus models without changing the empirical parameters. We anticipate that a future deterministic implementation of the hybrid model will be fast enough to process multiangle thermal imagery in a practical tomographic reconstruction of 3-D cirrus fields.

radiative transfer↗

Vacuum ultraviolet absorption in a hydrogen arcjet

Atomic absorption spectroscopy was utilized to measure the ground state atomic hydrogen number density in the plasma produced in a low power hydrogen arcjet. A microwave driven hydrogen plasma was used as the source of radiation resonant with the vacuum ultraviolet Lyman alpha transition. The suitability of this radiation source is discussed. The optical depth of this transition prevented measurements at locations where the ground state atomic hydrogen number density was larger than 3 x 10 exp 19/cu m. These results indicate that other single-photon optical diagnostic techniques are equally ineffective in locations of higher hydrogen number density unless the spectral line shape of the atomic hydrogen absorbers is known.

Manzella, David H.↗

Fast two-stream method for computing diurnal-mean actinic flux in vertically inhomogeneous atmospheres

Based on a derivation of the two-stream daytime-mean equations of radiative flux transfer, a method for computing the daytime-mean actinic fluxes in the absorbing and scattering vertically inhomogeneous atmosphere is suggested. The method applies direct daytime integration of the particular solutions of the two-stream approximations or the source functions. It is valid for any duration of period of averaging. The merit of the method is that the multiple scattering computation is carried out only once for the whole averaging period. It can be implemented with a number of widely used two-stream approximations. The method agrees with the results obtained with 200-point multiple scattering calculations. The method was also tested in runs with a 1-km cloud layer with optical depth of 10, as well as with aerosol background. Comparison of the results obtained for a cloud subdivided into 20 layers with those obtained for a one-layer cloud with the same optical parameters showed that direct integration of particular solutions possesses an 'analytical' accuracy. In the case of the source function interpolation, the actinic fluxes calculated above the one-layer and 20-layer clouds agreed within 1%-1.5%, while below the cloud they may differ up to 5% (in the worst case). The ways of enhancing the accuracy (in a 'two-stream sense') and computational efficiency of the method are discussed.

Filyushkin, V. V.↗

The lunar environment and its effect on optical astronomy

The Moon's geologic environment features: (1) gravity field one-sixth that of Earth; (2) sidereal rotation period of 27.3 days; (3) surface with greater curvature than Earth's surface (a chord along a 10 km baseline would have a bulge of 7.2 m); (4) seismically and tidally stable platform on which to make astronomical observations (most moonquakes have magnitudes of 1 to 2 on the Richter scale, within the earth's seismic noise, resulting in ground motions only 1 nm); (5) tenuous atmosphere (the total mass at night is only 10(exp 4) kg) that has an optical depth of 10(exp -6) and does not cause wind induced stresses and vibrations on structures; (6) large diurnal temperature variation (100 to 385 K in equatorial regions), which telescopes must be designed to withstand; (7) weak magnetic field, ranging from 3 to 330 x 10(exp -9) T, compared to 3 x 10(exp -5) T on Earth at the equator; (8) surface exposed to radiation, the most dangerous of which are high energy (1 to 100 Mev) particles resulting from solar flares; (9) high flux of micrometeorites which are not slowed down from their cosmic velocities because of the lack of air (data indicate that microcraters greater than 10 microns across will form at the rate of 3000/sq m/yr); (10) regolith 2 to 30 m thick which blankets the entire lunar surface (this layer is fine-grained (average grain sizes range from 40 to 268 microns), has a low density (800 to 1000 kg/cu m in the upper few mm, rising to 1500 to 1800 kg/cu m at depths of 10 to 20 cm), is porous (35 to 45 pct), cohesive (0.1 to 1.0 kN/sq m), and has a low thermal diffusivity (0.7 to 1.0 x 110-8 sq m/sec); about 29 pct of the regolith is less than 20 micron in size (this dust could pose a hazard to optical telescopes); (11) rubbly upper several hundred meters in which intact bedrock is uncommon, especially in the lunar highlands; and (12) craters with diameter-to-depth ratios of 5 if fresh and less than km across (larger and eroded craters have diameter-to-depth ratios greater than 5).

Taylor, G. Jeffrey↗

Optical properties of marine stratocumulus clouds modified by ships

Results are presented of an application of the diffusion domain method to multispectral solar radiation measurements obtained deep within a marine stratocumulus cloud layer modified by pollution from ships. In situ airborne measurements of the relative angular distribution of scattered radiation are compared to known asymptotic expressions for the intensity field deep within an optically thick cloud layer. Analytical expressions relating the ratio of the nadir-to-zenith intensities to surface reflectance, similarity parameter, and scaled optical depth beneath the aircraft flight level are used to analyze measurements obtained with the cloud absorption radiometer mounted on the University of Washington's C-131A research aircraft. It is shown that the total optical thickness of the cloud layer increased in the ship tracks, in contrast to the similarity parameter, which decreased. The decrease in absorption was a direct consequence of the reduction in cloud droplet size that occurred within the ship tracks.

King, Michael D.↗

A Generalised Porosity Formalism for Isotropic and Anisotropic Effective Opacity and its Effects on X-ray Line Attenuation in Clumped O Star Winds

We present a generalised formalism for treating the porosity-associated reduction in continuum opacity that occurs when individual clumps in a stochastic medium become optically thick. As in previous work, we concentrate on developing bridging laws between the limits of optically thin and thick clumps. We consider geometries resulting in either isotropic or anisotropic effective opacity, and, in addition to an idealised model in which all clumps have the same local overdensity and scale, we also treat an ensemble of clumps with optical depths set by Markovian statistics. This formalism is then applied to the specific case of bound-free absorption of X- rays in hot star winds, a process not directly affected by clumping in the optically thin limit. We find that the Markov model gives surprisingly similar results to those found previously for the single clump model, suggesting that porous opacity is not very sensitive to details of the assumed clump distribution function. Further, an anisotropic effective opacity favours escape of X-rays emitted in the tangential direction (the venetian blind effect), resulting in a bump of higher flux close to line centre as compared to profiles computed from isotropic porosity models. We demonstrate how this characteristic line shape may be used to diagnose the clump geometry, and we confirm previous results that for optically thick clumping to significantly influence X-ray line profiles, very large porosity lengths, defined as the mean free path between clumps, are required. Moreover, we present the first X-ray line profiles computed directly from line-driven instability simulations using a 3-D patch method, and find that porosity effects from such models also are very small. This further supports the view that porosity has, at most, a marginal effect on X-ray line diagnostics in O stars, and therefore that these diagnostics do indeed provide a good clumping insensitive method for deriving O star mass-loss rates.

Sundqvist, Jon O.↗

A Generalised Porosity Formalism for Isotropic and Anisotropic Effective Opacity and Its Effects on X-ray Line Attenuation in Clumped O Star Winds

We present a generalised formalism for treating the porosity-associated reduction in continuum opacity that occurs when individual clumps in a stochastic medium become optically thick. As in previous work, we concentrate on developing bridging laws between the limits of optically thin and thick clumps. We consider geometries resulting in either isotropic or anisotropic effective opacity, and, in addition to an idealised model in which all clumps have the same local overdensity and scale, we also treat an ensemble of clumps with optical depths set by Markovian statistics. This formalism is then applied to the specific case of bound-free absorption of X- rays in hot star winds, a process not directly affected by clumping in the optically thin limit. We find that the Markov model gives surprisingly similar results to those found previously for the single clump model, suggesting that porous opacity is not very sensitive to details of the assumed clump distribution function. Further, an anisotropic effective opacity favours escape of X-rays emitted in the tangential direction (the venetian blind effect), resulting in a bump of higher flux close to line centre as compared to profiles computed from isotropic porosity models. We demonstrate how this characteristic line shape may be used to diagnose the clump geometry, and we confirm previous results that for optically thick clumping to significantly influence X-ray line profiles, very large porosity lengths, defined as the mean free path between clumps, are required. Moreover, we present the first X-ray line profiles computed directly from line-driven instability simulations using a 3-D patch method, and find that porosity effects from such models also are very small. This further supports the view that porosity has, at most, a marginal effect on X-ray line diagnostics in O stars, and therefore that these diagnostics do indeed provide a good clumping insensitive method for deriving O star mass-loss rates.

generalised↗

Low-velocity variability in the stellar wind of HD 152408 (O8: Iafpe)

We describe high-quality, spectroscopic time series observations of variability at low velocities in the stellar wind of the extreme O-supergiant HD 152408. These observations were obtained during a monitoring campaign coordinated between Australia and Chile in 1992 July. Systematic variability on hourly time scales is particularly apparent in the He I lambda 5876 P Cygni profile, which diagnoses the deeper, denser region of the wind. These changes indicate the presence of evolving wind structure, which takes the form of blueward-migrating, discrete optical depth enhancements. Four distinct features are identified over approximately 5 days, spanning a velocity range of about -50 km/s at formation to about -500 km/s (i.e., greater than or approximately equal to 0.5 of the terminal velocity) at the blue edge of the He I absorption trough. Sympathetic variations are also apparent in the Balmer emission lines of HD 152408. The characteristics of these features, including their widths, column densities, and accelerations, suggest similarities to discrete absorption components commonly seen at larger velocities in UV P Cygni profiles of other O-type stars. These optical results demonstrate that frequent, systematic wind variability is present down to very large depths, and provide constraints on the stability of the low-velocity regime of hot-star winds.

Prinja, Raman K.↗

An Overview of the Tropospheric Aerosol Radiative Forcing Observational Experiment

Aerosol effects on atmospheric radiation are a leading source of uncertainty in predicting future climate. As a result, the International Global Atmospheric Chemistry Program has established a Focus on Atmospheric Aerosols (IGAC/FAA) and endorsed a series of aerosol field campaigns. TARFOX, the second in the IGAC/FAA series, was designed to reduce this uncertainty by measuring aerosol properties and effects in the US eastern seaboard, where one of the world's major plumes of industrial haze moves from the continent over the Atlantic Ocean. TARFOX's objectives are to: 1. Make simultaneous measurements of: (a) aerosol effects on radiation fields, and (b) the chemical, physical, and optical properties of the aerosols causing those effects. 2. Perform a variety of closure studies by using overdetermined data sets to test the mutual consistency of measurements and calculations of a wide range of aerosol properties and effects. 3. Use the results of the closure studies to assess and reduce uncertainties in estimates of aerosol radiative forcing, as well as to guide future field programs. An important subset of the closure studies is tests and improvements of algorithms used to derive aerosol properties and radiative effects from satellite measurements. The TARFOX Intensive Field Period (IFP) was conducted July 10-31, 1996. It included coordinated measurements from four satellites (GOES-8, NOAA-14, ERS-2, LANDSAT), four aircraft (ER-2, C-130, C-131, and a modified Cessna), land sites, and ships. A variety of aerosol conditions was sampled, ranging from relatively clean behind frontal passages to moderately polluted with aerosol optical depths exceeding 0.5 at mid-visible wavelengths. The latter conditions included separate incidents of enhancements caused primarily by anthropogenic sources and another incident of enhancement apparently influenced by recent fog processing. Spatial gradients of aerosol optical thickness were sampled to aid in isolating aerosol effects from other radiative effects and to more tightly constrain closure tests, including those of satellite retrievals. This talk gives an overview of TARFOX goals, rationale, methods, and initial key findings.

Russell, P. B.↗

Energy-dependent Orbital Modulation of X-rays and Constraints on Emission of the Jet in Cyg X-3

We study orbital modulation of X-rays from Cyg X-3, using data from Swift, INTEGRAL and RXTE. Using the wealth of the presently available data and an improved averaging method, we obtain energy-dependent folded and averaged light curves with unprecedented accuracy. We find that above ∼5 keV, the modulation depth decreases with the increasing energy, which is consistent with the modulation being caused by both bound-free absorption and Compton scattering in the stellar wind of the donor, with minima corresponding to the highest optical depth, which occurs around the superior conjunction. We find a decrease of the depth below ∼3 keV, which appears to be due to re-emission of the absorbed continuum by the wind in soft X-ray lines. Based on the shape of the folded light curves, any X-ray contribution from the jet in Cyg X-3, which emits γ-rays detected at energies > 0.1 GeV in soft spectral states, is found to be minor up to ∼100 keV. This implies the presence of a rather sharp low-energy break in the jet MeV-range spectrum.We also calculate phase-resolved RXTE X-ray spectra, and show the difference between the spectra corresponding to phases around the superior and inferior conjunctions can indeed be accounted for by a combined effect of bound-free absorption in an ionized medium and Compton scattering.

Energy-dependent Orbital↗

Accretion disk coronae

Recent observations of partial X-ray eclipses from 4U1822-37 have shown that the central X-ray source in this system is diffused by a large Compton-thick accretion disk corona (ADC). Another binary, 4U2129-47, also displays a partial eclipse and contains an ADC. The possible origin of an ADC is discussed and a simple hydrostatic evaporated ADC model is developed which, when applied to 4U1822-37, 4U2129+47 and Cyg X-3, can explain their temporal and spectral properties. The quasi-sinusoidal modulation of all three sources can be reconciled with the partial occultation of the ADC by a bulge at the edge of the accretion disk which is caused by the inflowing material. The height of this bulge is an order of magnitude larger than the hydrostatic disk height and is the result of turbulence in the outer region of the disk. The spectral properties of all three sources can be understood in terms of Compton scattering of the original source spectrum by the ADC. Spectral variations with epoch in Cyg X-3 are probably caused by changes in the optical depth of the corona. A consequence of our model is that any accreting neutron star X-ray source in a semi-detached binary system which is close to its Eddington limit most likely contains an optically thick ADC.

White, N. E.↗

Twenty years of balloon-borne tropospheric aerosol measurements at Laramie, Wyoming

The paper examines the tropospheric aerosol record obtained over the period 1971 to 1990, during which high-altitude balloons with optical particle counters were launched at Laramie, Wyoming, in a long-term study of the stratospheric sulfate aerosol layer. All aerosol particle size ranges display pronounced seasonal variations, with the condensation nuclei concentration and the optically active component showing a summer maximum throughout the troposphere. Mass estimates, assuming spherical sulfate particles, indicate an average column mass between altitudes of 2.5 and 10 km of about 4 and 16 mg/sq m in winter and summer, respectively. Calculated optical depths vary between 0.01 and 0.04 from winter to summer; the estimated mass scattering cross section is about 3 sq m/g throughout the troposphere. There is evidence for a decreasing trend of 1.6-1.8 percent/yr in the optically active tropospheric aerosol over the past 20 yr, which may be related to a similar reduction in SO2 emission in the U.S. over this period.

Hofmann, David J.↗

Global Lidar Measurements of Clouds and Aerosols from Space Using the Geoscience Laser Altimeter System (GLAS)

The Geoscience Laser Altimeter System (GLAS) is scheduled for launch on the ICESat satellite as part of the NASA EOS mission in 2002. GLAS will be used to perform high resolution surface altimetry and will also provide a continuously operating atmospheric lidar to profile clouds, aerosols, and the planetary boundary layer with horizontal and vertical resolution of 175 and 76.8 m, respectively. GLAS is the first active satellite atmospheric profiler to provide global coverage. Data products include direct measurements of the heights of aerosol and cloud layers, and the optical depth of transmissive layers. In this poster we provide an overview of the GLAS atmospheric data products, present a simulated GLAS data set, and show results from the simulated data set using the GLAS data processing algorithm. Optical results from the ER-2 Cloud Physics Lidar (CPL), which uses many of the same processing algorithms as GLAS, show algorithm performance with real atmospheric conditions during the Southern African Regional Science Initiative (SAFARI 2000).

Hlavka, Dennis L.↗

Extensive Characterization of Aerosol Optical Properties and Chemical Component Concentrations: Application of the GRASP/Component Approach to Long-term AERONET Measurements

A recently developed GRASP/Component approach (GRASP: Generalized Retrieval of Atmosphere and Surface Properties) was applied to AERONET (Aeronet Robotic Network) sun photometer measurements in this study. Unlike traditional aerosol component retrieval, this approach allows the inference of some information about aerosol composition directly from measured radiance, rather than indirectly through the inversion of optical parameters, and has been integrated into the GRASP algorithm. The newly developed GRASP/Component approach was applied to 13 AERONET sites for different aerosol types under the assumption of aerosol internal mixing rules to analyze the characteristics of aerosol components and their distribution patterns. The results indicate that the retrievals can characterize well the spatial and temporal variability of the component concentration for different aerosol types. A reasonable agreement between GRASP BC retrievals and MERRA-2 BC products is found for all different aerosol types. In addition, the relationships between aerosol component content and aerosol optical parameters such as aerosol optical depth (AOD), fine-mode fraction (FMF), absorption Ångström exponent (AAE), scattering Ångström exponent (SAE), and single scattering albedo (SSA) are also analyzed for indirect verifying the reliability of the component retrieval. It was demonstrated the GRASP/Component optical retrievals are in good agreement with AERONET standard products [e.g., correlation coefficient (R) of 0.93–1.0 for AOD, fine-mode AOD (AODF), coarse-mode AOD (AODC) and Ångström exponent (AE); R = ~ 0.8 for absorption AOD (AAOD) and SSA; RMSE (root mean square error) < 0.03 for AOD, AODF, AODC, AAOD and SSA]. Thus, it is demonstrated the GRASP/Component approach can provide aerosol optical products with comparable accuracy as the AERONET standard products from the ground-based sun photometer measurements as well as some additional important inside on aerosol composition.

Xindan Zhang↗