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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 865 records · Page 48
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Electron density measurement using a partially covered hairpin resonator in an inductively coupled plasma

Hairpin probes are used to determine electron densities via measuring the shift of the resonant frequency of the probe structure when immersed in a plasma. This manuscript presents new developments in hairpin probe hardware and theory that have enabled measurements in a high electron density plasma, up to approximately 10 12 cm -3 , corresponding to a plasma frequency of about 9 GHz. Hardware developments include the use of both quarter-wavelength and three-quarter-wavelength partially covered hairpin probes in a transmission mode together with an easily reproducible implementation of the associated microwave electronics using commercial off-the-shelf components. The three-quarter-wavelength structure is operated at its second harmonic with the purpose of measuring higher electron densities. New theory developments for interpreting the probe measurements include the use of a transmission line model to find an accurate relationship between the resonant frequency of the probe and the electron density, including effects of partially covering the probes with epoxy. Measurements are taken in an inductively coupled plasma sustained in argon at pressures below 50 mTorr. Results are compared with Langmuir probe and interferometry measurements.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Temperature effects on the nanoscale thermoelastic response of a SiO2 membrane

We crossed two femtosecond extreme ultraviolet (EUV) pulses on a 100 nm thick amorphous membrane of SiO2, generating transient gratings (TGs) of light intensity with 84 nm spatial periodicity. The EUV TG excitation gave rise to the efficient generation of Lamb waves (LWs) and of a temperature grating, whose dynamics was studied at two different initial sample temperatures, 50 and 300 K. The short penetration depth of the EUV excitation pulses turned into a strong non-uniformity in the actual temperature as a function of the depth from the sample surface. At the lowest temperature, the LW frequencies presented a sizable shift in time due to the thermal equilibration along the membrane thickness. The analysis of the EUV TG waveforms allowed us to determine the decay time of the thermal grating and the sound attenuation coefficient, both found in reasonable agreement with the literature. The results show how EUV TG can provide information of non-equilibrium thermoelastic dynamics in thin membranes transparent to optical radiation.

Materials Science↗
DOE OSTI2013

Self-diffraction of ultrashort laser pulses under resonant excitation of excitons in a colloidal solution of CdSe/ZnS quantum dots

We report self-diffraction processes of two types under resonant excitation of the fundamental electron – hole (exciton) transition in a strongly absorbing colloidal solution of CdSe/ZnS quantum dots (QDs) by high-power picosecond laser pulses. In the first case the absorption saturation (bleaching) at the exciton transition frequency and the Stark shift of exciton absorption line lead to the formation of a transparency channel and self-diffraction of the laser beam from the thus induced round diaphragm. In the second case, self-diffraction of two laser beams, intersecting in a cell with a colloidal QD solution, occurs on the diffraction grating induced by these beams. The physical processes responsible for the nonlinear optical properties of CdSe/ZnS QDs and the found selfaction effects are analysed. (nonlinear optical phenomena)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Rabi spectroscopy of the clock transition in thulium atoms in a one-dimensional optical lattice

The clock transition at a wavelength of 1.14 μm in thulium atoms in an optical lattice in the Lamb – Dick regime is studied. The capture of thulium atoms makes it possible to suppress completely both the transition broadening due to the first-order Doppler effect and the shift of the transition frequency caused by the recoil effect. The excitation spectra of sideband oscillation frequencies and Rabi oscillations of population between the clock transition levels upon resonance excitation are investigated. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

POSSIBLE EVIDENCE OF ALFVEN-CYCLOTRON WAVES IN THE ANGLE DISTRIBUTION OF MAGNETIC HELICITY OF SOLAR WIND TURBULENCE

The fluctuating magnetic helicity is considered an important parameter in diagnosing the characteristic modes of solar wind turbulence. Among them is the Alfven-cyclotron wave, which is probably responsible for the solar wind plasma heating, but has not yet been identified from the magnetic helicity of solar wind turbulence. Here, we present the possible signatures of Alfven-cyclotron waves in the distribution of magnetic helicity as a function of {theta}{sub VB}, which is the angle between the solar wind velocity and local mean magnetic field. We use magnetic field data from the STEREO spacecraft to calculate the {theta}{sub VB} distribution of the normalized reduced fluctuating magnetic helicity {sigma}{sub m}. We find a dominant negative {sigma}{sub m} for 1 s < p < 4 s (p is time period) and for {theta}{sub VB} < 30 deg. in the solar wind outward magnetic sector, and a dominant positive {sigma}{sub m} for 0.4 s < p < 4 s and for {theta}{sub VB}>150 deg. in the solar wind inward magnetic sector. These features of {sigma}{sub m} appearing around the Doppler-shifted ion-cyclotron frequencies may be consistent with the existence of Alfven-cyclotron waves among the outward propagating fluctuations. Moreover, right-handed polarized waves at larger propagation angles, which might be kinetic Alfven waves or whistler waves, have also been identified on the basis of the {sigma}{sub m} features in the angular range 40 deg. < {theta}{sub VB} < 140 deg. Our findings suggest that Alfven-cyclotron waves (together with other wave modes) play a prominent role in turbulence cascading and plasma heating of the solar wind.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Relativistic general-order coupled-cluster method for high-precision calculations: Application to the Al{sup +} atomic clock

We report the implementation of a general-order relativistic coupled-cluster method for performing high-precision calculations of atomic and molecular properties. As a first application, the black-body radiation shift of the Al{sup +} clock has been estimated precisely. The computed shift relative to the frequency of the 3s{sup 2} {sup 1}S{sub 0}{sup e}{yields}3s3p {sup 3}P{sub 0}{sup o} clock transition given by (-3.66{+-}0.60)x10{sup -18} calls for an improvement over the recent measurement with a reported result of (-9{+-}3)x10{sup -18}[Phys. Rev. Lett. 104, 070802 (2010)].

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2011

Casimir force between a microfabricated elliptic cylinder and a plate

We investigate the Casimir force between a microfabricated elliptic cylinder (cylindrical lens) and a plate made of real materials. After a brief discussion of the fabrication procedure, which typically results in elliptic rather than circular cylinders, the Lifshitz-type formulas for the Casimir force and for its gradient are derived. In the specific case of equal semiaxes, the resulting formulas coincide with those derived previously for circular cylinders. The nanofabrication procedure may also result in asymmetric cylindrical lenses obtained from parts of two different cylinders, or rotated through some angle about the axis of the cylinder. In these cases, the Lifshitz-type formulas for the Casimir force between a lens and a plate and for its gradient are also derived, and the influence of lens asymmetry is determined. Additionally, we obtain an expression for the shift of the natural frequency of a micromachined oscillator with an attached elliptic cylindrical lens interacting with a plate via the Casimir force in a nonlinear regime.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Effects of Lorentz-symmetry violation on the spectra of rare-earth ions in a crystal field

Here, we demonstrate that experiments measuring the transition energies of rare-earth ions doped in crystalline lattices are sensitive to violations of local Lorentz invariance and Einstein's equivalence principle. Using the crystal field of LaCl 3 as an example, we calculate the frame-dependent energy shifts of the transition frequencies between low-lying states of Ce 3+ , Nd 3+ , and Er 3+ dopants in the context of the standard model extension, and show that they have high sensitivity to electron anomalies that break rotational invariance.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Observation of cupratelike nonlinear terahertz responses in superconducting infinite-layer nickelates via two-dimensional coherent spectroscopy

The 𝑑-wave pairing symmetry in newly discovered infinite-layer nickelates remains highly debated compared to the widely accepted 𝑑-wave superconductivity in cuprates, despite recent intense efforts using equilibrium optical and electrical transport measurements. A complementary approach involves characterizing THz coherent nonlinear responses, which is currently lacking but needed, as it would offer new insights into the superconducting gap structure by characterizing Higgs modes and quasiparticle excitations. Here, in this study, we report THz 2D coherent spectroscopy (THz-2DCS) responses from the superconducting state in an infinite-layer nickelate. The 2D spectra clearly demonstrate the absence of hallmark signatures of 𝑠-wave pairing symmetry, such as resonant 2⁢Δ peaks at superconducting gaps. Instead, we observe gapless 2D spectra in the nickelate, centered around the THz driving frequency, with no noticeable shift as the temperature increases. These findings closely resemble the nodal superconductivity behavior expected in cuprates. Together with our simulations, these findings suggest that 2⁢Δ signatures in the 2D spectra of 𝑑-wave gap structures can be obscured by significant nodal quasiparticle excitations at arbitrarily low energies. This contrasts with the long-lived Higgs modes, observed as distinct 2⁢Δ peaks in a controlled THz-2DCS experiment on niobium, a representative example of dirty-limit s-wave superconductors. Our results have implications for understanding the unconventional superconductivity in nickelates and highlight the need to explore their coherent nonlinear dynamics.

Pairing mechanisms↗
DOE OSTI2016

Nonlinear and time-resolved optical study of the 112-type iron-based superconductor parent Ca 1 – x La x FeAs 2 across its structural phase transition

The newly discovered 112-type ferropnictide superconductors contain chains of As atoms that break the tetragonal symmetry between the a and b axes. This feature eliminates the need for uniaxial strain that is usually required to stabilize large single domains in the electronic nematic state that exists in the vicinity of magnetic order in the iron-based superconductors. We report detailed structural symmetry measurements of 112-type Ca 0.73⁢ La 0.27 ⁢FeAs 2 using rotational anisotropy optical second-harmonic generation. This technique is complementary to diffraction experiments and enables a precise determination of the point-group symmetry of a crystal. By combining our measurements with density functional theory calculations, we uncover a strong optical second-harmonic response of bulk electric dipole origin from the Fe and Ca 3⁢d-derived states that enables us to assign C 2 as the crystallographic point group. This makes the 112-type materials high-temperature superconductors without a center of inversion, allowing for the possible mixing of singlet and triplet Cooper pairs in the superconducting state. We also perform pump-probe transient reflectivity experiments that reveal a 4.6-THz phonon mode associated with the out-of-plane motion of As atoms in the FeAs layers. We do not observe any suppression of the optical second-harmonic response or shift in the phonon frequency upon cooling through the reported monoclinic-to-triclinic transition at 58 K. Furthermore, this allows us to identify C 1 as the low-temperature crystallographic point group but suggests that structural changes induced by long-range magnetic order are subtle and do not significantly affect electronic states near the Fermi level.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Experimental observation of electron-phonon coupling enhancement in Sn nanowires caused by phonon confinement effects

Reducing the size of a superconductor below its characteristic length scales can either enhance or suppress its critical temperature ( T c ). Depending on the bulk value of the electron-phonon coupling strength, electronic and phonon confinement effects will play different roles in the modification of T c . Experimentally disentangling each contribution has remained a challenge. We have measured both the phonon density of states and T c of Sn nanowires with diameters of 18, 35, and 100 nm in order to quantify the effects of phonon confinement on superconductivity. Furthermore, we observe a shift of the phonon frequency towards the low-energy region and an increase in the electron-phonon coupling constant that can account for the measured increase in T c .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Probing new spin-independent interactions through precision spectroscopy in atoms with few electrons

The very high precision of current measurements and theory predictions of spectral lines in few-electron atoms allows us to efficiently probe the existence of exotic forces between electrons, neutrons and protons. We investigate here the sensitivity to new spin-independent interactions in transition frequencies (and their isotopic shifts) of hydrogen, helium and some heliumlike ions. We find that present data probe new regions of the force-carrier couplings to electrons and neutrons around the MeV mass range. We also find that, below few keV, the sensitivity to the electron coupling in precision spectroscopy of helium and positronium is comparable to that of the anomalous magnetic moment of the electron. Finally, we interpret our results in the dark-photon model where a new gauge boson is kinetically mixed with the photon. There, we show that helium transitions, combined with the anomalous magnetic moment of the electron, provide the strongest indirect bound from laboratory experiments above 100 keV.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Single-electron detection and spectroscopy via relativistic cyclotron radiation

It has been understood since 1897 that accelerating charges should emit electromagnetic radiation. Cyclotron radiation, the particular form of radiation emitted by an electron orbiting in a magnetic field, was first derived in 1904. Despite the simplicity of this concept, and the enormous utility of electron spectroscopy in nuclear and particle physics, single-electron cyclotron radiation has never been observed directly. Here we demonstrate single-electron detection in a novel radiofrequency spectrometer. We observe the cyclotron radiation emitted by individual electrons that are produced with mildly-relativistic energies by a gaseous radioactive source and are magnetically trapped. The relativistic shift in the cyclotron frequency permits a precise electron energy measurement. Precise beta electron spectroscopy from gaseous radiation sources is a key technique in modern efforts to measure the neutrino mass via the tritium decay endpoint, and this work is a proof-of-concept for future neutrino mass experiments using this technique.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Antiferromagnetic Resonance and Terahertz Continuum in α - RuCl 3

We report measurements of optical absorption in the zigzag antiferromagnet α-RuCl 3 as a function of temperature T , magnetic field B , and photon energy ℏ ω in the range ~ 0.3 –8.3 meV, using time-domain terahertz spectroscopy. Polarized measurements show that threefold rotational symmetry is broken in the honeycomb plane from 2 to 300 K. We find a sharp absorption peak at 2.56 meV upon cooling below the Néel temperature of 7 K at B = 0 that we identify as the magnetic-dipole excitation of a zero-wave-vector magnon, or antiferromagnetic resonance (AFMR). With the application of B , the AFMR broadens and shifts to a lower frequency as long-range magnetic order is lost in a manner consistent with transitioning to a spin-disordered phase. From a direct, internally calibrated measurement of the AFMR spectral weight, we place an upper bound on the contribution to the dc susceptibility from a magnetic excitation continuum.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Evaluation of Lattice Light Shift at Low 10 -19 Uncertainty for a Shallow Lattice Sr Optical Clock

A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. Here, we present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an accurate atomic clock. With precise control of the atomic motional states in the lattice, we report accurate measurements of the multipolar and the hyperpolar contributions and the operational lattice light shift with a fractional frequency uncertainty of 3.5×10 -19 .

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Converse magnetoelectric effects in composites of liquid phase epitaxy grown nickel zinc ferrite films and lead zirconate titanate: Studies on the influence of ferrite film parameters

The interactions among electric and magnetic subsystems in a ferroelectric-ferromagnetic composite occur through mechanical forces. In this work, we discuss results of a systematic investigation on the strength of the magnetic response of the composite to an applied electric field, known as the converse magnetoelectric (CME) effect, and its dependence on the ferroic order parameters and volume fraction for the two phases. Studies were carried out on composites of lead zirconate titanate and 2-30-μm m-thick nickel zinc ferrite (NZFO) films grown by liquid phase epitaxy on lattice matched (100) and (111) MgO substrates. Ferromagnetic resonance was utilized to determine the strength of CME from data on electric field E induced shift in the resonance frequency and its dependence on ferrite film orientation and thickness as well as MgO substrate thickness. The CME coupling coefficient A was found to be a factor of 2 to 4 higher in samples with NZFO films with (100) orientation than for (111) films. A decrease in A was measured with increasing ferrite film thickness and a very significant enhancement in the strength of CME was measured for decreasing MgO thickness. A model for CME that takes into consideration the influence of nonferroic MgO substrate was developed, and estimated A values are in very good agreement with the data. The findings presented here are also of importance for a new class of electric field tunable ferrite microwave devices.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Probing electromagnetic nonreciprocity with quantum geometry of photonic states

Reciprocal and nonreciprocal effects in dielectric and magnetic materials provide crucial information about the microscopic properties of electrons. However, experimentally distinguishing the two has proven to be challenging, especially when the associated effects are extremely small. To this end, we propose a contactless detection using a cross-cavity device where a material of interest is placed at its center. We show that the optical properties of the material, such as Kerr and Faraday rotation, or birefringence, manifest in the coupling between the cavity's electromagnetic modes and in the shift of their resonant frequencies. By calculating the dynamics of a geometrical photonic state, we formulate a measurement protocol based on the quantum metric and quantum process tomography that isolates the individual components of the material's complex refractive index and minimizes the quantum mechanical Cramér-Rao bound on the variance of the associated parameter estimation. Our approach is expected to be applicable across a broad spectrum of experimental platforms including Fock states in optical cavities, or coherent states in microwave and THz resonators. Published by the American Physical Society 2025

Petrides, Ioannis (ORCID:0000000174842444)↗
DOE OSTI2024

Aerosol-Jet Printed Transferable Millimeter-Wave Circuits

Printed millimeter wave (mmW) electronics have been of high interest in the field of communications for some time now due to the potential ability to fabricate mmW systems that utilize 3-Dimension Heterogeneous Integration (3DHI) to improve performance beyond traditional systems. Here, in this paper, a method for fabricating transferable mmW structures via aerosol-jet printing (AJP) is presented. A PDMS stamp assisted liftoff procedure is developed to separate the printed part from a rigid printing support surface and apply it to an adhesive target surface. Several microstrip (MS) line structures are demonstrated to characterize the effect of stamp transfer on the RF performance of the printed circuits. The effects of printed vias on RF probe pads and shifts in the resonant frequencies of a Beatty standard line after transfer are considered and characterized using S-parameter measurements.

42 ENGINEERING↗