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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 865 records · Page 48
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Long-lived coherences: Improved dispersion in the frequency domain using continuous-wave and reduced-power windowed sustaining irradiation

Long-lived coherences (LLC’s) are detectable magnetisation modes with favourable relaxation times that translate as sharp resonances upon Fourier transform. The frequency domain of LLC's was previously limited to the range of J-couplings within pairs of homonuclear spins. LLC evolution at high magnetic fields needs to be sustained by radio-frequency irradiation. We show that LLC-based spectral dispersion can be extended beyond the J-couplings domain using adapted carrier offsets and introduce a new reduced-power sustaining method to preserve LLC's within the required range of offsets. Spectral resolution is enhanced as the natively narrow lines of LLC's are further dispersed, making them potential probes for the study of biomolecules featuring strong resonance overlap and for media where NMR spectroscopy is commonly hindered by line broadening.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Mid-infrared intersubband polaritons in dispersive metal-insulator-metal resonators

We demonstrate room-temperature strong coupling between a mid-infrared (λ = 9.9 μm) intersubband transition and the fundamental cavity mode of a metal-insulator-metal resonator. Patterning of the resonator surface enables surface-coupling of the radiation and introduces an energy dispersion which can be probed with angle-resolved reflectivity. In particular, the polaritonic dispersion presents an accessible energy minimum at k = 0 where—potentially—polaritons can accumulate. We also show that it is possible to maximize the coupling of photons into the polaritonic states and—simultaneously—to engineer the position of the minimum Rabi splitting at a desired value of the in-plane wavevector. This can be precisely accomplished via a simple post-processing technique. The results are confirmed using the temporal coupled mode theory formalism and their significance in the context of the strong critical coupling concept is highlighted.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Dispersion of the linear and nonlinear optical susceptibilities of the CuAl(S{sub 1–x}Se{sub x})₂ mixed chaclcopyrite compounds

Based on the electronic band structure, we have calculated the dispersion of the linear and nonlinear optical susceptibilities for the mixed CuAl(S{sub 1–x}Se{sub x})₂ chaclcopyrite compounds with x=0.0, 0.25, 0.5, 0.75, and 1.0. Calculations are performed within the Perdew-Becke-Ernzerhof general gradient approximation. The investigated compounds possess a direct band gap of about 2.2 eV (CuAlS₂), 1.9 eV (CuAl(S₀.₇₅Se₀.₂₅)₂), 1.7 eV (CuAl(S₀.₅Se₀.₅)₂), 1.5 eV (CuAl(S₀.₂₅Se₀.₇₅)₂), and 1.4 eV (CuAlSe₂) which tuned to make them optically active for the optoelectronics and photovoltaic applications. These results confirm that substituting S by Se causes significant band gaps' reduction. The optical function's dispersion ε₂{sup xx}(ω) and ε₂{sup zz}(ω)/ε₂{sup xx}(ω), ε₂{sup yy}(ω), and ε₂{sup zz}(ω) was calculated and discussed in detail. To demonstrate the effect of substituting S by Se on the complex second-order nonlinear optical susceptibility tensors, we performed detailed calculations for the complex second-order nonlinear optical susceptibility tensors, which show that the neat parents compounds CuAlS₂ and CuAlSe₂ exhibit | χ₁₂₂²}(-2ω;ω;ω) | as the dominant component, while the mixed alloys exhibit | χ₁₁₁²(-2ω;ω;ω) | as the dominant component. The features of | χ₁₂₃²}(-2ω;ω;ω) | and | χ{sub 111}²}(-2ω;ω;ω) | spectra were analyzed on the basis of the absorptive part of the corresponding dielectric function ε₂(ω) as a function of both ω/2 and ω.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Dispersion relations for electromagnetic wave propagation in chiral plasmas

The dispersion relations for electromagnetic wave propagation in chiral plasmas are derived using a simplified method and investigated in detail. With the help of the dispersion relations for each eignwave, we explore how the chiral plasmas exhibit negative refraction and investigate the frequency region for negative refraction. The results show that chirality can induce negative refraction in plasmas. Moreover, both the degree of chirality and the external magnetic field have a significant effect on the critical frequency and the bandwidth of the frequency for negative refraction in chiral plasmas. The parameter dependence of the effects is calculated and discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Nonlinear dispersion and transverse profile of intense electromagnetic waves, propagating through electron-positron-ion hot magnetoplasma

Self-guided nonlinear propagation of intense circularly-polarized electromagnetic waves in a hot electron-positron-ion magnetoplasma is studied. Using a relativistic fluid model, a nonlinear equation is derived, which describes the interaction of the electromagnetic wave with the plasma in the quasi-neutral approximation. Transverse Eigen modes, the nonlinear dispersion relation and the group velocity are obtained. Results show that the transverse profile in the case of magnetized plasma with cylindrical symmetry has a radially damping oscillatory form. Effect of applying external magnetic fields, existence of the electron-positron pairs, changing the amplitude of the electromagnetic wave, and its polarization on the nonlinear dispersion relation and Eigen modes are studied.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Dispersion relations and polarizations of low-frequency waves in two-fluid plasmas

Analytical expressions for the dispersion relations and polarizations of low-frequency waves in magnetized plasmas based on two-fluid model are obtained. The properties of waves propagating at different angles (to the ambient magnetic field B{sub 0}) and β (the ratio of the plasma to magnetic pressures) values are investigated. It is shown that two linearly polarized waves—namely, the fast and Alfvén modes in the low-β (β≪1) plasmas, the fast and slow modes in the β∼1 plasmas, and the Alfvén and slow modes in the high-β (β≫1) plasmas—become circularly polarized at the near-parallel (to B{sub 0}) propagation. The negative magnetic-helicity of the Alfvén mode occurs only at small or moderate angles in the low-β plasmas, and the ion cross-helicity of the slow mode is nearly the same as that of the Alfvén mode in the high-β plasmas. It is also shown that the electric polarization δE{sub z}/δE{sub y} decreases with the temperature ratio T{sub e}/T{sub i} for the long-wavelength waves, and the transition between left- and right-hand polarizations of the Alfvén mode in T{sub e}/T{sub i}≠0 plasmas can disappear when T{sub e}/T{sub i}=0. The approximate dispersion relations in the near-perpendicular propagation, low-β, and high-β limits can quite accurately describe the three modes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Magnetic and nonthermal effects on the dispersion properties of ion-cyclotron surface wave in a semi-bounded generalized Lorentzian plasma

The magnetic field strength and the nonthermal effects on the dispersion properties of ion-cyclotron surface wave propagating along the interface of a semi-bounded Lorentzian plasma and a vacuum are kinetically investigated. The direction of external magnetic field is applied in parallel to the interface. By employing the specular reflection boundary condition, the dispersion relation of the ion-cyclotron surface wave is derived in the long wavelength limit. The result shows that the phase velocity of the ion-cyclotron surface wave decreases with an increase of the strength of magnetic field. It is found that the increase of suprathermal particle population suppresses the phase velocity of the surface wave. In addition, it is found that the wave velocity increases with increasing ion mass in a semi-bounded Lorentzian plasma.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2015

Dispersion, spatial growth rate, and start current of a Cherenkov free-electron laser with negative-index material

We present an analysis of a Cherenkov free-electron laser based on a single slab made from negative-index materials. In this system, a flat electron beam with finite thickness travelling close to the surface of the slab interacts with the copropagating electromagnetic surface mode. The dispersion equation for a finitely thick slab is worked out and solved numerically to study the dispersion relation of surface modes supported by negative-index materials, and the calculations are in good agreement with the simulation results from a finite difference time domain code. We find that under suitable conditions there is inherent feedback in such a scheme due to the characteristics of negative-index materials, which means that the system can oscillate without external reflectors when the beam current exceeds a threshold value, i.e., start current. Using the hydrodynamic approach, we setup coupled equations for this system, and solve these equations analytically in the small signal regime to obtain formulas for the spatial growth rate and start current.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Dispersive Alfvén waves in a plasma with anisotropic superthermal particles

The dispersion of dispersive Alfvén wave in a low β plasma with anisotropic superthermal particles modeled by a bi-nonextensive distribution is derived from a kinetic way. The effect of anisotropic temperature on inertial Alfvén wave is so small that it is negligible. However, it will play an important role on the property of kinetic Alfvén wave (KAW). The numerical results reveal that the presence of superthermal electrons in the small wavenumber limit will lead the damping rate of the KAW bigger than the one with Maxwellian distribution. Whereas, the damping rate of KAW in the large wavenumber limit will decrease with the presence of superthermal electrons. When the effect of electron anisotropic temperature overwhelms the effect of finite ion gyroradius in the small wavenumber regime, the damping rate of KAW grows with the presence of electron temperature anisotropy. On the other hand, when the effects of finite ion gyroradius play a dominant role in the large wavenumber regime, the damping rate of KAW increases with the effective perpendicular and parallel electron temperatures.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Determination of dispersion parameters of thermally deposited CdTe thin film

Cadmium Telluride (CdTe) thin film was deposited onto glass substrates under a vacuum of 5 × 10{sup −6} torr by using thermal evaporation technique. The prepared film was characterized for dispersion analysis from reflectance spectra within the wavelength range of 300 nm – 1100 nm which was recorded by using UV-Visible spectrophotometer. The dispersion parameters (oscillator strength, oscillator wavelength, high frequency dielectric constant, long wavelength refractive index, lattice dielectric constant and plasma resonance frequency) of CdTe thin film were investigated using single sellimeir oscillator model.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

The effects of nanoparticles and organic additives with controlled dispersion on dielectric properties of polymers: Charge trapping and impact excitation

This work presents a comprehensive investigation into the effects of nanoparticles and organic additives on the dielectric properties of insulating polymers using reinforced silicone rubber as a model system. TiO{sub 2} and ZrO{sub 2} nanoparticles (d = 5 nm) were well dispersed into the polymer via a bimodal surface modification approach. Organic molecules with the potential of voltage stabilization were further grafted to the nanoparticle to ensure their dispersion. These extrinsic species were found to provide deep traps for charge carriers and exhibited effective charge trapping properties at a rather small concentration (∼10{sup 17} cm{sup −3}). The charge trapping is found to have the most significant effect on breakdown strength when the electrical stressing time is long enough that most charges are trapped in the deep states. To establish a quantitative correlation between the trap depth and the molecular properties, the electron affinity and ionization energy of each species were calculated by an ab initio method and were compared with the experimentally measured values. The correlation however remains elusive and is possibly complicated by the field effect and the electronic interactions between different species that are not considered in this computation. At high field, a super-linear increase of current density was observed for TiO{sub 2} filled composites and is likely caused by impact excitation due to the low excitation energy of TiO{sub 2} compared to ZrO{sub 2}. It is reasoned that the hot charge carriers with energies greater than the excitation energy of TiO{sub 2} may excite an electron-hole pair upon collision with the NP, which later will be dissociated and contribute to free charge carriers. This mechanism can enhance the energy dissipation and may account for the retarded electrical degradation and breakdown of TiO{sub 2} composites.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Aging kinetics of levoglucosan orientational glass as a rate dispersion process and consequences for the heterogeneous dynamics view

Aging kinetics of a glass is currently modeled in terms of slowing of its α-relaxation dynamics, whose features are interpreted in terms of dynamic heterogeneity, i.e., formation and decay of spatially and temporally distinct nm-size regions. To test the merits of this view, we studied the calorimetric effects of aging an orientational glass of levoglucosan crystal in which such regions would not form in the same way as they form in liquids, and persist in structural glasses, because there is no liquid-like molecular diffusion in the crystal. By measuring the heat capacity, C{sub p}, we determined the change in the enthalpy, H, and the entropy, S, during two aging-protocols: (a) keeping the samples isothermally at temperature, T{sub a}, and measuring the changes after different aging times, t{sub a}, and (b) keeping the samples at different T{sub a}s and measuring the changes after the same t{sub a}. A model-free analysis of the data shows that as t{sub a} is increased (procedure (a)), H and S decrease according to a dispersive rate kinetics, and as T{sub a} is increased (procedure (b)), H and S first increase, reach a local maximum at a certain T{sub a}, and then decrease. Even though there is no translational diffusion to produce (liquid-like) free volume, and no translational-rotational decoupling, the aging features are indistinguishable from those of structural glasses. We also find that the Kohlrausch parameter, originally fitted to the glass-aging data, decreases with decrease in T{sub a}, which is incompatible with the current use of the aging data for estimating the α-relaxation time. We argue that the vibrational state of a glass is naturally incompatible with its configurational state, and both change on aging until they are compatible, in the equilibrium liquid. So, dipolar fluctuations seen as the α-relaxation would not be the same motions that cause aging. We suggest that aging kinetics is intrinsically dispersive with its own characteristic rate constant and it does not yield the α-relaxation rate. In this view, thermodynamic and other properties define the fictive temperature; the real or imaginary components of a dynamic property do not define it. While particles’ overall motions may still play a crucial role in (structural) glass physics, we conclude that translational diffusion alone is not a requirement for structure stabilization on aging of a kinetically frozen state.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2013

Mathematical modelling of dispersion-managed thulium/holmium fibre lasers

The mathematical model of a dispersion-managed thulium/holmium fibre laser is described; the results of numerical calculations and their comparison with the experimental data are presented. Qualitative agreement of the results of the mathematical modelling with those of the experiment is obtained. Using the methods of mathematical modelling, the variation in the characteristics of the optical pulses due to the change in the average cavity dispersion is analysed. (control of laser radiation parameters)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Cross modulation instability in normal-dispersion fibre lasers and amplifiers

This paper examines instability resulting from cross phase modulation interaction between signal and pump waves in normal-dispersion fibre lasers and amplifiers. From analysis of the dispersion relation for the wave vector of small harmonic perturbations, we derive dynamic spectral characteristics of the modulation gain coefficient. Its dependence on the group velocity difference between signal and pump waves is investigated. Analytical results are compared to numerical simulation data. We discuss how the general relationships obtained in this study can be used in practical applications. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Dispersion management of the SULF front end

To manage dispersion of the front end in the Shanghai Superintense Ultrafast Laser Facility (SULF), which is a large-scale project aimed at delivering 10 PW laser pulses, a stretcher based on a combination of a grating and a prism (grism) pair is inserted between an Öffner-triplet-type stretcher and a regenerative amplifier to reduce high-order dispersion introduced by optical materials at the amplification stage. The alignment of the grism pair is implemented by controlling the far-field pattern of the output beam of the grism pair. The energy of the front end reaches up to 7 J at a 1-Hz repetition rate. Experimental results show that the pulse duration can be compressed to 22.4 fs and the spectral distortion over the spectrum is less than 2.25 rad. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Nonlinear noise suppression in a high-rate optical channel with phase modulation and dispersion compensation

We have performed a numerical simulation of transmission of optical DP QPSK signals at a rate of 40 Gbaud over a distance of 2000 km. It is shown that a channel with large negative dispersion and preliminary large positive pulse chirping significantly reduces nonlinear distortion and improves the signal quality. To further reduce the probability of recognition error, it is proposed, instead of a negative dispersion fibre, to use compensators with low attenuation. (fibre-optic communication lines)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Numerical simulation of dispersion and nonlinear characteristics of microstructured silica fibres with a thin suspended core in a wide range of their parameters

Dispersion and nonlinear characteristics of microstructured silica fibres with a thin suspended core surrounded by three, four or six air holes have been studied theoretically in the wavelength range 1 – 2 μm. It has been shown that, owing to strong fundamental mode confinement near the core, the Kerr nonlinearity coefficient can exceed the nonlinearity coefficient of standard telecom fibre SMF28e by two orders of magnitude. The large waveguide contribution allows for effective group velocity dispersion management. Estimates are presented that demonstrate the feasibility of using suspended core fibre exhibiting Kerr nonlinearity for generating non-classical light: a state with squeezed quantum fluctuations in one of the quadrature components of a cw laser signal at a wavelength near 1.55 μm. (paper)

36 MATERIALS SCIENCE↗
DOE OSTI2023

hpMCA: A Python-based Graphical Program for Energy Dispersive X-Ray Diffraction Data Collection and Analysis

Energy-dispersive X-ray diffraction (EDXD) at synchrotron beamlines is commonly used for the study of material properties under high pressure and/or high temperature. Experimenters typically rely on the availability of robust data collection and analysis at a beamline, but this has become increasingly difficult, especially with the introduction of multi-element detectors that generate complex, multi-dimensional data sets. These data sets have energy resolution, and they can also be resolved in relation to sample position, diffraction angle, or different external stimuli. We report a new Python-based graphical program, hpMCA, for EDXD data collection and analysis that streamlines the experimental process for the beamline users. The program features a user-friendly interface, capability for online viewing and analyzing data from multi-element energy-dispersive detectors, and includes features useful for working with samples under high pressure and/or high temperature, such as crystal phase identification, real-time unit cell lattice refinement, and pressure determination based on an equation of state.

data analysis software↗